Articles | Volume 21, issue 16
https://doi.org/10.5194/acp-21-12243-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-12243-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 Aug 2021
Research article |
| 16 Aug 2021
| 16 Aug 2021
Kinetics and impacting factors of HO2 uptake onto submicron atmospheric aerosols during the 2019 Air QUAlity Study (AQUAS) in Yokohama, Japan
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Guangzhou 511443, China
Graduate School of Global Environmental Studies, Kyoto University,
Kyoto 606-8501, Japan
Center for Regional Environmental Research, National Institute for
Environmental Studies, Ibaraki 305-8506, Japan
Yu Bai
Graduate School of Human and Environmental Studies, Kyoto University,
Kyoto 606-8316, Japan
Yukiko Fukusaki
Yokohama Environmental Science Research Institute, Yokohama Kanagawa
221-0024, Japan
Yuka Kousa
Yokohama Environmental Science Research Institute, Yokohama Kanagawa
221-0024, Japan
Sathiyamurthi Ramasamy
Center for Regional Environmental Research, National Institute for
Environmental Studies, Ibaraki 305-8506, Japan
Akinori Takami
Center for Regional Environmental Research, National Institute for
Environmental Studies, Ibaraki 305-8506, Japan
Ayako Yoshino
Center for Regional Environmental Research, National Institute for
Environmental Studies, Ibaraki 305-8506, Japan
Tomoki Nakayama
Faculty of Environmental Science and Graduate School of Fisheries and
Environmental Sciences, Nagasaki University, Nagasaki 852-8521, Japan
Yasuhiro Sadanaga
Graduate School of Engineering, Osaka Prefecture University, Osaka 599-8531, Japan
Yoshihiro Nakashima
Graduate School of Agriculture, Tokyo University of Agriculture and
Technology, Tokyo 183-8538, Japan
Graduate School of Global Environmental Studies, Kyoto University,
Kyoto 606-8501, Japan
Kentaro Murano
Graduate School of Global Environmental Studies, Kyoto University,
Kyoto 606-8501, Japan
Nanase Kohno
Graduate School of Global Environmental Studies, Kyoto University,
Kyoto 606-8501, Japan
Yosuke Sakamoto
Graduate School of Global Environmental Studies, Kyoto University,
Kyoto 606-8501, Japan
Center for Regional Environmental Research, National Institute for
Environmental Studies, Ibaraki 305-8506, Japan
Graduate School of Human and Environmental Studies, Kyoto University,
Kyoto 606-8316, Japan
Yoshizumi Kajii
CORRESPONDING AUTHOR
Graduate School of Global Environmental Studies, Kyoto University,
Kyoto 606-8501, Japan
Center for Regional Environmental Research, National Institute for
Environmental Studies, Ibaraki 305-8506, Japan
Graduate School of Human and Environmental Studies, Kyoto University,
Kyoto 606-8316, Japan
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Cited
18 citations as recorded by crossref.
- Heterogeneous Uptake onto Deliquesced Particles as an Atmospheric Fate of Isoprene-Derived Hydroxy-RO2 Y. Sakamoto et al. 10.1021/acsestair.4c00165
- Suppression of surface ozone by an aerosol-inhibited photochemical ozone regime P. Ivatt et al. 10.1038/s41561-022-00972-9
- OH, HO2, and RO2 radical chemistry in a rural forest environment: measurements, model comparisons, and evidence of a missing radical sink B. Bottorff et al. 10.5194/acp-23-10287-2023
- Seasonal dependency of the atmospheric oxidizing capacity of the marine boundary layer of Bermuda Y. Elshorbany et al. 10.1016/j.atmosenv.2022.119326
- Effects of hydroperoxy radical heterogeneous loss on the summertime ozone formation in the North China Plain R. Wang et al. 10.1016/j.scitotenv.2022.153993
- Opinion: Atmospheric multiphase chemistry – past, present, and future J. Abbatt & A. Ravishankara 10.5194/acp-23-9765-2023
- Investigation of HO2 uptake mechanisms onto multiple-component ambient aerosols collected in summer and winter time in Yokohama, Japan J. Zhou et al. 10.1016/j.jes.2023.02.030
- Potential Factors Contributing to Ozone Production in AQUAS–Kyoto Campaign in Summer 2020: Natural Source-Related Missing OH Reactivity and Heterogeneous HO2/RO2 Loss J. Li et al. 10.1021/acs.est.2c03628
- Radical chemistry in the Pearl River Delta: observations and modeling of OH and HO2 radicals in Shenzhen in 2018 X. Yang et al. 10.5194/acp-22-12525-2022
- Fractal analysis of impact of PM2.5 on surface O3 sensitivity regime based on field observations C. Liu et al. 10.1016/j.scitotenv.2022.160136
- Impact of HO2 aerosol uptake on radical levels and O3 production during summertime in Beijing J. Dyson et al. 10.5194/acp-23-5679-2023
- Intercomparison of measured and modelled photochemical ozone production rates: Suggestion of chemistry hypothesis regarding unmeasured VOCs J. Zhou et al. 10.1016/j.scitotenv.2024.175290
- Global Impact of Particulate Nitrate Photolysis on Fine Sulfate Aerosol L. Liu et al. 10.1021/acs.estlett.4c00416
- The number fraction of iron-containing particles affects OH, HO2 and H2O2 budgets in the atmospheric aqueous phase A. Khaled et al. 10.5194/acp-22-1989-2022
- Towards a better understanding of the HO2uptake coefficient to aerosol particles measured during laboratory experiments P. Lakey et al. 10.1039/D4EA00025K
- A quantitative understanding of total OH reactivity and ozone production in a coastal industrial area during the Yokohama air quality study (AQUAS) campaign of summer 2019 J. Li et al. 10.1016/j.atmosenv.2021.118754
- Peroxy radical chemistry during ozone photochemical pollution season at a suburban site in the boundary of Jiangsu–Anhui–Shandong–Henan region, China N. Wei et al. 10.1016/j.scitotenv.2023.166355
- Reduced Aerosol Uptake of Hydroperoxyl Radical May Increase the Sensitivity of Ozone Production to Volatile Organic Compounds H. Song et al. 10.1021/acs.estlett.1c00893
18 citations as recorded by crossref.
