Articles | Volume 22, issue 17
https://doi.org/10.5194/acp-22-11359-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-11359-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 Sep 2022
Research article |
| 05 Sep 2022
| 05 Sep 2022
Contribution of wood burning to exposures of PAHs and oxy-PAHs in Eastern Sweden
Hwanmi Lim
Department of Materials and Environmental Chemistry, Stockholm
University, 106 91 Stockholm, Sweden
Sanna Silvergren
Environment and Health Administration, SLB, 104 20 Stockholm, Sweden
Silvia Spinicci
Waters Sverige AB, 171 65 Solna, Sweden
Farshid Mashayekhy Rad
Department of Chemistry, Uppsala University, Post Box 576, 751 23 Uppsala, Sweden
Ulrika Nilsson
Department of Materials and Environmental Chemistry, Stockholm
University, 106 91 Stockholm, Sweden
Roger Westerholm
Department of Materials and Environmental Chemistry, Stockholm
University, 106 91 Stockholm, Sweden
Christer Johansson
CORRESPONDING AUTHOR
Environment and Health Administration, SLB, 104 20 Stockholm, Sweden
Department of Environmental Science, Stockholm University, 106 91 Stockholm, Sweden
Related authors
No articles found.
Zhiguo Zhang, Christer Johansson, Magnuz Engardt, Massimo Stafoggia, and Xiaoliang Ma
Atmos. Chem. Phys., 24, 807–851, https://doi.org/10.5194/acp-24-807-2024, https://doi.org/10.5194/acp-24-807-2024, 2024
Short summary
Short summary
Up-to-date information on present and near-future air quality help people avoid exposure to high levels of air pollution. We apply different machine learning models to significantly improve traditional forecasts of PM10, NOx, and O3 in Stockholm, Sweden. It is shown that forecasts of all air pollutants are improved by the input of lagged measurements and taking calendar information into account. The final modelled errors are substantially smaller than uncertainties in the measurements.
Henrik Olstrup, Bertil Forsberg, Hans Orru, Mårten Spanne, Hung Nguyen, Peter Molnár, and Christer Johansson
Atmos. Chem. Phys., 18, 15705–15723, https://doi.org/10.5194/acp-18-15705-2018, https://doi.org/10.5194/acp-18-15705-2018, 2018
Short summary
Short summary
This article analyzes the health effects caused by changes in air pollution concentrations during the period of 1990–2015 in Stockholm, Gothenburg, and Malmö: the three largest cities in Sweden. The air pollutants that have been measured and analyzed are NOx, NO2, O3, and PM10. NOx and NO2 exhibit decreasing trends during this period, with beneficial effects on public health. An overall conclusion is that public health can largely benefit from reduced air pollution levels.
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic
Short-term source apportionment of fine particulate matter with time-dependent profiles using SoFi Pro: exploring the reliability of rolling positive matrix factorization (PMF) applied to bihourly molecular and elemental tracer data
Particulate-bound alkyl nitrate pollution and formation mechanisms in Beijing, China
Characterization of water-soluble brown carbon chromophores from wildfire plumes in the western USA using size-exclusion chromatography
Marine carbohydrates in Arctic aerosol particles and fog – diversity of oceanic sources and atmospheric transformations
Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 1: Observational data analysis
Measurement report: Brown carbon aerosol in polluted urban air of the North China Plain – day–night differences in the chromophores and optical properties
Source apportionment of soot particles and aqueous-phase processing of black carbon coatings in an urban environment
Seasonal variations in composition and sources of atmospheric ultrafine particles in urban Beijing based on near-continuous measurements
Summertime response of ozone and fine particulate matter to mixing layer meteorology over the North China Plain
Trace elements in PM2.5 aerosols in East Asian outflow in the spring of 2018: emission, transport, and source apportionment
Measurement Report: Investigation on the sources and formation processes of dicarboxylic acids and related species in urban aerosols before and during the COVID-19 lockdown in Jinan, East China
pH dependence of brown-carbon optical properties in cloud water
Oxidative potential in rural, suburban and city centre atmospheric environments in central Europe
Secondary aerosol formation during a special dust transport event: impacts from unusually enhanced ozone and dust backflows over the ocean
Intra-event evolution of elemental and ionic concentrations in wet deposition in an urban environment
Spatial and diurnal variations of aerosol organosulfates in summertime Shanghai, China: potential influence of photochemical processes and anthropogenic sulfate pollution
Chemical characterization of atmospheric aerosols at a high-altitude mountain site: a study of source apportionment
Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes
Chemical composition-dependent hygroscopic behavior of individual ambient aerosol particles collected at a coastal site
Gas–particle partitioning of semivolatile organic compounds when wildfire smoke comes to town
Enrichment of calcium in sea spray aerosol: insights from bulk measurements and individual particle analysis during the R/V Xuelong cruise in the summertime in Ross Sea, Antarctica
Elucidating the mechanisms of atmospheric new particle formation in the highly polluted Po Valley, Italy
Source apportionment study on particulate air pollution in two high-altitude Bolivian cities: La Paz and El Alto
Morphological features and water solubility of iron in aged fine aerosol particles over the Indian Ocean
What chemical species are responsible for new particle formation and growth in the Netherlands? A hybrid positive matrix factorization (PMF) analysis using aerosol composition (ACSM) and size (SMPS)
Physicochemical and Temporal Characteristics of Individual Atmospheric Aerosol Particles in Urban Seoul during KORUS-AQ Campaign: Insights from Single-Particle Analysis
Measurement report: Stoichiometry of dissolved iron and aluminum as an indicator of the factors controlling the fractional solubility of aerosol iron – results of the annual observations of size-fractionated aerosol particles in Japan
Variation in chemical composition and volatility of oxygenated organic aerosol in different rural, urban, and remote environments
In-depth study of the formation processes of single atmospheric particles in the south-eastern margin of the Tibetan Plateau
Climatology of aerosol properties at an atmospheric monitoring site on the northern California coast
Concurrent photochemical whitening and darkening of ambient brown carbon
High-time-resolution chemical composition and source apportionment of PM2.5 in northern Chinese cities: implications for policy
Measurement report: New insights into the mixing structures of black carbon on the eastern Tibetan Plateau – soot redistribution and fractal dimension enhancement by liquid–liquid phase separation
Seasonal variations in the production of singlet oxygen and organic triplet excited states in aqueous PM2.5 in Hong Kong SAR, South China
Fractional solubility of iron in mineral dust aerosols over coastal Namibia: a link with marine biogenic emissions?
Nighttime NO emissions strongly suppress chlorine and nitrate radical formation during the winter in Delhi
Influence of natural and anthropogenic aerosols on cloud base droplet size distributions in clouds over the South China Sea and West Pacific
The important contribution of secondary formation and biomass burning to oxidized organic nitrogen (OON) in a polluted urban area: insights from in situ measurements of a chemical ionization mass spectrometer (CIMS)
Measurement report: A 1-year study to estimate maritime contributions to PM10 in a coastal area in northern France
Morphological and optical properties of carbonaceous aerosol particles from ship emissions and biomass burning during a summer cruise measurement in the South China Sea
Tropical tropospheric aerosol sources and chemical composition observed at high-altitude in the Bolivian Andes
Evolution and chemical characteristics of organic aerosols during wintertime PM2.5 episodes in Shanghai, China: insights gained from online measurements of organic molecular markers
Arctic observations of hydroperoxymethyl thioformate (HPMTF) – seasonal behavior and relationship to other oxidation products of dimethyl sulfide at the Zeppelin Observatory, Svalbard
A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz
Contributions of primary emissions and secondary formation to nitrated aromatic compounds in themountain background region of Southeast China
Mist cannon trucks can exacerbate the formation of water-soluble organic aerosol and PM2.5 pollution in the road environment
Amino acids, carbohydrates, and lipids in the tropical oligotrophic Atlantic Ocean: sea-to-air transfer and atmospheric in situ formation
Measurement report: Atmospheric Ice Nuclei at Changbai Mountain (2623 m a.s.l.) in Northeastern Asia
Ambient carbonaceous aerosol levels in Cyprus and the role of pollution transport from the Middle East
Eric Schneider, Hendryk Czech, Olga Popovicheva, Marina Chichaeva, Vasily Kobelev, Nikolay Kasimov, Tatiana Minkina, Christopher Paul Rüger, and Ralf Zimmermann
Atmos. Chem. Phys., 24, 553–576, https://doi.org/10.5194/acp-24-553-2024, https://doi.org/10.5194/acp-24-553-2024, 2024
Short summary
Short summary
This study provides insights into the complex chemical composition of long-range-transported wildfire plumes from Yakutia, which underwent different levels of atmospheric processing. With complementary mass spectrometric techniques, we improve our understanding of the chemical processes and atmospheric fate of wildfire plumes. Unprecedented high levels of carbonaceous aerosols crossed the polar circle with implications for the Arctic ecosystem and consequently climate.
Qiongqiong Wang, Shuhui Zhu, Shan Wang, Cheng Huang, Yusen Duan, and Jian Zhen Yu
Atmos. Chem. Phys., 24, 475–486, https://doi.org/10.5194/acp-24-475-2024, https://doi.org/10.5194/acp-24-475-2024, 2024
Short summary
Short summary
We investigated short-term source apportionment of PM2.5 utilizing rolling positive matrix factorization (PMF) and online PM chemical speciation data, which included source-specific organic tracers collected over a period of 37 d during the winter of 2019–2020 in suburban Shanghai, China. The findings highlight that by imposing constraints on the primary source profiles, short-term PMF analysis successfully replicated both the individual primary sources and the total secondary sources.
Jiyuan Yang, Guoyang Lei, Jinfeng Zhu, Yutong Wu, Chang Liu, Kai Hu, Junsong Bao, Zitong Zhang, Weili Lin, and Jun Jin
Atmos. Chem. Phys., 24, 123–136, https://doi.org/10.5194/acp-24-123-2024, https://doi.org/10.5194/acp-24-123-2024, 2024
Short summary
Short summary
The atmospheric pollution and formation mechanisms of particulate-bound alkyl nitrate in Beijing were studied. C9–C16 long-chain n-alkyl nitrates negatively correlated with O3 but positively correlated with PM2.5 and NO2, so they may not be produced during gas-phase homogeneous reactions in the photochemical process but form through reactions between alkanes and nitrates on PM surfaces. Particulate-bound n-alkyl nitrates strongly affect both haze pollution and atmospheric visibility.
