Articles | Volume 19, issue 15
https://doi.org/10.5194/acp-19-9887-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-9887-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Aug 2019
Research article |
| 07 Aug 2019
| 07 Aug 2019
Photochemical aging of atmospherically reactive organic compounds involving brown carbon at the air–aqueous interface
Siyang Li
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
Xiaotong Jiang
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
Marie Roveretto
University of Lyon, Université Claude Bernard Lyon 1, CNRS,
IRCELYON, 69626 Villeurbanne, France
Christian George
School of Environmental Science and Engineering, Shandong University,
Binhai Road 72, Qingdao 266237, China
University of Lyon, Université Claude Bernard Lyon 1, CNRS,
IRCELYON, 69626 Villeurbanne, France
Ling Liu
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
Wei Jiang
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
Qingzhu Zhang
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
Wenxing Wang
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
State Key Laboratory for Structural Chemistry of Unstable and Stable
Species, CAS Research/Education Center for Excellence in Molecular Sciences,
Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
Environment Research Institute, Shandong University, Binhai Road 72,
Qingdao 266237, China
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Cited
15 citations as recorded by crossref.
- Naphthalene‐Derived Secondary Organic Aerosols Interfacial Photosensitizing Properties X. Wang et al. 10.1029/2021GL093465
- Research progress on secondary formation, photosensitive reaction mechanism and human health effects of chromophoric brown carbon B. Chen et al. 10.1016/j.jes.2024.04.003
- Insoluble lipid film mediates transfer of soluble saccharides from the sea to the atmosphere: the role of hydrogen bonding M. Xu et al. 10.5194/acp-23-2235-2023
- Atmospheric chemical processes of microcystin-LR at the interface of sea spray aerosol M. Xu et al. 10.1016/j.chemosphere.2022.133726
- Photosensitization mechanisms at the air–water interface of aqueous aerosols M. Martins-Costa et al. 10.1039/D1SC06866K
- Spatiotemporal distribution, light absorption characteristics, and source apportionments of black and brown carbon in China N. Cao et al. 10.1016/j.scitotenv.2024.170796
- Enhanced sulfate formation in mixed biomass burning and sea-salt interactions mediated by photosensitization: effects of chloride, nitrogen-containing compounds, and atmospheric aging R. Tang et al. 10.5194/acp-25-425-2025
- The reaction of oleic acid monolayers with gas-phase ozone at the air water interface: the effect of sub-phase viscosity, and inert secondary components M. King et al. 10.1039/D0CP03934A
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Impact of Environmental Conditions on Secondary Organic Aerosol Production from Photosensitized Humic Acid A. Fankhauser et al. 10.1021/acs.est.9b07485
- Emission and optical characteristics of brown carbon in size-segregated particles from three types of Chinese ships F. Yang et al. 10.1016/j.jes.2023.05.045
- New Analytical Paradigm to Determine Concentration of Brown Carbon and Its Sample-by-Sample Mass Absorption Efficiency K. Liao et al. 10.1021/acs.est.4c06831
- Links between the optical properties and chemical compositions of brown carbon chromophores in different environments: Contributions and formation of functionalized aromatic compounds X. Li et al. 10.1016/j.scitotenv.2021.147418
- Exploring the influence of particle phase in the ozonolysis of oleic and elaidic acid R. Kaur Kohli et al. 10.1080/02786826.2023.2226183
- Oligomerization Mechanism of Methylglyoxal Regulated by the Methyl Groups in Reduced Nitrogen Species: Implications for Brown Carbon Formation Q. Shi et al. 10.1021/acs.est.3c05983
15 citations as recorded by crossref.
- Naphthalene‐Derived Secondary Organic Aerosols Interfacial Photosensitizing Properties X. Wang et al. 10.1029/2021GL093465
- Research progress on secondary formation, photosensitive reaction mechanism and human health effects of chromophoric brown carbon B. Chen et al. 10.1016/j.jes.2024.04.003
- Insoluble lipid film mediates transfer of soluble saccharides from the sea to the atmosphere: the role of hydrogen bonding M. Xu et al. 10.5194/acp-23-2235-2023
- Atmospheric chemical processes of microcystin-LR at the interface of sea spray aerosol M. Xu et al. 10.1016/j.chemosphere.2022.133726
- Photosensitization mechanisms at the air–water interface of aqueous aerosols M. Martins-Costa et al. 10.1039/D1SC06866K
- Spatiotemporal distribution, light absorption characteristics, and source apportionments of black and brown carbon in China N. Cao et al. 10.1016/j.scitotenv.2024.170796
- Enhanced sulfate formation in mixed biomass burning and sea-salt interactions mediated by photosensitization: effects of chloride, nitrogen-containing compounds, and atmospheric aging R. Tang et al. 10.5194/acp-25-425-2025
- The reaction of oleic acid monolayers with gas-phase ozone at the air water interface: the effect of sub-phase viscosity, and inert secondary components M. King et al. 10.1039/D0CP03934A
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Impact of Environmental Conditions on Secondary Organic Aerosol Production from Photosensitized Humic Acid A. Fankhauser et al. 10.1021/acs.est.9b07485
- Emission and optical characteristics of brown carbon in size-segregated particles from three types of Chinese ships F. Yang et al. 10.1016/j.jes.2023.05.045
- New Analytical Paradigm to Determine Concentration of Brown Carbon and Its Sample-by-Sample Mass Absorption Efficiency K. Liao et al. 10.1021/acs.est.4c06831
- Links between the optical properties and chemical compositions of brown carbon chromophores in different environments: Contributions and formation of functionalized aromatic compounds X. Li et al. 10.1016/j.scitotenv.2021.147418
- Exploring the influence of particle phase in the ozonolysis of oleic and elaidic acid R. Kaur Kohli et al. 10.1080/02786826.2023.2226183
- Oligomerization Mechanism of Methylglyoxal Regulated by the Methyl Groups in Reduced Nitrogen Species: Implications for Brown Carbon Formation Q. Shi et al. 10.1021/acs.est.3c05983
Latest update: 01 Jun 2025
Short summary
We stimulated the photochemical aging of organic film coated on aqueous aerosol in the presence of imidazole-2-carboxaldehyde, humic acid, an atmospheric PM2.5 sample, and a secondary organic aerosol sample from the lab. The unsaturated lipid mixed with photosensitizer under UV irradiation produced hydroperoxides, leading to surface area increase in organic film. Our results reveal the modification of organic film on aqueous aerosol has potential influence on the hygroscopic growth of droplets.
We stimulated the photochemical aging of organic film coated on aqueous aerosol in the presence...
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