- Heterogeneous Uptake onto Deliquesced Particles as an Atmospheric Fate of Isoprene-Derived Hydroxy-RO2 Y. Sakamoto et al. 10.1021/acsestair.4c00165
- Suppression of surface ozone by an aerosol-inhibited photochemical ozone regime P. Ivatt et al. 10.1038/s41561-022-00972-9
- OH, HO2, and RO2 radical chemistry in a rural forest environment: measurements, model comparisons, and evidence of a missing radical sink B. Bottorff et al. 10.5194/acp-23-10287-2023
- Seasonal dependency of the atmospheric oxidizing capacity of the marine boundary layer of Bermuda Y. Elshorbany et al. 10.1016/j.atmosenv.2022.119326
- Effects of hydroperoxy radical heterogeneous loss on the summertime ozone formation in the North China Plain R. Wang et al. 10.1016/j.scitotenv.2022.153993
- Opinion: Atmospheric multiphase chemistry – past, present, and future J. Abbatt & A. Ravishankara 10.5194/acp-23-9765-2023
- Investigation of HO2 uptake mechanisms onto multiple-component ambient aerosols collected in summer and winter time in Yokohama, Japan J. Zhou et al. 10.1016/j.jes.2023.02.030
- Potential Factors Contributing to Ozone Production in AQUAS–Kyoto Campaign in Summer 2020: Natural Source-Related Missing OH Reactivity and Heterogeneous HO2/RO2 Loss J. Li et al. 10.1021/acs.est.2c03628
- Radical chemistry in the Pearl River Delta: observations and modeling of OH and HO2 radicals in Shenzhen in 2018 X. Yang et al. 10.5194/acp-22-12525-2022
- Fractal analysis of impact of PM2.5 on surface O3 sensitivity regime based on field observations C. Liu et al. 10.1016/j.scitotenv.2022.160136
- Impact of HO2 aerosol uptake on radical levels and O3 production during summertime in Beijing J. Dyson et al. 10.5194/acp-23-5679-2023
- Intercomparison of measured and modelled photochemical ozone production rates: Suggestion of chemistry hypothesis regarding unmeasured VOCs J. Zhou et al. 10.1016/j.scitotenv.2024.175290
- Global Impact of Particulate Nitrate Photolysis on Fine Sulfate Aerosol L. Liu et al. 10.1021/acs.estlett.4c00416
- The number fraction of iron-containing particles affects OH, HO2 and H2O2 budgets in the atmospheric aqueous phase A. Khaled et al. 10.5194/acp-22-1989-2022
- Towards a better understanding of the HO2uptake coefficient to aerosol particles measured during laboratory experiments P. Lakey et al. 10.1039/D4EA00025K
- A quantitative understanding of total OH reactivity and ozone production in a coastal industrial area during the Yokohama air quality study (AQUAS) campaign of summer 2019 J. Li et al. 10.1016/j.atmosenv.2021.118754
- Peroxy radical chemistry during ozone photochemical pollution season at a suburban site in the boundary of Jiangsu–Anhui–Shandong–Henan region, China N. Wei et al. 10.1016/j.scitotenv.2023.166355
- Reduced Aerosol Uptake of Hydroperoxyl Radical May Increase the Sensitivity of Ozone Production to Volatile Organic Compounds H. Song et al. 10.1021/acs.estlett.1c00893
Latest update: 08 May 2025
Short summary
HO2 radicals play key roles in tropospheric chemistry, their levels in ambient air not yet fully explained by sophisticated models. Here we measured HO2 uptake kinetics onto ambient aerosols in real time using a self-built online system and investigated the impacting factors on such processes by coupling with other instrumentations. The role of the HO2 uptake process in O3 formation is also discussed. Results give useful information for coordinated control of aerosol and ozone pollutants.
HO2 radicals play key roles in tropospheric chemistry, their levels in ambient air not yet fully...
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