Articles | Volume 20, issue 12
https://doi.org/10.5194/acp-20-7291-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-7291-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Jun 2020
Research article |
| 24 Jun 2020
| 24 Jun 2020
Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China
Jingyi Li
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science & Technology, Nanjing 210044, China
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and
Pollution Control, School of Environmental Science and Engineering, Nanjing
University of Information Science & Technology, Nanjing 210044, China
Haowen Zhang
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and
Pollution Control, School of Environmental Science and Engineering, Nanjing
University of Information Science & Technology, Nanjing 210044, China
Qi Ying
CORRESPONDING AUTHOR
Zachry Department of Civil and Environmental Engineering, Texas
A & M University, College Station, Texas 77843-3136, USA
Zhijun Wu
State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science & Technology, Nanjing 210044, China
Yanli Zhang
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640,
China
Center for Excellence in Regional Atmospheric Environment,
Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Xinming Wang
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640,
China
Center for Excellence in Regional Atmospheric Environment,
Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
Xinghua Li
School of Space & Environment, Beihang University, Beijing
100191, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science & Technology, Nanjing 210044, China
Yuanhang Zhang
State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science & Technology, Nanjing 210044, China
Jianlin Hu
CORRESPONDING AUTHOR
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science & Technology, Nanjing 210044, China
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and
Pollution Control, School of Environmental Science and Engineering, Nanjing
University of Information Science & Technology, Nanjing 210044, China
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Cited
15 citations as recorded by crossref.
- Impacts of emissions along the lower Yangtze River on air quality and public health in the Yangtze River delta, China L. Sheng et al. 10.1016/j.apr.2022.101420
- Spatial and Temporal Variations in the Atmospheric Age Distribution of Primary and Secondary Inorganic Aerosols in China X. Xie et al. 10.1016/j.eng.2022.03.013
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Nitrate-Enhanced Gas-to-Particle-Phase Partitioning of Water-Soluble Organic Compounds in Chinese Urban Atmosphere: Implications for Secondary Organic Aerosol Formation S. Lv et al. 10.1021/acs.estlett.2c00894
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- Assessing the Impacts of Climate Change on Meteorology and Air Stagnation in China Using a Dynamical Downscaling Method A. Hu et al. 10.3389/fenvs.2022.894887
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- Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US S. Kakavas et al. 10.5194/acp-23-13555-2023
- Pollution levels and health risk assessment of potentially toxic metals of size-segregated particulate matter in rural residential areas of high lung cancer incidence in Fuyuan, China K. Xiao et al. 10.1007/s10653-022-01374-x
- Secondary organic aerosol formation via multiphase reaction of hydrocarbons in urban atmospheres using CAMx integrated with the UNIPAR model Z. Yu et al. 10.5194/acp-22-9083-2022
- Improving the accuracy of O3 prediction from a chemical transport model with a random forest model in the Yangtze River Delta region, China K. Xiong et al. 10.1016/j.envpol.2022.120926
- Assessing the Uncertainties in Ozone and SOA Predictions due to Different Branching Ratios of the Cresol Pathway in the Toluene-OH Oxidation Mechanism J. Zhang et al. 10.1021/acsearthspacechem.1c00092
- Estimation of Aromatic Secondary Organic Aerosol Using a Molecular Tracer—A Chemical Transport Model Assessment J. Zhang et al. 10.1021/acs.est.1c03670
- Capturing the Relative‐Humidity‐Sensitive Gas–Particle Partitioning of Organic Aerosols in a 2D Volatility Basis Set C. Serrano Damha et al. 10.1029/2023GL106095
15 citations as recorded by crossref.
- Impacts of emissions along the lower Yangtze River on air quality and public health in the Yangtze River delta, China L. Sheng et al. 10.1016/j.apr.2022.101420
- Spatial and Temporal Variations in the Atmospheric Age Distribution of Primary and Secondary Inorganic Aerosols in China X. Xie et al. 10.1016/j.eng.2022.03.013
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Nitrate-Enhanced Gas-to-Particle-Phase Partitioning of Water-Soluble Organic Compounds in Chinese Urban Atmosphere: Implications for Secondary Organic Aerosol Formation S. Lv et al. 10.1021/acs.estlett.2c00894
- Improved O3 predictions in China by combining chemical transport model and multi-source data with machining learning techniques K. Xiong et al. 10.1016/j.atmosenv.2023.120269
- Assessing the Impacts of Climate Change on Meteorology and Air Stagnation in China Using a Dynamical Downscaling Method A. Hu et al. 10.3389/fenvs.2022.894887
- Contrasting impacts of humidity on the ozonolysis of monoterpenes: insights into the multi-generation chemical mechanism S. Zhang et al. 10.5194/acp-23-10809-2023
- Characterization and source analysis of water-soluble inorganic ionic species in PM2.5 during a wintertime particle pollution episode in Nanjing, China Y. Zhan et al. 10.1016/j.atmosres.2021.105769
- Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US S. Kakavas et al. 10.5194/acp-23-13555-2023
- Pollution levels and health risk assessment of potentially toxic metals of size-segregated particulate matter in rural residential areas of high lung cancer incidence in Fuyuan, China K. Xiao et al. 10.1007/s10653-022-01374-x
- Secondary organic aerosol formation via multiphase reaction of hydrocarbons in urban atmospheres using CAMx integrated with the UNIPAR model Z. Yu et al. 10.5194/acp-22-9083-2022
- Improving the accuracy of O3 prediction from a chemical transport model with a random forest model in the Yangtze River Delta region, China K. Xiong et al. 10.1016/j.envpol.2022.120926
- Assessing the Uncertainties in Ozone and SOA Predictions due to Different Branching Ratios of the Cresol Pathway in the Toluene-OH Oxidation Mechanism J. Zhang et al. 10.1021/acsearthspacechem.1c00092
- Estimation of Aromatic Secondary Organic Aerosol Using a Molecular Tracer—A Chemical Transport Model Assessment J. Zhang et al. 10.1021/acs.est.1c03670
- Capturing the Relative‐Humidity‐Sensitive Gas–Particle Partitioning of Organic Aerosols in a 2D Volatility Basis Set C. Serrano Damha et al. 10.1029/2023GL106095
Latest update: 13 Dec 2024
Short summary
Large gaps still exist in modeled and observed secondary organic aerosol (SOA) mass loading and properties. Here we investigated the impacts of water partitioning into organic aerosol and nonideality of the organic–water mixture on SOA over eastern China using a regional 3D model. SOA is increased more significantly in humid and hot environments. Increases in SOA further cause an enhancement of the cooling effects of aerosols. It is crucial to consider the above processes in modeling SOA.
Large gaps still exist in modeled and observed secondary organic aerosol (SOA) mass loading and...
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