Articles | Volume 22, issue 20
https://doi.org/10.5194/acp-22-13467-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-13467-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Oct 2022
Research article |
| 19 Oct 2022
| 19 Oct 2022
Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface
Tao Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Yangyang Liu
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Hanyun Cheng
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Zhenzhen Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Hongbo Fu
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Jianmin Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Shanghai Institute of Pollution Control and Ecological Security, Shanghai,
200092, Peoples' Republic of China
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24 citations as recorded by crossref.
- Impact of SO2 and light on chemical morphology and hygroscopicity of natural salt aerosols X. Kong et al. 10.1016/j.atmosenv.2024.120373
- Heterogeneous photochemical uptake of SO2 on typical brown carbon species: A significant sulfate source H. Yang et al. 10.1016/j.atmosenv.2024.120425
- Analysis of secondary inorganic aerosols over the greater Athens area using the EPISODE–CityChem source dispersion and photochemistry model S. Myriokefalitakis et al. 10.5194/acp-24-7815-2024
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- Measurements of Water-Soluble Ions in Particulate Matter 2.5 in Polish Rural Areas: Identifying Possible Sources D. Chyzhykov & B. Mathews 10.1007/s11270-024-07265-4
- Modelling the European wind-blown dust emissions and their impact on particulate matter (PM) concentrations M. Liaskoni et al. 10.5194/acp-23-3629-2023
- Unveiling the Role of Carbonate Radical Anions in Dust‐Driven SO2 Oxidation Y. Liu et al. 10.1029/2023JD040017
- Black carbon and PM0.49 characterization in manila north harbour port, Metro Manila, Philippines J. Cadondon et al. 10.1016/j.envadv.2024.100526
- Nitrate formation and iron dissolution in the heterogeneous reactions of NH3 on nano α-Fe2O3 R. Wang et al. 10.1039/D3EN00494E
- Sink, Source or Something In‐Between? Net Effects of Precipitation on Aerosol Particle Populations T. Khadir et al. 10.1029/2023GL104325
- Rethinking urban haze formation: Atmospheric sulfite conversion rate scales with aerosol surface area, not volume L. Li et al. 10.1016/j.oneear.2024.05.007
- Nighttime–daytime PM10 source apportionment and toxicity in a remoteness inland city of the Iberian Peninsula Y. Cipoli et al. 10.1016/j.atmosenv.2023.119771
- Model Simulations and Predictions of Hydroxymethanesulfonate (HMS) in the Beijing-Tianjin-Hebei Region, China: Roles of Aqueous Aerosols and Atmospheric Acidity H. Wang et al. 10.1021/acs.est.3c07306
- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
- Characteristics of PM2.5 and secondary inorganic pollution formation during the heating season of 2021 in Beijing J. Wang et al. 10.3389/fenvs.2022.1028468
- Key Factors Determining the Formation of Sulfate Aerosols Through Multiphase Chemistry—A Kinetic Modeling Study Based on Beijing Conditions T. Wang et al. 10.1029/2022JD038382
- A CAPRAM Modeling Study on the Role of Heterogeneous Reactions on Dust in Tropospheric Chemistry M. Aiyuk et al. 10.1021/acsearthspacechem.4c00154
- Atmospheric fates of SO2 at the gas–solid interface of iron oxyhydroxide (FeOOH) minerals: effects of crystal structure, oxalate coating and light irradiance W. Wang et al. 10.1039/D2EN00874B
- Evaluating coarse PM composition and sources based on bulk and molecular speciation of PM2.5 and PM10 in Nanjing, East China W. Cui et al. 10.1016/j.jes.2024.04.038
- Interaction of Acrylic Acid and SO2 on the Surface of Mineral Dust Aerosol R. Wang et al. 10.1021/acsearthspacechem.2c00323
- Ambient PM2.5 and its components associated with 10-year atherosclerotic cardiovascular disease risk in Chinese adults J. Li et al. 10.1016/j.ecoenv.2023.115371
- Single Droplet Tweezer Revealing the Reaction Mechanism of Mn(II)-Catalyzed SO2 Oxidation X. Cao et al. 10.1021/acs.est.4c00309
- Classification and sources of extremely severe sandstorms mixed with haze pollution in Beijing T. Liu et al. 10.1016/j.envpol.2023.121154
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Latest update: 13 Dec 2024
Short summary
This study compared the gas-phase, aqueous-phase, and heterogeneous SO2 oxidation pathways by combining laboratory work with a modelling study. The heterogeneous oxidation, particularly that induced by the dust surface drivers, presents positive implications for the removal of airborne SO2 and formation of sulfate aerosols. This work highlighted the atmospheric significance of heterogeneous oxidation and suggested a comparison model to evaluate the following heterogeneous laboratory research.
This study compared the gas-phase, aqueous-phase, and heterogeneous SO2 oxidation pathways by...
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