Articles | Volume 19, issue 10
https://doi.org/10.5194/acp-19-6701-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-6701-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
The unintended consequence of SO2 and NO2 regulations over China: increase of ammonia levels and impact on PM2.5 concentrations
Mathieu Lachatre
CORRESPONDING AUTHOR
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil, Université de Paris, Institut Pierre Simon
Laplace, Créteil, France
Audrey Fortems-Cheiney
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil, Université de Paris, Institut Pierre Simon
Laplace, Créteil, France
now at: Laboratoire des Sciences du Climat et de l'Environnement, LSCE-IPSL (CEA-CNRS-UVSQ), Université Paris-Saclay, 91191 Gif-sur-Yvette, France
Gilles Foret
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil, Université de Paris, Institut Pierre Simon
Laplace, Créteil, France
Guillaume Siour
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil, Université de Paris, Institut Pierre Simon
Laplace, Créteil, France
Gaëlle Dufour
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil, Université de Paris, Institut Pierre Simon
Laplace, Créteil, France
Lieven Clarisse
Université libre de Bruxelles (ULB), Spectroscopie Atmosphérique, Service de Chimie Quantique et Photophysique, Brussels, Belgium
Cathy Clerbaux
LATMOS/IPSL, Sorbonne Université, UVSQ, CNRS, Paris, France
Université libre de Bruxelles (ULB), Spectroscopie Atmosphérique, Service de Chimie Quantique et Photophysique, Brussels, Belgium
Pierre-François Coheur
Université libre de Bruxelles (ULB), Spectroscopie Atmosphérique, Service de Chimie Quantique et Photophysique, Brussels, Belgium
Martin Van Damme
Université libre de Bruxelles (ULB), Spectroscopie Atmosphérique, Service de Chimie Quantique et Photophysique, Brussels, Belgium
Matthias Beekmann
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil, Université de Paris, Institut Pierre Simon
Laplace, Créteil, France
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Cited
67 citations as recorded by crossref.
- Summertime Urban Ammonia Emissions May Be Substantially Underestimated in Beijing, China J. Xu et al. 10.1021/acs.est.3c05266
- Impact of emissions from a single urban source on air quality estimated from mobile observation and WRF-STILT model simulations H. Fan et al. 10.1007/s11869-021-01023-9
- Global agricultural ammonia emissions simulated with the ORCHIDEE land surface model M. Beaudor et al. 10.5194/gmd-16-1053-2023
- Changes of nitrogen deposition in China from 1980 to 2018 Z. Wen et al. 10.1016/j.envint.2020.106022
- Impact of SOx, NOx and NH3 emission reductions on PM2.5 concentrations across Europe: Hints for future measure development A. Clappier et al. 10.1016/j.envint.2021.106699
- Ammonia and PM2.5 Air Pollution in Paris during the 2020 COVID Lockdown C. Viatte et al. 10.3390/atmos12020160
- Changes in ammonia and its effects on PM2.5 chemical property in three winter seasons in Beijing, China Z. Meng et al. 10.1016/j.scitotenv.2020.142208
- Simulation of organic aerosol, its precursors, and related oxidants in the Landes pine forest in southwestern France: accounting for domain-specific land use and physical conditions A. Cholakian et al. 10.5194/acp-23-3679-2023
- Estimation of surface ammonia concentrations and emissions in China from the polar-orbiting Infrared Atmospheric Sounding Interferometer and the FY-4A Geostationary Interferometric Infrared Sounder P. Liu et al. 10.5194/acp-22-9099-2022
- The IASI NH3 version 4 product: averaging kernels and improved consistency L. Clarisse et al. 10.5194/amt-16-5009-2023
- Atmospheric reactive nitrogen concentration and deposition trends from 2011 to 2018 at an urban site in north China X. Luo et al. 10.1016/j.atmosenv.2020.117298
- Possible underestimation of the coal-fired power plants to air pollution in China Z. Weng et al. 10.1016/j.resconrec.2023.107208
