the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Technical note: AQMEII4 Activity 1: evaluation of wet and dry deposition schemes as an integral part of regional-scale air quality models
Stefano Galmarini
Paul Makar
Olivia E. Clifton
Christian Hogrefe
Jesse O. Bash
Roberto Bellasio
Roberto Bianconi
Johannes Bieser
Tim Butler
Jason Ducker
Johannes Flemming
Alma Hodzic
Christopher D. Holmes
Ioannis Kioutsioukis
Richard Kranenburg
Aurelia Lupascu
Juan Luis Perez-Camanyo
Jonathan Pleim
Young-Hee Ryu
Roberto San Jose
Donna Schwede
Sam Silva
Ralf Wolke
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- Final revised paper (published on 20 Oct 2021)
- Preprint (discussion started on 12 May 2021)
Interactive discussion
Status: closed
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RC1: 'Comment on acp-2021-313', Anonymous Referee #1, 24 May 2021
General Comments
This technical note describes the research protocol for Activity 1 of AQMEII-4. AQMEII-4 has been set up to examine the deposition processes in regional air quality models with the aim of assessing differences in the models’ deposition parameterizations and how these differences impact atmospheric composition predictions. The technical note reports the models that will participate in AQMEII4 and defines a standard reporting framework for dry deposition parameters. Importantly, this technical note defines the ‘Effective Conductance’ and ‘Effective Flux’ parameter(s) and how they should be calculated so that dry deposition can be meaningfully compared across modelling systems.
This Technical Note is well written and provides a clear overview of Activity 1 as well as detailed descriptions of the calculations that will be used to compare dry deposition across the model ensemble. The Technical Note will provide a useful reference for Activity 1, bringing the technical information together in a single ‘point of reference’.
I recommend that this Technical Note is published once the following comments and technical corrections have been addressed.
Specific Comments and technical corrections
L203: It would be useful to have a figure to illustrate the European and North American domains.
L229-231: I do not understand what the authors mean by ‘hourly speciated files’. Please clarify.
L320-330: Suggested text modification from (units s cm-1) to (units = s cm-1)
Figure 3:
- The resolution of this figure is generally poor and in particular the text for the x-axes tick labels is difficult to read (in fact unintelligible for 3a and 3d). This should be improved before final publication.
- Can the authors explain why there is a smaller effective conductance for soil (and possibly lcan and cut, although it is difficult to tell from the figure) at 06:00?
Table 5: The format of this table should be improved. It might be better in landscape as all the columns could do with being a bit wider.
Tables 5 and 6: For ease of comparison, would it possible to situate Fig 2a in closer proximity to Table 5?
L524-526: ‘In this example, note that the branch containing the rdc term has been designated as the lower canopy pathway, due to the presence of the canopy buoyant convection term rdc (i.e., closest analogy to Wesely’s setup is to have the pathway involving deposition to “soil” pathway is designated as a “lower canopy” pathway).‘
=> Consider re-wording this sentence from ‘the branch containing the rdc term’ to ‘the branch representing deposition to soil’ or similar to avoid confusion about the two slightly different usages of rdc in this sentence.
Table A1: Should the units for the water vapour column be changed from cm3 cm-2 to cm3 cm-2? Units for RHO (Air density of lowest model layer)?
Table A2: Change ‘Number concentration of PM2.5at ground, cm-3' to ‘Number concentration of PM2.5 at ground, cm-3'. Units of eq ha -1?
Table A2: Could the authors please provide a description of the units eq ha -1.
Appendix tables B1 – B7: I think the formatting could be improved across these tables and importantly, made consistent. E.g. Font formatting, equation layout (for preference, the equations should be as in Table B6, represented as fractions rather than as (xxxx)-1, but consistency is the main thing). In some cases the tables may be better displayed in landscape so that equations can be presented on one line. Table B6 is nicely laid out, although the text in column one is too small to read easily.
Table B2 and B3: Should RES – SURF be RES-SURF?
Figure B3 and B4: Shold these be the same?
Appendix C, Equations 8 and 9: These are hard to decipher, please consider improving their layout
L958: Fix reference formatting for Yi (2008) and Bash et al., (2010)
Citation: https://doi.org/10.5194/acp-2021-313-RC1 - AC1: 'Comment on acp-2021-313', Stefano Galmarini, 08 Sep 2021
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RC2: 'Comment on acp-2021-313', Anonymous Referee #2, 16 Jun 2021
The Air Quality Model Evaluation International Initiative (AQMEII) aims to evaluate regional-scale air quality models used for research and regulatory applications. The fourth phase (AQMEII4) focuses on wet and dry deposition processes and their effects on model predictions and performance. A primary activity of the fourth phase is to conduct a diagnostic comparison of air quality model predictions of deposition fields and to evaluate model concentrations and wet deposition fluxes against surface observations in North America and Europe. The purpose of this technical note is to provide background information about the dry deposition schemes from the modeling systems included in the study and the protocols that will be used for their intercomparison. The technical note describes the harmonization of the spatial domains, emissions, chemical boundary conditions, and output across the modeling efforts. It provides detailed representations of the dry deposition scheme for each air quality model included in the study. It describes the use of effective conductance and effective flux as a basis for cross-comparisons of dry deposition pathways between models, as well as land use/land cover and other diagnostics reported for each model. The technical note is well written and will be an important resource of background material for future publications of AQMEII results. I highly recommend publication with consideration of the following:
- Versions and references for the modeling systems should be identified in Table 1.
- Maps of the European, North American, and combined domains should be added.
- Please explain what is meant in lines 194-196 on page 7 regarding “past use in policy-relevant emissions scenario simulation, with changes in emissions policies that may affect the deposition”.
- It would be helpful to know which emissions models were used, not only the source of the data, i.e., 2011v6.3 and 2016 beta, in the unified approach for forest fire emissions in North America and Canada.
- In lines 338-346 on page 13, consider summarizing and briefly explaining some of the key motivating factors that have led to the development of different resistance frameworks. For example, is it the evolution of measurement systems, availability of observational data, inclusion of missing deposition pathways, etc.
- Please describe the characteristics that are used to guide the mapping to each generic land use/land cover category. For example, what are the definitions of mixed forest or herbaceous cover?
- Check the references as well as the definitions of variables in Appendix B (which should be at the first instance) for completeness.
Citation: https://doi.org/10.5194/acp-2021-313-RC2 - AC3: 'Comment on acp-2021-313', Stefano Galmarini, 08 Sep 2021