Articles | Volume 21, issue 7
https://doi.org/10.5194/acp-21-5549-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-5549-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Apr 2021
Research article |
| 12 Apr 2021
| 12 Apr 2021
Atmospheric conditions and composition that influence PM2.5 oxidative potential in Beijing, China
Steven J. Campbell
CORRESPONDING AUTHOR
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Department of Chemistry, University of Cambridge, Cambridge, UK
Kate Wolfer
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Battist Utinger
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Joe Westwood
Department of Chemistry, University of Cambridge, Cambridge, UK
Zhi-Hui Zhang
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Department of Chemistry, University of Cambridge, Cambridge, UK
Nicolas Bukowiecki
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Sarah S. Steimer
Department of Chemistry, University of Cambridge, Cambridge, UK
now at: Department of Environmental Science, Stockholm
University, Stockholm, Sweden
Tuan V. Vu
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
also at: Department of Environmental Sciences/Center of
Excellence in Environmental Studies, King Abdulaziz University, P.O. Box 80203, Jeddah, 21589, Saudi Arabia
Jingsha Xu
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
Nicholas Straw
Centre for Cardiovascular Science, Queen's Medical Research Institute,
University of Edinburgh, Edinburgh, UK
Steven Thomson
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
Atallah Elzein
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing, China
Di Liu
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing, China
Linjie Li
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing, China
Pingqing Fu
Institute of Surface Earth System Science, Tianjin University,
Tianjin, China
Alastair C. Lewis
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
National Centre for Atmospheric Science, University of York, York, UK
Roy M. Harrison
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
now at: School of Public Health, Imperial College London, London, UK
William J. Bloss
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
Miranda Loh
Institute of Occupational Medicine, Edinburgh, UK
Mark R. Miller
Centre for Cardiovascular Science, Queen's Medical Research Institute,
University of Edinburgh, Edinburgh, UK
Zongbo Shi
School of Geography, Earth and Environmental Sciences, University of
Birmingham, Birmingham, UK
Markus Kalberer
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Department of Chemistry, University of Cambridge, Cambridge, UK
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53 citations as recorded by crossref.
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- Assessing the chemical composition, potential toxicity and cancer risk of airborne fine particulate matter (PM2.5) near a petrochemical industrial area S. Caumo et al. 10.1016/j.etap.2023.104170
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- Wintertime oxidative potential of PM2.5 over a big urban city in the central Indo-Gangetic Plain A. Singh et al. 10.1016/j.scitotenv.2023.167155
- Source apportionment of oxidative potential: What we know so far S. Stevanovic et al. 10.2298/TSCI221107111S
- Size distribution and lung-deposition of ambient particulate matter oxidative potential: A contrast between dithiothreitol and ascorbic acid assays L. Famiyeh et al. 10.1016/j.envpol.2023.122437
- Examining the structural properties of hydrophilic and hydrophobic organic aerosols using 1H NMR: diurnal variations and source apportionment. A. Sam et al. 10.1016/j.apr.2024.102363
- Oxidative potential induced by metal-organic interaction from PM2.5 in simulated biological fluids N. Wu et al. 10.1016/j.scitotenv.2022.157768
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- Health risk assessment in atmosphere near a petrochemical industrial complex: Measuring oxidative potential and oxidative burden S. Caumo et al. 10.1016/j.apr.2022.101457