Lisa Azzarello, Rebecca A. Washenfelder, Michael A. Robinson, Alessandro Franchin, Caroline C. Womack, Christopher D. Holmes, Steven S. Brown, Ann Middlebrook, Tim Newberger, Colm Sweeney, and Cora J. Young
Atmos. Chem. Phys., 23, 15643–15654, https://doi.org/10.5194/acp-23-15643-2023, https://doi.org/10.5194/acp-23-15643-2023, 2023
Short summary
Short summary
We present a molecular size-resolved offline analysis of water-soluble brown carbon collected on an aircraft during FIREX-AQ. The smoke plumes were aged 0 to 5 h, where absorption was dominated by small molecular weight molecules, brown carbon absorption downwind did not consistently decrease, and the measurements differed from online absorption measurements of the same samples. We show how differences between online and offline absorption could be related to different measurement conditions.
Sebastian Zeppenfeld, Manuela van Pinxteren, Markus Hartmann, Moritz Zeising, Astrid Bracher, and Hartmut Herrmann
Atmos. Chem. Phys., 23, 15561–15587, https://doi.org/10.5194/acp-23-15561-2023, https://doi.org/10.5194/acp-23-15561-2023, 2023
Short summary
Short summary
Marine carbohydrates are produced in the surface of the ocean, enter the atmophere as part of sea spray aerosol particles, and potentially contribute to the formation of fog and clouds. Here, we present the results of a sea–air transfer study of marine carbohydrates conducted in the high Arctic. Besides a chemo-selective transfer, we observed a quick atmospheric aging of carbohydrates, possibly as a result of both biotic and abiotic processes.
Xing Wei, Yanjie Shen, Xiao-Ying Yu, Yang Gao, Huiwang Gao, Ming Chu, Yujiao Zhu, and Xiaohong Yao
Atmos. Chem. Phys., 23, 15325–15350, https://doi.org/10.5194/acp-23-15325-2023, https://doi.org/10.5194/acp-23-15325-2023, 2023
Short summary
Short summary
We investigate the contribution of grown new particles to Nccn at a rural mountain site in the North China Plain. The total particle number concentrations (Ncn) observed on 8 new particle formation (NPF) days were higher compared to non-NPF days. The Nccn at 0.2 % supersaturation (SS) and 0.4 % SS on the NPF days was significantly lower than on non-NPF days. Only one of eight NPF events had detectable net contributions to Nccn at 0.4 % SS and 1.0 % SS with increased κ values.
Yuquan Gong, Ru-Jin Huang, Lu Yang, Ting Wang, Wei Yuan, Wei Xu, Wenjuan Cao, Yang Wang, and Yongjie Li
Atmos. Chem. Phys., 23, 15197–15207, https://doi.org/10.5194/acp-23-15197-2023, https://doi.org/10.5194/acp-23-15197-2023, 2023
Short summary
Short summary
This study reveals the large day–night differences in brown carbon (BrC) chromophore composition, which was not known previously. The results provide insights into the effects of atmospheric processes and emissions on BrC composition.
Ryan N. Farley, Sonya Collier, Christopher D. Cappa, Leah R. Williams, Timothy B. Onasch, Lynn M. Russell, Hwajin Kim, and Qi Zhang
Atmos. Chem. Phys., 23, 15039–15056, https://doi.org/10.5194/acp-23-15039-2023, https://doi.org/10.5194/acp-23-15039-2023, 2023
Short summary
Short summary
Soot particles, also known as black carbon (BC), have important implications for global climate and regional air quality. After the particles are emitted, BC can be coated with other material, impacting the aerosol properties. We selectively measured the composition of particles containing BC to explore their sources and chemical transformations in the atmosphere. We focus on a persistent, multiday fog event in order to study the effects of chemical reactions occurring within liquid droplets.
Xiaoxiao Li, Yijing Chen, Yuyang Li, Runlong Cai, Yiran Li, Chenjuan Deng, Jin Wu, Chao Yan, Hairong Cheng, Yongchun Liu, Markku Kulmala, Jiming Hao, James N. Smith, and Jingkun Jiang
Atmos. Chem. Phys., 23, 14801–14812, https://doi.org/10.5194/acp-23-14801-2023, https://doi.org/10.5194/acp-23-14801-2023, 2023
Short summary
Short summary
Near-continuous measurements show the composition, sources, and seasonal variations of ultrafine particles (UFPs) in urban Beijing. Vehicle and cooking emissions and new particle formation are the main sources of UFPs, and aqueous/heterogeneous processes increase UFP mode diameters. UFPs are the highest in winter due to the highest primary particle emission rates and new particle formation rates, and CHO fractions are the highest in summer due to the strongest photooxidation.
Jiaqi Wang, Jian Gao, Fei Che, Xin Yang, Yuanqin Yang, Lei Liu, Yan Xiang, and Haisheng Li
Atmos. Chem. Phys., 23, 14715–14733, https://doi.org/10.5194/acp-23-14715-2023, https://doi.org/10.5194/acp-23-14715-2023, 2023
Short summary
Short summary
Regional-scale observations of surface O3, PM2.5 and its major chemical species, mixing layer height (MLH), and other meteorological parameters were made in the North China Plain during summer. Unlike the cold season, synchronized increases in MDA8 O3 and PM2.5 under medium MLH conditions have been witnessed. The increasing trend of PM2.5 was associated with enhanced secondary chemical formation. The correlation between MLH and secondary air pollutants should be treated with care in hot seasons.
Takuma Miyakawa, Akinori Ito, Chunmao Zhu, Atsushi Shimizu, Erika Matsumoto, Yusuke Mizuno, and Yugo Kanaya
Atmos. Chem. Phys., 23, 14609–14626, https://doi.org/10.5194/acp-23-14609-2023, https://doi.org/10.5194/acp-23-14609-2023, 2023
Short summary
Short summary
This study conducted semi-continuous measurements of PM2.5 aerosols and their elemental composition in western Japan, during spring 2018. It analyzed the emissions, transport, and wet removal of elements such as Pb, Cu, Fe, and Mn. It also assessed the accuracy of modeled concentrations and found overestimations of BC and underestimations of Cu and anthropogenic Fe in East Asia. Insights into emissions, removals, and source apportionment of trace metals in the East Asian outflow were provided.
Jingjing Meng, Yachen Wang, Yuanyuan Li, Tonglin Huang, Zhifei Wang, Yiqiu Wang, Min Chen, Zhanfang Hou, Houhua Zhou, Keding Lu, Kimitaka Kawamura, and Pingqing Fu
Atmos. Chem. Phys., 23, 14481–14503, https://doi.org/10.5194/acp-23-14481-2023, https://doi.org/10.5194/acp-23-14481-2023, 2023
Short summary
Short summary
This study investigated the effect of COVID-19 lockdown (LCD) measures on the formation and evolutionary process of diacids and related compounds from field observations. Results demonstrate that more aged organic aerosols are observed during the LCD due to the enhanced photochemical oxidation. Our study also found that the reactivity of 13C was higher than that of 12C in the gaseous photochemical oxidation, leading to higher δ13C values of C2 during the LCD than before the LCD.
Christopher J. Hennigan, Michael McKee, Vikram Pratap, Bryanna Boegner, Jasper Reno, Lucia Garcia, Madison McLaren, and Sara M. Lance
Atmos. Chem. Phys., 23, 14437–14449, https://doi.org/10.5194/acp-23-14437-2023, https://doi.org/10.5194/acp-23-14437-2023, 2023
Short summary
Short summary
This study characterized the optical properties of light-absorbing organic compounds, called brown carbon (BrC), in atmospheric cloud water samples. In all samples, light absorption by BrC increased linearly with increasing pH. There was variability in the sensitivity of the absorption–pH relationship, depending on the degree of influence from fire emissions. Overall, these results show that the climate forcing of BrC is quite strongly affected by its pH-dependent absorption.
Máté Vörösmarty, Gaëlle Uzu, Jean-Luc Jaffrezo, Pamela Dominutti, Zsófia Kertész, Enikő Papp, and Imre Salma
Atmos. Chem. Phys., 23, 14255–14269, https://doi.org/10.5194/acp-23-14255-2023, https://doi.org/10.5194/acp-23-14255-2023, 2023
Short summary
Short summary
Poor air quality caused by high concentrations of particulate matter is one of the most severe public health concerns for humans worldwide. One of the most important biological mechanisms inducing adverse health effects is the oxidant–antioxidant imbalance. We showed that the oxidative stress changed substantially and in a complex manner with location and season. Biomass burning exhibited the dominant influence, while motor vehicles played an important role in the non-heating period.
Da Lu, Hao Li, Mengke Tian, Guochen Wang, Xiaofei Qin, Na Zhao, Juntao Huo, Fan Yang, Yanfen Lin, Jia Chen, Qingyan Fu, Yusen Duan, Xinyi Dong, Congrui Deng, Sabur F. Abdullaev, and Kan Huang
Atmos. Chem. Phys., 23, 13853–13868, https://doi.org/10.5194/acp-23-13853-2023, https://doi.org/10.5194/acp-23-13853-2023, 2023
Short summary
Short summary
Environmental conditions during dust are usually not favorable for secondary aerosol formation. However in this study, an unusual dust event was captured in a Chinese mega-city and showed “anomalous” meteorology and a special dust backflow transport pathway. The underlying formation mechanisms of secondary aerosols are probed in the context of this special dust event. This study shows significant implications for the varying dust aerosol chemistry in the future changing climate.
