Articles | Volume 21, issue 17
https://doi.org/10.5194/acp-21-13187-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-13187-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Chemical composition, optical properties, and oxidative potential of water- and methanol-soluble organic compounds emitted from the combustion of biomass materials and coal
Tao Cao
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Meiju Li
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Chunlin Zou
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Xingjun Fan
College of Resource and Environment, Anhui Science and Technology
University, Anhui 233100, China
Jianzhong Song
CORRESPONDING AUTHOR
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution
and Control, Guangzhou 510640, China
Wanglu Jia
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Chiling Yu
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Zhiqiang Yu
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Ping'an Peng
State Key Laboratory of Organic Geochemistry and Guangdong Provincial
Key Laboratory of Environmental Protection and Resources Utilization,
Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou
510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution
and Control, Guangzhou 510640, China
Viewed
Total article views: 3,937 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 23 Feb 2021)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
2,749 | 1,110 | 78 | 3,937 | 375 | 36 | 88 |
- HTML: 2,749
- PDF: 1,110
- XML: 78
- Total: 3,937
- Supplement: 375
- BibTeX: 36
- EndNote: 88
Total article views: 3,016 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 06 Sep 2021)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
2,247 | 708 | 61 | 3,016 | 242 | 33 | 78 |
- HTML: 2,247
- PDF: 708
- XML: 61
- Total: 3,016
- Supplement: 242
- BibTeX: 33
- EndNote: 78
Total article views: 921 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 23 Feb 2021)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
502 | 402 | 17 | 921 | 133 | 3 | 10 |
- HTML: 502
- PDF: 402
- XML: 17
- Total: 921
- Supplement: 133
- BibTeX: 3
- EndNote: 10
Viewed (geographical distribution)
Total article views: 3,937 (including HTML, PDF, and XML)
Thereof 3,920 with geography defined
and 17 with unknown origin.
Total article views: 3,016 (including HTML, PDF, and XML)
Thereof 3,007 with geography defined
and 9 with unknown origin.
Total article views: 921 (including HTML, PDF, and XML)
Thereof 913 with geography defined
and 8 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
38 citations as recorded by crossref.
- Molecular-level transformations of biomass burning-derived water-soluble organic carbon during dark aqueous OH oxidation: Insights from absorption, fluorescence, high-performance size exclusion chromatography and high-resolution mass spectrometry analysis X. Fan et al. 10.1016/j.scitotenv.2023.169290
- NMR spectroscopic applications to atmospheric organic aerosol analysis – Part 2: A review of existing methodologies and perspectives E. Tagliavini et al. 10.1016/j.trac.2024.117595
- The complexation of atmospheric Brown carbon surrogates on the generation of hydroxyl radical from transition metals in simulated lung fluid Y. Lyu et al. 10.1016/j.envint.2023.108240
- Key toxic components and sources affecting oxidative potential of atmospheric particulate matter using interpretable machine learning: Insights from fog episodes R. Li et al. 10.1016/j.jhazmat.2023.133175
- Molecular-level insights into the temperature-dependent formation dynamics and mechanism of water-soluble dissolved organic carbon derived from biomass pyrolysis smoke T. Li et al. 10.1016/j.watres.2024.121176
- Comparison of water-soluble and water-insoluble organic compositions attributing to different light absorption efficiency between residential coal and biomass burning emissions L. Zhang et al. 10.5194/acp-24-6323-2024
- Optical properties, molecular characterizations, and oxidative potentials of different polarity levels of water-soluble organic matters in winter PM2.5 in six China's megacities T. Zhang et al. 10.1016/j.scitotenv.2022.158600
- Variabilities in Primary N-Containing Aromatic Compound Emissions from Residential Solid Fuel Combustion and Implications for Source Tracers L. Zhang et al. 10.1021/acs.est.2c03000
- Source profiles of molecular structure and light absorption of PM2.5 brown carbon from residential coal combustion emission in Northwestern China Q. Zhang et al. 10.1016/j.envpol.2022.118866
- Connecting oxidative potential with organic carbon molecule composition and source-specific apportionment in PM2.5 in Xi'an, China Y. Luo et al. 10.1016/j.atmosenv.2023.119808