- Disentangling fine particles (PM2.5) composition in Hanoi, Vietnam: Emission sources and oxidative potential P. Dominutti et al. 10.1016/j.scitotenv.2024.171466
- Are reactive oxygen species (ROS) a suitable metric to predict toxicity of carbonaceous aerosol particles? Z. Zhang et al. 10.5194/acp-22-1793-2022
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- Redox-activity and in vitro effects of regional atmospheric aerosol pollution: Seasonal differences and correlation between oxidative potential and in vitro toxicity of PM1 G. Melzi et al. 10.1016/j.taap.2024.116913
- Source apportionment of oxidative potential depends on the choice of the assay: insights into 5 protocols comparison and implications for mitigation measures P. Dominutti et al. 10.1039/D3EA00007A
- Iron and Copper Alter the Oxidative Potential of Secondary Organic Aerosol: Insights from Online Measurements and Model Development S. Campbell et al. 10.1021/acs.est.3c01975
- New health index derived from oxidative potential and cell toxicity of fine particulate matter to assess its potential health effect M. Park et al. 10.1016/j.heliyon.2024.e25310
- Key toxic components and sources affecting oxidative potential of atmospheric particulate matter using interpretable machine learning: Insights from fog episodes R. Li et al. 10.1016/j.jhazmat.2023.133175
- Sensitivity of PM10 oxidative potential to aerosol chemical composition at a Mediterranean urban site: ascorbic acid versus dithiothreitol measurements Á. Clemente et al. 10.1007/s11869-023-01332-1
- The interplay of Brown carbon (BrC) surrogates and copper: Implications for the oxidative potential of ambient particles D. Wu et al. 10.1016/j.jhazmat.2024.136276
- Investigating PM2.5 Oxidative Potential and Its Association with Chemical Constituents Measured outside of Urban Residences in Three Metropolitan Cities of India S. Dubey et al. 10.1289/JHP1007
- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
- Changes in source contributions to the oxidative potential of PM2.5 in urban Xiamen, China J. Li et al. 10.1016/j.jes.2024.02.003
- Variations in the oxidation potential of PM2.5 in an old industrial city in China from 2015 to 2018 Z. Wang et al. 10.1016/j.scitotenv.2024.174639
- Critical contribution of chemically diverse carbonyl molecules to the oxidative potential of atmospheric aerosols F. Li et al. 10.5194/acp-24-8397-2024
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- Chemical and oxidative properties of fine particulate matter from near-road traffic sources N. Raparthi et al. 10.1016/j.envpol.2023.122514
- Oxidative potential of atmospheric brown carbon in six Chinese megacities: Seasonal variation and source apportionment D. Wang et al. 10.1016/j.atmosenv.2023.119909
- Ascorbate oxidation driven by PM2.5-bound metal(loid)s extracted in an acidic simulated lung fluid in relation to their bioaccessibility A. Expósito et al. 10.1007/s11869-023-01436-8
- Origins of the seasonal variability of PM2.5 sources in a rural site in Northern France P. Espina-Martin et al. 10.1016/j.atmosenv.2024.120660
- Multiphase Radical Chemical Processes Induced by Air Pollutants and the Associated Health Effects Q. Wang et al. 10.1021/envhealth.4c00157
- Aerosol Oxidative Potential in the Greater Los Angeles Area: Source Apportionment and Associations with Socioeconomic Position J. Shen et al. 10.1021/acs.est.2c02788
- Source apportionment of water-soluble oxidative potential of PM2.5 in a port city of Xiamen, Southeast China J. Li et al. 10.1016/j.atmosenv.2023.120122
- An automated online field instrument to quantify the oxidative potential of aerosol particles via ascorbic acid oxidation B. Utinger et al. 10.5194/amt-16-2641-2023
- Optical properties, chemical functional group, and oxidative activity of different polarity levels of water-soluble organic matter in PM2.5 from biomass and coal combustion in rural areas in Northwest China S. Huang et al. 10.1016/j.atmosenv.2022.119179