Thomas Audoux, Benoit Laurent, Karine Desboeufs, Gael Noyalet, Franck Maisonneuve, Olivier Lauret, and Servanne Chevaillier
Atmos. Chem. Phys., 23, 13485–13503, https://doi.org/10.5194/acp-23-13485-2023, https://doi.org/10.5194/acp-23-13485-2023, 2023
Short summary
Short summary
In the Paris region, a campaign was conducted to study wet deposition of aerosol particles during rainfall events. Simultaneous measurements of aerosol and wet deposition allowed us to discuss their transfer from the atmosphere to rain. Chemical evolution within events revealed meteorology, atmospheric conditions and local vs. long range sources as key factors. This study highlights the variability of wet deposition and the need to consider event-specific factors to understand its mechanisms.
Ting Yang, Yu Xu, Qing Ye, Yi-Jia Ma, Yu-Chen Wang, Jian-Zhen Yu, Yu-Sen Duan, Chen-Xi Li, Hong-Wei Xiao, Zi-Yue Li, Yue Zhao, and Hua-Yun Xiao
Atmos. Chem. Phys., 23, 13433–13450, https://doi.org/10.5194/acp-23-13433-2023, https://doi.org/10.5194/acp-23-13433-2023, 2023
Short summary
Short summary
In this study, 130 OS species were quantified in ambient fine particulate matter (PM2.5) collected in urban and suburban Shanghai (East China) in the summer of 2021. The daytime OS formation was concretized based on the interactions among OSs, ultraviolet (UV), ozone (O3), and sulfate. Our finding provides field evidence for the influence of photochemical process and anthropogenic sulfate on OS formation and has important implications for the mitigation of organic particulate pollution.
Elena Barbaro, Matteo Feltracco, Fabrizio De Blasi, Clara Turetta, Marta Radaelli, Warren Cairns, Giulio Cozzi, Giovanna Mazzi, Marco Casula, Jacopo Gabrieli, Carlo Barbante, and Andrea Gambaro
EGUsphere, https://doi.org/10.5194/egusphere-2023-2346, https://doi.org/10.5194/egusphere-2023-2346, 2023
Short summary
Short summary
The study analyzed a year of atmospheric aerosol composition at Col Margherita in the Italian Alps. Over 100 chemical markers were identified, including major ions, organic compounds, and trace elements. It revealed sources of aerosol, highlighted impacts of Saharan Dust events, and showed anthropogenic pollution's influence despite the site's remoteness. Enrichment factors emphasized non-natural sources of trace elements. Source apportionment identified four key factors affecting the area.
Miao Zhong, Jianzhong Xu, Huiqin Wang, Li Gao, Haixia Zhu, Lixiang Zhai, Xinghua Zhang, and Wenhui Zhao
Atmos. Chem. Phys., 23, 12609–12630, https://doi.org/10.5194/acp-23-12609-2023, https://doi.org/10.5194/acp-23-12609-2023, 2023
Short summary
Short summary
This study focus on coal-combustion-dominated aerosol in urban areas in northwestern China and combines the results of optical measurement and chemical analysis to deduce the evolution of these characteristics in the atmosphere, which has previously been unknown. The results provide insights into the effects of atmospheric processes and emissions on brown carbon properties.
Li Wu, Hyo-Jin Eom, Hanjin Yoo, Dhrubajyoti Gupta, Hye-Rin Cho, Pingqing Fu, and Chul-Un Ro
Atmos. Chem. Phys., 23, 12571–12588, https://doi.org/10.5194/acp-23-12571-2023, https://doi.org/10.5194/acp-23-12571-2023, 2023
Short summary
Short summary
Hygroscopicity of ambient marine aerosols is of critical relevance to investigate their atmospheric impacts, which, however, remain uncertain due to their complex compositions and mixing states. Therefore, a study on the hygroscopic behavior of ambient marine aerosols for understanding the phase states when interacting with water vapor at different RH levels and their subsequent impacts on the heterogeneous chemical reactions, atmospheric environment, and human health is of vital importance.
Yutong Liang, Rebecca A. Wernis, Kasper Kristensen, Nathan M. Kreisberg, Philip L. Croteau, Scott C. Herndon, Arthur W. H. Chan, Nga L. Ng, and Allen H. Goldstein
Atmos. Chem. Phys., 23, 12441–12454, https://doi.org/10.5194/acp-23-12441-2023, https://doi.org/10.5194/acp-23-12441-2023, 2023
Short summary
Short summary
We measured the gas–particle partitioning behaviors of biomass burning markers and examined the effect of wildfire organic aerosol on the partitioning of semivolatile organic compounds. Most compounds measured are less volatile than model predictions. Wildfire aerosol enhanced the condensation of polar compounds and caused some nonpolar (e.g., polycyclic aromatic hydrocarbons) compounds to partition into the gas phase, thus affecting their lifetimes in the atmosphere and the mode of exposure.
Bojiang Su, Xinhui Bi, Zhou Zhang, Yue Liang, Congbo Song, Tao Wang, Yaohao Hu, Lei Li, Zhen Zhou, Jinpei Yan, Xinming Wang, and Guohua Zhang
Atmos. Chem. Phys., 23, 10697–10711, https://doi.org/10.5194/acp-23-10697-2023, https://doi.org/10.5194/acp-23-10697-2023, 2023
Short summary
Short summary
During the R/V Xuelong cruise observation over the Ross Sea, Antarctica, the mass concentrations of water-soluble Ca2+ and the mass spectra of individual calcareous particles were measured. Our results indicated that lower temperature, lower wind speed, and the presence of sea ice may facilitate Ca2+ enrichment in sea spray aerosols and highlighted the potential contribution of organically complexed calcium to calcium enrichment, which is inaccurate based solely on water-soluble Ca2+ estimation.
Jing Cai, Juha Sulo, Yifang Gu, Sebastian Holm, Runlong Cai, Steven Thomas, Almuth Neuberger, Fredrik Mattsson, Marco Paglione, Stefano Decesari, Matteo Rinaldi, Rujing Yin, Diego Aliaga, Wei Huang, Yuanyuan Li, Yvette Gramlich, Giancarlo Ciarelli, Lauriane Quéléver, Nina Sarnela, Katrianne Lehtipalo, Nora Zannoni, Cheng Wu, Wei Nie, Claudia Mohr, Markku Kulmala, Qiaozhi Zha, Dominik Stolzenburg, and Federico Bianchi
EGUsphere, https://doi.org/10.5194/egusphere-2023-1803, https://doi.org/10.5194/egusphere-2023-1803, 2023
Short summary
Short summary
By combining field measurements, simulations, and recent chamber experiments, we investigate new particle formation (NPF) and its growth in Po Valley, where both haze and frequent NPF occurred. Our results showed sulfuric acid, ammonia, and amines are the dominant NPF precursors there. A high formation rate of NPF and a lower condensation sink lead to a greater survival probability for newly formed particles, highlighting the importance of gas-to-particle conversion to aerosol concentrations.
Valeria Mardoñez, Marco Pandolfi, Lucille Joanna S. Borlaza, Jean-Luc Jaffrezo, Andrés Alastuey, Jean-Luc Besombes, Isabel Moreno R., Noemi Perez, Griša Močnik, Patrick Ginot, Radovan Krejci, Vladislav Chrastny, Alfred Wiedensohler, Paolo Laj, Marcos Andrade, and Gaëlle Uzu
Atmos. Chem. Phys., 23, 10325–10347, https://doi.org/10.5194/acp-23-10325-2023, https://doi.org/10.5194/acp-23-10325-2023, 2023
Short summary
Short summary
La Paz and El Alto are two fast-growing, high-altitude Bolivian cities forming the second-largest metropolitan area in the country. The sources of particulate matter (PM) in this conurbation were not previously investigated. This study identified 11 main sources of PM, of which dust and vehicular emissions stand out as the main ones. The influence of regional biomass combustion and local waste combustion was also observed, with the latter being a major source of hazardous compounds.
Sayako Ueda, Yoko Iwamoto, Fumikazu Taketani, Mingxu Liu, and Hitoshi Matsui
Atmos. Chem. Phys., 23, 10117–10135, https://doi.org/10.5194/acp-23-10117-2023, https://doi.org/10.5194/acp-23-10117-2023, 2023
Short summary
Short summary
We examine iron in atmospheric fine aerosol particles collected over the Indian Ocean during shipborne observations in November 2018. Transmission electron microscopy analysis with water dialysis shows that various types of iron (fly ash, iron oxide, and mineral dust) co-exist with ammonium sulfate and that their solubility differs depending on the iron type. Using PM2.5 bulk samples and global model simulations, we elucidate their origins, aging, and implications for present iron simulations.
Farhan R. Nursanto, Roy Meinen, Rupert Holzinger, Maarten C. Krol, Xinya Liu, Ulrike Dusek, Bas Henzing, and Juliane L. Fry
Atmos. Chem. Phys., 23, 10015–10034, https://doi.org/10.5194/acp-23-10015-2023, https://doi.org/10.5194/acp-23-10015-2023, 2023
Short summary
Short summary
Particulate matter (PM) is a harmful air pollutant that depends on the complex mixture of natural and anthropogenic emissions into the atmosphere. Thus, in different regions and seasons, the way that PM is formed and grows can differ. In this study, we use a combined statistical analysis of the chemical composition and particle size distribution to determine what drives particle formation and growth across seasons, using varying wind directions to elucidate the role of different sources.
Hanjin Yoo, Li Wu, Hong Geng, and Chul-Un Ro
EGUsphere, https://doi.org/10.5194/egusphere-2023-1787, https://doi.org/10.5194/egusphere-2023-1787, 2023
Short summary
Short summary
We conducted an investigation of atmospheric aerosols collected in Seoul, Korea, during the KORUS-AQ campaign, on a single-particle basis. We were able to identify their sources, atmospheric fate, and the impacts of local emissions and long-range transport on aerosol composition. Additionally, we traced potential sources of non-exhaust heavy metal particles. This comprehensive analysis provides valuable insights into the complex dynamics of urban aerosols.
