Articles | Volume 21, issue 5
https://doi.org/10.5194/acp-21-3507-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-3507-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Mar 2021
Research article |
| 08 Mar 2021
| 08 Mar 2021
Inverse modelling of carbonyl sulfide: implementation, evaluation and implications for the global budget
Institute for Marine and Atmospheric Research, Utrecht University, Utrecht, the Netherlands
Linda M. J. Kooijmans
Meteorology and Air Quality, Wageningen University & Research, Wageningen, the Netherlands
Ara Cho
Meteorology and Air Quality, Wageningen University & Research, Wageningen, the Netherlands
Stephen A. Montzka
NOAA Global Monitoring Laboratory, National Oceanic and Atmospheric Administration, Boulder, Colorado, USA
Norbert Glatthor
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
John R. Worden
Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California, USA
Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California, USA
Elliot L. Atlas
Rosenstiel School of Marine and Atmospheric Science, University of Miami, Miami, Florida, USA
Maarten C. Krol
Institute for Marine and Atmospheric Research, Utrecht University, Utrecht, the Netherlands
Meteorology and Air Quality, Wageningen University & Research, Wageningen, the Netherlands
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Cited
34 citations as recorded by crossref.
- Efficient Production of Carbonyl Sulfide in the Low‐NOx Oxidation of Dimethyl Sulfide C. Jernigan et al. 10.1029/2021GL096838
- Intercomparison of Atmospheric Carbonyl Sulfide (TransCom‐COS): 2. Evaluation of Optimized Fluxes Using Ground‐Based and Aircraft Observations J. Ma et al. 10.1029/2023JD039198
- Variations of Carbonyl Sulfide During the Dry/Wet Seasons Over the Amazon X. Wang et al. 10.1029/2022GL101717
- Measurement report: Carbonyl sulfide production during dimethyl sulfide oxidation in the atmospheric simulation chamber SAPHIR M. von Hobe et al. 10.5194/acp-23-10609-2023
- Terrestrial photosynthesis inferred from plant carbonyl sulfide uptake J. Lai et al. 10.1038/s41586-024-08050-3
- Assimilation of carbonyl sulfide (COS) fluxes within the adjoint-based data assimilation system – Nanjing University Carbon Assimilation System (NUCAS v1.0) H. Zhu et al. 10.5194/gmd-17-6337-2024
- Plant gross primary production, plant respiration and carbonyl sulfide emissions over the globe inferred by atmospheric inverse modelling M. Remaud et al. 10.5194/acp-22-2525-2022
- Abiotic Production of Dimethyl Sulfide, Carbonyl Sulfide, and Other Organosulfur Gases via Photochemistry: Implications for Biosignatures and Metabolic Potential N. Reed et al. 10.3847/2041-8213/ad74da
- Carbonyl sulfide measurements from a South Pole ice core and implications for atmospheric variability since the last glacial period M. Aydin et al. 10.5194/cp-20-1885-2024
- Constraining the budget of atmospheric carbonyl sulfide using a 3-D chemical transport model M. Cartwright et al. 10.5194/acp-23-10035-2023
- The Z-2018 emissions inventory of COS in Europe: A semiquantitative multi-data-streams evaluation S. Belviso et al. 10.1016/j.atmosenv.2023.119689
- A GC-IRMS method for measuring sulfur isotope ratios of carbonyl sulfide from small air samples S. Baartman et al. 10.12688/openreseurope.13875.2
- Intercomparison of Atmospheric Carbonyl Sulfide (TransCom‐COS; Part One): Evaluating the Impact of Transport and Emissions on Tropospheric Variability Using Ground‐Based and Aircraft Data M. Remaud et al. 10.1029/2022JD037817
- Carbonyl sulfide removal from refinery tail-gas streams: Experimental and kinetic study of the hydrolysis reaction S. Renda et al. 10.1016/j.seppur.2023.124417
- Sources and sinks of carbonyl sulfide inferred from tower and mobile atmospheric observations in the Netherlands A. Zanchetta et al. 10.5194/bg-20-3539-2023
- Long-term fluxes of carbonyl sulfide and their seasonality and interannual variability in a boreal forest T. Vesala et al. 10.5194/acp-22-2569-2022
- Optimizing the terrestrial ecosystem gross primary productivity using carbonyl sulfide (COS) within a two-leaf modeling framework H. Zhu et al. 10.5194/bg-21-3735-2024
- Mitigating methane emissions and promoting acetogenesis in ruminant livestock R. Mrutu et al. 10.3389/fanim.2025.1489212
