Research article
| Highlight paper
03 Apr 2019
Research article
| Highlight paper
| 03 Apr 2019
Permafrost nitrous oxide emissions observed on a landscape scale using the airborne eddy-covariance method
Jordan Wilkerson et al.
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Jordan Wilkerson, David S. Sayres, Jessica B. Smith, Norton Allen, Marco Rivero, Mike Greenberg, Terry Martin, and James G. Anderson
Atmos. Meas. Tech., 14, 3597–3613, https://doi.org/10.5194/amt-14-3597-2021, https://doi.org/10.5194/amt-14-3597-2021, 2021
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The ozone layer in the stratosphere protects life from harmful UV light, but chlorine-based pollution threatens to damage it. We developed an instrument that couples a laser with highly reflective mirrors and advanced electronics to measure an important residue of this pollution: hydrogen chloride. Our instrument has an improved, more modern layout that we successfully tested in flight. This paves the way for future, advanced techniques that seek to evaluate the health of Earth’s ozone layer.
David S. Sayres, Ronald Dobosy, Claire Healy, Edward Dumas, John Kochendorfer, Jason Munster, Jordan Wilkerson, Bruce Baker, and James G. Anderson
Atmos. Chem. Phys., 17, 8619–8633, https://doi.org/10.5194/acp-17-8619-2017, https://doi.org/10.5194/acp-17-8619-2017, 2017
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Arctic temperatures have risen faster than the global average, causing the depth of melting of the frozen ground to increase. Previously frozen organic carbon, once exposed to air, water, and microbes, is turned into carbon dioxide and methane, both of which are important greenhouse gases. Due to the large and varied surface area of the Arctic and the difficulty of making measurements there we use a low flying aircraft (<25 m) to measure the amount of methane released from different regions.
Temple R. Lee, Travis J. Schuyler, Michael Buban, Edward J. Dumas, Tilden P. Meyers, and C. Bruce Baker
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-93, https://doi.org/10.5194/essd-2022-93, 2022
Preprint under review for ESSD
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Small uncrewed aircraft systems (sUxS), or drones, can be used to sample temperature, moisture, and wind in the lowest part of the atmosphere. In this study, we performed nearly 250 flights with our sUxS at a site about 20 miles northwest of Knoxville, Tennessee. We provided these datasets to forecasters at the local National Weather Service Weather Forecast Office to assist them with making their weather forecasts.
Jordan Wilkerson, David S. Sayres, Jessica B. Smith, Norton Allen, Marco Rivero, Mike Greenberg, Terry Martin, and James G. Anderson
Atmos. Meas. Tech., 14, 3597–3613, https://doi.org/10.5194/amt-14-3597-2021, https://doi.org/10.5194/amt-14-3597-2021, 2021
Short summary
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The ozone layer in the stratosphere protects life from harmful UV light, but chlorine-based pollution threatens to damage it. We developed an instrument that couples a laser with highly reflective mirrors and advanced electronics to measure an important residue of this pollution: hydrogen chloride. Our instrument has an improved, more modern layout that we successfully tested in flight. This paves the way for future, advanced techniques that seek to evaluate the health of Earth’s ozone layer.
John Kochendorfer, Rodica Nitu, Mareile Wolff, Eva Mekis, Roy Rasmussen, Bruce Baker, Michael E. Earle, Audrey Reverdin, Kai Wong, Craig D. Smith, Daqing Yang, Yves-Alain Roulet, Tilden Meyers, Samuel Buisan, Ketil Isaksen, Ragnar Brækkan, Scott Landolt, and Al Jachcik
Hydrol. Earth Syst. Sci., 22, 1437–1452, https://doi.org/10.5194/hess-22-1437-2018, https://doi.org/10.5194/hess-22-1437-2018, 2018
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Due to the effects of wind, precipitation gauges typically underestimate the amount of precipitation that occurs as snow. Measurements recorded during a World Meteorological Organization intercomparison of precipitation gauges were used to evaluate and improve the adjustments that are available to address this issue. Adjustments for specific types of precipitation gauges and wind shields were tested and recommended.
David S. Sayres, Ronald Dobosy, Claire Healy, Edward Dumas, John Kochendorfer, Jason Munster, Jordan Wilkerson, Bruce Baker, and James G. Anderson
Atmos. Chem. Phys., 17, 8619–8633, https://doi.org/10.5194/acp-17-8619-2017, https://doi.org/10.5194/acp-17-8619-2017, 2017
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Arctic temperatures have risen faster than the global average, causing the depth of melting of the frozen ground to increase. Previously frozen organic carbon, once exposed to air, water, and microbes, is turned into carbon dioxide and methane, both of which are important greenhouse gases. Due to the large and varied surface area of the Arctic and the difficulty of making measurements there we use a low flying aircraft (<25 m) to measure the amount of methane released from different regions.
John Kochendorfer, Rodica Nitu, Mareile Wolff, Eva Mekis, Roy Rasmussen, Bruce Baker, Michael E. Earle, Audrey Reverdin, Kai Wong, Craig D. Smith, Daqing Yang, Yves-Alain Roulet, Samuel Buisan, Timo Laine, Gyuwon Lee, Jose Luis C. Aceituno, Javier Alastrué, Ketil Isaksen, Tilden Meyers, Ragnar Brækkan, Scott Landolt, Al Jachcik, and Antti Poikonen
Hydrol. Earth Syst. Sci., 21, 3525–3542, https://doi.org/10.5194/hess-21-3525-2017, https://doi.org/10.5194/hess-21-3525-2017, 2017
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Precipitation measurements were combined from eight separate precipitation testbeds to create multi-site transfer functions for the correction of unshielded and single-Alter-shielded precipitation gauge measurements. Site-specific errors and more universally applicable corrections were created from these WMO-SPICE measurements. The importance and magnitude of such wind speed corrections were demonstrated.
John Kochendorfer, Roy Rasmussen, Mareile Wolff, Bruce Baker, Mark E. Hall, Tilden Meyers, Scott Landolt, Al Jachcik, Ketil Isaksen, Ragnar Brækkan, and Ronald Leeper
Hydrol. Earth Syst. Sci., 21, 1973–1989, https://doi.org/10.5194/hess-21-1973-2017, https://doi.org/10.5194/hess-21-1973-2017, 2017
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Snowfall measurements recorded using precipitation gauges are subject to significant underestimation due to the effects of wind. Using measurements recorded at two different precipitation test beds, corrections for unshielded gauges and gauges within different types of windshields were developed and tested. Using the new corrections, uncorrectable errors were quantified, and measurement biases were successfully eliminated.