- Molecular compositions and optical properties of water-soluble brown carbon during the autumn and winter in Guangzhou, China T. He et al. 10.1016/j.atmosenv.2022.119573
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- Deconvolving light absorption properties and influencing factors of carbonaceous aerosol in Shanghai Y. Zhou et al. 10.1016/j.scitotenv.2022.156280
- Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China Y. Luo et al. 10.1016/j.scitotenv.2023.168273
- Compositional and optical characteristics of aqueous brown carbon and HULIS in the eastern Indo-Gangetic Plain using a coupled EEM PARAFAC, FT-IR and 1H NMR approach S. Dey & S. Sarkar 10.1016/j.scitotenv.2024.171084
- Exploring the relationship between personal exposure to multiple water-soluble components and ROS in size-resolved PMs in solid fuel combustion households B. Zhang et al. 10.1016/j.envpol.2024.125075
- Atmospheric humic-like substances (HULIS) in Chongqing, Southwest China: Abundance, light absorption properties, and potential sources T. Tang et al. 10.1016/j.atmosres.2023.107016
- Insight into the Role of NH3/NH4+ and NOx/NO3– in the Formation of Nitrogen-Containing Brown Carbon in Chinese Megacities D. Wang et al. 10.1021/acs.est.3c10374
- Insights into dissolved organics in non-urban areas - Optical properties and sources F. Yu et al. 10.1016/j.envpol.2023.121641
- Field evidence for enhanced generation of reactive oxygen species in atmospheric aerosol containing quinoline components W. Zhang et al. 10.1016/j.atmosenv.2022.119406
- Mixing states and secondary formation processes of organic nitrogen-containing single particles in Guangzhou, China L. Yun et al. 10.1016/j.jes.2023.02.053
- Investigating the molecular weight distribution of atmospheric water-soluble brown carbon using high-performance size exclusion chromatography coupled with diode array and fluorescence detectors X. Fan et al. 10.1016/j.chemosphere.2023.139517
- Optical properties, chemical functional group, and oxidative activity of different polarity levels of water-soluble organic matter in PM2.5 from biomass and coal combustion in rural areas in Northwest China S. Huang et al. 10.1016/j.atmosenv.2022.119179
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
- Research progress on the characteristics, sources, and environmental and potential health effects of water-soluble organic compounds in atmospheric particulate matter L. Wang et al. 10.1007/s11356-023-31723-x
- Oxidative potential of fine particulate matter emitted from traditional and improved biomass cookstoves B. Isenor et al. 10.1039/D3EA00135K
- Dynamic Wood Smoke Aerosol Toxicity during Oxidative Atmospheric Aging S. Wang et al. 10.1021/acs.est.2c05929
- Characteristics and Oxidative Potential of Ambient PM2.5 in the Yangtze River Delta Region: Pollution Level and Source Apportionment Y. Cui et al. 10.3390/atmos14030425
- Contribution of Physical and Chemical Properties to Dithiothreitol-Measured Oxidative Potentials of Atmospheric Aerosol Particles at Urban and Rural Sites in Japan K. Kurihara et al. 10.3390/atmos13020319
- Winter brown carbon over six of China's megacities: light absorption, molecular characterization, and improved source apportionment revealed by multilayer perceptron neural network D. Wang et al. 10.5194/acp-22-14893-2022
- NMR spectroscopic applications to atmospheric organic aerosol analysis – Part 1: A critical review of data source and analysis, potentialities and limitations S. Decesari et al. 10.1016/j.trac.2023.117516
- Variations in optical properties of water- and methanol-soluble organic carbon in PM2.5 in Tianjin and Handan over the Wintertime of 2018–2020 H. Chen et al. 10.1016/j.atmosres.2024.107332
- Distribution, chemical, and molecular composition of high and low molecular weight humic-like substances in ambient aerosols X. Fan et al. 10.5194/acp-24-3769-2024
- Oxidative potential of atmospheric brown carbon in six Chinese megacities: Seasonal variation and source apportionment D. Wang et al. 10.1016/j.atmosenv.2023.119909
- Chemical composition of PM10 at a rural site in the western Mediterranean and its relationship with the oxidative potential N. Gómez-Sánchez et al. 10.1016/j.chemosphere.2024.142880
- Seasonal changes in water-soluble brown carbon (BrC) at Nanling background station in South China B. Zhang et al. 10.3389/fenvs.2024.1360453
- Technical note: Chemical composition and source identification of fluorescent components in atmospheric water-soluble brown carbon by excitation–emission matrix spectroscopy with parallel factor analysis – potential limitations and applications T. Cao et al. 10.5194/acp-23-2613-2023
- Compositions and sources of fluorescent water-soluble and water-insoluble organic aerosols H. Ma et al. 10.1016/j.scitotenv.2024.174627
38 citations as recorded by crossref.
