Articles | Volume 19, issue 9
https://doi.org/10.5194/acp-19-6107-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-6107-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Heterogeneous sulfate aerosol formation mechanisms during wintertime Chinese haze events: air quality model assessment using observations of sulfate oxygen isotopes in Beijing
Jingyuan Shao
Laboratory for Climate and Ocean-Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing 100871, China
Department of Atmospheric Sciences, University of Washington, Seattle, WA 98195, USA
Qianjie Chen
Department of Atmospheric Sciences, University of Washington, Seattle, WA 98195, USA
Department of Chemistry, University of Michigan, Ann Arbor, MI 48109, USA
Yuxuan Wang
Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX 77204, USA
Laboratory for Climate and Ocean-Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing 100871, China
Pengzhen He
Anhui Province Key Laboratory of Polar Environment and Global Change, School of Earth and Space Sciences, University of Science and Technology of China, Hefei 230026, China
State Key Laboratory of Atmospheric Boundary Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Viral Shah
Department of Atmospheric Sciences, University of Washington, Seattle, WA 98195, USA
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA
Randall V. Martin
Department of Physics and Atmospheric Science, Dalhousie University, Halifax, Nova Scotia, Canada
Sajeev Philip
NASA postdoctoral program, NASA Ames Research Center, Moffett Field, CA 94035, USA
Shaojie Song
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA
School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China
Zhouqing Xie
CORRESPONDING AUTHOR
Anhui Province Key Laboratory of Polar Environment and Global Change, School of Earth and Space Sciences, University of Science and Technology of China, Hefei 230026, China
Lin Zhang
CORRESPONDING AUTHOR
Laboratory for Climate and Ocean-Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing 100871, China
Department of Atmospheric Sciences, University of Washington, Seattle, WA 98195, USA
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Latest update: 06 Dec 2024
Short summary
Sulfate is a key species contributing to particle formation and growth during wintertime Chinese haze events. This study combines observations and modeling of oxygen isotope signatures in sulfate aerosol to investigate its formation mechanisms, with a focus on heterogeneous production on aerosol surface via H2O2, O3, and NO2 and trace metal catalyzed oxidation. Contributions from different formation pathways are presented.
Sulfate is a key species contributing to particle formation and growth during wintertime Chinese...
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