Related subject area
Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Temporary pause in the growth of atmospheric ethane and propane in 2015–2018
Colm Sweeney, Abhishek Chatterjee, Sonja Wolter, Kathryn McKain, Robert Bogue, Stephen Conley, Tim Newberger, Lei Hu, Lesley Ott, Benjamin Poulter, Luke Schiferl, Brad Weir, Zhen Zhang, and Charles E. Miller
Atmos. Chem. Phys., 22, 6347–6364, https://doi.org/10.5194/acp-22-6347-2022, https://doi.org/10.5194/acp-22-6347-2022, 2022
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The Arctic Carbon Atmospheric Profiles (Arctic-CAP) project demonstrates the utility of aircraft profiles for independent evaluation of model-derived emissions and uptake of atmospheric CO2, CH4, and CO from land and ocean. Comparison with the Goddard Earth Observing System (GEOS) modeling system suggests that fluxes of CO2 are very consistent with observations, while those of CH4 have some regional and seasonal biases, and that CO comparison is complicated by transport errors.
Roseline C. Thakur, Lubna Dada, Lisa J. Beck, Lauriane L. J. Quéléver, Tommy Chan, Marjan Marbouti, Xu-Cheng He, Carlton Xavier, Juha Sulo, Janne Lampilahti, Markus Lampimäki, Yee Jun Tham, Nina Sarnela, Katrianne Lehtipalo, Alf Norkko, Markku Kulmala, Mikko Sipilä, and Tuija Jokinen
Atmos. Chem. Phys., 22, 6365–6391, https://doi.org/10.5194/acp-22-6365-2022, https://doi.org/10.5194/acp-22-6365-2022, 2022
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Every year intense cyanobacterial and macroalgal blooms occur in the Baltic Sea and in the coastal areas surrounding Helsinki, yet no studies have addressed the impact of biogenic emissions from these blooms on gas vapor concentrations, which in turn could influence new particle formation. This is the first study of its kind to address the chemistry driving new particle formation (NPF) during a bloom period in this region, highlighting the role of biogenic sulfuric acid and iodic acid.
Gordon A. Novak, Delaney B. Kilgour, Christopher M. Jernigan, Michael P. Vermeuel, and Timothy H. Bertram
Atmos. Chem. Phys., 22, 6309–6325, https://doi.org/10.5194/acp-22-6309-2022, https://doi.org/10.5194/acp-22-6309-2022, 2022
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We describe field measurements of the mixing ratio and oceanic emission flux of dimethyl sulfide (DMS) and methanethiol (MeSH) from a coastal ocean site. DMS is known to impact aerosol formation and growth in the marine atmosphere, influencing cloud formation and climate. Measurements of MeSH, which is produced by the same oceanic source as DMS, are rare. We show that MeSH emissions are large and must be measured alongside DMS to understand marine sulfur chemistry and aerosol formation.
Yuting Zhu, Youfeng Wang, Xianliang Zhou, Yasin F. Elshorbany, Chunxiang Ye, Matthew Hayden, and Andrew J. Peters
Atmos. Chem. Phys., 22, 6327–6346, https://doi.org/10.5194/acp-22-6327-2022, https://doi.org/10.5194/acp-22-6327-2022, 2022
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The daytime chemistry of nitrous acid (HONO), which plays an important role in the oxidation capacity of the troposphere, is not well understood. In this work, we report new field measurement results of HONO and the relevant parameters in the marine boundary layer at Tudor Hill Marine Atmospheric Observatory in Bermuda. We evaluate the daytime HONO budgets in air masses under different types of interaction with the island and examine the strengths of different HONO formation and loss mechanisms.
Clara M. Nussbaumer, Andrea Pozzer, Ivan Tadic, Lenard Röder, Florian Obersteiner, Hartwig Harder, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 22, 6151–6165, https://doi.org/10.5194/acp-22-6151-2022, https://doi.org/10.5194/acp-22-6151-2022, 2022
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The European COVID-19 lockdowns have significantly reduced the emission of primary pollutants such as NOx, which impacts the tropospheric photochemical processes and the abundance of O3. In this study, we present how the lockdowns have affected tropospheric trace gases and ozone production based on in situ observations and modeling simulations. We additionally show that the chemical regime shifted from a transition point to a NOx limitation in the upper troposphere.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Lisa Kaser, Arianna Peron, Martin Graus, Marcus Striednig, Georg Wohlfahrt, Stanislav Juráň, and Thomas Karl
Atmos. Chem. Phys., 22, 5603–5618, https://doi.org/10.5194/acp-22-5603-2022, https://doi.org/10.5194/acp-22-5603-2022, 2022
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Biogenic volatile organic compounds (e.g., terpenoids) play an essential role in atmospheric chemistry. Urban greening activities need to consider the ozone- and aerosol-forming potential of these compounds released from vegetation. NMVOC emissions in urban environments are complex, and the biogenic component remains poorly quantified. For summer conditions biogenic emissions dominate terpene emissions and heat waves can significantly modulate urban biogenic terpenoid emissions.
Hannah Walker, Daniel Stone, Trevor Ingham, Sina Hackenberg, Danny Cryer, Shalini Punjabi, Katie Read, James Lee, Lisa Whalley, Dominick V. Spracklen, Lucy J. Carpenter, Steve R. Arnold, and Dwayne E. Heard
Atmos. Chem. Phys., 22, 5535–5557, https://doi.org/10.5194/acp-22-5535-2022, https://doi.org/10.5194/acp-22-5535-2022, 2022
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Glyoxal is a ubiquitous reactive organic compound in the atmosphere, which may form organic aerosol and impact the atmosphere's oxidising capacity. There are limited measurements of glyoxal's abundance in the remote marine atmosphere. We made new measurements of glyoxal using a highly sensitive technique over two 4-week periods in the tropical Atlantic atmosphere. We show that daytime measurements are mostly consistent with our chemical understanding but a potential missing source at night.
Haklim Choi, Mi-Kyung Park, Paul J. Fraser, Hyeri Park, Sohyeon Geum, Jens Mühle, Jooil Kim, Ian Porter, Peter K. Salameh, Christina M. Harth, Bronwyn L. Dunse, Paul B. Krummel, Ray F. Weiss, Simon O'Doherty, Dickon Young, and Sunyoung Park
Atmos. Chem. Phys., 22, 5157–5173, https://doi.org/10.5194/acp-22-5157-2022, https://doi.org/10.5194/acp-22-5157-2022, 2022
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We observed 12-year continuous CH3Br pollution signals at Gosan and estimated anthropogenic CH3Br emissions in eastern China. The analysis revealed a significant discrepancy between top-down estimates and the bottom-up emissions from the fumigation usage reported to the United Nations Environment Programme, likely due to unreported or inaccurately reported fumigation usage. This result provides information to monitor international compliance with the Montreal Protocol.
Shenglun Wu, Hyung Joo Lee, Andrea Anderson, Shang Liu, Toshihiro Kuwayama, John H. Seinfeld, and Michael J. Kleeman
Atmos. Chem. Phys., 22, 4929–4949, https://doi.org/10.5194/acp-22-4929-2022, https://doi.org/10.5194/acp-22-4929-2022, 2022
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An ozone control experiment usually conducted in the laboratory was installed in a trailer and moved to the outdoor environment to directly confirm that we are controlling the right sources in order to lower ambient ozone concentrations. Adding small amounts of precursor oxides of nitrogen and volatile organic compounds to ambient air showed that the highest ozone concentrations are best controlled by reducing concentrations of oxides of nitrogen. The results confirm satellite measurements.
