Articles | Volume 21, issue 3
https://doi.org/10.5194/acp-21-1565-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-1565-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| Highlight paper
| 
04 Feb 2021
Research article | Highlight paper |
| 04 Feb 2021
| 04 Feb 2021
Mass accommodation and gas–particle partitioning in secondary organic aerosols: dependence on diffusivity, volatility, particle-phase reactions, and penetration depth
Department of Chemistry, University of California, Irvine, CA 92697, USA
Multiphase Chemistry Department, Max Planck Institute for Chemistry,
55128 Mainz, Germany
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Cited
32 citations as recorded by crossref.
- Phase State, Surface Tension, Water Activity, and Accommodation Coefficient of Water–Organic Clusters Near the Critical Size for Atmospheric New Particle Formation X. Li & I. Bourg 10.1021/acs.est.2c09627
- The persistence of smoke VOCs indoors: Partitioning, surface cleaning, and air cleaning in a smoke-contaminated house J. Li et al. 10.1126/sciadv.adh8263
- Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics D. Knopf et al. 10.5194/acp-24-3445-2024
- Simulated phase state and viscosity of secondary organic aerosols over China Z. Zhang et al. 10.5194/acp-24-4809-2024
- Evaluating BC Aging Processes in the Community Atmosphere Model Version 6 (CAM6) W. Shen et al. 10.1029/2022JD037427
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Secondary organic aerosols derived from intermediate-volatility n-alkanes adopt low-viscous phase state T. Galeazzo et al. 10.5194/acp-24-5549-2024
- Technical note: Adsorption and desorption equilibria from statistical thermodynamics and rates from transition state theory D. Knopf & M. Ammann 10.5194/acp-21-15725-2021
- Estimation of secondary organic aerosol viscosity from explicit modeling of gas-phase oxidation of isoprene and <i>α</i>-pinene T. Galeazzo et al. 10.5194/acp-21-10199-2021
- Microphysics of liquid water in sub-10 nm ultrafine aerosol particles X. Li & I. Bourg 10.5194/acp-23-2525-2023
- The relative humidity-dependent viscosity of single quasi aerosol particles and possible implications for atmospheric aerosol chemistry Y. Tong et al. 10.1039/D2CP00740A
- Unexpected concentration dependence of the mass accommodation coefficient of water on aqueous triethylene glycol droplets M. Gleichweit et al. 10.1039/D4CP00966E
- Molecular-Level Study of the Photo-Oxidation of Aqueous-Phase Guaiacyl Acetone in the Presence of 3C*: Formation of Brown Carbon Products M. Misovich et al. 10.1021/acsearthspacechem.1c00103
- Applying a Phase-Separation Parameterization in Modeling Secondary Organic Aerosol Formation from Acid-Driven Reactive Uptake of Isoprene Epoxydiols under Humid Conditions Y. Chen et al. 10.1021/acsestair.4c00002
- Measurement report: Water diffusion in single suspended phase-separated aerosols Y. Tong et al. 10.5194/acp-24-2937-2024
- Volatility distribution of primary organic aerosol emissions from household crop waste combustion in China P. Chen et al. 10.1016/j.envpol.2023.121353
- Molecular-scale description of interfacial mass transfer in phase-separated aqueous secondary organic aerosol M. Lbadaoui-Darvas et al. 10.5194/acp-21-17687-2021
- How should we define an indoor surface? J. Abbatt et al. 10.1111/ina.12955
- Oxidation of Phenolic Aldehydes by Ozone and Hydroxyl Radicals at the Air–Solid Interface M. Rana & M. Guzman 10.1021/acsearthspacechem.2c00206
- A kinetic partitioning method for simulating the condensation mass flux of organic vapors in a wide volatility range Y. Li et al. 10.1016/j.jaerosci.2024.106400
- Species-specific effect of particle viscosity and particle-phase reactions on the formation of secondary organic aerosol Z. Luo et al. 10.1016/j.scitotenv.2024.175207
- Effective mass accommodation for partitioning of organic compounds into surface films with different viscosities P. Lakey et al. 10.1039/D3EM00213F
- The Significant Role of New Particle Composition and Morphology on the HNO3-Driven Growth of Particles down to Sub-10 nm Y. Li et al. 10.1021/acs.est.3c09454
- Effects of Nitrogen Oxides on the Production of Reactive Oxygen Species and Environmentally Persistent Free Radicals from α-Pinene and Naphthalene Secondary Organic Aerosols K. Edwards et al. 10.1021/acs.jpca.2c05532
- Composition of indoor organic surface films in residences: simulating the influence of sources, partitioning, particle deposition, and air exchange B. Cummings et al. 10.1039/D3EM00399J
- Humidity Dependence of the Condensational Growth of α-Pinene Secondary Organic Aerosol Particles Y. Qin et al. 10.1021/acs.est.1c01738
- Insufficient Condensable Organic Vapors Lead to Slow Growth of New Particles in an Urban Environment X. Li et al. 10.1021/acs.est.2c01566
- Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Y. Li et al. 10.1021/acsearthspacechem.1c00094
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al. 10.1021/acs.est.2c06377
- Kinetic multilayer models for surface chemistry in indoor environments P. Lakey & M. Shiraiwa 10.1039/D4EM00549J
- Heterogeneous Nucleation Drives Particle Size Segregation in Sequential Ozone and Nitrate Radical Oxidation of Catechol L. Garofalo et al. 10.1021/acs.est.1c02984
- Phase state of organic aerosols may limit temperature-driven thermodynamic repartitioning following outdoor-to-indoor transport B. Cummings et al. 10.1039/D2EM00093H
31 citations as recorded by crossref.