- Source Sectoral Impacts on Provincial PM<SUB>2.5</SUB> Concentrations based on the CAPSS 2016 using the CMAQ Model Y. Kang et al. 10.5572/KOSAE.2021.37.1.017
- Overall Characteristics of Nationwide High PM2.5 Episodes during 2013~2016 Y. Ghim et al. 10.5572/KOSAE.2019.35.5.609
- Tracking ammonia morning peak, sources and transport with 1 Hz measurements at a rural site in North China Plain Y. He et al. 10.1016/j.atmosenv.2020.117630
- Effect of global atmospheric aerosol emission change on PM2.5-related health impacts X. Seposo et al. 10.1080/16549716.2019.1664130
- Non-linear response of PM<sub>2.5</sub> to changes in NO<sub><i>x</i></sub> and NH<sub>3</sub> emissions in the Po basin (Italy): consequences for air quality plans P. Thunis et al. 10.5194/acp-21-9309-2021
- Spatiotemporal variations of atmospheric nitrogen deposition in China during 2008–2020 S. Chen et al. 10.1016/j.atmosenv.2023.120120
- Characteristics of PM2.5 and secondary inorganic pollution formation during the heating season of 2021 in Beijing J. Wang et al. 10.3389/fenvs.2022.1028468
- Bias in ammonia emission inventory and implications on emission control of nitrogen oxides over North China Plain Q. Zhang et al. 10.1016/j.atmosenv.2019.116869
- Spatiotemporal variations of nitrogen and phosphorus deposition across China Z. Wen et al. 10.1016/j.scitotenv.2022.154740
- Paradigm shift in aerosol chemical composition over regions downwind of China I. Uno et al. 10.1038/s41598-020-63592-6
- Does Ambient Secondary Conversion or the Prolonged Fast Conversion in Combustion Plumes Cause Severe PM2.5 Air Pollution in China? Y. Shen et al. 10.3390/atmos13050673
- Changes of precipitation acidity related to sulfur and nitrogen deposition in forests across three continents in north hemisphere over last two decades C. Chang et al. 10.1016/j.scitotenv.2021.150552
- Sources, Variations, and Effects on Air Quality of Atmospheric Ammonia Z. Lan et al. 10.1007/s40726-023-00291-6
- Contrasting change trends in dry and wet nitrogen depositions during 2011 to 2020: Evidence from an agricultural catchment in subtropical Central China W. Jiang et al. 10.1016/j.scitotenv.2023.168094
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- Direct and cross impacts of upwind emission control on downwind PM2.5 under various NH3 conditions in Northeast Asia E. Kim et al. 10.1016/j.envpol.2020.115794
- Role of Ammonia on the Feedback Between AWC and Inorganic Aerosol Formation During Heavy Pollution in the North China Plain B. Ge et al. 10.1029/2019EA000799
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- Simple Framework to Quantify the Contributions from Different Factors Influencing Aerosol pH Based on NHx Phase-Partitioning Equilibrium Y. Tao & J. Murphy 10.1021/acs.est.1c03103
- Reduction potential of ammonia emissions and impact on PM2.5 in a megacity of central China M. Zheng et al. 10.1016/j.envpol.2023.123172
- Understanding the Simulated Ammonia Increasing Trend from 2008 to 2015 over Europe with CHIMERE and Comparison with IASI Observations A. Fortems-Cheiney et al. 10.3390/atmos13071101
- Assessing the emission sources and reduction potential of atmospheric ammonia at an urban site in Northeast China X. Sun et al. 10.1016/j.envres.2021.111230
- Control of particulate nitrate air pollution in China S. Zhai et al. 10.1038/s41561-021-00726-z
- Meteorological variations impeded the benefits of recent NOx mitigation in reducing atmospheric nitrate deposition in the Pearl River Delta region, Southeast China B. Zhong et al. 10.1016/j.envpol.2020.115076
- Long-term spatiotemporal variations of ammonia in the Yangtze River Delta region of China and its driving factors J. Xue et al. 10.1016/j.jes.2024.02.021
- The formation of secondary inorganic aerosols: A data-driven investigation of Lombardy's secondary inorganic aerosol problem F. Granella et al. 10.1016/j.atmosenv.2024.120480