- Oxidative potential of ambient PM2.5 from São Paulo, Brazil: Variations, associations with chemical components and source apportionment E. Serafeim et al. 10.1016/j.atmosenv.2023.119593
- Oxidative potential of fine particulate matter emitted from traditional and improved biomass cookstoves B. Isenor et al. 10.1039/D3EA00135K
- Associations of Exposure to Fine Particulate Matter Mass and Constituents with Systemic Inflammation: A Cross-Sectional Study of Urban Older Adults in China B. Han et al. 10.1021/acs.est.1c04488
- Particulate Matter 2.5 – Muddling the Healthy Brain A. Menon et al. 10.4103/jopsys.jopsys_7_23
- Impact of anthropogenic emission control in reducing future PM2.5 concentrations and the related oxidative potential across different regions of China J. Liu et al. 10.1016/j.scitotenv.2024.170638
- Pollution characteristics and oxidative potential of atmospheric particles at a typical rural area: A case study during the Chinese Lunar New Year S. Jia et al. 10.1016/j.apr.2024.102251
- Characterization of Oxidative Potential and Ecotoxicity of the Organic Fraction of Particulate Matter in a Coastal City in China: Implications for Human Respiratory Health K. Chen et al. 10.1021/acsestair.4c00177
- Impact of PM 2.5 filter extraction solvent on oxidative potential and chemical analysis A. Craze et al. 10.1080/10962247.2024.2417736
- Oxidation potential of PM2.5 in a mechanical processing plant and its association with metal composition J. Ma et al. 10.1016/j.atmosenv.2023.120318
- Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China Y. Luo et al. 10.1016/j.scitotenv.2023.168273
- Effets de la pollution de l'air sur les évènements cardiovasculaires en unité de soins intensifs cardiologiques J. Argacha 10.1016/j.ancard.2023.101663
- Atmospheric evolution of environmentally persistent free radicals in the rural North China Plain: effects on water solubility and PM2.5 oxidative potential X. Yang et al. 10.5194/acp-24-11029-2024
- Particulate matter-induced oxidative stress – Mechanistic insights and antioxidant approaches reported in in vitro studies V. Vilas-Boas et al. 10.1016/j.etap.2024.104529
53 citations as recorded by crossref.
- Spatially resolved chemical data for PM10 and oxidative potential source apportionment in urban-industrial settings L. Massimi et al. 10.1016/j.uclim.2024.102113
- High time resolution quantification of PM2.5 oxidative potential at a Central London roadside supersite S. Campbell et al. 10.1016/j.envint.2024.109102
- Updated World Health Organization Air Quality Guidelines Highlight the Importance of Non-anthropogenic PM2.5 S. Pai et al. 10.1021/acs.estlett.2c00203
- Assessing the chemical composition, potential toxicity and cancer risk of airborne fine particulate matter (PM2.5) near a petrochemical industrial area S. Caumo et al. 10.1016/j.etap.2023.104170
- Effect of Biomass Burning, Diwali Fireworks, and Polluted Fog Events on the Oxidative Potential of Fine Ambient Particulate Matter in Delhi, India J. Puthussery et al. 10.1021/acs.est.2c02730
- Dynamic Wood Smoke Aerosol Toxicity during Oxidative Atmospheric Aging S. Wang et al. 10.1021/acs.est.2c05929
- Chemical constituents, driving factors, and source apportionment of oxidative potential of ambient fine particulate matter in a Port City in East China K. Chen et al. 10.1016/j.jhazmat.2022.129864
- Major source categories of PM2.5 oxidative potential in wintertime Beijing and surroundings based on online dithiothreitol-based field measurements R. Cheung et al. 10.1016/j.scitotenv.2024.172345
- Wintertime oxidative potential of PM2.5 over a big urban city in the central Indo-Gangetic Plain A. Singh et al. 10.1016/j.scitotenv.2023.167155
- Source apportionment of oxidative potential: What we know so far S. Stevanovic et al. 10.2298/TSCI221107111S
