Articles | Volume 21, issue 21
https://doi.org/10.5194/acp-21-16093-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-16093-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Nov 2021
Research article |
| 02 Nov 2021
| 02 Nov 2021
Influence of atmospheric in-cloud aqueous-phase chemistry on the global simulation of SO2 in CESM2
Wendong Ge
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Junfeng Liu
CORRESPONDING AUTHOR
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Kan Yi
Institute of Science and Technology, China Three Gorges Corporation, Beijing 100038, China
Jiayu Xu
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Yizhou Zhang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Xiurong Hu
College of Economics and Management, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, China
Jianmin Ma
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Xuejun Wang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Yi Wan
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Jianying Hu
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Zhaobin Zhang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Xilong Wang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
Shu Tao
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
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9 citations as recorded by crossref.
- A novel pathway of atmospheric sulfate formation through carbonate radicals Y. Liu et al. 10.5194/acp-22-9175-2022
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- Impacts of coal use phase-out in China on the atmospheric environment: (1) emissions, surface concentrations and exceedance of air quality standards W. Ge et al. 10.1016/j.atmosenv.2023.120163
- Impacts of coal use phase-out in China on the atmospheric environment: (2) public health and global radiative forcing Y. Zhou et al. 10.1016/j.atmosenv.2023.120280
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- Stratospheric Aerosol and Ozone Responses to the Hunga Tonga‐Hunga Ha'apai Volcanic Eruption J. Lu et al. 10.1029/2022GL102315
- Elucidating the Mechanism on the Transition-Metal Ion-Synergetic-Catalyzed Oxidation of SO2 with Implications for Sulfate Formation in Beijing Haze S. Zhang et al. 10.1021/acs.est.3c08411
- Global sensitivities of reactive N and S gas and particle concentrations and deposition to precursor emissions reductions Y. Ge et al. 10.5194/acp-23-6083-2023
- Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China J. Lu et al. 10.5194/acp-23-8021-2023
1 citations as recorded by crossref.
Latest update: 17 Jul 2024
Short summary
Compared with the observations, the results incorporating detailed cloud aqueous-phase chemistry greatly reduced SO2 overestimation. The biases in annual simulated SO2 concentrations (or mixing ratios) decreased by 46 %, 41 %, and 22 % in Europe, the USA, and China, respectively. Fe chemistry and HOx chemistry contributed more to SO2 oxidation than N chemistry. Higher concentrations of soluble Fe and higher pH values could further enhance the oxidation capacity.
Compared with the observations, the results incorporating detailed cloud aqueous-phase chemistry...
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