- Global, regional and national trends of atmospheric ammonia derived from a decadal (2008–2018) satellite record M. Van Damme et al. 10.1088/1748-9326/abd5e0
- Increased Aerosol Extinction Efficiency Hinders Visibility Improvement in Eastern China J. Liu et al. 10.1029/2020GL090167
- Effects of reactive nitrogen gases on the aerosol formation in Beijing from late autumn to early spring Z. Wen et al. 10.1088/1748-9326/abd973
- Are Cyclic Volatile Methylsiloxanes POPs? For Rigorous Science in Regulatory Decision Making M. McLachlan & F. Wania 10.1021/acs.est.4c02428
- Self-regulated catalysis for the selective synthesis of primary amines from carbonyl compounds M. Gao et al. 10.1039/D1GC01275D
- Multiscale observations of NH<sub>3</sub> around Toronto, Canada S. Yamanouchi et al. 10.5194/amt-14-905-2021
- Estimating global ammonia (NH3) emissions based on IASI observations from 2008 to 2018 Z. Luo et al. 10.5194/acp-22-10375-2022
- Global estimates of dry ammonia deposition inferred from space-measurements L. Liu et al. 10.1016/j.scitotenv.2020.139189
- Air quality and health co-benefits of China’s carbon dioxide emissions peaking before 2030 R. Tang et al. 10.1038/s41467-022-28672-3
- A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements W. Zhou et al. 10.1039/D0EM00212G
- Societal benefits of halving agricultural ammonia emissions in China far exceed the abatement costs X. Zhang et al. 10.1038/s41467-020-18196-z
- Spatio-temporal patterns of air pollution in China from 2015 to 2018 and implications for health risks M. Kuerban et al. 10.1016/j.envpol.2019.113659
- Sensitivity of fine particulate matter concentrations in South Korea to regional ammonia emissions in Northeast Asia E. Kim et al. 10.1016/j.envpol.2021.116428
- Regional Transport Increases Ammonia Concentration in Beijing, China Q. Wang et al. 10.3390/atmos11060563
- Atmospheric ammonia point source detection technique at regional scale using high resolution satellite imagery and deep learning M. Lei et al. 10.1016/j.atmosres.2021.105587
- Evidence and causes of recent decreases in nitrogen deposition in temperate forests in Northeast China Y. Wang et al. 10.1016/j.scitotenv.2024.172472
- 10-year satellite-constrained fluxes of ammonia improve performance of chemistry transport models N. Evangeliou et al. 10.5194/acp-21-4431-2021
- Evidence for global increases in urban ammonia pollution and their drivers S. Liu et al. 10.1016/j.scitotenv.2024.176846
- Enhanced Wet Deposition of Nitrogen Induced by a Landfalling Typhoon over East Asia: Implications for the Marine Eco-Environment Y. Zhang et al. 10.1021/acs.estlett.2c00762
- Tracking down global NH<sub>3</sub> point sources with wind-adjusted superresolution L. Clarisse et al. 10.5194/amt-12-5457-2019
- Frontiers of graphene and 2D material-based gas sensors for environmental monitoring D. Buckley et al. 10.1088/2053-1583/ab7bc5
- Air Quality Degradation by Mineral Dust over Beijing, Chengdu and Shanghai Chinese Megacities M. Lachatre et al. 10.3390/atmos11070708
- Estimation and variation analysis of secondary inorganic aerosols across the Greater Bay Area in 2005 and 2015 Y. Chen et al. 10.1016/j.chemosphere.2021.133393
- Record high levels of atmospheric ammonia over India: Spatial and temporal analyses J. Kuttippurath et al. 10.1016/j.scitotenv.2020.139986
- Responses of sulfate and nitrate to anthropogenic emission changes in eastern China - in perspective of long-term variations L. Qi et al. 10.1016/j.scitotenv.2022.158875
- Responses of nitrogen and sulfur deposition to NH3 emission control in the Yangtze River Delta, China Z. Dong et al. 10.1016/j.envpol.2022.119646
- Lower tropospheric ozone over the North China Plain: variability and trends revealed by IASI satellite observations for 2008–2016 G. Dufour et al. 10.5194/acp-18-16439-2018
66 citations as recorded by crossref.