Andrew J. Lindsay, Daniel C. Anderson, Rebecca A. Wernis, Yutong Liang, Allen H. Goldstein, Scott C. Herndon, Joseph R. Roscioli, Christoph Dyroff, Ed C. Fortner, Philip L. Croteau, Francesca Majluf, Jordan E. Krechmer, Tara I. Yacovitch, Walter B. Knighton, and Ezra C. Wood
Atmos. Chem. Phys., 22, 4909–4928, https://doi.org/10.5194/acp-22-4909-2022, https://doi.org/10.5194/acp-22-4909-2022, 2022
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Wildfire smoke dramatically impacts air quality and often has elevated concentrations of ozone. We present measurements of ozone and its precursors at a rural site periodically impacted by wildfire smoke. Measurements of total peroxy radicals, key ozone precursors that have been studied little within wildfires, compare well with chemical box model predictions. Our results indicate no serious issues with using current chemistry mechanisms to model chemistry in aged wildfire plumes.
Kun Zhang, Zhiqiang Liu, Xiaojuan Zhang, Qing Li, Andrew Jensen, Wen Tan, Ling Huang, Yangjun Wang, Joost de Gouw, and Li Li
Atmos. Chem. Phys., 22, 4853–4866, https://doi.org/10.5194/acp-22-4853-2022, https://doi.org/10.5194/acp-22-4853-2022, 2022
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A significant increase in O3 concentrations was found during the lockdown period of COVID-19 in most areas of China. By field measurements coupled with machine learning, an observation-based model (OBM) and sensitivity analysis, we found the changes in the NOx / VOC ratio were a key reason for the significant rise in O3. To restrain O3 pollution, more efforts should be devoted to the control of anthropogenic OVOCs, alkenes and aromatics.
Amy Foulds, Grant Allen, Jacob T. Shaw, Prudence Bateson, Patrick A. Barker, Langwen Huang, Joseph R. Pitt, James D. Lee, Shona E. Wilde, Pamela Dominutti, Ruth M. Purvis, David Lowry, James L. France, Rebecca E. Fisher, Alina Fiehn, Magdalena Pühl, Stéphane J. B. Bauguitte, Stephen A. Conley, Mackenzie L. Smith, Tom Lachlan-Cope, Ignacio Pisso, and Stefan Schwietzke
Atmos. Chem. Phys., 22, 4303–4322, https://doi.org/10.5194/acp-22-4303-2022, https://doi.org/10.5194/acp-22-4303-2022, 2022
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We measured CH4 emissions from 21 offshore oil and gas facilities in the Norwegian Sea in 2019. Measurements compared well with operator-reported emissions but were greatly underestimated when compared with a 2016 global fossil fuel inventory. This study demonstrates the need for up-to-date and accurate inventories for use in research and policy and the important benefits of best-practice reporting methods by operators. Airborne measurements are an effective tool to validate such inventories.
Hisahiro Takashima, Yugo Kanaya, Saki Kato, Martina M. Friedrich, Michel Van Roozendael, Fumikazu Taketani, Takuma Miyakawa, Yuichi Komazaki, Carlos A. Cuevas, Alfonso Saiz-Lopez, and Takashi Sekiya
Atmos. Chem. Phys., 22, 4005–4018, https://doi.org/10.5194/acp-22-4005-2022, https://doi.org/10.5194/acp-22-4005-2022, 2022
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We have undertaken atmospheric iodine monoxide (IO) observations in the global marine boundary layer with a wide latitudinal coverage and sea surface temperature (SST) range. We conclude that atmospheric iodine is abundant over the Western Pacific warm pool, appearing as an iodine fountain, where ozone (O3) minima occur. Our study also found negative correlations between IO and O3 concentrations over IO maxima, which requires reconsideration of the initiation process of halogen activation.
Wenjie Wang, Bin Yuan, Yuwen Peng, Hang Su, Yafang Cheng, Suxia Yang, Caihong Wu, Jipeng Qi, Fengxia Bao, Yibo Huangfu, Chaomin Wang, Chenshuo Ye, Zelong Wang, Baolin Wang, Xinming Wang, Wei Song, Weiwei Hu, Peng Cheng, Manni Zhu, Junyu Zheng, and Min Shao
Atmos. Chem. Phys., 22, 4117–4128, https://doi.org/10.5194/acp-22-4117-2022, https://doi.org/10.5194/acp-22-4117-2022, 2022
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From thorough measurements of numerous oxygenated volatile organic compounds, we show that their photodissociation can be important for radical production and ozone formation in the atmosphere. This effect was underestimated in previous studies, as measurements of them were lacking.
Helen L. Fitzmaurice, Alexander J. Turner, Jinsol Kim, Katherine Chan, Erin R. Delaria, Catherine Newman, Paul Wooldridge, and Ronald C. Cohen
Atmos. Chem. Phys., 22, 3891–3900, https://doi.org/10.5194/acp-22-3891-2022, https://doi.org/10.5194/acp-22-3891-2022, 2022
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On-road emissions are thought to vary widely from existing predictions, as the effects of the age of the vehicle fleet, the performance of emission control systems, and variations in speed are difficult to assess under ambient driving conditions. We present an observational approach to characterize on-road emissions and show that the method is consistent with other approaches to within ~ 3 %.
Danilo Custódio, Katrine Aspmo Pfaffhuber, T. Gerard Spain, Fidel F. Pankratov, Iana Strigunova, Koketso Molepo, Henrik Skov, Johannes Bieser, and Ralf Ebinghaus
Atmos. Chem. Phys., 22, 3827–3840, https://doi.org/10.5194/acp-22-3827-2022, https://doi.org/10.5194/acp-22-3827-2022, 2022
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As a poison in the air that we breathe and the food that we eat, mercury is a human health concern for society as a whole. In that regard, this work deals with monitoring and modelling mercury in the environment, improving wherewithal, identifying the strength of the different components at play, and interpreting information to support the efforts that seek to safeguard public health.
Xiaorui Chen, Haichao Wang, and Keding Lu
Atmos. Chem. Phys., 22, 3525–3533, https://doi.org/10.5194/acp-22-3525-2022, https://doi.org/10.5194/acp-22-3525-2022, 2022
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We use a complete set of simulations to evaluate whether equilibrium and steady state are appropriate for a chemical system involving several reactive nitrogen-containing species (NO2, NO3, and N2O5) under various conditions. A previously neglected bias for the coefficient applied for interpreting their effects is disclosed, and the relevant ambient factors are examined. We therefore provide a good solution to an accurate representation of nighttime chemistry in high-aerosol areas.
