Articles | Volume 22, issue 20
https://doi.org/10.5194/acp-22-13467-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-13467-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Oct 2022
Research article |
| 19 Oct 2022
| 19 Oct 2022
Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface
Tao Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Yangyang Liu
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Hanyun Cheng
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Zhenzhen Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Hongbo Fu
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Jianmin Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,
National Observations and Research Station for Wetland Ecosystems of the
Yangtze Estuary, IRDR international Center of Excellence on Risk
Interconnectivity and Governance on Weather, Department of Environmental
Science & Engineering, Fudan University, Shanghai, 200433, Peoples'
Republic of China
Shanghai Institute of Pollution Control and Ecological Security, Shanghai,
200092, Peoples' Republic of China
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33 citations as recorded by crossref.
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- Atmospheric fates of SO2 at the gas–solid interface of iron oxyhydroxide (FeOOH) minerals: effects of crystal structure, oxalate coating and light irradiance W. Wang et al. 10.1039/D2EN00874B
- Interaction of Acrylic Acid and SO2 on the Surface of Mineral Dust Aerosol R. Wang et al. 10.1021/acsearthspacechem.2c00323
- Single Droplet Tweezer Revealing the Reaction Mechanism of Mn(II)-Catalyzed SO2 Oxidation X. Cao et al. 10.1021/acs.est.4c00309
- Atmospheric Hydroxyl Radical Route Revealed: Interface-Mediated Effects of Mineral-Bearing Microdroplet Aerosol L. Yang et al. 10.1021/jacs.4c14149
- Analysis of secondary inorganic aerosols over the greater Athens area using the EPISODE–CityChem source dispersion and photochemistry model S. Myriokefalitakis et al. 10.5194/acp-24-7815-2024
- Unveiling the intricate dynamics of PM2.5 sulfate aerosols in the urban boundary layer: A pioneering two-year vertical profiling and machine learning-enhanced analysis in global Mega-City H. Li et al. 10.1016/j.uclim.2025.102424
- Atmospheric environment characteristic of severe dust storms and its impact on sulfate formation in downstream city N. Sun et al. 10.1016/j.scitotenv.2024.171128
- Rapid Sulfate Formation via Mn2+-Catalyzed SO2 Oxidation on the Surface of NaCl Microdroplets X. Jing et al. 10.1021/acs.jpcc.3c02839
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- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
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Latest update: 30 May 2025
Short summary
This study compared the gas-phase, aqueous-phase, and heterogeneous SO2 oxidation pathways by combining laboratory work with a modelling study. The heterogeneous oxidation, particularly that induced by the dust surface drivers, presents positive implications for the removal of airborne SO2 and formation of sulfate aerosols. This work highlighted the atmospheric significance of heterogeneous oxidation and suggested a comparison model to evaluate the following heterogeneous laboratory research.
This study compared the gas-phase, aqueous-phase, and heterogeneous SO2 oxidation pathways by...
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