Measurement report: dual-carbon isotopic characterization of carbonaceous aerosol reveals different primary and secondary sources in Beijing and Xi'an during severe haze events
Haiyan Ni,Ru-Jin Huang,Max M. Cosijn,Lu Yang,Jie Guo,Junji Cao,and Ulrike Dusek
Haiyan Ni
State Key Laboratory of Loess and Quaternary Geology, Center for
Excellence in Quaternary Science and Global Change, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an, 710061, China
Centre for Isotope Research (CIO), Energy and Sustainability Research
Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG,
the Netherlands
State Key Laboratory of Loess and Quaternary Geology, Center for
Excellence in Quaternary Science and Global Change, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an, 710061, China
Institute of Global Environmental Change, Xi'an Jiaotong University,
Xi'an, 710049, China
Max M. Cosijn
Centre for Isotope Research (CIO), Energy and Sustainability Research
Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG,
the Netherlands
Lu Yang
State Key Laboratory of Loess and Quaternary Geology, Center for
Excellence in Quaternary Science and Global Change, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an, 710061, China
Jie Guo
State Key Laboratory of Loess and Quaternary Geology, Center for
Excellence in Quaternary Science and Global Change, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an, 710061, China
Junji Cao
State Key Laboratory of Loess and Quaternary Geology, Center for
Excellence in Quaternary Science and Global Change, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an, 710061, China
Ulrike Dusek
Centre for Isotope Research (CIO), Energy and Sustainability Research
Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG,
the Netherlands
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We investigated sources of carbonaceous aerosols in Beijing and Xi'an during severe winter haze. Elemental carbon (EC) was dominated by vehicle emissions in Xi’an and coal burning in Beijing. Organic carbon (OC) increment during haze days was driven by the increase in primary and secondary OC (SOC). SOC was more from fossil sources in Beijing than Xi’an, especially during haze days. In Xi’an, no strong day–night differences in EC or OC sources suggest a large accumulation of particles.
We investigated sources of carbonaceous aerosols in Beijing and Xi'an during severe winter haze....