Jens Mühle, Lambert J. M. Kuijpers, Kieran M. Stanley, Matthew Rigby, Luke M. Western, Jooil Kim, Sunyoung Park, Christina M. Harth, Paul B. Krummel, Paul J. Fraser, Simon O'Doherty, Peter K. Salameh, Roland Schmidt, Dickon Young, Ronald G. Prinn, Ray H. J. Wang, and Ray F. Weiss
Atmos. Chem. Phys., 22, 3371–3378, https://doi.org/10.5194/acp-22-3371-2022, https://doi.org/10.5194/acp-22-3371-2022, 2022
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Emissions of the strong greenhouse gas perfluorocyclobutane (c-C4F8) into the atmosphere have been increasing sharply since the early 2000s. These c-C4F8 emissions are highly correlated with the amount of hydrochlorofluorocarbon-22 produced to synthesize polytetrafluoroethylene (known for its non-stick properties) and related chemicals. From this process, c-C4F8 by-product is vented to the atmosphere. Avoiding these unnecessary c-C4F8 emissions could reduce the climate impact of this industry.
Chaoyang Xue, Can Ye, Jörg Kleffmann, Chenglong Zhang, Valéry Catoire, Fengxia Bao, Abdelwahid Mellouki, Likun Xue, Jianmin Chen, Keding Lu, Yong Zhao, Hengde Liu, Zhaoxin Guo, and Yujing Mu
Atmos. Chem. Phys., 22, 3149–3167, https://doi.org/10.5194/acp-22-3149-2022, https://doi.org/10.5194/acp-22-3149-2022, 2022
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Summertime measurements of nitrous acid (HONO) and related parameters were conducted at the foot and the summit of Mt. Tai (1534 m above sea level). We proposed a rapid vertical air mass exchange between the foot and the summit level, which enhances the role of HONO in the oxidizing capacity of the upper boundary layer. Kinetics for aerosol-derived HONO sources were constrained. HONO formation from different paths was quantified and discussed.
Patrick Dewald, Clara M. Nussbaumer, Jan Schuladen, Akima Ringsdorf, Achim Edtbauer, Horst Fischer, Jonathan Williams, Jos Lelieveld, and John N. Crowley
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-163, https://doi.org/10.5194/acp-2022-163, 2022
Revised manuscript accepted for ACP
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We measured the gas-phase reactivity of the NO3 radical on the summit (825 m a.s.l.) of a semi-rural mountain in south-west Germany in July 2021. The impact of VOC-induced NO3 losses (mostly monoterpenes) in competition to loss by reaction with NO and photolysis throughout the diel cycle was estimated. Beside chemistry, boundary layer dynamics and plant-physiological processes presumably have a great impact on our observations, which were compared to previous NO3 measurements on the same site.
Kathryn D. Kulju, Stephen M. McNamara, Qianjie Chen, Hannah S. Kenagy, Jacinta Edebeli, Jose D. Fuentes, Steven B. Bertman, and Kerri A. Pratt
Atmos. Chem. Phys., 22, 2553–2568, https://doi.org/10.5194/acp-22-2553-2022, https://doi.org/10.5194/acp-22-2553-2022, 2022
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N2O5 uptake by chloride-containing surfaces produces ClNO2, which photolyzes, producing NO2 and highly reactive Cl radicals that impact air quality. In the inland urban atmosphere, ClNO2 was elevated during lower air turbulence and over snow-covered ground, from snowpack ClNO2 production. N2O5 and ClNO2 levels were lowest, on average, during rainfall and fog because of scavenging, with N2O5 scavenging by fog droplets likely contributing to observed increased particulate nitrate concentrations.
Huiming Lin, Yindong Tong, Chenghao Yu, Long Chen, Xiufeng Yin, Qianggong Zhang, Shichang Kang, Lun Luo, James Schauer, Benjamin de Foy, and Xuejun Wang
Atmos. Chem. Phys., 22, 2651–2668, https://doi.org/10.5194/acp-22-2651-2022, https://doi.org/10.5194/acp-22-2651-2022, 2022
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The Tibetan Plateau is known as
The Third Poleand is generally considered to be a clean area owing to its high altitude. However, it may receive be impacted by air pollutants transported from the Indian subcontinent. Pollutants generally enter the Tibetan Plateau in several ways. Among them is the Yarlung Zangbu–Brahmaputra Grand Canyon. In this study, we identified the influence of the Indian summer monsoon on the origin, transport, and behavior of mercury in this area.
Dominique Rust, Ioannis Katharopoulos, Martin K. Vollmer, Stephan Henne, Simon O'Doherty, Daniel Say, Lukas Emmenegger, Renato Zenobi, and Stefan Reimann
Atmos. Chem. Phys., 22, 2447–2466, https://doi.org/10.5194/acp-22-2447-2022, https://doi.org/10.5194/acp-22-2447-2022, 2022
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Artificial halocarbons contribute to ozone layer depletion and to global warming. We measured the atmospheric concentrations of halocarbons at the Beromünster tower, modelled the Swiss emissions, and compared the results to the internationally reported Swiss emissions inventory. For most of the halocarbons, we found good agreement, whereas one refrigerant might be overestimated in the inventory. In addition, we present first emission estimates of the newest types of halocarbons.
Tuija Jokinen, Katrianne Lehtipalo, Roseline Cutting Thakur, Ilona Ylivinkka, Kimmo Neitola, Nina Sarnela, Totti Laitinen, Markku Kulmala, Tuukka Petäjä, and Mikko Sipilä
Atmos. Chem. Phys., 22, 2237–2254, https://doi.org/10.5194/acp-22-2237-2022, https://doi.org/10.5194/acp-22-2237-2022, 2022
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New particle formation is an important source of cloud condensation nuclei; however, long-term measurements of aerosol-forming vapors are close to nonexistent in the Arctic. Here, we report 7 months of CI-APi-TOF measurements of sulfuric acid, iodic acid, methane sulfonic acid and the sum of highly oxygenated organic molecules from the SMEAR I station in the Finnish subarctic. The results help us to understand atmospheric chemical processes and aerosol formation in this rapidly changing area.
Andrew O. Langford, Christoph J. Senff, Raul J. Alvarez II, Ken C. Aikin, Sunil Baidar, Timothy A. Bonin, W. Alan Brewer, Jerome Brioude, Steven S. Brown, Joel D. Burley, Dani J. Caputi, Stephen A. Conley, Patrick D. Cullis, Zachary C. J. Decker, Stéphanie Evan, Guillaume Kirgis, Meiyun Lin, Mariusz Pagowski, Jeff Peischl, Irina Petropavlovskikh, R. Bradley Pierce, Thomas B. Ryerson, Scott P. Sandberg, Chance W. Sterling, Ann M. Weickmann, and Li Zhang
Atmos. Chem. Phys., 22, 1707–1737, https://doi.org/10.5194/acp-22-1707-2022, https://doi.org/10.5194/acp-22-1707-2022, 2022
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The Fires, Asian, and Stratospheric Transport–Las Vegas Ozone Study (FAST-LVOS) combined lidar, aircraft, and in situ measurements with global models to investigate the contributions of stratospheric intrusions, regional and Asian pollution, and wildfires to background ozone in the southwestern US during May and June 2017 and demonstrated that these processes contributed to background ozone levels that exceeded 70 % of the US National Ambient Air Quality Standard during the 6-week campaign.