Kohei Sakata, Aya Sakaguchi, Yoshiaki Yamakawa, Chihiro Miyamoto, Minako Kurisu, and Yoshio Takahashi
Atmos. Chem. Phys., 23, 9815–9836, https://doi.org/10.5194/acp-23-9815-2023, https://doi.org/10.5194/acp-23-9815-2023, 2023
Short summary
Short summary
Anthropogenic iron is the dominant source of dissolved Fe in aerosol particles, but its contribution to dissolved Fe in aerosol particles has not been quantitatively evaluated. We established the molar concentration ratio of dissolved Fe to dissolved Al as a new indicator to evaluate the contribution of anthropogenic iron. As a result, about 10 % of dissolved Fe in aerosol particles was derived from anthropogenic iron when aerosol particles were transported from East Asia to the Pacific Ocean.
Wei Huang, Cheng Wu, Linyu Gao, Yvette Gramlich, Sophie L. Haslett, Joel Thornton, Felipe D. Lopez-Hilfiker, Ben H. Lee, Junwei Song, Harald Saathoff, Xiaoli Shen, Ramakrishna Ramisetty, Sachchida N. Tripathi, Dilip Ganguly, Feng Jiang, Magdalena Vallon, Siegfried Schobesberger, Taina Yli-Juuti, and Claudia Mohr
EGUsphere, https://doi.org/10.5194/egusphere-2023-1821, https://doi.org/10.5194/egusphere-2023-1821, 2023
Short summary
Short summary
We present distinct molecular composition and volatility of oxygenated organic aerosol particles in different rural, urban, and remote environments across the globe. We did a comprehensive investigation of the relationship between chemical composition and volatility of oxygenated organic aerosol particles across different systems and environments. This study provides implications for volatility descriptions of oxygenated organic aerosol particles in different model frameworks.
Li Li, Qiyuan Wang, Jie Tian, Huikun Liu, Yong Zhang, Steven Sai Hang Ho, Weikang Ran, and Junji Cao
Atmos. Chem. Phys., 23, 9597–9612, https://doi.org/10.5194/acp-23-9597-2023, https://doi.org/10.5194/acp-23-9597-2023, 2023
Short summary
Short summary
The Tibetan Plateau has a unique geographical location, but there is a lack of detailed research on the real-time characteristics of full aerosol composition. This study elaborates the changes in chemical characteristics between transport and local fine particles during the pre-monsoon, reveals the size distribution and the mixing states of different individual particles, and highlights the contributions of photooxidation and aqueous reaction to the formation of the secondary species.
Erin K. Boedicker, Elisabeth Andrews, Patrick J. Sheridan, and Patricia K. Quinn
Atmos. Chem. Phys., 23, 9525–9547, https://doi.org/10.5194/acp-23-9525-2023, https://doi.org/10.5194/acp-23-9525-2023, 2023
Short summary
Short summary
We present 15 years of measurements from a marine site on the northern California coast and characterize the seasonal trends of aerosol ion composition and optical properties at the site. We investigate the relationship between the chemical and optical properties and show that they both support similar seasonal variations in aerosol sources at the site. Additionally, we show through comparisons to other marine aerosol observations that the site is representative of a clean marine environment.
Qian Li, Dantong Liu, Xiaotong Jiang, Ping Tian, Yangzhou Wu, Siyuan Li, Kang Hu, Quan Liu, Mengyu Huang, Ruijie Li, Kai Bi, Shaofei Kong, Deping Ding, and Chenjie Yu
Atmos. Chem. Phys., 23, 9439–9453, https://doi.org/10.5194/acp-23-9439-2023, https://doi.org/10.5194/acp-23-9439-2023, 2023
Short summary
Short summary
By attributing the shortwave absorption from black carbon, primary organic aerosol and secondary organic aerosol in a suburban environment, we firstly observed that the photochemically produced nitrogen-containing secondary organic aerosol may contribute to the enhancement of brown carbon absorption, partly compensating for some bleaching effect on the absorption of primary organic aerosol, hereby exerting radiative impacts.
Yong Zhang, Jie Tian, Qiyuan Wang, Lu Qi, Manousos Ioannis Manousakas, Yuemei Han, Weikang Ran, Yele Sun, Huikun Liu, Renjian Zhang, Yunfei Wu, Tianqu Cui, Kaspar Rudolf Daellenbach, Jay Gates Slowik, André S. H. Prévôt, and Junji Cao
Atmos. Chem. Phys., 23, 9455–9471, https://doi.org/10.5194/acp-23-9455-2023, https://doi.org/10.5194/acp-23-9455-2023, 2023
Short summary
Short summary
PM2.5 pollution still frequently occurs in northern China during winter, and it is necessary to figure out the causes of air pollution based on intensive real-time measurement. The findings elaborate the chemical characteristics and source contributions of PM2.5 in three pilot cities, reveal potential formation mechanisms of secondary aerosols, and highlight the importance of controlling biomass burning and inhibiting generation of secondary aerosol for air quality improvement.
Qi Yuan, Yuanyuan Wang, Yixin Chen, Siyao Yue, Jian Zhang, Yinxiao Zhang, Liang Xu, Wei Hu, Dantong Liu, Pingqing Fu, Huiwang Gao, and Weijun Li
Atmos. Chem. Phys., 23, 9385–9399, https://doi.org/10.5194/acp-23-9385-2023, https://doi.org/10.5194/acp-23-9385-2023, 2023
Short summary
Short summary
This study for the first time found large amounts of liquid–liquid phase separation particles with soot redistributing in organic coatings instead of sulfate cores in the eastern Tibetan Plateau atmosphere. The particle size and the ratio of the organic matter coating thickness to soot size are two of the major possible factors that likely affect the soot redistribution process. The soot redistribution process promoted the morphological compaction of soot particles.
Yuting Lyu, Yin Hau Lam, Yitao Li, Nadine Borduas-Dedekind, and Theodora Nah
Atmos. Chem. Phys., 23, 9245–9263, https://doi.org/10.5194/acp-23-9245-2023, https://doi.org/10.5194/acp-23-9245-2023, 2023
Short summary
Short summary
We measured singlet oxygen (1O2*) and triplet excited states of organic matter (3C*) in illuminated aqueous extracts of PM2.5 collected in different seasons at different sites in Hong Kong SAR, South China. In contrast to the locations, seasonality had significant effects on 3C* and 1O2* production due to seasonal variations in long-range air mass transport. The steady-state concentrations of 3C* and 1O2* correlated with the concentration and absorbance of water-soluble organic carbon.
Karine Desboeufs, Paola Formenti, Raquel Torres-Sánchez, Kerstin Schepanski, Jean-Pierre Chaboureau, Hendrik Andersen, Jan Cermak, Stefanie Feuerstein, Benoit Laurent, Danitza Klopper, Andreas Namwoonde, Mathieu Cazaunau, Servanne Chevaillier, Anaïs Feron, Cecile Mirande-Bret, Sylvain Triquet, and Stuart J. Piketh
EGUsphere, https://doi.org/10.5194/egusphere-2023-1736, https://doi.org/10.5194/egusphere-2023-1736, 2023
Short summary
Short summary
This study investigates the fractional solubility of iron (Fe) in dust particles along the coast of Namibia, a critical region for the atmospheric Fe supply of the Southern Atlantic Ocean. Our results suggest a possible two-way interplay whereby marine biogenic emissions from the coastal marine ecosystems to the atmosphere would increase the solubility of Fe-bearing dust by photo-reduction processes. The subsequent deposition of soluble Fe could act to further enhance marine biogenic emissions.
Sophie L. Haslett, David M. Bell, Varun Kumar, Jay G. Slowik, Dongyu S. Wang, Suneeti Mishra, Neeraj Rastogi, Atinderpal Singh, Dilip Ganguly, Joel Thornton, Feixue Zheng, Yuanyuan Li, Wei Nie, Yongchun Liu, Wei Ma, Chao Yan, Markku Kulmala, Kaspar R. Daellenbach, David Hadden, Urs Baltensperger, Andre S. H. Prevot, Sachchida N. Tripathi, and Claudia Mohr
Atmos. Chem. Phys., 23, 9023–9036, https://doi.org/10.5194/acp-23-9023-2023, https://doi.org/10.5194/acp-23-9023-2023, 2023
Short summary
Short summary
In Delhi, some aspects of daytime and nighttime atmospheric chemistry are inverted, and parodoxically, vehicle emissions may be limiting other forms of particle production. This is because the nighttime emissions of nitrogen oxide (NO) by traffic and biomass burning prevent some chemical processes that would otherwise create even more particles and worsen the urban haze.
Rose Marie Miller, Robert M. Rauber, Larry Di Girolamo, Matthew Rilloraza, Dongwei Fu, Greg M. McFarquhar, Stephen W. Nesbitt, Luke D. Ziemba, Sarah Woods, and Kenneth Lee Thornhill
Atmos. Chem. Phys., 23, 8959–8977, https://doi.org/10.5194/acp-23-8959-2023, https://doi.org/10.5194/acp-23-8959-2023, 2023
Short summary
Short summary
The influence of human-produced aerosols on clouds remains one of the uncertainties in radiative forcing of Earth’s climate. Measurements of aerosol chemistry from sources around the Philippines illustrate the linkage between aerosol chemical composition and cloud droplet characteristics. Differences in aerosol chemical composition in the marine layer from biomass burning, industrial, ship-produced, and marine aerosols are shown to impact cloud microphysical structure just above cloud base.
Yiyu Cai, Chenshuo Ye, Wei Chen, Weiwei Hu, Wei Song, Yuwen Peng, Shan Huang, Jipeng Qi, Sihang Wang, Chaomin Wang, Caihong Wu, Zelong Wang, Baolin Wang, Xiaofeng Huang, Lingyan He, Sasho Gligorovski, Bin Yuan, Min Shao, and Xinming Wang
Atmos. Chem. Phys., 23, 8855–8877, https://doi.org/10.5194/acp-23-8855-2023, https://doi.org/10.5194/acp-23-8855-2023, 2023
Short summary
Short summary
We studied the variability and molecular composition of ambient oxidized organic nitrogen (OON) in both gas and particle phases using a state-of-the-art online mass spectrometer in urban air. Biomass burning and secondary formation were found to be the two major sources of OON. Daytime nitrate radical chemistry for OON formation was more important than previously thought. Our results improved the understanding of the sources and molecular composition of OON in the polluted urban atmosphere.