- Summertime Urban Ammonia Emissions May Be Substantially Underestimated in Beijing, China J. Xu et al. 10.1021/acs.est.3c05266
- Impact of emissions from a single urban source on air quality estimated from mobile observation and WRF-STILT model simulations H. Fan et al. 10.1007/s11869-021-01023-9
- Global agricultural ammonia emissions simulated with the ORCHIDEE land surface model M. Beaudor et al. 10.5194/gmd-16-1053-2023
- Changes of nitrogen deposition in China from 1980 to 2018 Z. Wen et al. 10.1016/j.envint.2020.106022
- Impact of SOx, NOx and NH3 emission reductions on PM2.5 concentrations across Europe: Hints for future measure development A. Clappier et al. 10.1016/j.envint.2021.106699
- Ammonia and PM2.5 Air Pollution in Paris during the 2020 COVID Lockdown C. Viatte et al. 10.3390/atmos12020160
- Changes in ammonia and its effects on PM2.5 chemical property in three winter seasons in Beijing, China Z. Meng et al. 10.1016/j.scitotenv.2020.142208
- Simulation of organic aerosol, its precursors, and related oxidants in the Landes pine forest in southwestern France: accounting for domain-specific land use and physical conditions A. Cholakian et al. 10.5194/acp-23-3679-2023
- Estimation of surface ammonia concentrations and emissions in China from the polar-orbiting Infrared Atmospheric Sounding Interferometer and the FY-4A Geostationary Interferometric Infrared Sounder P. Liu et al. 10.5194/acp-22-9099-2022
- The IASI NH3 version 4 product: averaging kernels and improved consistency L. Clarisse et al. 10.5194/amt-16-5009-2023
- Atmospheric reactive nitrogen concentration and deposition trends from 2011 to 2018 at an urban site in north China X. Luo et al. 10.1016/j.atmosenv.2020.117298
- Possible underestimation of the coal-fired power plants to air pollution in China Z. Weng et al. 10.1016/j.resconrec.2023.107208
- Source Sectoral Impacts on Provincial PM<SUB>2.5</SUB> Concentrations based on the CAPSS 2016 using the CMAQ Model Y. Kang et al. 10.5572/KOSAE.2021.37.1.017
- Overall Characteristics of Nationwide High PM2.5 Episodes during 2013~2016 Y. Ghim et al. 10.5572/KOSAE.2019.35.5.609
- Tracking ammonia morning peak, sources and transport with 1 Hz measurements at a rural site in North China Plain Y. He et al. 10.1016/j.atmosenv.2020.117630
- Effect of global atmospheric aerosol emission change on PM2.5-related health impacts X. Seposo et al. 10.1080/16549716.2019.1664130
- Non-linear response of PM<sub>2.5</sub> to changes in NO<sub><i>x</i></sub> and NH<sub>3</sub> emissions in the Po basin (Italy): consequences for air quality plans P. Thunis et al. 10.5194/acp-21-9309-2021
- Spatiotemporal variations of atmospheric nitrogen deposition in China during 2008–2020 S. Chen et al. 10.1016/j.atmosenv.2023.120120
- Characteristics of PM2.5 and secondary inorganic pollution formation during the heating season of 2021 in Beijing J. Wang et al. 10.3389/fenvs.2022.1028468
- Bias in ammonia emission inventory and implications on emission control of nitrogen oxides over North China Plain Q. Zhang et al. 10.1016/j.atmosenv.2019.116869
- Spatiotemporal variations of nitrogen and phosphorus deposition across China Z. Wen et al. 10.1016/j.scitotenv.2022.154740
- Paradigm shift in aerosol chemical composition over regions downwind of China I. Uno et al. 10.1038/s41598-020-63592-6
- Does Ambient Secondary Conversion or the Prolonged Fast Conversion in Combustion Plumes Cause Severe PM2.5 Air Pollution in China? Y. Shen et al. 10.3390/atmos13050673
