Articles | Volume 21, issue 21
https://doi.org/10.5194/acp-21-16093-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-16093-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Nov 2021
Research article |
| 02 Nov 2021
| 02 Nov 2021
Influence of atmospheric in-cloud aqueous-phase chemistry on the global simulation of SO2 in CESM2
Wendong Ge
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Junfeng Liu
CORRESPONDING AUTHOR
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Kan Yi
Institute of Science and Technology, China Three Gorges Corporation, Beijing 100038, China
Jiayu Xu
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Yizhou Zhang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Xiurong Hu
College of Economics and Management, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, China
Jianmin Ma
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Xuejun Wang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Yi Wan
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Jianying Hu
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Zhaobin Zhang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Xilong Wang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Shu Tao
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
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Cited
17 citations as recorded by crossref.
- A novel pathway of atmospheric sulfate formation through carbonate radicals Y. Liu et al.
- Significantly Accelerated Hydroxyl Radical Generation by Fe(III)–Oxalate Photochemistry in Aerosol Droplets L. Wang et al.
- Impacts of coal use phase-out in China on the atmospheric environment: (1) emissions, surface concentrations and exceedance of air quality standards W. Ge et al.
- Effect of cloud chemistry on seasonal variations of sulfate and its precursors in China J. Lu et al.
- Improvement and Uncertainties of Global Simulation of Sulfate Concentration and Radiative Forcing in CESM2 W. Ge et al.
- The transport, removal, and formation of aerosols by a precipitating extratropical cyclone passing the Korean Peninsula Y. Jo et al.
- The short-term comprehensive impact of the phase-out of global coal combustion on air pollution and climate change W. Ge et al.
- Elucidating the Mechanism on the Transition-Metal Ion-Synergetic-Catalyzed Oxidation of SO2 with Implications for Sulfate Formation in Beijing Haze S. Zhang et al.
- Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China J. Lu et al.
- SO2 emissions derived from TROPOMI observations over India using a flux-divergence method with variable lifetimes Y. Chen et al.
- Impacts of coal use phase-out in China on the atmospheric environment: (2) public health and global radiative forcing Y. Zhou et al.
- An oxidation flow reactor for simulating and accelerating secondary aerosol formation in aerosol liquid water and cloud droplets N. Xu et al.
- A new NMVOCs emission inventory for China: Impact on O3 and PM2.5 regional simulations and assessment of recent industrial NMVOCs emission abatement policies W. Ge et al.
- The effect of organic nucleation on the indirect radiative forcing with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs) X. Shao et al.
- Stratospheric Aerosol and Ozone Responses to the Hunga Tonga‐Hunga Ha'apai Volcanic Eruption J. Lu et al.
- Global sensitivities of reactive N and S gas and particle concentrations and deposition to precursor emissions reductions Y. Ge et al.
- Atmospheric ozonolysis of allyl sulfides: Theoretical and experimental study of kinetics and product yields in the presence and absence of an OH radical scavenger A. Cardona et al.
17 citations as recorded by crossref.
- A novel pathway of atmospheric sulfate formation through carbonate radicals Y. Liu et al.
- Significantly Accelerated Hydroxyl Radical Generation by Fe(III)–Oxalate Photochemistry in Aerosol Droplets L. Wang et al.
- Impacts of coal use phase-out in China on the atmospheric environment: (1) emissions, surface concentrations and exceedance of air quality standards W. Ge et al.
- Effect of cloud chemistry on seasonal variations of sulfate and its precursors in China J. Lu et al.
- Improvement and Uncertainties of Global Simulation of Sulfate Concentration and Radiative Forcing in CESM2 W. Ge et al.
- The transport, removal, and formation of aerosols by a precipitating extratropical cyclone passing the Korean Peninsula Y. Jo et al.
- The short-term comprehensive impact of the phase-out of global coal combustion on air pollution and climate change W. Ge et al.
- Elucidating the Mechanism on the Transition-Metal Ion-Synergetic-Catalyzed Oxidation of SO2 with Implications for Sulfate Formation in Beijing Haze S. Zhang et al.
- Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China J. Lu et al.
- SO2 emissions derived from TROPOMI observations over India using a flux-divergence method with variable lifetimes Y. Chen et al.
- Impacts of coal use phase-out in China on the atmospheric environment: (2) public health and global radiative forcing Y. Zhou et al.
- An oxidation flow reactor for simulating and accelerating secondary aerosol formation in aerosol liquid water and cloud droplets N. Xu et al.
- A new NMVOCs emission inventory for China: Impact on O3 and PM2.5 regional simulations and assessment of recent industrial NMVOCs emission abatement policies W. Ge et al.
- The effect of organic nucleation on the indirect radiative forcing with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs) X. Shao et al.
- Stratospheric Aerosol and Ozone Responses to the Hunga Tonga‐Hunga Ha'apai Volcanic Eruption J. Lu et al.
- Global sensitivities of reactive N and S gas and particle concentrations and deposition to precursor emissions reductions Y. Ge et al.
- Atmospheric ozonolysis of allyl sulfides: Theoretical and experimental study of kinetics and product yields in the presence and absence of an OH radical scavenger A. Cardona et al.
Saved (final revised paper)
Latest update: 02 May 2026
Short summary
Compared with the observations, the results incorporating detailed cloud aqueous-phase chemistry greatly reduced SO2 overestimation. The biases in annual simulated SO2 concentrations (or mixing ratios) decreased by 46 %, 41 %, and 22 % in Europe, the USA, and China, respectively. Fe chemistry and HOx chemistry contributed more to SO2 oxidation than N chemistry. Higher concentrations of soluble Fe and higher pH values could further enhance the oxidation capacity.
Compared with the observations, the results incorporating detailed cloud aqueous-phase chemistry...
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