Articles | Volume 20, issue 7
https://doi.org/10.5194/acp-20-4105-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-4105-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
06 Apr 2020
Research article |
| 06 Apr 2020
| 06 Apr 2020
Bromine from short-lived source gases in the extratropical northern hemispheric upper troposphere and lower stratosphere (UTLS)
Timo Keber
CORRESPONDING AUTHOR
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Harald Bönisch
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
now at: Karlsruhe Institute of Technology, Institute of Meteorology and
Climate Research, Hermann-von-Helmholtz-Platz 1, 76344
Eggenstein-Leopoldshafen, Germany
Carl Hartick
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
now at: Research Centre Jülich, Institute for Agrosphere (IBG-3),
Wilhelm-Johnen-Straße, 52428 Jülich, Germany
Marius Hauck
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Fides Lefrancois
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Florian Obersteiner
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
now at: Karlsruhe Institute of Technology, Institute of Meteorology and
Climate Research, Hermann-von-Helmholtz-Platz 1, 76344
Eggenstein-Leopoldshafen, Germany
Akima Ringsdorf
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
now at: Atmospheric Chemistry Division, Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128
Mainz, Germany
Nils Schohl
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Tanja Schuck
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Ryan Hossaini
Lancaster Environment Centre, Lancaster University, Lancaster, LA1 4YQ, UK
Phoebe Graf
Institut für Physik der Atmosphäre, Deutsches Zentrum für
Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Patrick Jöckel
Institut für Physik der Atmosphäre, Deutsches Zentrum für
Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Andreas Engel
CORRESPONDING AUTHOR
Institute for Atmospheric and Environmental
Sciences, University of Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
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Cited
19 citations as recorded by crossref.
- Cloud-scale modelling of the impact of deep convection on the fate of oceanic bromoform in the troposphere: a case study over the west coast of Borneo P. Hamer et al. 10.5194/acp-21-16955-2021
- Changes in tropospheric air quality related to the protection of stratospheric ozone in a changing climate S. Madronich et al. 10.1007/s43630-023-00369-6
- Intercomparison Between Surrogate, Explicit, and Full Treatments of VSL Bromine Chemistry Within the CAM‐Chem Chemistry‐Climate Model R. Fernandez et al. 10.1029/2020GL091125
- Investigating the radiative effect of Arctic cirrus measured in situ during the winter 2015–2016 A. Marsing et al. 10.5194/acp-23-587-2023
- In situ observations of CH<sub>2</sub>Cl<sub>2</sub> and CHCl<sub>3</sub> show efficient transport pathways for very short-lived species into the lower stratosphere via the Asian and the North American summer monsoon V. Lauther et al. 10.5194/acp-22-2049-2022
- Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere: insights into the transport pathways and total bromine M. Rotermund et al. 10.5194/acp-21-15375-2021
- Anthropogenic Bromoform at the Extratropical Tropopause Y. Jia et al. 10.1029/2023GL102894
- Atmospheric impacts of chlorinated very short-lived substances over the recent past – Part 1: Stratospheric chlorine budget and the role of transport E. Bednarz et al. 10.5194/acp-22-10657-2022
- Mean age from observations in the lowermost stratosphere: an improved method and interhemispheric differences T. Wagenhäuser et al. 10.5194/acp-23-3887-2023
- Environmental effects of stratospheric ozone depletion, UV radiation, and interactions with climate change: UNEP Environmental Effects Assessment Panel, Update 2020 R. Neale et al. 10.1007/s43630-020-00001-x
- Atmospheric impacts of chlorinated very short-lived substances over the recent past – Part 2: Impacts on ozone E. Bednarz et al. 10.5194/acp-23-13701-2023
- Global seasonal distribution of CH2Br2 and CHBr3 in the upper troposphere and lower stratosphere M. Jesswein et al. 10.5194/acp-22-15049-2022
- A convolution of observational and model data to estimate age of air spectra in the northern hemispheric lower stratosphere M. Hauck et al. 10.5194/acp-20-8763-2020
- Comparison of inorganic chlorine in the Antarctic and Arctic lowermost stratosphere by separate late winter aircraft measurements M. Jesswein et al. 10.5194/acp-21-17225-2021
- Seasonal Variations of SF6, CO2, CH4, and N2O in the UT/LS Region due to Emissions, Transport, and Chemistry J. Bisht et al. 10.1029/2020JD033541
- Measurements and Modeling of the Interhemispheric Differences of Atmospheric Chlorinated Very Short‐Lived Substances B. Roozitalab et al. 10.1029/2023JD039518
- The Michelson Interferometer for Passive Atmospheric Sounding global climatology of BrONO<sub>2</sub> 2002–2012: a test for stratospheric bromine chemistry M. Höpfner et al. 10.5194/acp-21-18433-2021
- The interhemispheric gradient of SF6 in the upper troposphere T. Schuck et al. 10.5194/acp-24-689-2024
- Stability of halocarbons in air samples stored in stainless- steel canisters T. Schuck et al. 10.5194/amt-13-73-2020
18 citations as recorded by crossref.