- Optimizing the carbonic anhydrase temperature response and stomatal conductance of carbonyl sulfide leaf uptake in the Simple Biosphere model (SiB4) A. Cho et al. 10.5194/bg-20-2573-2023
- Carbonyl sulfide: comparing a mechanistic representation of the vegetation uptake in a land surface model and the leaf relative uptake approach F. Maignan et al. 10.5194/bg-18-2917-2021
- ICLASS 1.1, a variational Inverse modelling framework for the Chemistry Land-surface Atmosphere Soil Slab model: description, validation, and application P. Bosman & M. Krol 10.5194/gmd-16-47-2023
- Evaluation of carbonyl sulfide biosphere exchange in the Simple Biosphere Model (SiB4) L. Kooijmans et al. 10.5194/bg-18-6547-2021
- Carbon and Water Fluxes of the Boreal Evergreen Needleleaf Forest Biome Constrained by Assimilating Ecosystem Carbonyl Sulfide Flux Observations C. Abadie et al. 10.1029/2023JG007407
- Covariation of Airborne Biogenic Tracers (CO2, COS, and CO) Supports Stronger Than Expected Growing Season Photosynthetic Uptake in the Southeastern US N. Parazoo et al. 10.1029/2021GB006956
- Carbonyl Sulfide Sulfur Isotope Fractionation During Uptake by C3 and C4 Plants C. Davidson et al. 10.1029/2022JG007035
- Leaf relative uptake of carbonyl sulfide to CO2 seen through the lens of stomatal conductance–photosynthesis coupling W. Sun et al. 10.1111/nph.18178
- A GC-IRMS method for measuring sulfur isotope ratios of carbonyl sulfide from small air samples S. Baartman et al. 10.12688/openreseurope.13875.1
- Recent Solutions for Efficient Carbonyl Sulfide Hydrolysis: A Review S. Renda et al. 10.1021/acs.iecr.2c00649
- Combined assimilation of NOAA surface and MIPAS satellite observations to constrain the global budget of carbonyl sulfide J. Ma et al. 10.5194/acp-24-6047-2024
- Carbonyl Sulfide (OCS) in the Upper Troposphere/Lowermost Stratosphere (UT/LMS) Region: Estimates of Lifetimes and Fluxes E. Karu et al. 10.1029/2023GL105826
- Carbonyl Sulfide (COS) in Terrestrial Ecosystem: What We Know and What We Do Not J. Li et al. 10.3390/atmos15070778
- Remotely Sensed Carbonyl Sulfide Constrains Model Estimates of Amazon Primary Productivity J. Stinecipher et al. 10.1029/2021GL096802
- Estimating emissions of methane consistent with atmospheric measurements of methane and δ13C of methane S. Basu et al. 10.5194/acp-22-15351-2022
- Global Atmospheric OCS Trend Analysis From 22 NDACC Stations J. Hannigan et al. 10.1029/2021JD035764
33 citations as recorded by crossref.
- Efficient Production of Carbonyl Sulfide in the Low‐NOx Oxidation of Dimethyl Sulfide C. Jernigan et al. 10.1029/2021GL096838
- Intercomparison of Atmospheric Carbonyl Sulfide (TransCom‐COS): 2. Evaluation of Optimized Fluxes Using Ground‐Based and Aircraft Observations J. Ma et al. 10.1029/2023JD039198
- Variations of Carbonyl Sulfide During the Dry/Wet Seasons Over the Amazon X. Wang et al. 10.1029/2022GL101717
- Measurement report: Carbonyl sulfide production during dimethyl sulfide oxidation in the atmospheric simulation chamber SAPHIR M. von Hobe et al. 10.5194/acp-23-10609-2023
- Terrestrial photosynthesis inferred from plant carbonyl sulfide uptake J. Lai et al. 10.1038/s41586-024-08050-3
- Assimilation of carbonyl sulfide (COS) fluxes within the adjoint-based data assimilation system – Nanjing University Carbon Assimilation System (NUCAS v1.0) H. Zhu et al. 10.5194/gmd-17-6337-2024
- Plant gross primary production, plant respiration and carbonyl sulfide emissions over the globe inferred by atmospheric inverse modelling M. Remaud et al. 10.5194/acp-22-2525-2022
- Abiotic Production of Dimethyl Sulfide, Carbonyl Sulfide, and Other Organosulfur Gases via Photochemistry: Implications for Biosignatures and Metabolic Potential N. Reed et al. 10.3847/2041-8213/ad74da
- Carbonyl sulfide measurements from a South Pole ice core and implications for atmospheric variability since the last glacial period M. Aydin et al. 10.5194/cp-20-1885-2024
- Constraining the budget of atmospheric carbonyl sulfide using a 3-D chemical transport model M. Cartwright et al. 10.5194/acp-23-10035-2023
- The Z-2018 emissions inventory of COS in Europe: A semiquantitative multi-data-streams evaluation S. Belviso et al. 10.1016/j.atmosenv.2023.119689
