Articles | Volume 20, issue 16
https://doi.org/10.5194/acp-20-9837-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-9837-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
An inversion of NOx and non-methane volatile organic compound (NMVOC) emissions using satellite observations during the KORUS-AQ campaign and implications for surface ozone over East Asia
Amir H. Souri
CORRESPONDING AUTHOR
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Caroline R. Nowlan
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Gonzalo González Abad
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen, China
Donald R. Blake
Department of Chemistry, University of California, Irvine, Irvine, CA, USA
Alan Fried
Institute of Arctic & Alpine Research, University of Colorado,
Boulder, CO, USA
Andrew J. Weinheimer
National Center for Atmospheric Research, Boulder, CO, USA
Armin Wisthaler
Institute for Ion Physics and Applied Physics, University of Innsbruck, Technikerstrasse 25, 6020 Innsbruck, Austria
Department of Chemistry, University of Oslo, P.O. box 1033, Blindern, 0315 Oslo, Norway
Jung-Hun Woo
Department of Advanced Technology Fusion, Konkuk University, Seoul,
South Korea
Qiang Zhang
Department of Earth System Science, Tsinghua University, Beijing,
China
Christopher E. Chan Miller
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Xiong Liu
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Kelly Chance
Atomic and Molecular Physics (AMP) Division, Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Data sets
Data outputs from the joint inversion study A. H. Souri, C. R. Nowlan, G. González Abad, L. Zhu, D. R. Blake, A. Fried, A. J. Weinheimer, A. Wisthaler, J.-H. Woo, Q. Zhang, C. E. Chan Miller, X. Liu, and K. Chance https://doi.org/10.17632/8s4jscy93m.1
Short summary
For the first time, we provide a joint nonlinear optimal estimate of NOx and NMVOC emissions during the KORUS-AQ campaign by simultaneously incorporating SAO's new product of HCHO columns from OMPS and OMI tropospheric NO2 columns into a regional model. Results demonstrate a promising improvement in the performance of the model in terms of HCHO and NO2 concentrations, which in turn enables us to quantify the impact of the emission changes on different pathways of ozone formation and loss.
For the first time, we provide a joint nonlinear optimal estimate of NOx and NMVOC emissions...
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