Frédéric Ledoux, Cloé Roche, Gilles Delmaire, Gilles Roussel, Olivier Favez, Marc Fadel, and Dominique Courcot
Atmos. Chem. Phys., 23, 8607–8622, https://doi.org/10.5194/acp-23-8607-2023, https://doi.org/10.5194/acp-23-8607-2023, 2023
Short summary
Short summary
We quantify the emissions from the marine sector in northern France, whether from natural or human-made sources. Therefore, a 1-year PM10 sampling campaign was conducted at a French coastal site. Results showed that sea salts contributed 37 %, while secondary nitrate and sulfate contributed 42 %, biomass burning 8 %, and heavy-fuel-oil combustion from shipping emissions 5 %. Sources contributing more than 80 % of PM10 are of regional and/or long-range origin.
Cuizhi Sun, Yongyun Zhang, Baoling Liang, Min Gao, Xi Sun, Fei Li, Xue Ni, Qibin Sun, Hengjia Ou, Dexian Chen, Shengzhen Zhou, and Jun Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2023-1589, https://doi.org/10.5194/egusphere-2023-1589, 2023
Short summary
Short summary
Black and brown carbon particles contribute significantly to light absorption and hence heat the atmosphere. However, their contribution is currently not well known, especially in the South China Sea. We conduct a ship-based cruise campaign in this region to measure the properties of these particles using advanced instruments. The results show that the properties differed depending on their origins, and the size, shape, and fractal dimensions changed little after they spent some time in the air.
C. Isabel Moreno, Radovan Krejci, Jean-Luc Jaffrezo, Gaëlle Uzu, Andrés Alastuey, Marcos F. Andrade, Valeria Mardóñez, Alkuin Maximilian Koenig, Diego Aliaga, Claudia Mohr, Laura Ticona, Fernando Velarde, Luis Blacutt, Ricardo Forno, David N. Whiteman, Alfred Wiedensohler, Patrick Ginot, and Paolo Laj
EGUsphere, https://doi.org/10.5194/egusphere-2023-1298, https://doi.org/10.5194/egusphere-2023-1298, 2023
Short summary
Short summary
Aerosol chemical composition (ions, sugars, carbonaceous matter) from 2011 to 2020 was studied at Mt. Chacaltaya (5380 masl, Bolivian Andes), in a region lacking data. Minimum concentrations occur in the rainy season and maxima in the dry-transition seasons. The origins of the aerosol are located in a radius of hundreds of kilometers: nearby urban and rural areas; natural biogenic emissions; vegetation burning from Amazonia and Chaco; Pacific Ocean emissions; soil dust; and Peruvian volcanism.
Shuhui Zhu, Min Zhou, Liping Qiao, Dan Dan Huang, Qiongqiong Wang, Shan Wang, Yaqin Gao, Shengao Jing, Qian Wang, Hongli Wang, Changhong Chen, Cheng Huang, and Jian Zhen Yu
Atmos. Chem. Phys., 23, 7551–7568, https://doi.org/10.5194/acp-23-7551-2023, https://doi.org/10.5194/acp-23-7551-2023, 2023
Short summary
Short summary
Organic aerosol (OA) is increasingly important in urban PM2.5 pollution as inorganic ions are becoming lower. We investigated the chemical characteristics of OA during nine episodes in Shanghai. The availability of bi-hourly measured molecular markers revealed that the control of local urban sources such as vehicular and cooking emissions lessened the severity of local episodes. Regional control of precursors and biomass burning would reduce PM2.5 episodes influenced by regional transport.
Karolina Siegel, Yvette Gramlich, Sophie L. Haslett, Gabriel Freitas, Radovan Krejci, Paul Zieger, and Claudia Mohr
Atmos. Chem. Phys., 23, 7569–7587, https://doi.org/10.5194/acp-23-7569-2023, https://doi.org/10.5194/acp-23-7569-2023, 2023
Short summary
Short summary
Hydroperoxymethyl thioformate (HPMTF) is a recently discovered oxidation product of dimethyl sulfide (DMS). We present a full year of concurrent gas- and particle-phase observations of HPMTF and other DMS oxidation products from the Arctic. We did not observe significant amounts of HPMTF in the particle phase but a good agreement between gas-phase HMPTF and methanesulfonic acid in the summer. Our study provides information about the relationship between HPMTF and other DMS oxidation products.
Samira Atabakhsh, Laurent Poulain, Gang Chen, Francesco Canonaco, André S. H. Prévôt, Mira Pöhlker, Alfred Wiedensohler, and Hartmut Herrmann
Atmos. Chem. Phys., 23, 6963–6988, https://doi.org/10.5194/acp-23-6963-2023, https://doi.org/10.5194/acp-23-6963-2023, 2023
Short summary
Short summary
The study focuses on the aerosol chemical variations found in the rural-background station of Melpitz based on ACSM and MAAP measurements. Source apportionment on both organic aerosol (OA) and black carbon (eBC) was performed, and source seasonality was also linked to air mass trajectories. Overall, three anthropogenic sources were identified in OA and eBC plus two additional aged OA. Our results demonstrate the influence of transported coal-combustion-related OA even during summer time.
Yanqin Ren, Gehui Wang, Jie Wei, Jun Tao, Zhisheng Zhang, and Hong Li
Atmos. Chem. Phys., 23, 6835–6848, https://doi.org/10.5194/acp-23-6835-2023, https://doi.org/10.5194/acp-23-6835-2023, 2023
Short summary
Short summary
Nine quantified nitrated aromatic compounds (NACs) in PM2.5 were examined at the peak of Mt. Wuyi. They manifested a significant rise in overall abundance in the winter and autumn. The transport of contaminants had a significant impact on NACs. Under low-NOx conditions, the formation of NACs was comparatively sensitive to NO2, suggesting that NACs would become significant in the aerosol characteristics when nitrate concentrations decreased as a result of emission reduction measures.
Yu Xu, Xin-Ni Dong, Chen He, Dai-She Wu, Hong-Wei Xiao, and Hua-Yun Xiao
Atmos. Chem. Phys., 23, 6775–6788, https://doi.org/10.5194/acp-23-6775-2023, https://doi.org/10.5194/acp-23-6775-2023, 2023
Short summary
Short summary
The air pollution associated with fine particles and secondary organic aerosol is not weakened by the application of mist cannon trucks but rather is aggravated. Our results provide not only new insights into the formation processes of aerosol water-soluble organic compounds associated with the water mist sprayed by mist cannon trucks in the road atmospheric environment but also crucial information for the decision makers to regulate the operation of mist cannon trucks in many cities in China.
Manuela van Pinxteren, Sebastian Zeppenfeld, Khanneh Wadinga Fomba, Nadja Triesch, Sanja Frka, and Hartmut Herrmann
Atmos. Chem. Phys., 23, 6571–6590, https://doi.org/10.5194/acp-23-6571-2023, https://doi.org/10.5194/acp-23-6571-2023, 2023
Short summary
Short summary
Important marine organic carbon compounds were identified in the Atlantic Ocean and marine aerosol particles. These compounds were strongly enriched in the atmosphere. Their enrichment was, however, not solely explained via sea-to-air transfer but also via atmospheric in situ formation. The identified compounds constituted about 50 % of the organic carbon on the aerosol particles, and a pronounced coupling between ocean and atmosphere for this oligotrophic region could be concluded.
Yue Sun, Yujiao Zhu, Yanbin Qi, Lanxiadi Chen, Jiangshan Mu, Ye Shan, Yu Yang, Yanqiu Nie, Ping Liu, Can Cui, Ji Zhang, Mingxuan Liu, Lingli Zhang, Yufei Wang, Xinfeng Wang, Mingjin Tang, Wenxing Wang, and Likun Xue
EGUsphere, https://doi.org/10.5194/egusphere-2023-925, https://doi.org/10.5194/egusphere-2023-925, 2023
Short summary
Short summary
Field observations were conducted at the top of Changbai Mountain in Northeast Asia. Our findings indicate that the ice-nucleating particles (INPs) were mainly dominated by biological sources, accounting for over 90 % above the freezing temperature of −13.0 °C. Biological INPs were found to attached to soil dust surfaces, and their concentrations influenced by a combination of factors, such as the planetary boundary layer height, valley breezes, and long-distance transport of air mass.
Aliki Christodoulou, Iasonas Stavroulas, Mihalis Vrekoussis, Maximillien Desservettaz, Michael Pikridas, Elie Bimenyimana, Jonilda Kushta, Matic Ivančič, Martin Rigler, Philippe Goloub, Konstantina Oikonomou, Roland Sarda-Estève, Chrysanthos Savvides, Charbel Afif, Nikos Mihalopoulos, Stéphane Sauvage, and Jean Sciare
Atmos. Chem. Phys., 23, 6431–6456, https://doi.org/10.5194/acp-23-6431-2023, https://doi.org/10.5194/acp-23-6431-2023, 2023
Short summary
Short summary
Our study presents, for the first time, a detailed source identification of aerosols at an urban background site in Cyprus (eastern Mediterranean), a region strongly impacted by climate change and air pollution. Here, we identify an unexpected high contribution of long-range transported pollution from fossil fuel sources in the Middle East, highlighting an urgent need to further characterize these fast-growing emissions and their impacts on regional atmospheric composition, climate, and health.
Cited articles
Ahmed, T. M., Bergvall, C., Åberg, M., and Westerholm, R.: Determination
of oxygenated and native polycyclic aromatic hydrocarbons in urban dust and
diesel particulate matter standard reference materials using pressurized
liquid extraction and LC–GC/MS, Anal. Bioanal. Chem., 407, 427–438,
https://doi.org/10.1007/s00216-014-8304-8, 2015.
