Articles | Volume 21, issue 21
Atmos. Chem. Phys., 21, 16093–16120, 2021
https://doi.org/10.5194/acp-21-16093-2021
Atmos. Chem. Phys., 21, 16093–16120, 2021
https://doi.org/10.5194/acp-21-16093-2021
Research article
02 Nov 2021
Research article | 02 Nov 2021

Influence of atmospheric in-cloud aqueous-phase chemistry on the global simulation of SO2 in CESM2

Wendong Ge et al.

Viewed

Total article views: 1,486 (including HTML, PDF, and XML)
HTML PDF XML Total Supplement BibTeX EndNote
1,170 296 20 1,486 98 12 18
  • HTML: 1,170
  • PDF: 296
  • XML: 20
  • Total: 1,486
  • Supplement: 98
  • BibTeX: 12
  • EndNote: 18
Views and downloads (calculated since 16 Jun 2021)
Cumulative views and downloads (calculated since 16 Jun 2021)

Viewed (geographical distribution)

Total article views: 1,492 (including HTML, PDF, and XML) Thereof 1,492 with geography defined and 0 with unknown origin.
Country # Views %
  • 1
1
 
 
 
 
Latest update: 29 Jun 2022
Download
Short summary
Compared with the observations, the results incorporating detailed cloud aqueous-phase chemistry greatly reduced SO2 overestimation. The biases in annual simulated SO2 concentrations (or mixing ratios) decreased by 46 %, 41 %, and 22 % in Europe, the USA, and China, respectively. Fe chemistry and HOx chemistry contributed more to SO2 oxidation than N chemistry. Higher concentrations of soluble Fe and higher pH values could further enhance the oxidation capacity.
Altmetrics
Final-revised paper
Preprint