Articles | Volume 20, issue 8
https://doi.org/10.5194/acp-20-4757-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-20-4757-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Apr 2020
Research article |
| 24 Apr 2020
| 24 Apr 2020
Influx of African biomass burning aerosol during the Amazonian dry season through layered transatlantic transport of black carbon-rich smoke
Bruna A. Holanda
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Instituto de Fisica, Universidade de Sao Paulo, 05508-090, Sao Paulo, SP, Brazil
Mira L. Pöhlker
CORRESPONDING AUTHOR
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
David Walter
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Max Planck Institute for Biogeochemistry, 07701 Jena, Germany
Jorge Saturno
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
now at: Physikalisch-Technische Bundesanstalt, 38116 Braunschweig, Germany
Matthias Sörgel
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Atmospheric Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Jeannine Ditas
Institute for Environmental and Climate Research (ECI), Jinan University, Guangzhou, 511443, China
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Florian Ditas
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
now at: Hessisches Landesamt für Naturschutz, Umwelt und Geologie, 65203 Wiesbaden, Germany
Christiane Schulz
Experimental Aerosol and Cloud Microphysics Department, TROPOS, Leibniz-Institute for Tropospheric Research, Leipzig, Germany
Particle Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Marco Aurélio Franco
Instituto de Fisica, Universidade de Sao Paulo, 05508-090, Sao Paulo, SP, Brazil
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Qiaoqiao Wang
Institute for Environmental and Climate Research (ECI), Jinan University, Guangzhou, 511443, China
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Tobias Donth
Leipzig Institute for Meteorology, Leipzig University, Leipzig, Germany
Paulo Artaxo
Instituto de Fisica, Universidade de Sao Paulo, 05508-090, Sao Paulo, SP, Brazil
Henrique M. J. Barbosa
Instituto de Fisica, Universidade de Sao Paulo, 05508-090, Sao Paulo, SP, Brazil
Stephan Borrmann
Particle Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Institute for Physics of the Atmosphere, Johannes Gutenberg University, 55128 Mainz, Germany
Ramon Braga
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Joel Brito
Instituto de Fisica, Universidade de Sao Paulo, 05508-090, Sao Paulo, SP, Brazil
now at: IMT Lille Douai, Univ. Lille, SAGE, 59000 Lille, France
Yafang Cheng
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Maximilian Dollner
University of Vienna, Faculty of Physics, Aerosol Physics and Environmental Physics, 1090 Vienna, Austria
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Johannes W. Kaiser
Atmospheric Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
now at: Deutscher Wetterdienst, 63067 Offenbach, Germany
Thomas Klimach
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Christoph Knote
Meteorological Institute, Ludwig-Maximilians-Universität, Munich, Germany
Ovid O. Krüger
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Daniel Fütterer
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Jošt V. Lavrič
Max Planck Institute for Biogeochemistry, 07701 Jena, Germany
Nan Ma
Institute for Environmental and Climate Research (ECI), Jinan University, Guangzhou, 511443, China
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Luiz A. T. Machado
National Institute for Space Research (INPE), São José Dos Campos, Brazil
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Jing Ming
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Fernando G. Morais
Instituto de Fisica, Universidade de Sao Paulo, 05508-090, Sao Paulo, SP, Brazil
Hauke Paulsen
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Daniel Sauer
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Hans Schlager
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Johannes Schneider
Particle Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Bernadett Weinzierl
University of Vienna, Faculty of Physics, Aerosol Physics and Environmental Physics, 1090 Vienna, Austria
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Adrian Walser
University of Vienna, Faculty of Physics, Aerosol Physics and Environmental Physics, 1090 Vienna, Austria
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Meteorological Institute, Ludwig-Maximilians-Universität, Munich, Germany
Manfred Wendisch
Leipzig Institute for Meteorology, Leipzig University, Leipzig, Germany
Helmut Ziereis
Institute for Atmospheric Physics, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Martin Zöger
Flight experiments, German Aerospace Center (DLR), 82234 Oberpfaffenhofen, Germany
Ulrich Pöschl
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Meinrat O. Andreae
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Scripps Institution of Oceanography, University of California San Diego, La Jolla, California 92093, USA
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Biogeochemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
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Cited
32 citations as recorded by crossref.