- A GC-IRMS method for measuring sulfur isotope ratios of carbonyl sulfide from small air samples S. Baartman et al. 10.12688/openreseurope.13875.2
- Intercomparison of Atmospheric Carbonyl Sulfide (TransCom‐COS; Part One): Evaluating the Impact of Transport and Emissions on Tropospheric Variability Using Ground‐Based and Aircraft Data M. Remaud et al. 10.1029/2022JD037817
- Carbonyl sulfide removal from refinery tail-gas streams: Experimental and kinetic study of the hydrolysis reaction S. Renda et al. 10.1016/j.seppur.2023.124417
- Sources and sinks of carbonyl sulfide inferred from tower and mobile atmospheric observations in the Netherlands A. Zanchetta et al. 10.5194/bg-20-3539-2023
- Long-term fluxes of carbonyl sulfide and their seasonality and interannual variability in a boreal forest T. Vesala et al. 10.5194/acp-22-2569-2022
- Optimizing the terrestrial ecosystem gross primary productivity using carbonyl sulfide (COS) within a two-leaf modeling framework H. Zhu et al. 10.5194/bg-21-3735-2024
- Mitigating methane emissions and promoting acetogenesis in ruminant livestock R. Mrutu et al. 10.3389/fanim.2025.1489212
- Optimizing the carbonic anhydrase temperature response and stomatal conductance of carbonyl sulfide leaf uptake in the Simple Biosphere model (SiB4) A. Cho et al. 10.5194/bg-20-2573-2023
- Carbonyl sulfide: comparing a mechanistic representation of the vegetation uptake in a land surface model and the leaf relative uptake approach F. Maignan et al. 10.5194/bg-18-2917-2021
- ICLASS 1.1, a variational Inverse modelling framework for the Chemistry Land-surface Atmosphere Soil Slab model: description, validation, and application P. Bosman & M. Krol 10.5194/gmd-16-47-2023
- Evaluation of carbonyl sulfide biosphere exchange in the Simple Biosphere Model (SiB4) L. Kooijmans et al. 10.5194/bg-18-6547-2021
- Carbon and Water Fluxes of the Boreal Evergreen Needleleaf Forest Biome Constrained by Assimilating Ecosystem Carbonyl Sulfide Flux Observations C. Abadie et al. 10.1029/2023JG007407
- Covariation of Airborne Biogenic Tracers (CO2, COS, and CO) Supports Stronger Than Expected Growing Season Photosynthetic Uptake in the Southeastern US N. Parazoo et al. 10.1029/2021GB006956
- Carbonyl Sulfide Sulfur Isotope Fractionation During Uptake by C3 and C4 Plants C. Davidson et al. 10.1029/2022JG007035
- Leaf relative uptake of carbonyl sulfide to CO2 seen through the lens of stomatal conductance–photosynthesis coupling W. Sun et al. 10.1111/nph.18178
- A GC-IRMS method for measuring sulfur isotope ratios of carbonyl sulfide from small air samples S. Baartman et al. 10.12688/openreseurope.13875.1
- Recent Solutions for Efficient Carbonyl Sulfide Hydrolysis: A Review S. Renda et al. 10.1021/acs.iecr.2c00649
- Combined assimilation of NOAA surface and MIPAS satellite observations to constrain the global budget of carbonyl sulfide J. Ma et al. 10.5194/acp-24-6047-2024
- Carbonyl Sulfide (OCS) in the Upper Troposphere/Lowermost Stratosphere (UT/LMS) Region: Estimates of Lifetimes and Fluxes E. Karu et al. 10.1029/2023GL105826
- Carbonyl Sulfide (COS) in Terrestrial Ecosystem: What We Know and What We Do Not J. Li et al. 10.3390/atmos15070778
- Remotely Sensed Carbonyl Sulfide Constrains Model Estimates of Amazon Primary Productivity J. Stinecipher et al. 10.1029/2021GL096802
- Estimating emissions of methane consistent with atmospheric measurements of methane and δ13C of methane S. Basu et al. 10.5194/acp-22-15351-2022
1 citations as recorded by crossref.
Latest update: 17 Apr 2025
Short summary
Carbonyl sulfide is an important trace gas in the atmosphere and useful to estimating gross primary productivity in ecosystems, but its sources and sinks remain highly uncertain. Therefore, we applied inverse model system TM5-4DVAR to better constrain the global budget. Our finding is in line with earlier studies, pointing to missing sources in the tropics and more uptake in high latitudes. We also stress the necessity of more ground-based observations and satellite data assimilation in future.
Carbonyl sulfide is an important trace gas in the atmosphere and useful to estimating gross...
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