- Size distribution and lung-deposition of ambient particulate matter oxidative potential: A contrast between dithiothreitol and ascorbic acid assays L. Famiyeh et al. 10.1016/j.envpol.2023.122437
- Examining the structural properties of hydrophilic and hydrophobic organic aerosols using 1H NMR: diurnal variations and source apportionment. A. Sam et al. 10.1016/j.apr.2024.102363
- Oxidative potential induced by metal-organic interaction from PM2.5 in simulated biological fluids N. Wu et al. 10.1016/j.scitotenv.2022.157768
- Chemical Constituents, Driving Factors, and Source Apportionment of Oxidative Potential of Ambient Fine Particulate Matter in a Port City in East China K. Chen et al. 10.2139/ssrn.4113951
- Health risk assessment in atmosphere near a petrochemical industrial complex: Measuring oxidative potential and oxidative burden S. Caumo et al. 10.1016/j.apr.2022.101457
- Disentangling fine particles (PM2.5) composition in Hanoi, Vietnam: Emission sources and oxidative potential P. Dominutti et al. 10.1016/j.scitotenv.2024.171466
- Are reactive oxygen species (ROS) a suitable metric to predict toxicity of carbonaceous aerosol particles? Z. Zhang et al. 10.5194/acp-22-1793-2022
- Effects of personal exposure to the oxidative potential of PM2.5 on oxidative stress biomarkers in pregnant women A. Marsal et al. 10.1016/j.scitotenv.2023.168475
- Redox-activity and in vitro effects of regional atmospheric aerosol pollution: Seasonal differences and correlation between oxidative potential and in vitro toxicity of PM1 G. Melzi et al. 10.1016/j.taap.2024.116913
- Source apportionment of oxidative potential depends on the choice of the assay: insights into 5 protocols comparison and implications for mitigation measures P. Dominutti et al. 10.1039/D3EA00007A
- Iron and Copper Alter the Oxidative Potential of Secondary Organic Aerosol: Insights from Online Measurements and Model Development S. Campbell et al. 10.1021/acs.est.3c01975
- New health index derived from oxidative potential and cell toxicity of fine particulate matter to assess its potential health effect M. Park et al. 10.1016/j.heliyon.2024.e25310
- Key toxic components and sources affecting oxidative potential of atmospheric particulate matter using interpretable machine learning: Insights from fog episodes R. Li et al. 10.1016/j.jhazmat.2023.133175
- Sensitivity of PM10 oxidative potential to aerosol chemical composition at a Mediterranean urban site: ascorbic acid versus dithiothreitol measurements Á. Clemente et al. 10.1007/s11869-023-01332-1
- The interplay of Brown carbon (BrC) surrogates and copper: Implications for the oxidative potential of ambient particles D. Wu et al. 10.1016/j.jhazmat.2024.136276
- Investigating PM2.5 Oxidative Potential and Its Association with Chemical Constituents Measured outside of Urban Residences in Three Metropolitan Cities of India S. Dubey et al. 10.1289/JHP1007
- Organic Peroxides in Aerosol: Key Reactive Intermediates for Multiphase Processes in the Atmosphere S. Wang et al. 10.1021/acs.chemrev.2c00430
- Changes in source contributions to the oxidative potential of PM2.5 in urban Xiamen, China J. Li et al. 10.1016/j.jes.2024.02.003
- Variations in the oxidation potential of PM2.5 in an old industrial city in China from 2015 to 2018 Z. Wang et al. 10.1016/j.scitotenv.2024.174639
- Critical contribution of chemically diverse carbonyl molecules to the oxidative potential of atmospheric aerosols F. Li et al. 10.5194/acp-24-8397-2024
- Impact of meteorology and aerosol sources on PM2.5 and oxidative potential variability and levels in China J. Liu et al. 10.5194/acp-24-10849-2024
- Chemical and oxidative properties of fine particulate matter from near-road traffic sources N. Raparthi et al. 10.1016/j.envpol.2023.122514
- Oxidative potential of atmospheric brown carbon in six Chinese megacities: Seasonal variation and source apportionment D. Wang et al. 10.1016/j.atmosenv.2023.119909