- Changes of precipitation acidity related to sulfur and nitrogen deposition in forests across three continents in north hemisphere over last two decades C. Chang et al. 10.1016/j.scitotenv.2021.150552
- Sources, Variations, and Effects on Air Quality of Atmospheric Ammonia Z. Lan et al. 10.1007/s40726-023-00291-6
- Contrasting change trends in dry and wet nitrogen depositions during 2011 to 2020: Evidence from an agricultural catchment in subtropical Central China W. Jiang et al. 10.1016/j.scitotenv.2023.168094
- Atmospheric NH3 in urban Beijing: long-term variations and implications for secondary inorganic aerosol control Z. Lan et al. 10.5194/acp-24-9355-2024
- Direct and cross impacts of upwind emission control on downwind PM2.5 under various NH3 conditions in Northeast Asia E. Kim et al. 10.1016/j.envpol.2020.115794
- Role of Ammonia on the Feedback Between AWC and Inorganic Aerosol Formation During Heavy Pollution in the North China Plain B. Ge et al. 10.1029/2019EA000799
- Trends of inorganic and organic aerosols and precursor gases in Europe: insights from the EURODELTA multi-model experiment over the 1990–2010 period G. Ciarelli et al. 10.5194/gmd-12-4923-2019
- Temporal variations and spatial distributions of gaseous and particulate air pollutants and their health risks during 2015–2019 in China W. Zhou et al. 10.1016/j.envpol.2020.116031
- Ground-based measurements of atmospheric NH3 by Fourier transform infrared spectrometry at Hefei and comparisons with IASI data W. Wang et al. 10.1016/j.atmosenv.2022.119256
- Simple Framework to Quantify the Contributions from Different Factors Influencing Aerosol pH Based on NHx Phase-Partitioning Equilibrium Y. Tao & J. Murphy 10.1021/acs.est.1c03103
- Reduction potential of ammonia emissions and impact on PM2.5 in a megacity of central China M. Zheng et al. 10.1016/j.envpol.2023.123172
- Understanding the Simulated Ammonia Increasing Trend from 2008 to 2015 over Europe with CHIMERE and Comparison with IASI Observations A. Fortems-Cheiney et al. 10.3390/atmos13071101
- Assessing the emission sources and reduction potential of atmospheric ammonia at an urban site in Northeast China X. Sun et al. 10.1016/j.envres.2021.111230
- Control of particulate nitrate air pollution in China S. Zhai et al. 10.1038/s41561-021-00726-z
- Meteorological variations impeded the benefits of recent NOx mitigation in reducing atmospheric nitrate deposition in the Pearl River Delta region, Southeast China B. Zhong et al. 10.1016/j.envpol.2020.115076
- Long-term spatiotemporal variations of ammonia in the Yangtze River Delta region of China and its driving factors J. Xue et al. 10.1016/j.jes.2024.02.021
- The formation of secondary inorganic aerosols: A data-driven investigation of Lombardy's secondary inorganic aerosol problem F. Granella et al. 10.1016/j.atmosenv.2024.120480
- Global, regional and national trends of atmospheric ammonia derived from a decadal (2008–2018) satellite record M. Van Damme et al. 10.1088/1748-9326/abd5e0
- Increased Aerosol Extinction Efficiency Hinders Visibility Improvement in Eastern China J. Liu et al. 10.1029/2020GL090167
- Effects of reactive nitrogen gases on the aerosol formation in Beijing from late autumn to early spring Z. Wen et al. 10.1088/1748-9326/abd973
- Are Cyclic Volatile Methylsiloxanes POPs? For Rigorous Science in Regulatory Decision Making M. McLachlan & F. Wania 10.1021/acs.est.4c02428
- Self-regulated catalysis for the selective synthesis of primary amines from carbonyl compounds M. Gao et al. 10.1039/D1GC01275D
- Multiscale observations of NH<sub>3</sub> around Toronto, Canada S. Yamanouchi et al. 10.5194/amt-14-905-2021
