Articles | Volume 22, issue 5
https://doi.org/10.5194/acp-22-3469-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-3469-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 Mar 2022
Research article |
| 16 Mar 2022
| 16 Mar 2022
Occurrence and growth of sub-50 nm aerosol particles in the Amazonian boundary layer
Institute of Physics, University of São Paulo, São Paulo 05508-900, Brazil
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Florian Ditas
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
now at: Hessian Agency for Nature Conservation, Environment and Geology, 65203 Wiesbaden, Germany
Leslie A. Kremper
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Luiz A. T. Machado
Institute of Physics, University of São Paulo, São Paulo 05508-900, Brazil
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Meinrat O. Andreae
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Scripps Institution of Oceanography, University of California San Diego, La Jolla, CA 92037, USA
Department of Geology and Geophysics, King Saud University, Riyadh, Saudi Arabia
Alessandro Araújo
Empresa Brasileira de Pesquisa Agropecuária (Embrapa) Amazonia Oriental, CEP 66095-100, Belém, Brazil
Henrique M. J. Barbosa
Institute of Physics, University of São Paulo, São Paulo 05508-900, Brazil
Joel F. de Brito
IMT Lille Douai, Institut Mines-Télécom, Université de Lille, Centre for Energy and Environment, 59000 Lille, France
Samara Carbone
Agrarian Sciences Institute, Federal University of Uberlândia, Uberlândia-MG, 38408-100, Brazil
Bruna A. Holanda
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Fernando G. Morais
Institute of Physics, University of São Paulo, São Paulo 05508-900, Brazil
Janaína P. Nascimento
National Institute for Amazonian Research, Manaus, AM, 69.060-000, Brazil
now at: NOAA Global Systems Laboratory, Boulder, CO 80305, USA
Mira L. Pöhlker
CORRESPONDING AUTHOR
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Experimental Aerosol and Cloud Microphysics Department, Leibniz Institute for Tropospheric Research, Leipzig, Germany
Luciana V. Rizzo
Federal University of Sao Paulo, Department of Environmental Sciences, Diadema, Brazil
Marta Sá
National Institute for Amazonian Research, Manaus, AM, 69.060-000, Brazil
Jorge Saturno
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
now at: Department 3.4 Analytical Chemistry of the Gas Phase, Physikalisch-Technische Bundesanstalt, 38116 Braunschweig, Germany
David Walter
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Department of Biogeochemical Systems, Max Planck Institute for Biogeochemistry, 07701 Jena, Germany
now at: Climate Geochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Stefan Wolff
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Ulrich Pöschl
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Paulo Artaxo
Institute of Physics, University of São Paulo, São Paulo 05508-900, Brazil
Christopher Pöhlker
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
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Cited
24 citations as recorded by crossref.
- Numerical simulation and evaluation of global ultrafine particle concentrations at the Earth's surface M. Kohl et al. 10.5194/acp-23-13191-2023
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- Satellite‐Based Detection of Secondary Droplet Activation in Convective Clouds A. Efraim et al. 10.1029/2022JD036519
- Particle Number Size Distribution of Wintertime Alpine Aerosols and Their Activation as Cloud Condensation Nuclei in the Guanzhong Plain, Northwest China Y. Chen et al. 10.1029/2022JD037877
- Statistical analysis and environmental impact of pre-existing particle growth events in a Northern Chinese coastal megacity: A 725-day study in 2010–2018 X. Wei et al. 10.1016/j.scitotenv.2024.173227
- Nontrivial Impact of Relative Humidity on Organic New Particle Formation from Ozonolysis of cis-3-Hexenyl Acetate A. Flueckiger et al. 10.3390/air1040017
- Global variability in atmospheric new particle formation mechanisms B. Zhao et al. 10.1038/s41586-024-07547-1
- Sink, Source or Something In‐Between? Net Effects of Precipitation on Aerosol Particle Populations T. Khadir et al. 10.1029/2023GL104325
- Relationship between Land Use and Spatial Variability of Atmospheric Brown Carbon and Black Carbon Aerosols in Amazonia F. Morais et al. 10.3390/atmos13081328
- African biomass burning affects aerosol cycling over the Amazon B. Holanda et al. 10.1038/s43247-023-00795-5
- Secondary droplet activation during condensational growth in convective clouds and its detection from satellites A. Efraim et al. 10.1016/j.atmosres.2023.107196
- Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories G. Unfer et al. 10.5194/acp-24-3869-2024
- On the Sensitivity of a Ground-Based Tropospheric Lidar to Aitken Mode Particles in the Upper Troposphere M. Silva et al. 10.3390/rs14194913
- Process-evaluation of forest aerosol-cloud-climate feedback shows clear evidence from observations and large uncertainty in models S. Blichner et al. 10.1038/s41467-024-45001-y
- Aerosol optical depth and water vapor variability assessed through autocorrelation analysis M. Franco et al. 10.1007/s00703-024-01011-5
- Contribution of regional aerosol nucleation to low-level CCN in an Amazonian deep convective environment: results from a regionally nested global model X. Wang et al. 10.5194/acp-23-4431-2023
- Characterization of ultrafine particles and the occurrence of new particle formation events in an urban and coastal site of the Mediterranean area A. Dinoi et al. 10.5194/acp-23-2167-2023
- A comprehensive study on the validation and application of multi-lognormal distribution models for atmospheric particles K. Zhu & L. Wang 10.1016/j.atmosenv.2024.120813
- Frequent rainfall-induced new particle formation within the canopy in the Amazon rainforest L. Machado et al. 10.1038/s41561-024-01585-0
- Vertically resolved aerosol variability at the Amazon Tall Tower Observatory under wet-season conditions M. Franco et al. 10.5194/acp-24-8751-2024
- Analysis of the Influence of Deforestation on the Microphysical Parameters of Clouds in the Amazon H. da Silva et al. 10.3390/rs14215353
- Vertical Profiles of Particle Number Size Distribution and Variation Characteristics at the Eastern Slope of the Tibetan Plateau C. Shu et al. 10.3390/rs15225363
- Formation Process of Particles and Cloud Condensation Nuclei Over the Amazon Rainforest: The Role of Local and Remote New‐Particle Formation B. Zhao et al. 10.1029/2022GL100940
- How rainfall events modify trace gas mixing ratios in central Amazonia L. Machado et al. 10.5194/acp-24-8893-2024
24 citations as recorded by crossref.
