Articles | Volume 20, issue 20
https://doi.org/10.5194/acp-20-12223-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-12223-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Global modeling of cloud water acidity, precipitation acidity, and acid inputs to ecosystems
Harvard John A. Paulson School of Engineering and Applied Sciences,
Harvard University, Cambridge, MA, USA
Daniel J. Jacob
Harvard John A. Paulson School of Engineering and Applied Sciences,
Harvard University, Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University,
Cambridge, MA, USA
Jonathan M. Moch
Department of Earth and Planetary Sciences, Harvard University,
Cambridge, MA, USA
Xuan Wang
Harvard John A. Paulson School of Engineering and Applied Sciences,
Harvard University, Cambridge, MA, USA
now at: School of Energy and Environment, City University of
Hong Kong, Hong Kong SAR, China
Shixian Zhai
Harvard John A. Paulson School of Engineering and Applied Sciences,
Harvard University, Cambridge, MA, USA
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Latest update: 13 Dec 2024
Short summary
Cloud water pH affects atmospheric chemistry, and acid rain damages ecosystems. We use model simulations along with observations to present a global view of cloud water and precipitation pH. Sulfuric acid, nitric acid, and ammonia control the pH in the northern midlatitudes, but carboxylic acids and dust cations are important in the tropics and subtropics. The acid inputs to many nitrogen-saturated ecosystems are high enough to cause acidification, with ammonium as the main acidifying species.
Cloud water pH affects atmospheric chemistry, and acid rain damages ecosystems. We use model...
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