Qingqing Yin, Qianli Ma, Weili Lin, Xiaobin Xu, and Jie Yao
Atmos. Chem. Phys., 22, 1015–1033, https://doi.org/10.5194/acp-22-1015-2022, https://doi.org/10.5194/acp-22-1015-2022, 2022
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China has been experiencing rapid changes in emissions of air pollutants in recent decades. NOx and SO2 measurements from 2006 to 2016 at the Lin’an World Meteorological Organization Global Atmospheric Watch station were used to characterize the seasonal and diurnal variations and study the long-term trends. This study reaffirms China’s success in controlling both NOx and SO2 in the Yangtze River Delta but indicates at the same time a necessity to strengthen the NOx emission control.
Chaoyang Xue, Can Ye, Jörg Kleffmann, Wenjin Zhang, Xiaowei He, Pengfei Liu, Chenglong Zhang, Xiaoxi Zhao, Chengtang Liu, Zhuobiao Ma, Junfeng Liu, Jinhe Wang, Keding Lu, Valéry Catoire, Abdelwahid Mellouki, and Yujing Mu
Atmos. Chem. Phys., 22, 1035–1057, https://doi.org/10.5194/acp-22-1035-2022, https://doi.org/10.5194/acp-22-1035-2022, 2022
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Nitrous acid (HONO) and related parameters were measured at the foot and the summit of Mt. Tai in the summer of 2018. Based on measurements at the foot station, we utilized a box model to explore the roles of different sources in the HONO budget. We also studied radical chemistry in this high-ozone region.
Baoye Hu, Jun Duan, Youwei Hong, Lingling Xu, Mengren Li, Yahui Bian, Min Qin, Wu Fang, Pinhua Xie, and Jinsheng Chen
Atmos. Chem. Phys., 22, 371–393, https://doi.org/10.5194/acp-22-371-2022, https://doi.org/10.5194/acp-22-371-2022, 2022
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There has been a lack of research into HONO in coastal cities with low concentrations of PM2.5, but strong sunlight and high humidity. Insufficient research on coastal cities with good air quality has resulted in certain obstacles to assessing the photochemical processes in these areas. Furthermore, HONO contributes to the atmospheric photochemistry depending on the season. Therefore, observations of HONO across four seasons in the southeastern coastal area of China are urgently needed.
Will S. Drysdale, Adam R. Vaughan, Freya A. Squires, Sam J. Cliff, Stefan Metzger, David Durden, Natchaya Pingintha-Durden, Carole Helfter, Eiko Nemitz, C. Sue B. Grimmond, Janet Barlow, Sean Beevers, Gregor Stewart, David Dajnak, Ruth M. Purvis, and James D. Lee
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-982, https://doi.org/10.5194/acp-2021-982, 2022
Revised manuscript accepted for ACP
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Measurements of nitrogen oxide and nitrogen dioxide (NOx) emissions are important for a good understanding of air quality. While there are many direct measurements of NOx concentration, there are very few measurements of its emission. Measurements of emissions provide constraints to emissions inventories and air quality models. This article presents measurements of NOx emission from the BT Tower in central London in 2017, and compares them with inventories, finding they underestimate by ~1.48 x.
Xueli Liu, Liang Ran, Weili Lin, Xiaobin Xu, Zhiqiang Ma, Fan Dong, Di He, Liyan Zhou, Qingfeng Shi, and Yao Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-866, https://doi.org/10.5194/acp-2021-866, 2022
Revised manuscript accepted for ACP
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Significant decreases in the annual mean NOx from 2011 to 2016 and SO2 from 2008 to 2016 affirm the effectiveness of relevant control measures on the reduction in NOx and SO2 emissions in the North China Plain (NCP). NOx at SDZ had weaker influence than SO2 by the emission reduction in Beijing and other areas in NCP. The increase in the amount of motor vehicles and the weak traffic restrictions have caused vehicle emissions on NOx that indicated that NOx emission control should be strengthened.
Lian Zong, Yuanjian Yang, Haiyun Xia, Meng Gao, Zhaobin Sun, Zuofang Zheng, Xianxiang Li, Guicai Ning, Yubin Li, and Simone Lolli
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1095, https://doi.org/10.5194/acp-2021-1095, 2022
Revised manuscript accepted for ACP
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Heatwaves (HWs) paired with higher ozone (O3) concentration at surface level pose a serious threat to human health. Taking Beijing as an example, tree unfavourable synoptic weather patterns were identified to dominate the compound HWs and O3 pollution events. Under the synergistic stress of HWs and O3 pollution, the public mortality risk increased, and synoptic patterns and urbanization can enhance the compound risk of events in Beijing by 45.46 % and 8.08 %, respectively.
Xuefei Ma, Zhaofeng Tan, Keding Lu, Xinping Yang, Xiaorui Chen, Haichao Wang, Shiyi Chen, Xin Fang, Shule Li, Xin Li, Jingwei Liu, Ying Liu, Shengrong Lou, Wanyi Qiu, Hongli Wang, Limin Zeng, and Yuanhang Zhang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1021, https://doi.org/10.5194/acp-2021-1021, 2022
Revised manuscript accepted for ACP
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This paper presents the first OH and HO2 radicals observation made in Yangtze River Delta in China and strong oxidation capacity is discovered based on direct measurements. The impacts of new OH regeneration mechanism, monoterpene oxidation and HO2 uptake process are examined and discussed. The sources and the factors to sustain such strong oxidation is the key to understand the ozone pollutions formed in this area.
Lulu Cui, Di Wu, Shuxiao Wang, Qingcheng Xu, Ruolan Hu, and Jiming Hao
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-959, https://doi.org/10.5194/acp-2021-959, 2021
Revised manuscript accepted for ACP
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A one-year campaign was conducted to characterize VOCs at an urban site in Beijing during different episodes. VOCs from fuel evaporation and diesel exhaust particularly toluene, xylenes, trans-2-butene, acrolein, methyl methacrylate, vinyl acetate, 1-butene and 1-hexene were the main contributors. VOCs from diesel exhaust and coal/biomass combustion were found to be the dominant contributors for SOAFP, particularly the VOC species of toluene, 1-hexene, xylenes, ethylbenzene and styrene.
