Articles | Volume 22, issue 2
https://doi.org/10.5194/acp-22-1251-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-22-1251-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 Jan 2022
Research article |
| 25 Jan 2022
| 25 Jan 2022
Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing
Jing Cai
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Cheng Wu
Department of Environmental Science, Stockholm University, Stockholm,
11418, Sweden
Jiandong Wang
School of Atmospheric Physics, Nanjing University of Information
Science and Technology, Nanjing 210044, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Feixue Zheng
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Simo Hakala
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Xiaolong Fan
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of
Sciences, Beijing 100085, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Zemin Feng
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Yongchun Liu
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Jun Zheng
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and
Pollution Control, Nanjing University of Information Science and
Technology, Nanjing 210044, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Federico Bianchi
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Markku Kulmala
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing 210023, China
Faculty of Geography, Lomonosov Moscow State University, Moscow,
Russia
Department of Environmental Science, Stockholm University, Stockholm,
11418, Sweden
Kaspar R. Daellenbach
CORRESPONDING AUTHOR
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Institute for Atmospheric and Earth System Research, Faculty of
Science, University of Helsinki, Helsinki 00014, Finland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
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Cited
18 citations as recorded by crossref.
- Recent Advancement in Organic Aerosol Understanding: a Review of Their Sources, Formation, and Health Impacts S. Chaturvedi et al. 10.1007/s11270-023-06772-0
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al. 10.1038/s41561-024-01493-3
- Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region J. Wang et al. 10.1007/s11783-023-1714-0
- Nighttime NO emissions strongly suppress chlorine and nitrate radical formation during the winter in Delhi S. Haslett et al. 10.5194/acp-23-9023-2023
- Linking Precursors and Volatility of Ambient Oxygenated Organic Aerosols Using Thermal Desorption Measurement and Machine Learning X. Wang et al. 10.1021/acsestair.4c00076
- Development of a high-resolution emissions inventory of carbonaceous particulate matters and their growth during 2011–2018 over India P. Kumar et al. 10.1016/j.atmosenv.2023.119750
- Measurement report: Molecular-level investigation of atmospheric cluster ions at the tropical high-altitude research station Chacaltaya (5240 m a.s.l.) in the Bolivian Andes Q. Zha et al. 10.5194/acp-23-4559-2023
- Weakened Gas-to-Particle Partitioning of Oxygenated Organic Molecules in Liquified Aerosol Particles W. Ma et al. 10.1021/acs.estlett.2c00556
- Molecular composition of organic aerosols in urban and marine atmosphere: A comparison study using FIGAERO-I-CIMS, ESI-FT-ICR MS, and GC × GC-EI-ToF-MS X. Xin et al. 10.1080/02786826.2024.2377394
- Impacts of elevated anthropogenic emissions on physicochemical characteristics of black-carbon-containing particles over the Tibetan Plateau J. Wang et al. 10.5194/acp-24-11063-2024
- Quantifying New Sources of Ambient Organic Aerosol and Their Roles in Particle Growth Using Oxygenated Organic Molecule (OOM) Tracers Y. Zhao et al. 10.1021/acs.estlett.4c00536
- Elucidating the mechanisms of atmospheric new particle formation in the highly polluted Po Valley, Italy J. Cai et al. 10.5194/acp-24-2423-2024
- Dust event identification and characterization with one-year online observations in Beijing F. Zheng et al. 10.1016/j.scitotenv.2024.177296
- Contributions of different organic compounds to brown carbon light absorption in a river-valley region, China Y. Li et al. 10.1016/j.atmosenv.2024.120731
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
- Precursors and Pathways Leading to Enhanced Secondary Organic Aerosol Formation during Severe Haze Episodes Y. Zheng et al. 10.1021/acs.est.1c04255
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
15 citations as recorded by crossref.
- Recent Advancement in Organic Aerosol Understanding: a Review of Their Sources, Formation, and Health Impacts S. Chaturvedi et al. 10.1007/s11270-023-06772-0
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al. 10.1038/s41561-024-01493-3
- Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region J. Wang et al. 10.1007/s11783-023-1714-0
- Nighttime NO emissions strongly suppress chlorine and nitrate radical formation during the winter in Delhi S. Haslett et al. 10.5194/acp-23-9023-2023
- Linking Precursors and Volatility of Ambient Oxygenated Organic Aerosols Using Thermal Desorption Measurement and Machine Learning X. Wang et al. 10.1021/acsestair.4c00076
- Development of a high-resolution emissions inventory of carbonaceous particulate matters and their growth during 2011–2018 over India P. Kumar et al. 10.1016/j.atmosenv.2023.119750
- Measurement report: Molecular-level investigation of atmospheric cluster ions at the tropical high-altitude research station Chacaltaya (5240 m a.s.l.) in the Bolivian Andes Q. Zha et al. 10.5194/acp-23-4559-2023
- Weakened Gas-to-Particle Partitioning of Oxygenated Organic Molecules in Liquified Aerosol Particles W. Ma et al. 10.1021/acs.estlett.2c00556
- Molecular composition of organic aerosols in urban and marine atmosphere: A comparison study using FIGAERO-I-CIMS, ESI-FT-ICR MS, and GC × GC-EI-ToF-MS X. Xin et al. 10.1080/02786826.2024.2377394
- Impacts of elevated anthropogenic emissions on physicochemical characteristics of black-carbon-containing particles over the Tibetan Plateau J. Wang et al. 10.5194/acp-24-11063-2024
- Quantifying New Sources of Ambient Organic Aerosol and Their Roles in Particle Growth Using Oxygenated Organic Molecule (OOM) Tracers Y. Zhao et al. 10.1021/acs.estlett.4c00536
- Elucidating the mechanisms of atmospheric new particle formation in the highly polluted Po Valley, Italy J. Cai et al. 10.5194/acp-24-2423-2024
- Dust event identification and characterization with one-year online observations in Beijing F. Zheng et al. 10.1016/j.scitotenv.2024.177296
- Contributions of different organic compounds to brown carbon light absorption in a river-valley region, China Y. Li et al. 10.1016/j.atmosenv.2024.120731
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
3 citations as recorded by crossref.
- Precursors and Pathways Leading to Enhanced Secondary Organic Aerosol Formation during Severe Haze Episodes Y. Zheng et al. 10.1021/acs.est.1c04255
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
Latest update: 20 Nov 2024
Short summary
This study investigates the connection between organic aerosol (OA) molecular composition and particle absorptive properties in autumn in Beijing. We find that the molecular properties of OA compounds in different episodes influence particle light absorption properties differently: the light absorption enhancement of black carbon and light absorption coefficient of brown carbon were mostly related to more oxygenated OA (low C number and four O atoms) and aromatics/nitro-aromatics, respectively.
This study investigates the connection between organic aerosol (OA) molecular composition and...
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