Articles | Volume 21, issue 19
https://doi.org/10.5194/acp-21-14907-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-14907-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Oct 2021
Research article |
| 07 Oct 2021
| 07 Oct 2021
Photolytically induced changes in composition and volatility of biogenic secondary organic aerosol from nitrate radical oxidation during night-to-day transition
Cheng Wu
Department of Environmental Science, Stockholm University, Stockholm, Sweden
David M. Bell
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Emelie L. Graham
Department of Environmental Science, Stockholm University, Stockholm, Sweden
Sophie Haslett
Department of Environmental Science, Stockholm University, Stockholm, Sweden
Ilona Riipinen
Department of Environmental Science, Stockholm University, Stockholm, Sweden
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Amelie Bertrand
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Stamatios Giannoukos
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
now at: Department of Chemistry and Applied Biosciences, ETH Zurich, Zurich, Switzerland
Janne Schoonbaert
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Imad El Haddad
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Andre S. H. Prevot
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Wei Huang
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Department of Environmental Science, Stockholm University, Stockholm, Sweden
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Cited
15 citations as recorded by crossref.
- Particle-phase processing of α-pinene NO3 secondary organic aerosol in the dark D. Bell et al. 10.5194/acp-22-13167-2022
- The important contribution of secondary formation and biomass burning to oxidized organic nitrogen (OON) in a polluted urban area: insights from in situ measurements of a chemical ionization mass spectrometer (CIMS) Y. Cai et al. 10.5194/acp-23-8855-2023
- Contrasting Influence of Nitrogen Oxides on the Cloud Condensation Nuclei Activity of Monoterpene‐Derived Secondary Organic Aerosol in Daytime and Nighttime Oxidation C. Zhang et al. 10.1029/2022GL102110
- Time-Resolved Molecular Characterization of Secondary Organic Aerosol Formed from OH and NO3Radical Initiated Oxidation of a Mixture of Aromatic Precursors V. Kumar et al. 10.1021/acs.est.3c00225
- Sensitivity Constraints of Extractive Electrospray for a Model System and Secondary Organic Aerosol D. Bell et al. 10.1021/acs.analchem.3c00441
- Variation in chemical composition and volatility of oxygenated organic aerosol in different rural, urban, and mountain environments W. Huang et al. 10.5194/acp-24-2607-2024
- Sources of organic gases and aerosol particles and their roles in nighttime particle growth at a rural forested site in southwest Germany J. Song et al. 10.5194/acp-24-6699-2024
- Identification of highly oxygenated organic molecules and their role in aerosol formation in the reaction of limonene with nitrate radical Y. Guo et al. 10.5194/acp-22-11323-2022
- Volatility of aerosol particles from NO3 oxidation of various biogenic organic precursors E. Graham et al. 10.5194/acp-23-7347-2023
- Effects of Relative Humidity and Photoaging on the Formation, Composition, and Aging of Ethylbenzene SOA: Insights from Chamber Experiments on Chlorine Radical-Initiated Oxidation of Ethylbenzene L. Jahn et al. 10.1021/acsearthspacechem.3c00279
- Bidirectional selection of the functional properties and environmental friendliness of organophosphorus (OP) pesticide derivatives: Design, screening, and mechanism analysis Z. Wang et al. 10.1016/j.scitotenv.2023.163043
- Kinetics, SOA yields, and chemical composition of secondary organic aerosol from <i>β</i>-caryophyllene ozonolysis with and without nitrogen oxides between 213 and 313 K L. Gao et al. 10.5194/acp-22-6001-2022
- An experimental study of the reactivity of terpinolene and <i>β</i>-caryophyllene with the nitrate radical A. Fouqueau et al. 10.5194/acp-22-6411-2022
- Products and Mechanisms of Secondary Organic Aerosol Formation from the NO3 Radical-Initiated Oxidation of Cyclic and Acyclic Monoterpenes M. DeVault et al. 10.1021/acsearthspacechem.2c00130
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
15 citations as recorded by crossref.
- Particle-phase processing of α-pinene NO3 secondary organic aerosol in the dark D. Bell et al. 10.5194/acp-22-13167-2022
- The important contribution of secondary formation and biomass burning to oxidized organic nitrogen (OON) in a polluted urban area: insights from in situ measurements of a chemical ionization mass spectrometer (CIMS) Y. Cai et al. 10.5194/acp-23-8855-2023
- Contrasting Influence of Nitrogen Oxides on the Cloud Condensation Nuclei Activity of Monoterpene‐Derived Secondary Organic Aerosol in Daytime and Nighttime Oxidation C. Zhang et al. 10.1029/2022GL102110
- Time-Resolved Molecular Characterization of Secondary Organic Aerosol Formed from OH and NO3Radical Initiated Oxidation of a Mixture of Aromatic Precursors V. Kumar et al. 10.1021/acs.est.3c00225
- Sensitivity Constraints of Extractive Electrospray for a Model System and Secondary Organic Aerosol D. Bell et al. 10.1021/acs.analchem.3c00441
- Variation in chemical composition and volatility of oxygenated organic aerosol in different rural, urban, and mountain environments W. Huang et al. 10.5194/acp-24-2607-2024
- Sources of organic gases and aerosol particles and their roles in nighttime particle growth at a rural forested site in southwest Germany J. Song et al. 10.5194/acp-24-6699-2024
- Identification of highly oxygenated organic molecules and their role in aerosol formation in the reaction of limonene with nitrate radical Y. Guo et al. 10.5194/acp-22-11323-2022
- Volatility of aerosol particles from NO3 oxidation of various biogenic organic precursors E. Graham et al. 10.5194/acp-23-7347-2023
- Effects of Relative Humidity and Photoaging on the Formation, Composition, and Aging of Ethylbenzene SOA: Insights from Chamber Experiments on Chlorine Radical-Initiated Oxidation of Ethylbenzene L. Jahn et al. 10.1021/acsearthspacechem.3c00279
- Bidirectional selection of the functional properties and environmental friendliness of organophosphorus (OP) pesticide derivatives: Design, screening, and mechanism analysis Z. Wang et al. 10.1016/j.scitotenv.2023.163043
- Kinetics, SOA yields, and chemical composition of secondary organic aerosol from <i>β</i>-caryophyllene ozonolysis with and without nitrogen oxides between 213 and 313 K L. Gao et al. 10.5194/acp-22-6001-2022
- An experimental study of the reactivity of terpinolene and <i>β</i>-caryophyllene with the nitrate radical A. Fouqueau et al. 10.5194/acp-22-6411-2022
- Products and Mechanisms of Secondary Organic Aerosol Formation from the NO3 Radical-Initiated Oxidation of Cyclic and Acyclic Monoterpenes M. DeVault et al. 10.1021/acsearthspacechem.2c00130
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
Latest update: 29 Jun 2024
Short summary
Night-time reactions of biogenic volatile organic compounds and nitrate radicals can lead to the formation of secondary organic aerosol (BSOANO3). Here, we study the impacts of light exposure on the BSOANO3 from three biogenic precursors. Our results suggest that photolysis causes photodegradation of a substantial fraction of BSOANO3, changes the chemical composition and bulk volatility, and might be a potentially important loss pathway of BSOANO3 during the night-to-day transition.
Night-time reactions of biogenic volatile organic compounds and nitrate radicals can lead to the...
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