Articles | Volume 19, issue 12
https://doi.org/10.5194/acp-19-8003-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-8003-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
18 Jun 2019
Research article |
| 18 Jun 2019
| 18 Jun 2019
Interaction between succinic acid and sulfuric acid–base clusters
Department of Atmospheric Sciences and Department of Chemistry,
Texas A&M University, College Station, TX 77843, USA
Department of Atmospheric Sciences and Department of Chemistry,
Texas A&M University, College Station, TX 77843, USA
Guangzhou Key Laboratory Environmental Catalysis and Pollution Control, Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control, School of Environmental Science and Engineering, Institute of Environmental Health and Pollution Control, Guangdong University of Technology, Guangzhou 510006, China
Yixin Li
Department of Atmospheric Sciences and Department of Chemistry,
Texas A&M University, College Station, TX 77843, USA
Jeremiah Secrest
Department of Atmospheric Sciences and Department of Chemistry,
Texas A&M University, College Station, TX 77843, USA
Aerodyne Research Inc, Billerica, MA 01821, USA
Fei Xu
Environment Research Institute, Shandong University, Qingdao 266237, China
Yuan Wang
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA 91125, USA
Taicheng An
Guangzhou Key Laboratory Environmental Catalysis and Pollution Control, Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control, School of Environmental Science and Engineering, Institute of Environmental Health and Pollution Control, Guangdong University of Technology, Guangzhou 510006, China
Department of Atmospheric Sciences and Department of Chemistry,
Texas A&M University, College Station, TX 77843, USA
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34 citations as recorded by crossref.
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- The effect of water molecules and air humidity on the cluster formation from benzoic acid with sulfuric acid/ammonia/dimethylamine: A molecular-scale investigation H. Wang et al. 10.1016/j.molliq.2023.123001
- Effects of Amides on the Formation of Atmospheric HONO and the Nucleation of Nitric Acid Hydrates S. Ni et al. 10.2139/ssrn.3982283
- Synergistic effect of glutaric acid and ammonia/amine/amide on their hydrates in the clustering: A theoretical study S. Ni et al. 10.1016/j.chemosphere.2021.130063
- Methanesulfonic Acid-driven New Particle Formation Enhanced by Monoethanolamine: A Computational Study J. Shen et al. 10.1021/acs.est.9b05306
- Unveiling the conformational diversity of succinic acid: Insights from IR spectroscopy and quantum chemical calculations L. Da Silva Sa et al. 10.1063/10.0028183
- Contributions of alanine and serine to sulfuric acid-based homogeneous nucleation H. Cao et al. 10.1016/j.atmosenv.2020.118139
- Observational Evidence for the Involvement of Dicarboxylic Acids in Particle Nucleation X. Fang et al. 10.1021/acs.estlett.0c00270
- The nucleation mechanism of succinic acid involved sulfuric acid - Dimethylamine in new particle formation Z. Wang et al. 10.1016/j.atmosenv.2021.118683
- Extensive urban air pollution footprint evidenced by submicron organic aerosols molecular composition C. Salvador et al. 10.1038/s41612-022-00314-x
- Sulfuric acid–dimethylamine particle formation enhanced by functional organic acids: an integrated experimental and theoretical study C. Wang et al. 10.1039/D2CP01671K
- A quantum chemical investigation of the interaction of perfluoropropionic acid with monoethanolamine and sulfuric acid in the atmosphere F. Medeiros et al. 10.1016/j.comptc.2024.114485
- A theoretical study of hydrogen-bonded molecular clusters of sulfuric acid and organic acids with amides C. Zuo et al. 10.1016/j.jes.2020.07.022
- Understanding vapor nucleation on the molecular level: A review C. Li & R. Signorell 10.1016/j.jaerosci.2020.105676
