Articles | Volume 21, issue 19
https://doi.org/10.5194/acp-21-14983-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-14983-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
ACP Letters
| Highlight paper
| 
15 Oct 2021
ACP Letters | Highlight paper |
| 15 Oct 2021
| 15 Oct 2021
How alkaline compounds control atmospheric aerosol particle acidity
Vlassis A. Karydis
CORRESPONDING AUTHOR
Atmospheric Chemistry Dept., Max Planck Institute for Chemistry,
Mainz 55128, Germany
Inst. for Energy and Climate Research, IEK-8, Forschungszentrum Jülich, Jülich 52425, Germany
Alexandra P. Tsimpidi
Atmospheric Chemistry Dept., Max Planck Institute for Chemistry,
Mainz 55128, Germany
Inst. for Energy and Climate Research, IEK-8, Forschungszentrum Jülich, Jülich 52425, Germany
Inst. for Environmental Research and Sustainable Development, National Observatory of Athens, Athens, 15236, Greece
Andrea Pozzer
Atmospheric Chemistry Dept., Max Planck Institute for Chemistry,
Mainz 55128, Germany
International Centre for Theoretical Physics, Trieste, 34151, Italy
Jos Lelieveld
Atmospheric Chemistry Dept., Max Planck Institute for Chemistry,
Mainz 55128, Germany
The Cyprus Institute, Climate and Atmosphere Research Center,
Nicosia, 1645, Cyprus
Viewed
Total article views: 5,177 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 22 Dec 2020)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 3,912 | 1,187 | 78 | 5,177 | 301 | 64 | 117 |
- HTML: 3,912
- PDF: 1,187
- XML: 78
- Total: 5,177
- Supplement: 301
- BibTeX: 64
- EndNote: 117
Total article views: 4,355 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 15 Oct 2021)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 3,541 | 739 | 75 | 4,355 | 182 | 60 | 103 |
- HTML: 3,541
- PDF: 739
- XML: 75
- Total: 4,355
- Supplement: 182
- BibTeX: 60
- EndNote: 103
Total article views: 822 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 22 Dec 2020)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 371 | 448 | 3 | 822 | 119 | 4 | 14 |
- HTML: 371
- PDF: 448
- XML: 3
- Total: 822
- Supplement: 119
- BibTeX: 4
- EndNote: 14
Viewed (geographical distribution)
Total article views: 5,177 (including HTML, PDF, and XML)
Thereof 5,238 with geography defined
and -61 with unknown origin.
Total article views: 4,355 (including HTML, PDF, and XML)
Thereof 4,315 with geography defined
and 40 with unknown origin.
Total article views: 822 (including HTML, PDF, and XML)
Thereof 923 with geography defined
and -101 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
28 citations as recorded by crossref.
- Multiphase processes in the EC-Earth model and their relevance to the atmospheric oxalate, sulfate, and iron cycles S. Myriokefalitakis et al. 10.5194/gmd-15-3079-2022
- Perspective about gasoline soot combustion over ceria catalysts: A close look into the “active oxygen” enigma Z. Tu et al. 10.1016/j.jre.2024.08.017
- Summertime Airborne Measurements of Ammonia Emissions From Cattle Feedlots and Dairies in Northeastern Colorado J. Juncosa Calahorrano et al. 10.1029/2023JD039043
- Ph Modifies the Oxidative Potential and Peroxide Content of Biomass Burning Hulis Under Dark Aging C. Li et al. 10.2139/ssrn.4045471
- Field Evidence for Constraints of Nearly Dry and Weakly Acidic Aerosol Conditions on the Formation of Organosulfates T. Yang et al. 10.1021/acs.estlett.4c00522
- Mineral dust aerosol impacts on global climate and climate change J. Kok et al. 10.1038/s43017-022-00379-5