- Phase State, Surface Tension, Water Activity, and Accommodation Coefficient of Water–Organic Clusters Near the Critical Size for Atmospheric New Particle Formation X. Li & I. Bourg 10.1021/acs.est.2c09627
- The persistence of smoke VOCs indoors: Partitioning, surface cleaning, and air cleaning in a smoke-contaminated house J. Li et al. 10.1126/sciadv.adh8263
- Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics D. Knopf et al. 10.5194/acp-24-3445-2024
- Simulated phase state and viscosity of secondary organic aerosols over China Z. Zhang et al. 10.5194/acp-24-4809-2024
- Evaluating BC Aging Processes in the Community Atmosphere Model Version 6 (CAM6) W. Shen et al. 10.1029/2022JD037427
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Secondary organic aerosols derived from intermediate-volatility n-alkanes adopt low-viscous phase state T. Galeazzo et al. 10.5194/acp-24-5549-2024
- Technical note: Adsorption and desorption equilibria from statistical thermodynamics and rates from transition state theory D. Knopf & M. Ammann 10.5194/acp-21-15725-2021
- Estimation of secondary organic aerosol viscosity from explicit modeling of gas-phase oxidation of isoprene and <i>α</i>-pinene T. Galeazzo et al. 10.5194/acp-21-10199-2021
- Microphysics of liquid water in sub-10 nm ultrafine aerosol particles X. Li & I. Bourg 10.5194/acp-23-2525-2023
- The relative humidity-dependent viscosity of single quasi aerosol particles and possible implications for atmospheric aerosol chemistry Y. Tong et al. 10.1039/D2CP00740A
- Unexpected concentration dependence of the mass accommodation coefficient of water on aqueous triethylene glycol droplets M. Gleichweit et al. 10.1039/D4CP00966E
- Molecular-Level Study of the Photo-Oxidation of Aqueous-Phase Guaiacyl Acetone in the Presence of 3C*: Formation of Brown Carbon Products M. Misovich et al. 10.1021/acsearthspacechem.1c00103
- Applying a Phase-Separation Parameterization in Modeling Secondary Organic Aerosol Formation from Acid-Driven Reactive Uptake of Isoprene Epoxydiols under Humid Conditions Y. Chen et al. 10.1021/acsestair.4c00002
- Measurement report: Water diffusion in single suspended phase-separated aerosols Y. Tong et al. 10.5194/acp-24-2937-2024
- Volatility distribution of primary organic aerosol emissions from household crop waste combustion in China P. Chen et al. 10.1016/j.envpol.2023.121353
- Molecular-scale description of interfacial mass transfer in phase-separated aqueous secondary organic aerosol M. Lbadaoui-Darvas et al. 10.5194/acp-21-17687-2021
- How should we define an indoor surface? J. Abbatt et al. 10.1111/ina.12955
- Oxidation of Phenolic Aldehydes by Ozone and Hydroxyl Radicals at the Air–Solid Interface M. Rana & M. Guzman 10.1021/acsearthspacechem.2c00206
- A kinetic partitioning method for simulating the condensation mass flux of organic vapors in a wide volatility range Y. Li et al. 10.1016/j.jaerosci.2024.106400
- Species-specific effect of particle viscosity and particle-phase reactions on the formation of secondary organic aerosol Z. Luo et al. 10.1016/j.scitotenv.2024.175207
- Effective mass accommodation for partitioning of organic compounds into surface films with different viscosities P. Lakey et al. 10.1039/D3EM00213F
- The Significant Role of New Particle Composition and Morphology on the HNO3-Driven Growth of Particles down to Sub-10 nm Y. Li et al. 10.1021/acs.est.3c09454
- Effects of Nitrogen Oxides on the Production of Reactive Oxygen Species and Environmentally Persistent Free Radicals from α-Pinene and Naphthalene Secondary Organic Aerosols K. Edwards et al. 10.1021/acs.jpca.2c05532
- Composition of indoor organic surface films in residences: simulating the influence of sources, partitioning, particle deposition, and air exchange B. Cummings et al. 10.1039/D3EM00399J
- Humidity Dependence of the Condensational Growth of α-Pinene Secondary Organic Aerosol Particles Y. Qin et al. 10.1021/acs.est.1c01738
- Insufficient Condensable Organic Vapors Lead to Slow Growth of New Particles in an Urban Environment X. Li et al. 10.1021/acs.est.2c01566
- Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Y. Li et al. 10.1021/acsearthspacechem.1c00094
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al. 10.1021/acs.est.2c06377
- Kinetic multilayer models for surface chemistry in indoor environments P. Lakey & M. Shiraiwa 10.1039/D4EM00549J
- Heterogeneous Nucleation Drives Particle Size Segregation in Sequential Ozone and Nitrate Radical Oxidation of Catechol L. Garofalo et al. 10.1021/acs.est.1c02984
Latest update: 20 Nov 2024
Short summary
Mass accommodation is a crucial process in secondary organic aerosol partitioning that depends on volatility, diffusivity, reactivity, and particle penetration depth of the chemical species involved. For efficient kinetic modeling, we introduce an effective mass accommodation coefficient that accounts for the above influencing factors, can be applied in the common Fuchs–Sutugin approximation, and helps to resolve inconsistencies and shortcomings of earlier experimental and model investigations.
Mass accommodation is a crucial process in secondary organic aerosol partitioning that depends...
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