- Elucidating the Infrared Spectral Properties of Succinic Molecular Acid Crystals: Illustration of the Structure and the Hydrogen Bond Energies of the Crystal and Its Deuterated Analogs J. Hołaj-Krzak et al. 10.1021/acs.jpca.2c04440
- Enhancement of Atmospheric Nucleation Precursors on Iodic Acid-Induced Nucleation: Predictive Model and Mechanism F. Ma et al. 10.1021/acs.est.3c01034
- Spatio-temporal characteristics and source apportionment of water-soluble organic acids in PM2.5 in the North China Plain Y. Li et al. 10.1016/j.apr.2022.101540
- Hygroscopic behavior and aerosol chemistry of atmospheric particles containing organic acids and inorganic salts F. Tan et al. 10.1038/s41612-024-00752-9
- Enhancing acid–base–water ternary aerosol nucleation with organic acid: a case of tartaric acid C. Wang et al. 10.1039/D3CP00809F
- Interaction of Glutamic Acid/Protonated Glutamic Acid with Amide and Water Molecules: A Theoretical Study J. Liu et al. 10.1021/acs.jpca.2c05135
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- Modeling the formation and growth of atmospheric molecular clusters: A review J. Elm et al. 10.1016/j.jaerosci.2020.105621
- Introductory lecture: air quality in megacities L. Molina 10.1039/D0FD00123F
- The role of organic acids in new particle formation from methanesulfonic acid and methylamine R. Zhang et al. 10.5194/acp-22-2639-2022
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- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Roles of Amides on the Formation of Atmospheric HONO and the Nucleation of Nitric Acid Hydrates S. Ni et al. 10.1021/acs.jpca.3c01518
- Hydrazine and its Derivatives: Role on Nitrogen Dioxide Hydrolysis and Ensuing Nucleation in the Atmosphere S. Ni et al. 10.1002/slct.202304403
- Toward a Holistic Understanding of the Formation and Growth of Atmospheric Molecular Clusters: A Quantum Machine Learning Perspective J. Elm 10.1021/acs.jpca.0c09762
- The synergistic effect of organic and inorganic sulfonic acids promotes new particle formation Y. Ji et al. 10.1016/j.scitotenv.2023.163611
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- Quantum chemical modeling of organic enhanced atmospheric nucleation: A critical review J. Elm et al. 10.1002/wcms.1662
- Autoxidation mechanism for atmospheric oxidation of tertiary amines: Implications for secondary organic aerosol formation F. Ma et al. 10.1016/j.chemosphere.2020.129207
- Piperazine Enhancing Sulfuric Acid-Based New Particle Formation: Implications for the Atmospheric Fate of Piperazine F. Ma et al. 10.1021/acs.est.9b02117
33 citations as recorded by crossref.
- Computational chemistry of cluster: Understanding the mechanism of atmospheric new particle formation at the molecular level X. Zhang et al. 10.1016/j.chemosphere.2022.136109
- The effect of water molecules and air humidity on the cluster formation from benzoic acid with sulfuric acid/ammonia/dimethylamine: A molecular-scale investigation H. Wang et al. 10.1016/j.molliq.2023.123001
- Effects of Amides on the Formation of Atmospheric HONO and the Nucleation of Nitric Acid Hydrates S. Ni et al. 10.2139/ssrn.3982283
- Synergistic effect of glutaric acid and ammonia/amine/amide on their hydrates in the clustering: A theoretical study S. Ni et al. 10.1016/j.chemosphere.2021.130063
- Methanesulfonic Acid-driven New Particle Formation Enhanced by Monoethanolamine: A Computational Study J. Shen et al. 10.1021/acs.est.9b05306
- Unveiling the conformational diversity of succinic acid: Insights from IR spectroscopy and quantum chemical calculations L. Da Silva Sa et al. 10.1063/10.0028183
- Contributions of alanine and serine to sulfuric acid-based homogeneous nucleation H. Cao et al. 10.1016/j.atmosenv.2020.118139
- Observational Evidence for the Involvement of Dicarboxylic Acids in Particle Nucleation X. Fang et al. 10.1021/acs.estlett.0c00270
- The nucleation mechanism of succinic acid involved sulfuric acid - Dimethylamine in new particle formation Z. Wang et al. 10.1016/j.atmosenv.2021.118683