Alves, C. A., Vicente, A. M., Custódio, D., Cerqueira, M., Nunes, T.,
Pio, C., Lucarelli, F., Calzolai, G., Nava, S., Diapouli, E., Eleftheriadis,
K., Querol, X., and Bandowe, B. A. M.: Polycyclic aromatic hydrocarbons and
their derivatives (nitro-PAHs, oxygenated PAHs, and azaarenes) in PM2.5
from Southern European cities, Sci. Total Environ., 595, 494–504,
https://doi.org/10.1016/j.scitotenv.2017.03.256, 2017.
Andersson, S., Arvelius, J., Verbova, M., Omstedt, G., and Torstensson, M.:
Identifiering av potentiella riskområden för höga halter av
benso(a)pyren, Nationell kartering av emissioner och halter av B(a)P
från vedeldning i småhusområden, SMHI report 159, http://urn.kb.se/resolve?urn=urn%3Anbn%3Ase%3Asmhi%3Adiva-2815 or http://smhi.diva-portal.org/smash/get/diva2:948111/FULLTEXT01.pdf, (last access: 15 August 2022), 2015.
Andersson, S., Arvelius, J., Jones, J., Kindell, S., and Leung, W.:
Beräkningar av emissioner och halter av benso(a)pyren och partiklar
från småskalig vedeldning. Luftkvalitetsmodellering för
Skellefteå, Strömsunds och Alingsås kommuner, SMHI report 29, http://urn.kb.se/resolve?urn=urn%3Anbn%3Ase%3Asmhi%3Adiva-5169, or http://smhi.diva-portal.org/smash/get/diva2:1290201/FULLTEXT02.pdf (last access: 15 August 2022), 2018.
Apertum: Airviro user's reference, Working with the Dispersion Module, How
to simulate the dispersion of pollutants, Airviro version 4.0, Linköping, Sweden,
https://www.airviro.com/airviro/extras/pdffiles/UserRef_Volume2_Dispersion_v4.00.pdf, last access: 1 February 2021.
Apertum: Airviro, airviro [code], https://www.airviro.com/airviro, last access: 26 July 2022.
Bari, M. A., Baumbach, G., Kuch, B., and Scheffknecht, G.: Air pollution in
residential areas from wood-fired heating, Aerosol Air Qual. Res., 11,
749–757, https://doi.org/10.4209/aaqr.2010.09.0079, 2011.
Beekmann, M., Prévôt, A. S. H., Drewnick, F., Sciare, J., Pandis, S. N., Denier van der Gon, H. A. C., Crippa, M., Freutel, F., Poulain, L., Ghersi, V., Rodriguez, E., Beirle, S., Zotter, P., von der Weiden-Reinmüller, S.-L., Bressi, M., Fountoukis, C., Petetin, H., Szidat, S., Schneider, J., Rosso, A., El Haddad, I., Megaritis, A., Zhang, Q. J., Michoud, V., Slowik, J. G., Moukhtar, S., Kolmonen, P., Stohl, A., Eckhardt, S., Borbon, A., Gros, V., Marchand, N., Jaffrezo, J. L., Schwarzenboeck, A., Colomb, A., Wiedensohler, A., Borrmann, S., Lawrence, M., Baklanov, A., and Baltensperger, U.: In situ, satellite measurement and model evidence on the dominant regional contribution to fine particulate matter levels in the Paris megacity, Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, 2015.
Belis, C. A., Cancelinha, J., Duane, M., Forcina, V., Pedroni, V.,
Passarella, R., Tanet, G., Douglas, K., Piazzalunga, A., Bolzacchini, E.,
Sangiorgi, G., Perrone, M.-G., Ferrero, L., Fermo, P., and Larsen, B. R.:
Sources for PM air pollution in the Po Plain, Italy: I. Critical comparison
of methods for estimating biomass burning contributions to benzo(a)pyrene,
Atmos. Environ., 45, 7266–7275, https://doi.org/10.1016/j.atmosenv.2011.08.061,
2011.
Bi, X., Sheng, G., Peng, P., Chen, Y., Zhang, Z., and Fu, J.: Distribution
of particulate- and vapor-phase n-alkanes and polycyclic aromatic
hydrocarbons in urban atmosphere of Guangzhou, China, Atmos. Environ., 37, 289–298, https://doi.org/10.1016/S1352-2310(02)00832-4, 2003.
Boman, B. C., Forsberg, A. B., and Järvholm, B. G.: Adverse health effects
from ambient air pollution in relation to residential wood combustion in
modern society, Scand. J. Work Environ. Health, 29, 251–260,
https://doi.org/10.5271/sjweh.729, 2003.
Boström, C. E., Gerde, P., Hanberg, A., Jernström, B., Johansson, C.,
Kyrklund, T., Rannug, A., Törnqvist, M., Victorin, K., and Westerholm,
R.: Cancer risk assessment, indicators, and guidelines for polycyclic
aromatic hydrocarbons in the ambient air, Environ. Health Persp., 110, 451–488, https://doi.org/10.1289/ehp.110-1241197, 2002.
Caseiro, A., Bauer, H., Schmidl, C., Pio, C. A., and Puxbaum, H.: Wood
burning impact on PM10 in three Austrian regions, Atmos. Environ., 43, 2186–2195, https://doi.org/10.1016/j.atmosenv.2009.01.012, 2009.
Cordell, R. L., Mazet, M., Dechoux, C., Hama, S. M. L., Staelens, J., Hofman,
J., Stroobants, C., Roekens, E., Kos, G. P. A., Weijers, E. P., Frumau, K. F. A.,
Panteliadis, P., Delaunay, T., Wyche, K. P., and Monks, P. S.: Evaluation of
biomass burning across North West Europe and its impact on air quality,
Atmos. Environ., 141, 276–286, https://doi.org/10.1016/j.atmosenv.2016.06.065, 2016.
Danard, M.: A simple model for mesoscale effects of topography on surface
winds, Mon. Weather Rev., 99, 831–839, 1977.
Delgado-Saborit, J. M., Alam, M. S., Pollitt, K. J. G., Stark, C., and Harrison,
R. M.: Analysis of atmospheric concentrations of quinones and polycyclic
aromatic hydrocarbons in vapour and particulate phases, Atmos. Environ., 77,
974–982, https://doi.org/10.1016/j.atmosenv.2013.05.080, 2013.
Dreij, K., Mattsson, Å., Jarvis, I. W. H., Lim, H., Hurkmans, J.,
Gustafsson, J., Bergvall, C., Westerholm, R., Johansson, C., and Stenius,
U.: Cancer risk assessment of airborne PAHs based on in vitro mixture potency factors, Environ. Sci. Technol., 51, 8805–8814, https://doi.org/10.1021/acs.est.7b02963, 2017.
EEA: European Environment Agency Air quality standards,
https://www.eea.europa.eu/themes/air/air-quality-standards (last access: 7 November 2018), 2017.
EEA: Air quality in Europe – 2018 report, EEA Report, European Environment
Agency, Publications Office of the European Union, Luxembourg, https://www.eea.europa.eu/publications/air-quality-in-europe-2018, (last access: 25 July 2022) 2018a.
EEA: European Union emission inventory report 1990–2016 under the UNECE
convention on long-range transboundary air pollution (LRTAP), European
Environment Agency, Publications Office of the European Union, Luxembourg, https://www.eea.europa.eu/publications/european-union-emission-inventory-report-1990-2016 (last access: 25 July 2022), 2018b.
EMEP/EEA: EMEP/EEA air pollutant emission inventory guidebook 2013, EEA
technical report, No. 12/2013, A.4 Small
combustion Appendix D 20+13update of methodologies for Small combustion
(1A4), http://www.eea.europa.eu/publications/emep-eea-guidebook-2013, (last access: 15 August 2022), 2013.
EU: Directive 2004/107/EC of the European Parliament and of the Council of
15 December 2004 relating to arsenic, cadmium, mercury, nickel and
polycyclic aromatic hydrocarbons in ambient air, Official Journal of the
European Union, L23, 26 January 2005, https://eur-lex.europa.eu/LexUriServ/LexUriServ.do?uri=OJ:L:2005:023:0003:0016:EN:PDF (last access: 25 July 2022), 2005.
EU: Directive 2008/50/EC of the European Parliament and of the Council of 21
May 2008 on ambient air quality and cleaner air for Europe, Official Journal
of the European Union, L152, 11 June 2008, https://eur-lex.europa.eu/legal-content/EN/TXT/?uri=OJ%3AL%3A2008%3A152%3ATOC, (last access: 25 July 2022), 2008.
Fabbri, D., Torri, C., Simo.neit, B. R. T., Marynowski, L., Rushdi, A. I., and
Fabiańska, M. J.: Levoglucosan and other cellulose and lignin markers in
emissions from burning of Miocene lignites, Atmos. Environ., 43,
2286–2295, https://doi.org/10.1016/j.atmosenv.2009.01.030, 2009.
Favez, O., Cachier, H., Sciare, J., Sarda-Estève, R., and Martinon, L.:
Evidence for a significant contribution of wood burning aerosols to
PM2.5 during the winter season in Paris, France, Atmos. Environ., 43, 3640–3644, https://doi.org/10.1016/j.atmosenv.2009.04.035, 2009.
Fine, P. M., Cass, G. R., and Simoneit, B. R. T.: Chemical characterization of
fine particle emissions from the fireplace combustion of woods grown in the
southern United States, Environ. Sci. Technol., 36, 1442–1451,
https://doi.org/10.1021/es0108988, 2002.
Fine, P. M., Cass, G. R., and Simoneit, B. R. T.: Chemical characterization of
fine particle emissions from the fireplace combustion of wood types grown in
the midwestern and western United States, Environ. Eng. Sci., 21,
387–409, https://doi.org/10.1089/109287504323067021, 2004.
Fraser, M. P. and Lakshmanan, K.: Using levoglucosan as a molecular marker
for the long-range transport of biomass combustion aerosols, Environ. Sci.
Technol., 34, 4560–4564, https://doi.org/10.1021/es991229l, 2000.
Fuller, G. W., Tremper, A. H., Baker, T. D., Yttri, K. E., and Butterfield, D.:
Contribution of wood burning to PM10 in London, Atmos. Environ., 87,
87–94, https://doi.org/10.1016/j.atmosenv.2013.12.037, 2014.