- Molecular-level transformations of biomass burning-derived water-soluble organic carbon during dark aqueous OH oxidation: Insights from absorption, fluorescence, high-performance size exclusion chromatography and high-resolution mass spectrometry analysis X. Fan et al. 10.1016/j.scitotenv.2023.169290
- NMR spectroscopic applications to atmospheric organic aerosol analysis – Part 2: A review of existing methodologies and perspectives E. Tagliavini et al. 10.1016/j.trac.2024.117595
- The complexation of atmospheric Brown carbon surrogates on the generation of hydroxyl radical from transition metals in simulated lung fluid Y. Lyu et al. 10.1016/j.envint.2023.108240
- Key toxic components and sources affecting oxidative potential of atmospheric particulate matter using interpretable machine learning: Insights from fog episodes R. Li et al. 10.1016/j.jhazmat.2023.133175
- Molecular-level insights into the temperature-dependent formation dynamics and mechanism of water-soluble dissolved organic carbon derived from biomass pyrolysis smoke T. Li et al. 10.1016/j.watres.2024.121176
- Comparison of water-soluble and water-insoluble organic compositions attributing to different light absorption efficiency between residential coal and biomass burning emissions L. Zhang et al. 10.5194/acp-24-6323-2024
- Optical properties, molecular characterizations, and oxidative potentials of different polarity levels of water-soluble organic matters in winter PM2.5 in six China's megacities T. Zhang et al. 10.1016/j.scitotenv.2022.158600
- Variabilities in Primary N-Containing Aromatic Compound Emissions from Residential Solid Fuel Combustion and Implications for Source Tracers L. Zhang et al. 10.1021/acs.est.2c03000
- Source profiles of molecular structure and light absorption of PM2.5 brown carbon from residential coal combustion emission in Northwestern China Q. Zhang et al. 10.1016/j.envpol.2022.118866
- Connecting oxidative potential with organic carbon molecule composition and source-specific apportionment in PM2.5 in Xi'an, China Y. Luo et al. 10.1016/j.atmosenv.2023.119808
- Molecular compositions and optical properties of water-soluble brown carbon during the autumn and winter in Guangzhou, China T. He et al. 10.1016/j.atmosenv.2022.119573
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- Deconvolving light absorption properties and influencing factors of carbonaceous aerosol in Shanghai Y. Zhou et al. 10.1016/j.scitotenv.2022.156280
- Insights the dominant contribution of biomass burning to methanol-soluble PM2.5 bounded oxidation potential based on multilayer perceptron neural network analysis in Xi'an, China Y. Luo et al. 10.1016/j.scitotenv.2023.168273
- Compositional and optical characteristics of aqueous brown carbon and HULIS in the eastern Indo-Gangetic Plain using a coupled EEM PARAFAC, FT-IR and 1H NMR approach S. Dey & S. Sarkar 10.1016/j.scitotenv.2024.171084
- Exploring the relationship between personal exposure to multiple water-soluble components and ROS in size-resolved PMs in solid fuel combustion households B. Zhang et al. 10.1016/j.envpol.2024.125075
- Atmospheric humic-like substances (HULIS) in Chongqing, Southwest China: Abundance, light absorption properties, and potential sources T. Tang et al. 10.1016/j.atmosres.2023.107016
- Insight into the Role of NH3/NH4+ and NOx/NO3– in the Formation of Nitrogen-Containing Brown Carbon in Chinese Megacities D. Wang et al. 10.1021/acs.est.3c10374
- Insights into dissolved organics in non-urban areas - Optical properties and sources F. Yu et al. 10.1016/j.envpol.2023.121641
- Field evidence for enhanced generation of reactive oxygen species in atmospheric aerosol containing quinoline components W. Zhang et al. 10.1016/j.atmosenv.2022.119406
- Mixing states and secondary formation processes of organic nitrogen-containing single particles in Guangzhou, China L. Yun et al. 10.1016/j.jes.2023.02.053