- Estimating global ammonia (NH3) emissions based on IASI observations from 2008 to 2018 Z. Luo et al. 10.5194/acp-22-10375-2022
- Global estimates of dry ammonia deposition inferred from space-measurements L. Liu et al. 10.1016/j.scitotenv.2020.139189
- Air quality and health co-benefits of China’s carbon dioxide emissions peaking before 2030 R. Tang et al. 10.1038/s41467-022-28672-3
- A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements W. Zhou et al. 10.1039/D0EM00212G
- Societal benefits of halving agricultural ammonia emissions in China far exceed the abatement costs X. Zhang et al. 10.1038/s41467-020-18196-z
- Spatio-temporal patterns of air pollution in China from 2015 to 2018 and implications for health risks M. Kuerban et al. 10.1016/j.envpol.2019.113659
- Sensitivity of fine particulate matter concentrations in South Korea to regional ammonia emissions in Northeast Asia E. Kim et al. 10.1016/j.envpol.2021.116428
- Regional Transport Increases Ammonia Concentration in Beijing, China Q. Wang et al. 10.3390/atmos11060563
- Atmospheric ammonia point source detection technique at regional scale using high resolution satellite imagery and deep learning M. Lei et al. 10.1016/j.atmosres.2021.105587
- Evidence and causes of recent decreases in nitrogen deposition in temperate forests in Northeast China Y. Wang et al. 10.1016/j.scitotenv.2024.172472
- 10-year satellite-constrained fluxes of ammonia improve performance of chemistry transport models N. Evangeliou et al. 10.5194/acp-21-4431-2021
- Evidence for global increases in urban ammonia pollution and their drivers S. Liu et al. 10.1016/j.scitotenv.2024.176846
- Enhanced Wet Deposition of Nitrogen Induced by a Landfalling Typhoon over East Asia: Implications for the Marine Eco-Environment Y. Zhang et al. 10.1021/acs.estlett.2c00762
- Tracking down global NH<sub>3</sub> point sources with wind-adjusted superresolution L. Clarisse et al. 10.5194/amt-12-5457-2019
- Frontiers of graphene and 2D material-based gas sensors for environmental monitoring D. Buckley et al. 10.1088/2053-1583/ab7bc5
- Air Quality Degradation by Mineral Dust over Beijing, Chengdu and Shanghai Chinese Megacities M. Lachatre et al. 10.3390/atmos11070708
- Estimation and variation analysis of secondary inorganic aerosols across the Greater Bay Area in 2005 and 2015 Y. Chen et al. 10.1016/j.chemosphere.2021.133393
- Record high levels of atmospheric ammonia over India: Spatial and temporal analyses J. Kuttippurath et al. 10.1016/j.scitotenv.2020.139986
- Responses of sulfate and nitrate to anthropogenic emission changes in eastern China - in perspective of long-term variations L. Qi et al. 10.1016/j.scitotenv.2022.158875
- Responses of nitrogen and sulfur deposition to NH3 emission control in the Yangtze River Delta, China Z. Dong et al. 10.1016/j.envpol.2022.119646
Latest update: 23 Nov 2024
Short summary
It has been observed from satellite-based instruments that ammonia levels strongly increased between 2011 and 2015. We have used the CHIMERE CTM to understand what could explain such an increase. We first focused on meteorological condition variations, and it has been concluded that meteorology did not explain ammonia evolution. Then, we focused on SO2 and NOx emission evolution rates to evaluate their influences on ammonia. It appears that theses decreases were the main explanation.
It has been observed from satellite-based instruments that ammonia levels strongly increased...
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