Articles | Volume 21, issue 3
https://doi.org/10.5194/acp-21-2251-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-2251-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 Feb 2021
Research article |
| 16 Feb 2021
| 16 Feb 2021
Persistent residential burning-related primary organic particles during wintertime hazes in North China: insights into their aging and optical changes
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
Jian Zhang
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
Yinxiao Zhang
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
Yuanyuan Wang
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
Liang Xu
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
Qi Yuan
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
Dantong Liu
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Pingqing Fu
Institute of Surface-Earth System Science, Tianjin University, Tianjin 300072, China
Zongbo Shi
School of Geography, Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2TT, UK
Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang University, Hangzhou 310027, China
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Cited
19 citations as recorded by crossref.
- Source apportionment of fine organic carbon at an urban site of Beijing using a chemical mass balance model J. Xu et al. 10.5194/acp-21-7321-2021
- Organic aerosol volatility and viscosity in the North China Plain: contrast between summer and winter W. Xu et al. 10.5194/acp-21-5463-2021
- Chemical composition, sources, and processes of winter haze in Chengdu, China: Insights from integrating the bulk chemical and single particle approaches J. Zhang et al. 10.1016/j.atmosenv.2024.120371
- Significant coal combustion contribution to water-soluble brown carbon during winter in Xingtai, China: Optical properties and sources D. Li et al. 10.1016/j.jes.2022.02.026
- Chemical and morphological characterization by SEM–EDS of PM2.5 collected during winter in Ulaanbaatar, Mongolia J. Park et al. 10.1016/j.atmosenv.2023.119752
- Nonlinear Enhancement of Radiative Absorption by Black Carbon in Response to Particle Mixing Structure Y. Wang et al. 10.1029/2021GL096437
- Impact of COVID-19 lockdown on the optical properties and radiative effects of urban brown carbon aerosol Y. Zhang et al. 10.1016/j.gsf.2021.101320
- Unexpected molecular diversity of brown carbon formed by Maillard-like reactions in aqueous aerosols S. Tang et al. 10.1039/D2SC02857C
- Multi-modal chemical characterization of highly viscous submicrometer organic particles A. Morales et al. 10.1080/02786826.2023.2266494
- The effects of number and mass concentration of aerosol components on scattering coefficients in Xianghe, southeast of Beijing, China – A case study J. Zou et al. 10.1016/j.atmosenv.2022.118938
- Estimation of particulate organic nitrates from thermodenuder–aerosol mass spectrometer measurements in the North China Plain W. Xu et al. 10.5194/amt-14-3693-2021
- The density of ambient black carbon retrieved by a new method: implications for cloud condensation nuclei prediction J. Ren et al. 10.5194/acp-23-4327-2023
- Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts W. Li et al. 10.1038/s41612-024-00610-8
- On the fossil and non-fossil fuel sources of carbonaceous aerosol with radiocarbon and AMS-PMF methods during winter hazy days in a rural area of North China plain Y. Zhang et al. 10.1016/j.envres.2021.112672
- Chemical composition, sources and formation mechanism of urban PM2.5 in Southwest China: a case study at the beginning of 2023 J. Zhang et al. 10.5194/acp-24-2803-2024
- Significant Contribution of Coarse Black Carbon Particles to Light Absorption in North China Plain J. Wang et al. 10.1021/acs.estlett.1c00953
- Secondary Formation of Submicron and Supermicron Organic and Inorganic Aerosols in a Highly Polluted Urban Area Y. Zheng et al. 10.1029/2022JD037865
- Measurement report: Comparison of wintertime individual particles at ground level and above the mixed layer in urban Beijing W. Wang et al. 10.5194/acp-21-5301-2021
- Morphological and optical properties of carbonaceous aerosol particles from ship emissions and biomass burning during a summer cruise measurement in the South China Sea C. Sun et al. 10.5194/acp-24-3043-2024
19 citations as recorded by crossref.
- Source apportionment of fine organic carbon at an urban site of Beijing using a chemical mass balance model J. Xu et al. 10.5194/acp-21-7321-2021
- Organic aerosol volatility and viscosity in the North China Plain: contrast between summer and winter W. Xu et al. 10.5194/acp-21-5463-2021
- Chemical composition, sources, and processes of winter haze in Chengdu, China: Insights from integrating the bulk chemical and single particle approaches J. Zhang et al. 10.1016/j.atmosenv.2024.120371
- Significant coal combustion contribution to water-soluble brown carbon during winter in Xingtai, China: Optical properties and sources D. Li et al. 10.1016/j.jes.2022.02.026
- Chemical and morphological characterization by SEM–EDS of PM2.5 collected during winter in Ulaanbaatar, Mongolia J. Park et al. 10.1016/j.atmosenv.2023.119752
- Nonlinear Enhancement of Radiative Absorption by Black Carbon in Response to Particle Mixing Structure Y. Wang et al. 10.1029/2021GL096437
- Impact of COVID-19 lockdown on the optical properties and radiative effects of urban brown carbon aerosol Y. Zhang et al. 10.1016/j.gsf.2021.101320
- Unexpected molecular diversity of brown carbon formed by Maillard-like reactions in aqueous aerosols S. Tang et al. 10.1039/D2SC02857C
- Multi-modal chemical characterization of highly viscous submicrometer organic particles A. Morales et al. 10.1080/02786826.2023.2266494
- The effects of number and mass concentration of aerosol components on scattering coefficients in Xianghe, southeast of Beijing, China – A case study J. Zou et al. 10.1016/j.atmosenv.2022.118938
- Estimation of particulate organic nitrates from thermodenuder–aerosol mass spectrometer measurements in the North China Plain W. Xu et al. 10.5194/amt-14-3693-2021
- The density of ambient black carbon retrieved by a new method: implications for cloud condensation nuclei prediction J. Ren et al. 10.5194/acp-23-4327-2023
- Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts W. Li et al. 10.1038/s41612-024-00610-8
- On the fossil and non-fossil fuel sources of carbonaceous aerosol with radiocarbon and AMS-PMF methods during winter hazy days in a rural area of North China plain Y. Zhang et al. 10.1016/j.envres.2021.112672
- Chemical composition, sources and formation mechanism of urban PM2.5 in Southwest China: a case study at the beginning of 2023 J. Zhang et al. 10.5194/acp-24-2803-2024
- Significant Contribution of Coarse Black Carbon Particles to Light Absorption in North China Plain J. Wang et al. 10.1021/acs.estlett.1c00953
- Secondary Formation of Submicron and Supermicron Organic and Inorganic Aerosols in a Highly Polluted Urban Area Y. Zheng et al. 10.1029/2022JD037865
- Measurement report: Comparison of wintertime individual particles at ground level and above the mixed layer in urban Beijing W. Wang et al. 10.5194/acp-21-5301-2021
- Morphological and optical properties of carbonaceous aerosol particles from ship emissions and biomass burning during a summer cruise measurement in the South China Sea C. Sun et al. 10.5194/acp-24-3043-2024
Latest update: 16 Apr 2024
Short summary
We found that large numbers of light-absorbing primary organic particles with high viscosity, especially tarballs, from domestic coal and biomass burning occurred in rural and even urban hazes in the winter of North China. For the first time, we characterized the atmospheric aging process of these burning-related primary organic particles by microscopic analysis and further evaluated their light absorption enhancement resulting from the “lensing effect” of secondary inorganic coatings.
We found that large numbers of light-absorbing primary organic particles with high viscosity,...
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