Articles | Volume 21, issue 15
https://doi.org/10.5194/acp-21-12141-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-12141-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Aug 2021
Research article |
| 13 Aug 2021
| 13 Aug 2021
Gas–particle partitioning of polyol tracers at a suburban site in Nanjing, east China: increased partitioning to the particle phase
Chao Qin
Colleges of Resources and Environmental Sciences, Nanjing Agricultural University, Nanjing 210095, China
Yafeng Gou
Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, 219 Ningliu Road, Nanjing 210044, China
Yuhang Wang
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
Yuhao Mao
Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, 219 Ningliu Road, Nanjing 210044, China
Hong Liao
Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, 219 Ningliu Road, Nanjing 210044, China
Qin'geng Wang
State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Nanjing 210023, China
Mingjie Xie
CORRESPONDING AUTHOR
Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, 219 Ningliu Road, Nanjing 210044, China
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Cited
11 citations as recorded by crossref.
- Energetic description of the liquid–vapor interface of water with organic coating molecules J. Devémy et al. 10.1039/D4LF00037D
- Evaluating coarse PM composition and sources based on bulk and molecular speciation of PM2.5 and PM10 in Nanjing, East China W. Cui et al. 10.1016/j.jes.2024.04.038
- Estimation of the Volatility and Apparent Activity Coefficient of Levoglucosan in Wood-Burning Organic Aerosols J. Zhang et al. 10.1021/acs.estlett.4c00608
- Compilation of Henry's law constants (version 5.0.0) for water as solvent R. Sander 10.5194/acp-23-10901-2023
- Collocated Measurements of Light‐Absorbing Organic Carbon in PM2.5: Observation Uncertainty and Organic Tracer‐Based Source Apportionment M. Xie et al. 10.1029/2021JD035874
- Potential underestimation of ambient brown carbon absorption based on the methanol extraction method and its impacts on source analysis Z. Xu et al. 10.5194/acp-22-13739-2022
- Size-resolved light-absorbing organic carbon and organic molecular markers in Nanjing, east China: Seasonal variations and sources W. Feng et al. 10.1016/j.envpol.2023.122006
- Spatiotemporal variations of PM2.5 organic molecular markers in five central cities of the Yangtze River Delta, East China in autumn and winter: Implications for regional and local sources of organic aerosols W. Feng et al. 10.1016/j.envpol.2024.125227
- The C5–Alkene Triol Conundrum: Structural Characterization and Quantitation of Isoprene-Derived C5H10O3 Reactive Uptake Products M. Frauenheim et al. 10.1021/acs.estlett.2c00548
- Time‐Resolved Measurements of PM2.5 Chemical Composition and Brown Carbon Absorption in Nanjing, East China: Diurnal Variations and Organic Tracer‐Based PMF Analysis W. Feng et al. 10.1029/2023JD039092
- Partitioning of Ambient Organic Gases to Inorganic Salt Solutions: Influence of Salt Identity, Ionic Strength, and pH V. Pratap et al. 10.1029/2021GL095247
11 citations as recorded by crossref.
- Energetic description of the liquid–vapor interface of water with organic coating molecules J. Devémy et al. 10.1039/D4LF00037D
- Evaluating coarse PM composition and sources based on bulk and molecular speciation of PM2.5 and PM10 in Nanjing, East China W. Cui et al. 10.1016/j.jes.2024.04.038
- Estimation of the Volatility and Apparent Activity Coefficient of Levoglucosan in Wood-Burning Organic Aerosols J. Zhang et al. 10.1021/acs.estlett.4c00608
- Compilation of Henry's law constants (version 5.0.0) for water as solvent R. Sander 10.5194/acp-23-10901-2023
- Collocated Measurements of Light‐Absorbing Organic Carbon in PM2.5: Observation Uncertainty and Organic Tracer‐Based Source Apportionment M. Xie et al. 10.1029/2021JD035874
- Potential underestimation of ambient brown carbon absorption based on the methanol extraction method and its impacts on source analysis Z. Xu et al. 10.5194/acp-22-13739-2022
- Size-resolved light-absorbing organic carbon and organic molecular markers in Nanjing, east China: Seasonal variations and sources W. Feng et al. 10.1016/j.envpol.2023.122006
- Spatiotemporal variations of PM2.5 organic molecular markers in five central cities of the Yangtze River Delta, East China in autumn and winter: Implications for regional and local sources of organic aerosols W. Feng et al. 10.1016/j.envpol.2024.125227
- The C5–Alkene Triol Conundrum: Structural Characterization and Quantitation of Isoprene-Derived C5H10O3 Reactive Uptake Products M. Frauenheim et al. 10.1021/acs.estlett.2c00548
- Time‐Resolved Measurements of PM2.5 Chemical Composition and Brown Carbon Absorption in Nanjing, East China: Diurnal Variations and Organic Tracer‐Based PMF Analysis W. Feng et al. 10.1029/2023JD039092
- Partitioning of Ambient Organic Gases to Inorganic Salt Solutions: Influence of Salt Identity, Ionic Strength, and pH V. Pratap et al. 10.1029/2021GL095247
Latest update: 13 Dec 2024
Short summary
In this study, we found that the aqueous solution in aerosols is an important absorbing phase for gaseous polyols in the atmosphere, indicating that the dissolution in aerosol liquid water should not be ignored when investigating gas–particle partitioning of water-soluble organics. The exponential increase in effective partitioning coefficients of polyol tracers with sulfate ion concentrations could be attributed to organic–inorganic interactions in the particle phase.
In this study, we found that the aqueous solution in aerosols is an important absorbing phase...
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