- Investigating the molecular weight distribution of atmospheric water-soluble brown carbon using high-performance size exclusion chromatography coupled with diode array and fluorescence detectors X. Fan et al. 10.1016/j.chemosphere.2023.139517
- Optical properties, chemical functional group, and oxidative activity of different polarity levels of water-soluble organic matter in PM2.5 from biomass and coal combustion in rural areas in Northwest China S. Huang et al. 10.1016/j.atmosenv.2022.119179
- Characterizing water-soluble brown carbon in fine particles in four typical cities in northwestern China during wintertime: integrating optical properties with chemical processes M. Zhong et al. 10.5194/acp-23-12609-2023
- Research progress on the characteristics, sources, and environmental and potential health effects of water-soluble organic compounds in atmospheric particulate matter L. Wang et al. 10.1007/s11356-023-31723-x
- Oxidative potential of fine particulate matter emitted from traditional and improved biomass cookstoves B. Isenor et al. 10.1039/D3EA00135K
- Dynamic Wood Smoke Aerosol Toxicity during Oxidative Atmospheric Aging S. Wang et al. 10.1021/acs.est.2c05929
- Characteristics and Oxidative Potential of Ambient PM2.5 in the Yangtze River Delta Region: Pollution Level and Source Apportionment Y. Cui et al. 10.3390/atmos14030425
- Contribution of Physical and Chemical Properties to Dithiothreitol-Measured Oxidative Potentials of Atmospheric Aerosol Particles at Urban and Rural Sites in Japan K. Kurihara et al. 10.3390/atmos13020319
- Winter brown carbon over six of China's megacities: light absorption, molecular characterization, and improved source apportionment revealed by multilayer perceptron neural network D. Wang et al. 10.5194/acp-22-14893-2022
- NMR spectroscopic applications to atmospheric organic aerosol analysis – Part 1: A critical review of data source and analysis, potentialities and limitations S. Decesari et al. 10.1016/j.trac.2023.117516
- Variations in optical properties of water- and methanol-soluble organic carbon in PM2.5 in Tianjin and Handan over the Wintertime of 2018–2020 H. Chen et al. 10.1016/j.atmosres.2024.107332
- Distribution, chemical, and molecular composition of high and low molecular weight humic-like substances in ambient aerosols X. Fan et al. 10.5194/acp-24-3769-2024
- Oxidative potential of atmospheric brown carbon in six Chinese megacities: Seasonal variation and source apportionment D. Wang et al. 10.1016/j.atmosenv.2023.119909
- Chemical composition of PM10 at a rural site in the western Mediterranean and its relationship with the oxidative potential N. Gómez-Sánchez et al. 10.1016/j.chemosphere.2024.142880
- Seasonal changes in water-soluble brown carbon (BrC) at Nanling background station in South China B. Zhang et al. 10.3389/fenvs.2024.1360453
- Technical note: Chemical composition and source identification of fluorescent components in atmospheric water-soluble brown carbon by excitation–emission matrix spectroscopy with parallel factor analysis – potential limitations and applications T. Cao et al. 10.5194/acp-23-2613-2023
- Compositions and sources of fluorescent water-soluble and water-insoluble organic aerosols H. Ma et al. 10.1016/j.scitotenv.2024.174627
Latest update: 20 Nov 2024
Short summary
Brown carbon (BrC) fractions derived from biomass burning and coal combustion including water- and methanol-soluble organic carbon were comprehensively characterized for their optical and chemical properties, as well as oxidative potential. Moreover, the key components or functional groups that were responsible for the reactive oxygen species (ROS) generation capacity of BrC were also discussed. These findings are useful for estimation of their environmental, climate, and health impacts.
Brown carbon (BrC) fractions derived from biomass burning and coal combustion including water-...
Altmetrics
Final-revised paper
Preprint