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- Occurrence and growth of sub-50 nm aerosol particles in the Amazonian boundary layer M. Franco et al. 10.5194/acp-22-3469-2022
- African biomass burning affects aerosol cycling over the Amazon B. Holanda et al. 10.1038/s43247-023-00795-5
- Impact of biomass burning aerosols on radiation, clouds, and precipitation over the Amazon: relative importance of aerosol–cloud and aerosol–radiation interactions L. Liu et al. 10.5194/acp-20-13283-2020
- Global organic and inorganic aerosol hygroscopicity and its effect on radiative forcing M. Pöhlker et al. 10.1038/s41467-023-41695-8
- Overview: On the transport and transformation of pollutants in the outflow of major population centres – observational data from the EMeRGe European intensive operational period in summer 2017 M. Andrés Hernández et al. 10.5194/acp-22-5877-2022
- African smoke particles act as cloud condensation nuclei in the wintertime tropical North Atlantic boundary layer over Barbados H. Royer et al. 10.5194/acp-23-981-2023
- Aerosol optical depth and water vapor variability assessed through autocorrelation analysis M. Franco et al. 10.1007/s00703-024-01011-5
- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
- Long-term deposition and condensation ice-nucleating particle measurements from four stations across the globe J. Schrod et al. 10.5194/acp-20-15983-2020
- Extremely low-volatility organic coating leads to underestimation of black carbon climate impact Y. Zhang et al. 10.1016/j.oneear.2023.01.009
- Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations F. Kluge et al. 10.5194/acp-23-1369-2023
- Long-range transport and microscopy analysis of Sangay volcanic ashes in Ecuador D. Moran-Zuloaga et al. 10.1007/s11869-023-01434-w
- Isolating Large‐Scale Smoke Impacts on Cloud and Precipitation Processes Over the Amazon With Convection Permitting Resolution R. Herbert et al. 10.1029/2021JD034615
- An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic A. Dobracki et al. 10.5194/acp-23-4775-2023
- Acceleration of the southern African easterly jet driven by the radiative effect of biomass burning aerosols and its impact on transport during AEROCLO-sA J. Chaboureau et al. 10.5194/acp-22-8639-2022
- Black carbon aerosol reductions during COVID-19 confinement quantified by aircraft measurements over Europe O. Krüger et al. 10.5194/acp-22-8683-2022
- Vertical variability of the properties of highly aged biomass burning aerosol transported over the southeast Atlantic during CLARIFY-2017 H. Wu et al. 10.5194/acp-20-12697-2020
- Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories G. Unfer et al. 10.5194/acp-24-3869-2024
- Relationship between Land Use and Spatial Variability of Atmospheric Brown Carbon and Black Carbon Aerosols in Amazonia F. Morais et al. 10.3390/atmos13081328
- How weather events modify aerosol particle size distributions in the Amazon boundary layer L. Machado et al. 10.5194/acp-21-18065-2021
- Analysis of the Influence of Deforestation on the Microphysical Parameters of Clouds in the Amazon H. da Silva et al. 10.3390/rs14215353
- Vertical profiles of trace gas and aerosol properties over the eastern North Atlantic: variations with season and synoptic condition Y. Wang et al. 10.5194/acp-21-11079-2021
- Using the Black Carbon Particle Mixing State to Characterize the Lifecycle of Biomass Burning Aerosols A. Sedlacek et al. 10.1021/acs.est.2c03851
- Aerosols from anthropogenic and biogenic sources and their interactions – modeling aerosol formation, optical properties, and impacts over the central Amazon basin J. Nascimento et al. 10.5194/acp-21-6755-2021
- Relationship between El Niño-Southern Oscillation and Atmospheric Aerosols in the Legal Amazon A. Pereira et al. 10.3390/cli12020013
- Cloud droplet formation at the base of tropical convective clouds: closure between modeling and measurement results of ACRIDICON–CHUVA R. Braga et al. 10.5194/acp-21-17513-2021
- Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest R. Herbert & P. Stier 10.5194/acp-23-4595-2023
- Detrainment Dominates CCN Concentrations Around Non‐Precipitating Convective Clouds Over the Amazon R. Braga et al. 10.1029/2022GL100411
- Concentrations and biosphere–atmosphere fluxes of inorganic trace gases and associated ionic aerosol counterparts over the Amazon rainforest R. Ramsay et al. 10.5194/acp-20-15551-2020
- Transport and Variability of Tropospheric Ozone over Oceania and Southern Pacific during the 2019–20 Australian Bushfires N. Bègue et al. 10.3390/rs13163092
- Total OH reactivity over the Amazon rainforest: variability with temperature, wind, rain, altitude, time of day, season, and an overall budget closure E. Pfannerstill et al. 10.5194/acp-21-6231-2021
32 citations as recorded by crossref.
