Articles | Volume 22, issue 19
https://doi.org/10.5194/acp-22-12907-2022
© Author(s) 2022. This work is distributed under the Creative Commons Attribution 4.0 License.
NH3 spatiotemporal variability over Paris, Mexico City, and Toronto, and its link to PM2.5 during pollution events
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- Final revised paper (published on 07 Oct 2022)
- Supplement to the final revised paper
- Preprint (discussion started on 10 Jun 2022)
- Supplement to the preprint
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
| : Report abuse
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RC1: 'Comment on egusphere-2022-413', Anonymous Referee #1, 21 Jul 2022
- AC1: 'Reply on RC1', Camille Viatte, 02 Sep 2022
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RC2: 'Comment on egusphere-2022-413', Anonymous Referee #2, 22 Jul 2022
- AC2: 'Reply on RC2', Camille Viatte, 02 Sep 2022
Peer review completion
AR – Author's response | RR – Referee report | ED – Editor decision | EF – Editorial file upload
AR by Camille Viatte on behalf of the Authors (02 Sep 2022)
Author's response
Author's tracked changes
Manuscript
EF by Daria Karpachova (05 Sep 2022)
Supplement
EF by Daria Karpachova (05 Sep 2022)
Author's tracked changes
EF by Daria Karpachova (05 Sep 2022)
Supplement
ED: Publish subject to technical corrections (08 Sep 2022) by Jeffrey Geddes
AR by Camille Viatte on behalf of the Authors (09 Sep 2022)
Author's response
Manuscript
General comments:
The manuscript of egusphere-2022-413 presented the result of a unique project of the AmmonAQ that targeted different three areas of Paris, Toronto, and Mexico City. Towards better air quality by mitigating NH3 emissions, the finding of this study will contribute to improving the atmospheric environment. I generally agree with this manuscript being published; however, some points are concerned. Especially, I am wondering about the uncertainty of the satellite NH3 measurement dataset analyzed in this study. Please address the following specific points.
Specific comments:
P3, L52: Please specify these five countries.
P3, L65: Are these increasing trends explained by the expansion of NH3 emissions, or meteorological variability (e.g., temperature)?
P3, L77: Does “the standard” indicate the standard in Mexico? Because this study conducted the comparison over three regions, it will be better to explicitly state it.
P5, L111 (Section 2.1): Because of the recent progress in satellite NH3 measurement, I would like to strongly suggest including the discussion of the uncertainty of satellite data, such as the detection limit (https://doi.org/10.5194/acp-19-12261-2019).
P5, L115: What is the actual gridded data (e.g., Figure 2) analyzed in this study?
P5, L130: Although we can find the reason to choose the model simulation period of 2011 in P12, L344-P13, L349, it is better to be shortly explained here.
P6, L178: Are these three panels shown with the same horizontal distance? If different, the scaler might be helpful.
P6, L152: Too coarse reanalysis resolution to investigate air mass trajectories on 50 km radius-circle at each city?
P7, L188: Same to Europe and southern North America, source information of “(Canada)” or “(U.S.A.)” can be useful in this Table 1.
P13, L358: Should the denominator be “observations” when comparing observation and model? Why model is referred to as a criterion?
P13, L359: Are these values positive? If model underestimation, are these negative?
P14, L379: From the spatial mapping over Europe, this seems to be simply led to model overestimation, and this is not consistent with the timeseries and relevant discussion in the main text. Please confirm this figure.
P15, L413-418: From this comparison on PM2.5 component, I am suspicious about the result in other cities of Paris and Mexico City. When we considered this poor performance for PM2.5 components, the result in Figure 9 and the relevant discussion seems to be meaningless. Is this performance for PM2.5 component useful (worse or better than other studies)? If not, I would like to request to reconsider this final section in P14, L391-P16, L425.
Technical corrections:
P10, L281: 4.71 “×” 1015?
P12, L324 and L325: “m.s-1”? Does it need the period?