- Sources, Variations, and Effects on Air Quality of Atmospheric Ammonia Z. Lan et al. 10.1007/s40726-023-00291-6
- pH modifies the oxidative potential and peroxide content of biomass burning HULIS under dark aging C. Li et al. 10.1016/j.scitotenv.2022.155365
- An improved representation of aerosol in the ECMWF IFS-COMPO 49R1 through the integration of EQSAM4Climv12 – a first attempt at simulating aerosol acidity S. Rémy et al. 10.5194/gmd-17-7539-2024
- Rising Alkali-to-Acid Ratios in the Atmosphere May Correspond to Increased Aerosol Acidity G. Zheng et al. 10.1021/acs.est.4c06860
- Implementation of the ISORROPIA-lite aerosol thermodynamics model into the EMAC chemistry climate model (based on MESSy v2.55): implications for aerosol composition and acidity A. Milousis et al. 10.5194/gmd-17-1111-2024
- Acidity in rainwater and airborne suspended particles in the southwestern coast of the East Sea (Sea of Japan): Their potential impact on seawater total alkalinity G. Park et al. 10.1016/j.marpolbul.2023.115742
- Atmospheric NH3 in urban Beijing: long-term variations and implications for secondary inorganic aerosol control Z. Lan et al. 10.5194/acp-24-9355-2024
- Deciphering the key drivers of oxidative potential during ammonium nitrate-mediated aqueous-phase photoreaction of methoxyphenols R. Lai et al. 10.1016/j.atmosenv.2024.120895
- Characteristics of aerosol chemistry and acidity in Shanghai after PM2.5 satisfied national guideline: Insight into future emission control Z. Fu et al. 10.1016/j.scitotenv.2022.154319
- Unanswered questions on the airborne transmission of COVID-19 Z. Gu et al. 10.1007/s10311-022-01557-z
- Quantitative Decomposition of Influencing Factors to Aerosol pH Variation over the Coasts of the South China Sea, East China Sea, and Bohai Sea G. Wang et al. 10.1021/acs.estlett.2c00527
- Seasonal variation and sources of PM2.5 bound water‐soluble ions at Jammu city in the foothills of the North‐western Himalayas, India S. Gupta et al. 10.1002/gj.4835
- Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain Y. Liu et al. 10.1038/s41467-022-34733-4
- A fingerprint of source-specific health risk of PM2.5-bound components over a coastal industrial city J. dos Santos Silva et al. 10.1016/j.jhazmat.2024.136369
- Simulations of aerosol pH in China using WRF-Chem (v4.0): sensitivities of aerosol pH and its temporal variations during haze episodes X. Ruan et al. 10.5194/gmd-15-6143-2022
- A central arctic extreme aerosol event triggered by a warm air-mass intrusion L. Dada et al. 10.1038/s41467-022-32872-2
- Quantitative analysis of influencing factors to aerosol pH and its responses to PM2.5 and O3 pollution in a coastal city K. Xu et al. 10.1016/j.jes.2024.03.044
- Elucidating Decade-Long Trends and Diurnal Patterns in Aerosol Acidity in Shanghai Z. Lv et al. 10.3390/atmos15081004
- Review of health effects driven by aerosol acidity: Occurrence and implications for air pollution control X. Song et al. 10.1016/j.scitotenv.2024.176839
- Sources, Ionic Composition and Acidic Properties of Bulk and Wet Atmospheric Deposition in the Eastern Middle Adriatic Region V. Gluščić et al. 10.3390/toxics11070551
- Direct Observation of Particle-To-Particle Variability in Ambient Aerosol pH Using a Novel Analytical Approach Based on Surface-Enhanced Raman Spectroscopy H. Yoo et al. 10.1021/acs.est.4c00220
- Impacts of the East Asia Monsoon on the PM2.5 Acidity in Hanoi P. Hien et al. 10.1016/j.apr.2024.102304
27 citations as recorded by crossref.