- Ascorbate oxidation driven by PM2.5-bound metal(loid)s extracted in an acidic simulated lung fluid in relation to their bioaccessibility A. Expósito et al. 10.1007/s11869-023-01436-8
- Origins of the seasonal variability of PM2.5 sources in a rural site in Northern France P. Espina-Martin et al. 10.1016/j.atmosenv.2024.120660
- Multiphase Radical Chemical Processes Induced by Air Pollutants and the Associated Health Effects Q. Wang et al. 10.1021/envhealth.4c00157
- Aerosol Oxidative Potential in the Greater Los Angeles Area: Source Apportionment and Associations with Socioeconomic Position J. Shen et al. 10.1021/acs.est.2c02788
- Source apportionment of water-soluble oxidative potential of PM2.5 in a port city of Xiamen, Southeast China J. Li et al. 10.1016/j.atmosenv.2023.120122
- An automated online field instrument to quantify the oxidative potential of aerosol particles via ascorbic acid oxidation B. Utinger et al. 10.5194/amt-16-2641-2023
- Optical properties, chemical functional group, and oxidative activity of different polarity levels of water-soluble organic matter in PM2.5 from biomass and coal combustion in rural areas in Northwest China S. Huang et al. 10.1016/j.atmosenv.2022.119179
- Oxidative potential of ambient PM2.5 from São Paulo, Brazil: Variations, associations with chemical components and source apportionment E. Serafeim et al. 10.1016/j.atmosenv.2023.119593
- Oxidative potential of fine particulate matter emitted from traditional and improved biomass cookstoves B. Isenor et al. 10.1039/D3EA00135K
- Associations of Exposure to Fine Particulate Matter Mass and Constituents with Systemic Inflammation: A Cross-Sectional Study of Urban Older Adults in China B. Han et al. 10.1021/acs.est.1c04488
- Particulate Matter 2.5 – Muddling the Healthy Brain A. Menon et al. 10.4103/jopsys.jopsys_7_23
- Impact of anthropogenic emission control in reducing future PM2.5 concentrations and the related oxidative potential across different regions of China J. Liu et al. 10.1016/j.scitotenv.2024.170638
- Pollution characteristics and oxidative potential of atmospheric particles at a typical rural area: A case study during the Chinese Lunar New Year S. Jia et al. 10.1016/j.apr.2024.102251
- Characterization of Oxidative Potential and Ecotoxicity of the Organic Fraction of Particulate Matter in a Coastal City in China: Implications for Human Respiratory Health K. Chen et al. 10.1021/acsestair.4c00177
- Impact of PM 2.5 filter extraction solvent on oxidative potential and chemical analysis A. Craze et al. 10.1080/10962247.2024.2417736
- Oxidation potential of PM2.5 in a mechanical processing plant and its association with metal composition J. Ma et al. 10.1016/j.atmosenv.2023.120318
- Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China Y. Luo et al. 10.1016/j.scitotenv.2023.168273
- Effets de la pollution de l'air sur les évènements cardiovasculaires en unité de soins intensifs cardiologiques J. Argacha 10.1016/j.ancard.2023.101663
- Atmospheric evolution of environmentally persistent free radicals in the rural North China Plain: effects on water solubility and PM2.5 oxidative potential X. Yang et al. 10.5194/acp-24-11029-2024
- Particulate matter-induced oxidative stress – Mechanistic insights and antioxidant approaches reported in in vitro studies V. Vilas-Boas et al. 10.1016/j.etap.2024.104529
Latest update: 19 Nov 2024
Short summary
In this study, we quantify PM2.5 oxidative potential (OP), a metric widely suggested as a potential measure of particle toxicity, in Beijing in summer and winter using four acellular assays. We correlate PM2.5 OP with a comprehensive range of atmospheric and particle composition measurements, demonstrating inter-assay differences and seasonal variation of PM2.5 OP. Using multivariate statistical analysis, we highlight specific particle chemical components and sources that influence OP.
In this study, we quantify PM2.5 oxidative potential (OP), a metric widely suggested as a...
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