Glasius, M., Hansen, A. M. K., Claeys, M., Henzing, J. S., Jedynska A. D.,
Kasper-Giebl, A., Kistler, M., Kristensen, K., Martinsson, J., Maenhaut, W.,
Nøjgaard, J. K., Spindler, G., Stenström, K. E., Swietlicki, E.,
Szidat, S., Simpson, D., and Yttri, K. E.: Composition and sources of
carbonaceous aerosols in Northern Europe during winter, Atmos. Environ.,
173, 127–141, https://doi.org/10.1016/j.atmosenv.2017.11.005, 2018.
Hellén, H., Kangas, L., Kousa, A., Vestenius, M., Teinilä, K., Karppinen, A., Kukkonen, J., and Niemi, J. V.: Evaluation of the impact of wood combustion on benzo[a]pyrene (BaP) concentrations; ambient measurements and dispersion modeling in Helsinki, Finland, Atmos. Chem. Phys., 17, 3475–3487, https://doi.org/10.5194/acp-17-3475-2017, 2017.
Hong, Y., Cao, F., Fan, M.-Y., Lin, Y.-C., Gul, C., Yu, M., Wu, X., Zhai, X.
and Zhang, Y.-L.: Impacts of chemical degradation of levoglucosan on
quantifying biomass burning contribution to carbonaceous aerosols: A case
study in Northeast China, Sci. Total Environ., 819, 152007,
https://doi.org/10.1016/j.scitotenv.2021.152007, 2022.
Jedynska, A., Hoek, G., Wang, M., Eeftens, M., Cyrys, J., Beelen, R.,
Cirach, M., De Nazelle, A., Keuken, M., Visschedijk, A., Nystad, W.,
Akhlaghi, H. M., Meliefste, K., Nieuwenhuijsen, M., de Hoogh, K., Brunekreef,
B., and Kooter, I. M.: Spatial variations of levoglucosan in four European
study areas, Sci. Total Environ., 505, 1072–1081,
https://doi.org/10.1016/j.scitotenv.2014.10.091, 2015.
Johansson, C., Pettersson, M., Omstedt, G.: Metodik för utvärdering av den lokala
vedeldningens påverkan på luftkvalitet – Erfarenheter från BHM, ITM Report 118, Inst of Applied Environmental Research, Stockholm University, Sweden, http://www.aces.su.se/reflab/wp-content/uploads/itm_rapp118_2003-12-10.pdf (last access: 22 August, 2022), 2003.
Keyte, I. J., Harrison, R. M. and Lammel, G: Chemical reactivity and
long-range transport potential of polycyclic aromatic hydrocarbons – a
review, Chem. Soc. Rev., 42, 9333–9391, https://doi.org/10.1039/c3cs60147a,
2013.
Khan, M. B., Masiol, M., Bruno, C., Pasqualetto, A., Formenton, G. M.,
Agostinelli, C., and Pavoni, B.: Potential sources and meteorological
factors affecting PM2.5-bound polycyclic aromatic hydrocarbon levels in
six main cities of northeastern Italy: an assessment of the related
carcinogenic and mutagenic risks, Environ. Sci. Pollut. Res., 25,
31987–32000, https://doi.org/10.1007/s11356-018-2841-1, 2018.
Kocbach Bølling, A., Pagels, J., Yttri, K. E., Barregard, L., Sallsten,
G., Schwarze, P. E., and Boman, C.: Health effects of residential wood smoke
particles: the importance of combustion conditions and physicochemical
particle properties, Part. Fibre Toxicol., 6, 29,
https://doi.org/10.1186/1743-8977-6-29, 2009.
Lewtas, J.: Air pollution combustion emissions: Characterization of
causative agents and mechanisms associated with cancer, reproductive, and
cardiovascular effects, Mut. Res., 636, 95–133,
https://doi.org/10.1016/j.mrrev.2007.08.003, 2007.
Li, Y., Fu, T.-M., Yu, J. Z., Feng, X., Zhang, L., Chen, J., Boreddy, S. K. R.,
Kawamura, K., Fu, P., Yang, X., Zhu, L. and Zeng, Z.: Impacts of chemical
degradation on the global budget of atmospheric levoglucosan and its use as
a biomass burning tracer, Environ. Sci. Technol., 55, 5525–5536, https://doi.org/10.1021/acs.est.0c07313, 2021.
Lim, H., Mattsson, Å., Jarvis, I. W. H., Bergvall, C., Bottai, M.,
Morales, D. A., Kummrow, F., Umbuzeiro, G. A., Stenius, U., Westerholm, R.,
and Dreij, K.: Detection of benz[j]aceanthrylene in urban air and evaluation
of its genotoxic potential, Environ. Sci. Technol., 49, 3101–3109,
https://doi.org/10.1021/es505458g, 2015.
Maenhaut, W., Vermeylen, R., Claeys, M., Vercauteren, J., Matheeussen, C.,
and Roekens, E.: Assessment of the contribution from wood burning to the
PM10 aerosol in Flanders, Belgium, Sci. Total Environ., 437, 226–236,
https://doi.org/10.1016/j.scitotenv.2012.08.015, 2012.
Maenhaut, W., Vermeylen, R., Claeys, M., Vercauteren, J., and Roekens, E.:
Sources of the PM10 aerosol in Flanders, Belgium, and re-assessment of the
contribution from wood burning, Sci. Total Environ., 562, 550–560,
https://doi.org/10.1016/j.scitotenv.2016.04.074, 2016.
Manoli, E., Kouras, A., Karagkiozidou, O., Argyropoulos, G., Voutsa, D., and
Samara, C.: Polycyclic aromatic hydrocarbons (PAHs) at traffic and urban
background sites of northern Greece: source apportionment of ambient PAH
levels and PAH-induced lung cancer risk, Environ. Sci. Pollut. Res., 23,
3556–3568, https://doi.org/10.1007/s11356-015-5573-5, 2016.
Martinsson, J., Eriksson, A. C., Elbæk Nielsen, I., Berg Malmborg, V.,
Ahlberg, E., Andersen, C., Lindgren, R., Nyström, R.,
Nordin, E. Z., Brune, W. H., Svenningsson, B., Swietlicki, E., Boman, C. and
Pagels, J. H.: Impacts of combustion conditions and photochemical processing
on the light absorption of biomass combustion aerosol, Environ. Sci.
Technol., 49, 14663–14671, https://doi.org/10.1021/acs.est.5b03205, 2015.
Mashayekhy Rad, F., Spinicci, S., Silvergren, S., Nilsson, U., and
Westerholm, R.: Validation of a HILIC/ESI-MS/MS method for the wood burning
marker levoglucosan and its isomers in airborne particulate matter,
Chemosphere, 211, 617–623, https://doi.org/10.1016/j.chemosphere.2018.07.188, 2018.
MDH: Guidance for evaluating the cancer potency of polycyclic aromatic
hydrocarbon (PAH) mixtures in environmental samples, Minnesota Department of
Health, St. Paul, MN, USA, https://www.health.state.mn.us/communities/environment/risk/docs/guidance/pahguidance.pdf (last access: 25 July 2022), 2016.
Mitchell, J.: IARC Monographs on the evaluation of carcinogenic risks to humans,
Volume 92, Some Non-heterocyclic polycyclic aromatic hydrocarbons and some
related exposures, International Agency for Research on Cancer, Lyon,
France, https://publications.iarc.fr/Book-And-Report-Series/Iarc-Monographs-On-The-Identification-Of-Carcinogenic-Hazards-To-Humans/Some-Non-heterocyclic-Polycyclic-Aromatic-Hydrocarbons-And-Some-Related-Exposures-2010 (last access: 25 July 2022), 2010.
Mitchell, J.: IARC Monographs on the evaluation of carcinogenic risks to humans,
Volume 101, Some chemicals present in industrial and consumer products,
food and drinking-water, International Agency for Research on Cancer, Lyon,
France, https://publications.iarc.fr/Book-And-Report-Series/Iarc-Monographs-On-The-Identification-Of-Carcinogenic-Hazards-To-Humans/Some-Chemicals-Present-In-Industrial-And-Consumer-Products-Food-And-Drinking-water-2012 (last access: 25 July 2022), 2013.
Müller, K.: IARC Monographs on the evaluation of carcinogenic risks to humans,
Volume 109, Outdoor air pollution, International Agency for Research on
Cancer, Lyon, France, https://publications.iarc.fr/Book-And-Report-Series/Iarc-Monographs-On-The-Identification-Of-Carcinogenic-Hazards-To-Humans/Outdoor-Air-Pollution-2015 (last access: 25 July 2022), 2016.
Muller, P.: Scientific criteria document for multimedia standards
development, polycyclic aromatic hydrocarbons (PAH), Part 1, Hazard
identification and dose-response assessment, Ontario Ministry of Environment
and Energy, Ontario, Canada, https://www.osti.gov/etdeweb/biblio/607219 (last access: 26 July 2022), 1997.
Nisbet, I. C. T. and LaGoy, P. K.: Toxic equivalency factors (TEFs) for
polycyclic aromatic hydrocarbons (PAHs), Regul. Toxicol. Pharm., 16,
290–300, https://doi.org/10.1016/0273-2300(92)90009-X, 1992.
Nolte, C. G., Schauer, J. J., Cass, G. R., and Simoneit, B. R. T.: Highly polar
organic compounds present in wood smoke and in the ambient atmosphere,
Environ. Sci. Technol., 35, 1912–1919, https://doi.org/10.1021/es001420r, 2001.
Nyström, R., Sadiktsis, I., Ahmed, T. M., Westerholm, R., Koegler, J. H.,
Blomberg, A., Sandström, T., and Boman, C.: Physical and chemical
properties of RME biodiesel exhaust particles without engine modifications,
Fuel, 186, 261–269, https://doi.org/10.1016/j.fuel.2016.08.062, 2016.
Olsson, P., Sadiktsis, I., Holmbäck, J., and Westerholm, R.: Class
separation of lipids and polycyclic aromatic hydrocarbons in normal phase
high performance liquid chromatography – A prospect for analysis of
aromatics in edible vegeTable oils and biodiesel exhaust particulates, J.