Jin Liao, Glenn M. Wolfe, Reem A. Hannun, Jason M. St. Clair, Thomas F. Hanisco, Jessica B. Gilman, Aaron Lamplugh, Vanessa Selimovic, Glenn S. Diskin, John B. Nowak, Hannah S. Halliday, Joshua P. DiGangi, Samuel R. Hall, Kirk Ullmann, Christopher D. Holmes, Charles H. Fite, Anxhelo Agastra, Thomas B. Ryerson, Jeff Peischl, Ilann Bourgeois, Carsten Warneke, Matthew M. Coggon, Georgios I. Gkatzelis, Kanako Sekimoto, Alan Fried, Dirk Richter, Petter Weibring, Eric C. Apel, Rebecca S. Hornbrook, Steven S. Brown, Caroline C. Womack, Michael A. Robinson, Rebecca A. Washenfelder, Patrick R. Veres, and J. Andrew Neuman
Atmos. Chem. Phys., 21, 18319–18331, https://doi.org/10.5194/acp-21-18319-2021, https://doi.org/10.5194/acp-21-18319-2021, 2021
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Formaldehyde (HCHO) is an important oxidant precursor and affects the formation of O3 and other secondary pollutants in wildfire plumes. We disentangle the processes controlling HCHO evolution from wildfire plumes sampled by NASA DC-8 during FIREX-AQ. We find that OH abundance rather than normalized OH reactivity is the main driver of fire-to-fire variability in HCHO secondary production and estimate an effective HCHO yield per volatile organic compound molecule oxidized in wildfire plumes.
Clara M. Nussbaumer, John N. Crowley, Jan Schuladen, Jonathan Williams, Sascha Hafermann, Andreas Reiffs, Raoul Axinte, Hartwig Harder, Cheryl Ernest, Anna Novelli, Katrin Sala, Monica Martinez, Chinmay Mallik, Laura Tomsche, Christian Plass-Dülmer, Birger Bohn, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 21, 18413–18432, https://doi.org/10.5194/acp-21-18413-2021, https://doi.org/10.5194/acp-21-18413-2021, 2021
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HCHO is an important atmospheric trace gas influencing the photochemical processes in the Earth’s atmosphere, including the budget of HOx and the abundance of tropospheric O3. This research presents the photochemical calculations of HCHO and O3 based on three field campaigns across Europe. We show that HCHO production via the oxidation of only four volatile organic compound precursors, i.e., CH4, CH3CHO, C5H8 and CH3OH, can balance the observed loss at all sites well.
Leigh R. Crilley, Louisa J. Kramer, Francis D. Pope, Chris Reed, James D. Lee, Lucy J. Carpenter, Lloyd D. J. Hollis, Stephen M. Ball, and William J. Bloss
Atmos. Chem. Phys., 21, 18213–18225, https://doi.org/10.5194/acp-21-18213-2021, https://doi.org/10.5194/acp-21-18213-2021, 2021
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Nitrous acid (HONO) is a key source of atmospheric oxidants. We evaluate if the ocean surface is a source of HONO for the marine boundary layer, using measurements from two contrasting coastal locations. We observed no evidence for a night-time ocean surface source, in contrast to previous work. This points to significant geographical variation in the predominant HONO formation mechanisms in marine environments, reflecting possible variability in the sea-surface microlayer composition.
Ahsan Mozaffar, Yan-Lin Zhang, Yu-Chi Lin, Feng Xie, Mei-Yi Fan, and Fang Cao
Atmos. Chem. Phys., 21, 18087–18099, https://doi.org/10.5194/acp-21-18087-2021, https://doi.org/10.5194/acp-21-18087-2021, 2021
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We performed a long-term investigation of ambient volatile organic compounds (VOCs) in an industrial area in Nanjing, China. Followed by alkanes, halocarbons and aromatics were the most abundant VOC groups. Vehicle-related emissions were the major VOC sources in the study area. Aromatic and alkene VOCs were responsible for most of the atmospheric reactions.
Yulu Qiu, Zhiqiang Ma, Ke Li, Mengyu Huang, Jiujiang Sheng, Ping Tian, Jia Zhu, Weiwei Pu, Yingxiao Tang, Tingting Han, Huaigang Zhou, and Hong Liao
Atmos. Chem. Phys., 21, 17995–18010, https://doi.org/10.5194/acp-21-17995-2021, https://doi.org/10.5194/acp-21-17995-2021, 2021
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Photochemical pollution over the North China Plain (NCP) is attracting much concern. Our observations at a rural site in the NCP identified high peroxyacetyl nitrate (PAN) concentrations, even on cold days. Increased acetaldehyde concentration and hydroxyl radical production rates drive fast PAN formation. Moreover, our study emphasizes the importance of formaldehyde photolysis in PAN formation and calls for implementing strict volatile organic compound controls after summer over the NCP.
Ira Leifer, Christopher Melton, and Donald R. Blake
Atmos. Chem. Phys., 21, 17607–17629, https://doi.org/10.5194/acp-21-17607-2021, https://doi.org/10.5194/acp-21-17607-2021, 2021
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We demonstrate a novel application using air quality station data to derive 3-decade-averaged emissions from the Coal Oil Point (COP) seep field, a highly spatially and temporally variable geological migration system. Emissions were 19 Gg per year, suggesting that the COP seep field contributes 0.27 % of the global marine seep budget based on a recent estimate. This provides an advance over snapshot survey values by accounting for seasonal and interannual variations.
Dirk Dienhart, John N. Crowley, Efstratios Bourtsoukidis, Achim Edtbauer, Philipp G. Eger, Lisa Ernle, Hartwig Harder, Bettina Hottmann, Monica Martinez, Uwe Parchatka, Jean-Daniel Paris, Eva Y. Pfannerstill, Roland Rohloff, Jan Schuladen, Christof Stönner, Ivan Tadic, Sebastian Tauer, Nijing Wang, Jonathan Williams, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 21, 17373–17388, https://doi.org/10.5194/acp-21-17373-2021, https://doi.org/10.5194/acp-21-17373-2021, 2021
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We present the first ship-based in situ measurements of formaldehyde (HCHO), hydroxyl radicals (OH) and the OH reactivity around the Arabian Peninsula. Regression analysis of the HCHO production rate and the related OH chemistry revealed the regional HCHO yield αeff, which represents the different chemical regimes encountered. Highest values were found for the Arabian Gulf (also known as the Persian Gulf), which highlights this region as a hotspot of photochemical air pollution.
James M. Roberts
Atmos. Chem. Phys., 21, 16793–16795, https://doi.org/10.5194/acp-21-16793-2021, https://doi.org/10.5194/acp-21-16793-2021, 2021
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This comment provides evidence that recently reported measurements of the isotope composition of wildfire-derived oxides of nitrogen have a significant interference from other nitrogen compounds. In addition, the conceptual model used to interpret the results was missing several key reactions.
Shohei Nomura, Manish Naja, M. Kawser Ahmed, Hitoshi Mukai, Yukio Terao, Toshinobu Machida, Motoki Sasakawa, and Prabir K. Patra
Atmos. Chem. Phys., 21, 16427–16452, https://doi.org/10.5194/acp-21-16427-2021, https://doi.org/10.5194/acp-21-16427-2021, 2021
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Long-term measurements of greenhouse gases (GHGs) in India and Bangladesh unveiled specific characteristics in their variations in these regions. Plants including rice cultivated in winter and summer strongly affected seasonal variations and levels in CO2 and CH4. Long-term variability of GHGs showed quite different features in their growth rates from those in Mauna Loa. GHG trends in this region seemed to be hardly affected by El Niño–Southern Oscillation (ENSO).
