Articles | Volume 21, issue 4
https://doi.org/10.5194/acp-21-2457-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-2457-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Sulfuric acid–amine nucleation in urban Beijing
Runlong Cai
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Dongsen Yang
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science and Technology, Nanjing, 210044, China
Rujing Yin
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science and Engineering, Fudan University, Shanghai, 200433, China
Chenjuan Deng
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Yueyun Fu
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Jiaxin Ruan
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science and Technology, Nanjing, 210044, China
Xiaoxiao Li
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Jenni Kontkanen
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Qiang Zhang
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Juha Kangasluoma
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Yan Ma
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science and Technology, Nanjing, 210044, China
Jiming Hao
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
Douglas R. Worsnop
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Aerodyne Research, Inc., Billerica, Massachusetts 01821, USA
Federico Bianchi
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Pauli Paasonen
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Veli-Matti Kerminen
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Yongchun Liu
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science and Engineering, Fudan University, Shanghai, 200433, China
Jun Zheng
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science and Technology, Nanjing, 210044, China
Markku Kulmala
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, 100029, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, 00014, Finland
Jingkun Jiang
CORRESPONDING AUTHOR
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, 100084, China
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77 citations as recorded by crossref.
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- Sulfuric acid–dimethylamine particle formation enhanced by functional organic acids: an integrated experimental and theoretical study C. Wang et al. 10.1039/D2CP01671K
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76 citations as recorded by crossref.
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- Sulfuric acid–dimethylamine particle formation enhanced by functional organic acids: an integrated experimental and theoretical study C. Wang et al. 10.1039/D2CP01671K
- Formation mechanism of typical aromatic sulfuric anhydrides and their potential role in atmospheric nucleation process H. Zhang et al. 10.1016/j.jes.2022.01.015
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- Estimates of Future New Particle Formation under Different Emission Scenarios in Beijing J. Brean et al. 10.1021/acs.est.2c08348
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- Insights into the different mixing states and formation processes of amine-containing single particles in Guangzhou, China Q. Zhong et al. 10.1016/j.scitotenv.2022.157440
- Size-resolved effective density of ambient aerosols measured by an AAC–SMPS tandem system in Beijing J. Lu et al. 10.1016/j.atmosenv.2023.120226
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- The synergistic effect of organic and inorganic sulfonic acids promotes new particle formation Y. Ji et al. 10.1016/j.scitotenv.2023.163611
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- Overlooked significance of iodic acid in new particle formation in the continental atmosphere A. Ning et al. 10.1073/pnas.2404595121
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- High contribution of new particle formation to ultrafine particles in four seasons in an urban atmosphere in south China L. Tao et al. 10.1016/j.scitotenv.2023.164202
- Significant contributions of trimethylamine to sulfuric acid nucleation in polluted environments R. Cai et al. 10.1038/s41612-023-00405-3
- The striking effect of vertical mixing in the planetary boundary layer on new particle formation in the Yangtze River Delta S. Lai et al. 10.1016/j.scitotenv.2022.154607
- The effect of COVID-19 restrictions on atmospheric new particle formation in Beijing C. Yan et al. 10.5194/acp-22-12207-2022
- A dynamic parameterization of sulfuric acid–dimethylamine nucleation and its application in three-dimensional modeling Y. Li et al. 10.5194/acp-23-8789-2023
- Emissions of Ammonia and Other Nitrogen-Containing Volatile Organic Compounds from Motor Vehicles under Low-Speed Driving Conditions D. Yang et al. 10.1021/acs.est.2c00555
- A sulfuric acid nucleation potential model for the atmosphere J. Johnson & C. Jen 10.5194/acp-22-8287-2022
- Unexpectedly significant stabilizing mechanism of iodous acid on iodic acid nucleation under different atmospheric conditions L. Liu et al. 10.1016/j.scitotenv.2022.159832
- Vigorous New Particle Formation Above Polluted Boundary Layer in the North China Plain S. Lai et al. 10.1029/2022GL100301
- Characteristics and origins of fine particulate amines at a coastal mountain site in northern China in spring M. Liu et al. 10.1016/j.atmosenv.2024.120365
- Condensation sink of atmospheric vapors: the effect of vapor properties and the resulting uncertainties S. Tuovinen et al. 10.1039/D1EA00032B
- Formation Process of Particles and Cloud Condensation Nuclei Over the Amazon Rainforest: The Role of Local and Remote New‐Particle Formation B. Zhao et al. 10.1029/2022GL100940
- Review on main sources and impacts of urban ultrafine particles: Traffic emissions, nucleation, and climate modulation Q. Li et al. 10.1016/j.aeaoa.2023.100221
- Sulfur Dioxide Transported From the Residual Layer Drives Atmospheric Nucleation During Haze Periods in Beijing Y. Wang et al. 10.1029/2022GL100514
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
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Latest update: 20 Nov 2024
Short summary
Based on long-term measurements, we discovered that the collision of H2SO4–amine clusters is the governing mechanism that initializes fast new particle formation in the polluted atmospheric environment of urban Beijing. The mechanism and the governing factors for H2SO4–amine nucleation in the polluted atmosphere are quantitatively investigated in this study.
Based on long-term measurements, we discovered that the collision of H2SO4–amine clusters is...
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