Chromatogr. A., 1360, 39–46, https://doi.org/10.1016/j.chroma.2014.07.064, 2014.
Omstedt, G., Forsberg, M., Persson, K.: Vedrök i Västerbotten –
mätningar, beräkningar och hälsokonsekvenser, SMHI report 156, http://urn.kb.se/resolve?urn=urn%3Anbn%3Ase%3Asmhi%3Adiva-2792, or
https://www.diva-portal.org/smash/get/diva2:948088/FULLTEXT01.pdf (last access: 15 August 2022), 2014.
Pietrogrande, M. C., Bacco, D., Demaria, G., Russo, M., Scotto, F., and
Trentini, A.: Polycyclic aromatic hydrocarbons and their oxygenated
derivatives in urban aerosol: levels, chemical profiles, and contribution to
PM2.5 oxidative potential, Environ. Sci. Pollut. Res., 29, 54391–54406, https://doi.org/10.1007/s11356-021-16858-z, 2022.
Puxbaum, H., Caseiro, A., Sánchez-Ochoa, A., Kasper-Giebl, A., Claeys,
M., Gelencsér, A., Legrand, M., Preunkert, S., and Pio, C.: Levoglucosan
levels at background sites in Europe for assessing the impact of biomass
combustion on the European aerosol background, J. Geophys. Res., 112,
D23S05, https://doi.org/10.1029/2006JD008114, 2007.
Sadiktsis, I., Koegler, J. H., Benham, T., Bergvall, C., and Westerholm, R.:
Particulate associated polycyclic aromatic hydrocarbon exhaust emissions
from a porTable power generator fueled with three different fuels – A
comparison between petroleum diesel and two biodiesels, Fuel, 115, 573–580,
https://doi.org/10.1016/j.fuel.2013.07.062, 2014.
Saleh, R., Robinson, E. S., Tkacik, D. S., Ahern, A. T., Liu, S., Aiken, A. C.,
Sullivan, R. C., Presto, A. A., Dubey, M. K., Yokelson, R. J., Donahue, N. M., and
Robinson, A. L.: Brownness of organics in aerosols from biomass burning
linked to their black carbon content, Nat. Geosci., 7, 647–650,
https://doi.org/10.1038/ngeo2220, 2014.
Sarigiannis, D. A., Karakitsios, S. P., Zikopoulos, D., Nikolaki, S., and
Kermenidou, M.: Lung cancer risk from PAHs emitted from biomass combustion,
Environ. Res., 137, 147–156, https://doi.org/10.1016/j.envres.2014.12.009, 2015.
Schmidl, C., Marr, I. L., Caseiro, A., Kotianová, P., Berner, A., Bauer,
H., Kasper-Giebl, A., and Puxbaum, H.: Chemical characterisation of fine
particle emissions from wood stove combustion of common woods growing in
mid-European Alpine regions, Atmos. Environ., 42, 126–141,
https://doi.org/10.1016/j.atmosenv.2007.09.028, 2008.
Segersson, D., Eneroth, K., Engström Nylén, A., Gidhagen, L.,
Omstedt, G., Johansson, C., and Forsberg, B.: Health impact of PM10, PM2.5 and
BC exposure due to different source sectors in Stockholm, Gothenburg and
Umea, Sweden, Int. J. Environ. Res. Public Health, 14, 742,
https://doi.org/10.3390/ijerph14070742, 2017.
Shafizadeh, F.: Pyrolysis and combustion of cellulosic materials, Adv.
Carbohydr. Chem., 23, 419–474, https://doi.org/10.1016/S0096-5332(08)60173-3, 1968.
Sigsgaard, T., Forsberg, B., Annesi-Maesano, I., Blomberg, A., Bølling,
A., Boman, C., Bønløkke, J., Brauer, M., Bruce, N., Héroux, M. E.,
Hirvonen, M. R., Kelly, F., Künzli, N., Lundbäck, B., Moshammer, H.,
Noonan, C., Pagels, J., Sallsten, G., Sculier, J. P., and Brunekreef, B.:
Health impacts of anthropogenic biomass burning in the developed world, Eur.
Respir. J., 46, 1577–1588, https://doi.org/10.1183/13993003.01865-2014, 2015.
Simoneit, B. R. T.: Biomass burning – a review of organic tracers for smoke
from incomplete combustion, Appl. Geochem., 17, 129–162,
https://doi.org/10.1016/S0883-2927(01)00061-0, 2002.
Simoneit, B. R. T., Schauer, J. J., Nolte, C. G., Oros, D. R., Elias, V. O.,
Fraser, M. P., Rogge, W. F., and Cass, G. R.: Levoglucosan, a tracer for
cellulose in biomass burning and atmospheric particles, Atmos. Environ., 33, 173–182, https://doi.org/10.1016/S1352-2310(98)00145-9, 1999.
Singh, D. K., Kawamura, K., Yanase, A., and Barrie, L. A.: Distributions of
polycyclic aromatic hydrocarbons, aromatic ketones, carboxylic acids, and
trace metals in Arctic aerosols: Long-range atmospheric transport,
photochemical degradation/production at polar sunrise, Environ. Sci.
Technol., 51, 8992–9004, https://doi.org/10.1021/acs.est.7b01644, 2017.
SLB-analys: LVF 2010:06 Kartläggning av bens(a)pyrenhalter i Stockholms-
och Uppsala län samt tätorterna Gävle och Sandviken, Technical
report by Stockholm and Uppsala Air quality management association, https://www.slb.nu/slb/rapporter/pdf8/lvf2010_006.pdf (last access: 15 August 2022), 2010.
SLB-analys: Meteorological data/Meteorologi timdatabas, Meteorologi dygnsdatabas, slb.nu [data set], https://www.slb.nu/slbanalys/historiska-data-met, last access: 15 August 2022a.
SLB-analys: Measured air pollutant data/Luftkvalitet timdatabas, slb.nu [data set], https://www.slb.nu/slbanalys/historiska-data-luft, last access: 15 August 2022b.
Slezakova, K., Castro, D., Delerue-Matos, C., Alvim-Ferraz, M. C., Morais,
S., and Pereira, M. C.: Impact of vehicular traffic emissions on
particulate-bound PAHs: Levels and associated health risks, Atmos. Res.,
127, 141–147, https://doi.org/10.1016/j.atmosres.2012.06.009, 2013.
SMED and Naturvårdsverket: Informative Inventory Report Sweden 2017, Swedish Environmental Protection Agency, Stockholm, Sweden,
https://www.naturvardsverket.se/upload/sa-mar-miljon/klimat-och-luft/luft/luftfororeningar/informative-inventory-report-sweden-2017.pdf (last access: last access: 31 January 2019), 2017.
Taesler, R. and Andersson, C.: A method for solar radiation computations
using routine meteorological observations, Energy and Buildings, 7, 341–352, 1984.
Taesler, R., Andersson, C., Nord, M., Gollvik, L.: Analyses of impacts of
weather and climate on building energy performance with special regard to
urban climate characteristics, Preprint, 6th International Conference on
Urban Climate, Göteborg, Sweden, 12–16 June 2006, http://www.urban-climate.org/documents/ICUC6_Preprints.pdf (last access: 16 August 2022), 2006.
Todorovic, J., Broden, H., Padban, N., Lange, S, Gustafsson, L., Johansson,
L., Paulrud, S., and Löfgren, B. E.: Syntes och analys av
emissionsfaktorerer för småskalig biobränsleförbränning,
TPS Termiska Processer, SP Technical Research Institute of Sweden, IVL Swedish Environmental Research Institute, and ÄFAB, 2007.
Wagener, S., Langner, M., Hansen, U., Moriske, H. J., and Endlicher, W. R.:
Spatial and seasonal variations of biogenic tracer compounds in ambient
PM10 and PM1 samples in Berlin, Germany, Atmos. Environ., 47,
33–42, https://doi.org/10.1016/j.atmosenv.2011.11.044, 2012.
Wagner, F., Amann, M., Bertok, I., Cofala, J., Heyes, C., Klimont, Z.,
Rafaj, P., and Schöpp, W.: Baseline emission projections and further
cost-effective reductions of air pollution impacts in Europe – a 2010
perspective, IIASA, Austria, 2010.
Walgraeve, C., Demeestere, K., Dewulf, J., Zimmermann, R., and Van
Langenhove, H.: Oxygenated polycyclic aromatic hydrocarbons in atmospheric
particulate matter: Molecular characterization and occurrence, Atmos.
Environ., 44, 1831–1846, https://doi.org/10.1016/j.atmosenv.2009.12.004, 2010.
WHO: WHO Air quality guidelines for particulate matter, ozone, nitrogen
oxide and sulfur dioxide, Global update 2005, Summary of risk assessment,
World Health Organization, WHO Press, Geneva, Switzerland, https://apps.who.int/iris/handle/10665/69477 (last access: 26 July 2022), 2006.
Yttri, K. E., Dye, K., Slørdal, L. H., and Braathen, O. A.: Quantification
of monosaccharide anhydrides by liquid chromatography combined with mass
spectrometry: application to aerosol samples from an urban and a suburban
site influenced by small-scale wood burning, J. Air Waste Manag.
Assoc., 55, 1169–1177, https://doi.org/10.1080/10473289.2005.10464720, 2005.
Download
The requested paper has a corresponding corrigendum published. Please read the corrigendum first before downloading the article.
- Article
(3550 KB) - Full-text XML
- Corrigendum
-
Supplement
(595 KB) - BibTeX
- EndNote
Short summary
Air pollutants from wood burning become more important as other regulated emissions are being reduced, e.g. combustion of diesel. We analysed particles in residential areas and found that local wood burning was the most important source of polycyclic aromatic hydrocarbons (PAHs). Specific tracers were used to separate wood combustion from other contributions. Calculations of population exposure showed that the mix of PAHs may cause 13 cancer cases per 0.1 million inhabitants.
Air pollutants from wood burning become more important as other regulated emissions are being...
Altmetrics
Final-revised paper
Preprint