- Numerical simulation and evaluation of global ultrafine particle concentrations at the Earth's surface M. Kohl et al. 10.5194/acp-23-13191-2023
- Isoprene nitrates drive new particle formation in Amazon’s upper troposphere J. Curtius et al. 10.1038/s41586-024-08192-4
- Satellite‐Based Detection of Secondary Droplet Activation in Convective Clouds A. Efraim et al. 10.1029/2022JD036519
- Particle Number Size Distribution of Wintertime Alpine Aerosols and Their Activation as Cloud Condensation Nuclei in the Guanzhong Plain, Northwest China Y. Chen et al. 10.1029/2022JD037877
- Statistical analysis and environmental impact of pre-existing particle growth events in a Northern Chinese coastal megacity: A 725-day study in 2010–2018 X. Wei et al. 10.1016/j.scitotenv.2024.173227
- Nontrivial Impact of Relative Humidity on Organic New Particle Formation from Ozonolysis of cis-3-Hexenyl Acetate A. Flueckiger et al. 10.3390/air1040017
- Global variability in atmospheric new particle formation mechanisms B. Zhao et al. 10.1038/s41586-024-07547-1
- Sink, Source or Something In‐Between? Net Effects of Precipitation on Aerosol Particle Populations T. Khadir et al. 10.1029/2023GL104325
- Relationship between Land Use and Spatial Variability of Atmospheric Brown Carbon and Black Carbon Aerosols in Amazonia F. Morais et al. 10.3390/atmos13081328
- African biomass burning affects aerosol cycling over the Amazon B. Holanda et al. 10.1038/s43247-023-00795-5
- Secondary droplet activation during condensational growth in convective clouds and its detection from satellites A. Efraim et al. 10.1016/j.atmosres.2023.107196
- Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories G. Unfer et al. 10.5194/acp-24-3869-2024
- On the Sensitivity of a Ground-Based Tropospheric Lidar to Aitken Mode Particles in the Upper Troposphere M. Silva et al. 10.3390/rs14194913
- Process-evaluation of forest aerosol-cloud-climate feedback shows clear evidence from observations and large uncertainty in models S. Blichner et al. 10.1038/s41467-024-45001-y
- Aerosol optical depth and water vapor variability assessed through autocorrelation analysis M. Franco et al. 10.1007/s00703-024-01011-5
- Contribution of regional aerosol nucleation to low-level CCN in an Amazonian deep convective environment: results from a regionally nested global model X. Wang et al. 10.5194/acp-23-4431-2023
- Characterization of ultrafine particles and the occurrence of new particle formation events in an urban and coastal site of the Mediterranean area A. Dinoi et al. 10.5194/acp-23-2167-2023
- A comprehensive study on the validation and application of multi-lognormal distribution models for atmospheric particles K. Zhu & L. Wang 10.1016/j.atmosenv.2024.120813
- Frequent rainfall-induced new particle formation within the canopy in the Amazon rainforest L. Machado et al. 10.1038/s41561-024-01585-0
- Vertically resolved aerosol variability at the Amazon Tall Tower Observatory under wet-season conditions M. Franco et al. 10.5194/acp-24-8751-2024
- Analysis of the Influence of Deforestation on the Microphysical Parameters of Clouds in the Amazon H. da Silva et al. 10.3390/rs14215353
- Vertical Profiles of Particle Number Size Distribution and Variation Characteristics at the Eastern Slope of the Tibetan Plateau C. Shu et al. 10.3390/rs15225363
- Formation Process of Particles and Cloud Condensation Nuclei Over the Amazon Rainforest: The Role of Local and Remote New‐Particle Formation B. Zhao et al. 10.1029/2022GL100940
- How rainfall events modify trace gas mixing ratios in central Amazonia L. Machado et al. 10.5194/acp-24-8893-2024
Latest update: 13 Dec 2024
Short summary
In Central Amazonia, new particle formation in the planetary boundary layer is rare. Instead, there is the appearance of sub-50 nm aerosols with diameters larger than about 20 nm that eventually grow to cloud condensation nuclei size range. Here, 254 growth events were characterized which have higher predominance in the wet season. About 70 % of them showed direct relation to convective downdrafts, while 30 % occurred partly under clear-sky conditions, evidencing still unknown particle sources.
In Central Amazonia, new particle formation in the planetary boundary layer is rare. Instead,...
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