Zachary C. J. Decker, Michael A. Robinson, Kelley C. Barsanti, Ilann Bourgeois, Matthew M. Coggon, Joshua P. DiGangi, Glenn S. Diskin, Frank M. Flocke, Alessandro Franchin, Carley D. Fredrickson, Georgios I. Gkatzelis, Samuel R. Hall, Hannah Halliday, Christopher D. Holmes, L. Gregory Huey, Young Ro Lee, Jakob Lindaas, Ann M. Middlebrook, Denise D. Montzka, Richard Moore, J. Andrew Neuman, John B. Nowak, Brett B. Palm, Jeff Peischl, Felix Piel, Pamela S. Rickly, Andrew W. Rollins, Thomas B. Ryerson, Rebecca H. Schwantes, Kanako Sekimoto, Lee Thornhill, Joel A. Thornton, Geoffrey S. Tyndall, Kirk Ullmann, Paul Van Rooy, Patrick R. Veres, Carsten Warneke, Rebecca A. Washenfelder, Andrew J. Weinheimer, Elizabeth Wiggins, Edward Winstead, Armin Wisthaler, Caroline Womack, and Steven S. Brown
Atmos. Chem. Phys., 21, 16293–16317, https://doi.org/10.5194/acp-21-16293-2021, https://doi.org/10.5194/acp-21-16293-2021, 2021
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To understand air quality impacts from wildfires, we need an accurate picture of how wildfire smoke changes chemically both day and night as sunlight changes the chemistry of smoke. We present a chemical analysis of wildfire smoke as it changes from midday through the night. We use aircraft observations from the FIREX-AQ field campaign with a chemical box model. We find that even under sunlight typical
nighttimechemistry thrives and controls the fate of key smoke plume chemical processes.
Hannah Clark, Yasmine Bennouna, Maria Tsivlidou, Pawel Wolff, Bastien Sauvage, Brice Barret, Eric Le Flochmoën, Romain Blot, Damien Boulanger, Jean-Marc Cousin, Philippe Nédélec, Andreas Petzold, and Valérie Thouret
Atmos. Chem. Phys., 21, 16237–16256, https://doi.org/10.5194/acp-21-16237-2021, https://doi.org/10.5194/acp-21-16237-2021, 2021
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We examined 27 years of IAGOS (In-service Aircraft for a Global Observing System) profiles at Frankfurt to see if there were unusual features during the spring of 2020 related to COVID-19 lockdowns in Europe. Increased ozone near the surface was partly linked to the reduction in emissions. Carbon monoxide decreased near the surface, but the impact of the lockdowns was offset by polluted air masses from elsewhere. There were small reductions in ozone and carbon monoxide in the free troposphere.
Men Xia, Xiang Peng, Weihao Wang, Chuan Yu, Zhe Wang, Yee Jun Tham, Jianmin Chen, Hui Chen, Yujing Mu, Chenglong Zhang, Pengfei Liu, Likun Xue, Xinfeng Wang, Jian Gao, Hong Li, and Tao Wang
Atmos. Chem. Phys., 21, 15985–16000, https://doi.org/10.5194/acp-21-15985-2021, https://doi.org/10.5194/acp-21-15985-2021, 2021
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ClNO2 is an important precursor of chlorine radical that affects photochemistry. However, its production and impact are not well understood. Our study presents field observations of ClNO2 at three sites in northern China. These observations provide new insights into nighttime processes that produce ClNO2 and the significant impact of ClNO2 on secondary pollutions during daytime. The results improve the understanding of photochemical pollution in the lower part of the atmosphere.
Hui Zhang, Xuewu Fu, Ben Yu, Baoxin Li, Peng Liu, Guoqing Zhang, Leiming Zhang, and Xinbin Feng
Atmos. Chem. Phys., 21, 15847–15859, https://doi.org/10.5194/acp-21-15847-2021, https://doi.org/10.5194/acp-21-15847-2021, 2021
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Our observations of speciated atmospheric mercury at the Waliguan GAW Baseline Observatory show that concentrations of gaseous elemental mercury (GEM) and particulate bound mercury (PBM) were elevated compared to the Northern Hemisphere background. We propose that the major sources of GEM and PBM were mainly related to anthropogenic emissions and desert dust sources. This study highlights that dust-related sources played an important role in the variations of PBM in the Tibetan Plateau.
Deborah F. McGlynn, Laura E. R. Barry, Manuel T. Lerdau, Sally E. Pusede, and Gabriel Isaacman-VanWertz
Atmos. Chem. Phys., 21, 15755–15770, https://doi.org/10.5194/acp-21-15755-2021, https://doi.org/10.5194/acp-21-15755-2021, 2021
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We present 1 year of hourly measurements of chemically resolved Biogenic volatile organic compound (BVOCs) between 15 September 2019 and 15 September 2020, collected at a research tower in central Virginia. Concentrations of a range of BVOCs are described and examined for their impact on atmospheric reactivity. The majority of reactivity comes from α-pinene and limonene, highlighting the importance of both concentration and structure in assessing atmospheric impacts of emissions.
Adam R. Vaughan, James D. Lee, Stefan Metzger, David Durden, Alastair C. Lewis, Marvin D. Shaw, Will S. Drysdale, Ruth M. Purvis, Brian Davison, and C. Nicholas Hewitt
Atmos. Chem. Phys., 21, 15283–15298, https://doi.org/10.5194/acp-21-15283-2021, https://doi.org/10.5194/acp-21-15283-2021, 2021
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Validating emissions estimates of atmospheric pollutants is a vital pathway towards reducing urban concentrations of air pollution and ensuring effective legislative controls are implemented. The work presented here highlights a strategy capable of quantifying and spatially disaggregating NOx emissions over challenging urban terrain. This work shows great scope as a tool for emission inventory validation and independent generation of high-resolution surface emissions on a city-wide scale.
Hélène Angot, Connor Davel, Christine Wiedinmyer, Gabrielle Pétron, Jashan Chopra, Jacques Hueber, Brendan Blanchard, Ilann Bourgeois, Isaac Vimont, Stephen A. Montzka, Ben R. Miller, James W. Elkins, and Detlev Helmig
Atmos. Chem. Phys., 21, 15153–15170, https://doi.org/10.5194/acp-21-15153-2021, https://doi.org/10.5194/acp-21-15153-2021, 2021
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After a multidecadal global decline in atmospheric abundance of ethane and propane (precursors of tropospheric ozone and aerosols), previous work showed a reversal of this trend in 2009–2015 in the Northern Hemisphere due to the growth in oil and natural gas production in North America. Here we show a temporary pause in the growth of atmospheric ethane and propane in 2015–2018 and highlight the critical need for additional top-down studies to further constrain ethane and propane emissions.