- Extensive urban air pollution footprint evidenced by submicron organic aerosols molecular composition C. Salvador et al. 10.1038/s41612-022-00314-x
- Sulfuric acid–dimethylamine particle formation enhanced by functional organic acids: an integrated experimental and theoretical study C. Wang et al. 10.1039/D2CP01671K
- A quantum chemical investigation of the interaction of perfluoropropionic acid with monoethanolamine and sulfuric acid in the atmosphere F. Medeiros et al. 10.1016/j.comptc.2024.114485
- A theoretical study of hydrogen-bonded molecular clusters of sulfuric acid and organic acids with amides C. Zuo et al. 10.1016/j.jes.2020.07.022
- Understanding vapor nucleation on the molecular level: A review C. Li & R. Signorell 10.1016/j.jaerosci.2020.105676
- Elucidating the Infrared Spectral Properties of Succinic Molecular Acid Crystals: Illustration of the Structure and the Hydrogen Bond Energies of the Crystal and Its Deuterated Analogs J. Hołaj-Krzak et al. 10.1021/acs.jpca.2c04440
- Enhancement of Atmospheric Nucleation Precursors on Iodic Acid-Induced Nucleation: Predictive Model and Mechanism F. Ma et al. 10.1021/acs.est.3c01034
- Spatio-temporal characteristics and source apportionment of water-soluble organic acids in PM2.5 in the North China Plain Y. Li et al. 10.1016/j.apr.2022.101540
- Hygroscopic behavior and aerosol chemistry of atmospheric particles containing organic acids and inorganic salts F. Tan et al. 10.1038/s41612-024-00752-9
- Enhancing acid–base–water ternary aerosol nucleation with organic acid: a case of tartaric acid C. Wang et al. 10.1039/D3CP00809F
- Interaction of Glutamic Acid/Protonated Glutamic Acid with Amide and Water Molecules: A Theoretical Study J. Liu et al. 10.1021/acs.jpca.2c05135
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Modeling the formation and growth of atmospheric molecular clusters: A review J. Elm et al. 10.1016/j.jaerosci.2020.105621
- Introductory lecture: air quality in megacities L. Molina 10.1039/D0FD00123F
- The role of organic acids in new particle formation from methanesulfonic acid and methylamine R. Zhang et al. 10.5194/acp-22-2639-2022
- The homogeneous gas-phase formation mechanisms of PCPTs/PCDTs/PCDFs from the radical/radical cross-condensation of 2-CPR and 2-CTPR: a theoretical, mechanistic and kinetics study Y. Li et al. 10.1039/D1RA00599E
- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Roles of Amides on the Formation of Atmospheric HONO and the Nucleation of Nitric Acid Hydrates S. Ni et al. 10.1021/acs.jpca.3c01518
- Hydrazine and its Derivatives: Role on Nitrogen Dioxide Hydrolysis and Ensuing Nucleation in the Atmosphere S. Ni et al. 10.1002/slct.202304403
- Toward a Holistic Understanding of the Formation and Growth of Atmospheric Molecular Clusters: A Quantum Machine Learning Perspective J. Elm 10.1021/acs.jpca.0c09762
- The synergistic effect of organic and inorganic sulfonic acids promotes new particle formation Y. Ji et al. 10.1016/j.scitotenv.2023.163611
- Atmospheric oxidation mechanism and kinetics of indole initiated by ●OH and ●Cl: a computational study J. Xue et al. 10.5194/acp-22-11543-2022
- Quantum chemical modeling of organic enhanced atmospheric nucleation: A critical review J. Elm et al. 10.1002/wcms.1662
- Autoxidation mechanism for atmospheric oxidation of tertiary amines: Implications for secondary organic aerosol formation F. Ma et al. 10.1016/j.chemosphere.2020.129207
Latest update: 19 Nov 2024
Short summary
We have investigated the molecular interactions between succinic acid and sulfuric acid–base clusters in the presence of hydration, including ammonia and dimethylamine. Our results indicate that the multicomponent nucleation involving organic acids, sulfuric acid, and base species promotes new particle formation in the atmosphere, particularly under polluted conditions.
We have investigated the molecular interactions between succinic acid and sulfuric acid–base...
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