Articles | Volume 21, issue 13
https://doi.org/10.5194/acp-21-10215-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-10215-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Jul 2021
Research article |
| 07 Jul 2021
| 07 Jul 2021
Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts
Young-Chul Song
Department of Earth and Environmental Sciences, Jeonbuk National University, Jeonju, Republic of Korea
The Earth and Environmental Science System Research Center, Jeonbuk National University, Jeonju, Republic of Korea
Joseph Lilek
Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Quebec, Canada
Jae Bong Lee
Innovative System Safety Research Division, Korea Atomic Energy Research Institute, Daejeon, Republic of Korea
Man Nin Chan
Earth System Science Programme, Faculty of Science, The Chinese University of Hong Kong, Hong Kong, China
The Institute of Environment, Energy, and Sustainability, The Chinese University of Hong Kong, Hong Kong, China
Zhijun Wu
Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing, China
Andreas Zuend
Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Quebec, Canada
Mijung Song
CORRESPONDING AUTHOR
Department of Earth and Environmental Sciences, Jeonbuk National University, Jeonju, Republic of Korea
The Earth and Environmental Science System Research Center, Jeonbuk National University, Jeonju, Republic of Korea
Department of Environment and Energy, Jeonbuk National University, Jeonju, Republic of Korea
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24 citations as recorded by crossref.
- Accelerated Sulfur Oxidation by Ozone on Surfaces of Single Optically Trapped Aerosol Particles S. Hsu et al. 10.1021/acs.jpcc.2c06831
- Aqueous-phase formation of N-containing secondary organic compounds affected by the ionic strength Y. Gan et al. 10.1016/j.jes.2023.03.003
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al. 10.1016/j.scitotenv.2024.177298
- Influence of Relative Humidity and Composition on PM2.5 Phases in Northeast Asia C. Seong et al. 10.1021/acsearthspacechem.4c00019
- Tutorial: Electrodynamic balance methods for single particle levitation and the physicochemical analysis of aerosol R. Kaur Kohli et al. 10.1016/j.jaerosci.2023.106255
- Exploring the hygroscopicity and chemical composition evolution in organic-inorganic aerosols: A study on internally mixed malonic acid-metal (Na+, Ca2+, Mg2+) nitrates S. Saha & P. Mathi 10.1016/j.chemosphere.2023.139260
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- Particle phase-state variability in the North Atlantic free troposphere during summertime is determined by atmospheric transport patterns and sources Z. Cheng et al. 10.5194/acp-22-9033-2022
- Microscopic observation of a liquid-liquid-(semi)solid phase in polluted PM2.5 S. Gaikwad et al. 10.3389/fenvs.2022.947924
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- Enhanced Nitrate Fraction: Enabling Urban Aerosol Particles to Remain in a Liquid State at Reduced Relative Humidity Y. Liu et al. 10.1029/2023GL105505
- pH regulates the formation of organosulfates and inorganic sulfate from organic peroxide reaction with dissolved SO2 in aquatic media L. Du et al. 10.5194/acp-24-1841-2024
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- Probe molecular diffusivity in single ternary inorganic–organic microdroplets via interfacial ozonolysis of thiosulfate T. Hung et al. 10.1039/D4EA00072B
- Viscosity and physical state of sucrose mixed with ammonium sulfate droplets R. Jeong et al. 10.5194/acp-22-8805-2022
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al. 10.3389/fenvs.2023.1142941
- Correlating the Viscosity and Rate of Water Diffusion in Semisolid Gel-Forming Aerosol Particles C. Sheldon et al. 10.1021/acsearthspacechem.3c00241
- Single particle measurements of mixing between mimics for biomass burning and aged secondary organic aerosols L. Habib & N. Donahue 10.1039/D2EA00017B
- The relative humidity-dependent viscosity of single quasi aerosol particles and possible implications for atmospheric aerosol chemistry Y. Tong et al. 10.1039/D2CP00740A
- Glass Transition Temperatures of Organic Mixtures from Isoprene Epoxydiol-Derived Secondary Organic Aerosol B. Chen et al. 10.1021/acs.jpca.2c08936
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al. 10.1021/acs.est.2c06377
- Direct measurement of the viscosity of ternary aerosol mixtures S. Mahant et al. 10.1039/D2EA00160H
24 citations as recorded by crossref.