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- Occurrence and growth of sub-50 nm aerosol particles in the Amazonian boundary layer M. Franco et al. 10.5194/acp-22-3469-2022
- African biomass burning affects aerosol cycling over the Amazon B. Holanda et al. 10.1038/s43247-023-00795-5
- Impact of biomass burning aerosols on radiation, clouds, and precipitation over the Amazon: relative importance of aerosol–cloud and aerosol–radiation interactions L. Liu et al. 10.5194/acp-20-13283-2020
- Global organic and inorganic aerosol hygroscopicity and its effect on radiative forcing M. Pöhlker et al. 10.1038/s41467-023-41695-8
- Overview: On the transport and transformation of pollutants in the outflow of major population centres – observational data from the EMeRGe European intensive operational period in summer 2017 M. Andrés Hernández et al. 10.5194/acp-22-5877-2022
- African smoke particles act as cloud condensation nuclei in the wintertime tropical North Atlantic boundary layer over Barbados H. Royer et al. 10.5194/acp-23-981-2023
- Aerosol optical depth and water vapor variability assessed through autocorrelation analysis M. Franco et al. 10.1007/s00703-024-01011-5
- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
- Long-term deposition and condensation ice-nucleating particle measurements from four stations across the globe J. Schrod et al. 10.5194/acp-20-15983-2020
- Extremely low-volatility organic coating leads to underestimation of black carbon climate impact Y. Zhang et al. 10.1016/j.oneear.2023.01.009
- Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations F. Kluge et al. 10.5194/acp-23-1369-2023
- Long-range transport and microscopy analysis of Sangay volcanic ashes in Ecuador D. Moran-Zuloaga et al. 10.1007/s11869-023-01434-w
- Isolating Large‐Scale Smoke Impacts on Cloud and Precipitation Processes Over the Amazon With Convection Permitting Resolution R. Herbert et al. 10.1029/2021JD034615
- An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic A. Dobracki et al. 10.5194/acp-23-4775-2023
- Acceleration of the southern African easterly jet driven by the radiative effect of biomass burning aerosols and its impact on transport during AEROCLO-sA J. Chaboureau et al. 10.5194/acp-22-8639-2022
- Black carbon aerosol reductions during COVID-19 confinement quantified by aircraft measurements over Europe O. Krüger et al. 10.5194/acp-22-8683-2022
- Vertical variability of the properties of highly aged biomass burning aerosol transported over the southeast Atlantic during CLARIFY-2017 H. Wu et al. 10.5194/acp-20-12697-2020
- Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories G. Unfer et al. 10.5194/acp-24-3869-2024
- Relationship between Land Use and Spatial Variability of Atmospheric Brown Carbon and Black Carbon Aerosols in Amazonia F. Morais et al. 10.3390/atmos13081328
- How weather events modify aerosol particle size distributions in the Amazon boundary layer L. Machado et al. 10.5194/acp-21-18065-2021
- Analysis of the Influence of Deforestation on the Microphysical Parameters of Clouds in the Amazon H. da Silva et al. 10.3390/rs14215353
- Vertical profiles of trace gas and aerosol properties over the eastern North Atlantic: variations with season and synoptic condition Y. Wang et al. 10.5194/acp-21-11079-2021
- Using the Black Carbon Particle Mixing State to Characterize the Lifecycle of Biomass Burning Aerosols A. Sedlacek et al. 10.1021/acs.est.2c03851
- Aerosols from anthropogenic and biogenic sources and their interactions – modeling aerosol formation, optical properties, and impacts over the central Amazon basin J. Nascimento et al. 10.5194/acp-21-6755-2021
- Relationship between El Niño-Southern Oscillation and Atmospheric Aerosols in the Legal Amazon A. Pereira et al. 10.3390/cli12020013
- Cloud droplet formation at the base of tropical convective clouds: closure between modeling and measurement results of ACRIDICON–CHUVA R. Braga et al. 10.5194/acp-21-17513-2021
- Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest R. Herbert & P. Stier 10.5194/acp-23-4595-2023
- Detrainment Dominates CCN Concentrations Around Non‐Precipitating Convective Clouds Over the Amazon R. Braga et al. 10.1029/2022GL100411
- Concentrations and biosphere–atmosphere fluxes of inorganic trace gases and associated ionic aerosol counterparts over the Amazon rainforest R. Ramsay et al. 10.5194/acp-20-15551-2020
- Transport and Variability of Tropospheric Ozone over Oceania and Southern Pacific during the 2019–20 Australian Bushfires N. Bègue et al. 10.3390/rs13163092
- Total OH reactivity over the Amazon rainforest: variability with temperature, wind, rain, altitude, time of day, season, and an overall budget closure E. Pfannerstill et al. 10.5194/acp-21-6231-2021
Latest update: 29 Jun 2024
Short summary
Biomass burning smoke from African savanna and grassland is transported across the South Atlantic Ocean in defined layers within the free troposphere. The combination of in situ aircraft and ground-based measurements aided by satellite observations showed that these layers are transported into the Amazon Basin during the early dry season. The influx of aged smoke, enriched in black carbon and cloud condensation nuclei, has important implications for the Amazonian aerosol and cloud cycling.
Biomass burning smoke from African savanna and grassland is transported across the South...
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