- Multiphase processes in the EC-Earth model and their relevance to the atmospheric oxalate, sulfate, and iron cycles S. Myriokefalitakis et al. 10.5194/gmd-15-3079-2022
- Perspective about gasoline soot combustion over ceria catalysts: A close look into the “active oxygen” enigma Z. Tu et al. 10.1016/j.jre.2024.08.017
- Summertime Airborne Measurements of Ammonia Emissions From Cattle Feedlots and Dairies in Northeastern Colorado J. Juncosa Calahorrano et al. 10.1029/2023JD039043
- Ph Modifies the Oxidative Potential and Peroxide Content of Biomass Burning Hulis Under Dark Aging C. Li et al. 10.2139/ssrn.4045471
- Field Evidence for Constraints of Nearly Dry and Weakly Acidic Aerosol Conditions on the Formation of Organosulfates T. Yang et al. 10.1021/acs.estlett.4c00522
- Mineral dust aerosol impacts on global climate and climate change J. Kok et al. 10.1038/s43017-022-00379-5
- Sources, Variations, and Effects on Air Quality of Atmospheric Ammonia Z. Lan et al. 10.1007/s40726-023-00291-6
- pH modifies the oxidative potential and peroxide content of biomass burning HULIS under dark aging C. Li et al. 10.1016/j.scitotenv.2022.155365
- An improved representation of aerosol in the ECMWF IFS-COMPO 49R1 through the integration of EQSAM4Climv12 – a first attempt at simulating aerosol acidity S. Rémy et al. 10.5194/gmd-17-7539-2024
- Rising Alkali-to-Acid Ratios in the Atmosphere May Correspond to Increased Aerosol Acidity G. Zheng et al. 10.1021/acs.est.4c06860
- Implementation of the ISORROPIA-lite aerosol thermodynamics model into the EMAC chemistry climate model (based on MESSy v2.55): implications for aerosol composition and acidity A. Milousis et al. 10.5194/gmd-17-1111-2024
- Acidity in rainwater and airborne suspended particles in the southwestern coast of the East Sea (Sea of Japan): Their potential impact on seawater total alkalinity G. Park et al. 10.1016/j.marpolbul.2023.115742
- Atmospheric NH3 in urban Beijing: long-term variations and implications for secondary inorganic aerosol control Z. Lan et al. 10.5194/acp-24-9355-2024
- Deciphering the key drivers of oxidative potential during ammonium nitrate-mediated aqueous-phase photoreaction of methoxyphenols R. Lai et al. 10.1016/j.atmosenv.2024.120895
- Characteristics of aerosol chemistry and acidity in Shanghai after PM2.5 satisfied national guideline: Insight into future emission control Z. Fu et al. 10.1016/j.scitotenv.2022.154319
- Unanswered questions on the airborne transmission of COVID-19 Z. Gu et al. 10.1007/s10311-022-01557-z
- Quantitative Decomposition of Influencing Factors to Aerosol pH Variation over the Coasts of the South China Sea, East China Sea, and Bohai Sea G. Wang et al. 10.1021/acs.estlett.2c00527
- Seasonal variation and sources of PM2.5 bound water‐soluble ions at Jammu city in the foothills of the North‐western Himalayas, India S. Gupta et al. 10.1002/gj.4835
- Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain Y. Liu et al. 10.1038/s41467-022-34733-4
- A fingerprint of source-specific health risk of PM2.5-bound components over a coastal industrial city J. dos Santos Silva et al. 10.1016/j.jhazmat.2024.136369
- Simulations of aerosol pH in China using WRF-Chem (v4.0): sensitivities of aerosol pH and its temporal variations during haze episodes X. Ruan et al. 10.5194/gmd-15-6143-2022
- A central arctic extreme aerosol event triggered by a warm air-mass intrusion L. Dada et al. 10.1038/s41467-022-32872-2
- Quantitative analysis of influencing factors to aerosol pH and its responses to PM2.5 and O3 pollution in a coastal city K. Xu et al. 10.1016/j.jes.2024.03.044
- Elucidating Decade-Long Trends and Diurnal Patterns in Aerosol Acidity in Shanghai Z. Lv et al. 10.3390/atmos15081004
- Review of health effects driven by aerosol acidity: Occurrence and implications for air pollution control X. Song et al. 10.1016/j.scitotenv.2024.176839
- Sources, Ionic Composition and Acidic Properties of Bulk and Wet Atmospheric Deposition in the Eastern Middle Adriatic Region V. Gluščić et al. 10.3390/toxics11070551
- Direct Observation of Particle-To-Particle Variability in Ambient Aerosol pH Using a Novel Analytical Approach Based on Surface-Enhanced Raman Spectroscopy H. Yoo et al. 10.1021/acs.est.4c00220
1 citations as recorded by crossref.
Latest update: 13 Dec 2024
Short summary
Aerosol particle pH is well-buffered by alkaline compounds, notably NH3 and crustal elements. NH3 is found to supply remarkable buffering capacity on a global scale, from the polluted continents to the remote oceans. Potential future changes in agricultural NH3 must be accompanied by strong reductions of SO2 and NOx to avoid particles becoming highly acidic, with implications for human health (aerosol toxicity), ecosystems (acid deposition), clouds, and climate (aerosol hygroscopicity).
Aerosol particle pH is well-buffered by alkaline compounds, notably NH3 and crustal elements....
Altmetrics
Final-revised paper
Preprint