- Cloud-scale modelling of the impact of deep convection on the fate of oceanic bromoform in the troposphere: a case study over the west coast of Borneo P. Hamer et al. 10.5194/acp-21-16955-2021
- Changes in tropospheric air quality related to the protection of stratospheric ozone in a changing climate S. Madronich et al. 10.1007/s43630-023-00369-6
- Intercomparison Between Surrogate, Explicit, and Full Treatments of VSL Bromine Chemistry Within the CAM‐Chem Chemistry‐Climate Model R. Fernandez et al. 10.1029/2020GL091125
- Investigating the radiative effect of Arctic cirrus measured in situ during the winter 2015–2016 A. Marsing et al. 10.5194/acp-23-587-2023
- In situ observations of CH<sub>2</sub>Cl<sub>2</sub> and CHCl<sub>3</sub> show efficient transport pathways for very short-lived species into the lower stratosphere via the Asian and the North American summer monsoon V. Lauther et al. 10.5194/acp-22-2049-2022
- Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere: insights into the transport pathways and total bromine M. Rotermund et al. 10.5194/acp-21-15375-2021
- Anthropogenic Bromoform at the Extratropical Tropopause Y. Jia et al. 10.1029/2023GL102894
- Atmospheric impacts of chlorinated very short-lived substances over the recent past – Part 1: Stratospheric chlorine budget and the role of transport E. Bednarz et al. 10.5194/acp-22-10657-2022
- Mean age from observations in the lowermost stratosphere: an improved method and interhemispheric differences T. Wagenhäuser et al. 10.5194/acp-23-3887-2023
- Environmental effects of stratospheric ozone depletion, UV radiation, and interactions with climate change: UNEP Environmental Effects Assessment Panel, Update 2020 R. Neale et al. 10.1007/s43630-020-00001-x
- Atmospheric impacts of chlorinated very short-lived substances over the recent past – Part 2: Impacts on ozone E. Bednarz et al. 10.5194/acp-23-13701-2023
- Global seasonal distribution of CH2Br2 and CHBr3 in the upper troposphere and lower stratosphere M. Jesswein et al. 10.5194/acp-22-15049-2022
- A convolution of observational and model data to estimate age of air spectra in the northern hemispheric lower stratosphere M. Hauck et al. 10.5194/acp-20-8763-2020
- Comparison of inorganic chlorine in the Antarctic and Arctic lowermost stratosphere by separate late winter aircraft measurements M. Jesswein et al. 10.5194/acp-21-17225-2021
- Seasonal Variations of SF6, CO2, CH4, and N2O in the UT/LS Region due to Emissions, Transport, and Chemistry J. Bisht et al. 10.1029/2020JD033541
- Measurements and Modeling of the Interhemispheric Differences of Atmospheric Chlorinated Very Short‐Lived Substances B. Roozitalab et al. 10.1029/2023JD039518
- The Michelson Interferometer for Passive Atmospheric Sounding global climatology of BrONO<sub>2</sub> 2002–2012: a test for stratospheric bromine chemistry M. Höpfner et al. 10.5194/acp-21-18433-2021
- The interhemispheric gradient of SF6 in the upper troposphere T. Schuck et al. 10.5194/acp-24-689-2024
1 citations as recorded by crossref.
Latest update: 23 Nov 2024
Short summary
In this paper we summarize observations of short-lived halocarbons in the tropopause region. We show that, especially during winter, the levels of short-lived bromine gases at the extratropical tropopause are higher than at the tropical tropopause. We discuss the impact of the distributions on stratospheric bromine levels and compare our observations to two models with four different emission scenarios.
In this paper we summarize observations of short-lived halocarbons in the tropopause region. We...
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