- Accelerated Sulfur Oxidation by Ozone on Surfaces of Single Optically Trapped Aerosol Particles S. Hsu et al. 10.1021/acs.jpcc.2c06831
- Aqueous-phase formation of N-containing secondary organic compounds affected by the ionic strength Y. Gan et al. 10.1016/j.jes.2023.03.003
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al. 10.1016/j.scitotenv.2024.177298
- Influence of Relative Humidity and Composition on PM2.5 Phases in Northeast Asia C. Seong et al. 10.1021/acsearthspacechem.4c00019
- Tutorial: Electrodynamic balance methods for single particle levitation and the physicochemical analysis of aerosol R. Kaur Kohli et al. 10.1016/j.jaerosci.2023.106255
- Exploring the hygroscopicity and chemical composition evolution in organic-inorganic aerosols: A study on internally mixed malonic acid-metal (Na+, Ca2+, Mg2+) nitrates S. Saha & P. Mathi 10.1016/j.chemosphere.2023.139260
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- Particle phase-state variability in the North Atlantic free troposphere during summertime is determined by atmospheric transport patterns and sources Z. Cheng et al. 10.5194/acp-22-9033-2022
- Microscopic observation of a liquid-liquid-(semi)solid phase in polluted PM2.5 S. Gaikwad et al. 10.3389/fenvs.2022.947924
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- Enhanced Nitrate Fraction: Enabling Urban Aerosol Particles to Remain in a Liquid State at Reduced Relative Humidity Y. Liu et al. 10.1029/2023GL105505
- pH regulates the formation of organosulfates and inorganic sulfate from organic peroxide reaction with dissolved SO2 in aquatic media L. Du et al. 10.5194/acp-24-1841-2024
- A predictive viscosity model for aqueous electrolytes and mixed organic–inorganic aerosol phases J. Lilek & A. Zuend 10.5194/acp-22-3203-2022
- Role of WSOCs and pH on Ammonium Nitrate Aerosol Efflorescence: Insights into Secondary Aerosol Formation J. Sun et al. 10.1021/acs.est.3c07603
- Probe molecular diffusivity in single ternary inorganic–organic microdroplets via interfacial ozonolysis of thiosulfate T. Hung et al. 10.1039/D4EA00072B
- Viscosity and physical state of sucrose mixed with ammonium sulfate droplets R. Jeong et al. 10.5194/acp-22-8805-2022
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al. 10.3389/fenvs.2023.1142941
- Correlating the Viscosity and Rate of Water Diffusion in Semisolid Gel-Forming Aerosol Particles C. Sheldon et al. 10.1021/acsearthspacechem.3c00241
- Single particle measurements of mixing between mimics for biomass burning and aged secondary organic aerosols L. Habib & N. Donahue 10.1039/D2EA00017B
- The relative humidity-dependent viscosity of single quasi aerosol particles and possible implications for atmospheric aerosol chemistry Y. Tong et al. 10.1039/D2CP00740A
- Glass Transition Temperatures of Organic Mixtures from Isoprene Epoxydiol-Derived Secondary Organic Aerosol B. Chen et al. 10.1021/acs.jpca.2c08936
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al. 10.1021/acs.est.2c06377
- Direct measurement of the viscosity of ternary aerosol mixtures S. Mahant et al. 10.1039/D2EA00160H
Latest update: 20 Nov 2024
Short summary
We report viscosity of binary mixtures of organic material / H2O and inorganic salts / H2O, as well as ternary mixtures of organic material / inorganic salts/ H2O, over the atmospheric relative humidity (RH) range. The viscosity measurements indicate that the studied mixed organic–inorganic particles range in phase state from liquid to semi-solid or even solid across the atmospheric RH range at a temperature of 293 K.
We report viscosity of binary mixtures of organic material / H2O and inorganic salts / H2O, as...
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