Cited articles
Abbott, B. W. and Jones, J. B.: Permafrost collapse alters soil carbon
stocks, respiration, CH4, and N2O in upland tundra, Glob.
Change Biol., 21, 4570–4587, https://doi.org/10.1111/gcb.13069, 2015.
Anderson, B., Bartlett, K., Frolking, S., Hayhoe, K., Jenkins, J., and Salas,
W.: Methane and Nitrous Oxide Emissions from Natural Sources, Office of
Atmospheric Programs, US EPA, EPA 430-R-10-001, Washington DC, 2010.
Avis, C. A., Weaver, A. J., and Meissner, K. J.: Reduction in areal extent of
high-latitude wetlands in response to permafrost thaw, Nat. Geosci., 4,
444–448, https://doi.org/10.1038/ngeo1160, 2011.
Borge, A. F., Westermann, S., Solheim, I., and Etzelmüller, B.: Strong
degradation of palsas and peat plateaus in northern Norway during the last 60
years, The Cryosphere, 11, 1–16, https://doi.org/10.5194/tc-11-1-2017, 2017.
Butterbach-Bahl, K., Baggs, E. M., Dannenmann, M., Kiese, R., and
Zechmeister-Boltenstern, S.: Nitrous oxide emissions from soils: how well do
we understand the processes and their controls?, Philos. T. R. Soc. B, 368,
20130122–20130122, https://doi.org/10.1098/rstb.2013.0122, 2013.
Crawford, T., McMillen, R., Dobosy, R., and MacPherson, I.: Correcting
airborne flux measurements for aircraft speed variation, Bound.-Lay.
Meteorol., 66, 237–245, 1993.
Davidson, E. A. and Kanter, D.: Inventories and scenarios of nitrous oxide
emissions, Environ. Res. Lett., 9, 105012,
https://doi.org/10.1088/1748-9326/9/10/105012, 2014.
Dobosy, R., Dumas, E., and Senn, D.: Calibration and Quality Assurance of an
Airborne Turbulence Probe in an Aeronautical Wind Tunnel, J. Atmos. Ocean.
Tech., 30, 182–196, https://doi.org/10.1175/JTECH-D-11-00206.1, 2013.
Dobosy, R., Sayres, D., Healy, C., Dumas, E., Heuer, M., Kochendorfer, J.,
Baker, B., and Anderson, J. G.: Estimating random uncertainty in airborne
flux measurements over Alaskan tundra: Update in the Flux-Fragment Method, J.
Atmos. Ocean. Tech., 34, 1807–1822, https://doi.org/10.1175/JTECH-D-16-0187.1, 2017.
Elberling, B., Christiansen, H. H., and Hansen, B. U.: High nitrous oxide
production from thawing permafrost, Nat. Geosci., 3, 332–335,
https://doi.org/10.1038/ngeo893, 2010.
Eugster, W. and Merbold, L.: Eddy covariance for quantifying trace gas fluxes
from soils, SOIL, 1, 187–205, https://doi.org/10.5194/soil-1-187-2015, 2015.
Eugster, W., Zeyer, K., Zeeman, M., Michna, P., Zingg, A., Buchmann, N., and
Emmenegger, L.: Methodical study of nitrous oxide eddy covariance
measurements using quantum cascade laser spectrometery over a Swiss forest,
Biogeosciences, 4, 927–939, https://doi.org/10.5194/bg-4-927-2007, 2007.
Foken, T.: Micrometeorology, 2nd edn., Springer-Verlag, Bayreuth, Germany,
113–115, 2008.
Fuchs, M., Grosse, G., Strauss, J., Günther, F., Grigoriev, M., Maximov,
G. M., and Hugelius, G.: Carbon and nitrogen pools in thermokarst-affected
permafrost landscapes in Arctic Siberia, Biogeosciences, 15, 953–971,
https://doi.org/10.5194/bg-15-953-2018, 2018.
Garman, K., Hill, K. A., Wyss, P., Carlsen, M., Zimmerman, J. R., Stirm, B.
H., Carney, T. Q., Santini, R., and Shepson, P. B.: An airborne and wind
tunnel evaluation of a wind turbulence measurement system for aircraft-based
flux measurements, J. Atmos. Ocean. Tech., 23, 1696–1708,
https://doi.org/10.1175/JTECH1940, 2006.
Gioli, B., Miglietta, F., De Martino, B., Hutjes, R. W. A., Dolman, H. A. J.,
Lindroth, A., Schumacher, M., Sanz, M., Manca, G., Peressotti, A., and Dumas,
E.: Comparison between tower and aircraft-based eddy covariance fluxes in
five European regions, Agr. Forest Meteorol., 127, 1–16,
https://doi.org/10.1016/j.agrformet.2004.08.004, 2004.
Gu, L., Massman, W. J., Leuning, R., Pallardy, S. G., Meyers, T., Hanson, P.
J., Riggs, J. S., Hosman, K. P., and Yang, B.: The fundamental equation of
eddy covariance and its application in flux measurements, Agr. Forest
Meteorol., 152, 135–148, https://doi.org/10.1016/j.agrformet.2011.09.014, 2012.
Harden, J. W., Koven, C., Ping, C., Hugelius, G., McGuire, A. D., Camill, P.,
Jorgenson, T., Kuhry, P., Michaelson, G. J., O'Donnell, J. A., Schuur, E. A.
G., Tarnocai, C., Johnson, K., and Grosse, G..: Field information links
permafrost carbon to physical vulnerabilities of thawing, Geophys. Res.
Lett., 39, 71–6, https://doi.org/10.1029/2012GL051958, 2012.
Healy, C.: Mapping and Characterizing the Alaskan North Slope Methane Flux
With Airborne Eddy-Covariance Flux Measurements, PhD dissertation, Graduate
School of Arts & Sciences, Harvard University, 2016.
Hensen, A., Skiba, U., and Famulari, D.: Low cost and state of the art
methods to measure nitrous oxide emissions, Environ. Res. Lett., 8, 025022,
https://doi.org/10.1088/1748-9326/8/2/025022, 2013.
IPCC: Climate Change 2013: The Physical Science Basis. Contribution of
Working Group I to the Fifth Assessment Report of the Intergovernmental Panel
on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K.,
Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and
Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New
York, NY, USA, 1535 pp., https://doi.org/10.1017/CBO9781107415324, 2013.
Jansson, J. K. and Taş, N.: The microbial ecology of permafrost, Nat.
Rev. Microbiol., 12, 414–425, https://doi.org/10.1038/nrmicro3262, 2014.
Jones, B. M., Baughman, C. A., Romanovsky, V. E., Parsekian, A. D., Babcock,
E. L., Stephani, E., Jones, M. C., Grosse, G., and Berg, E. E.: Presence of
rapidly degrading permafrost plateaus in south-central Alaska, The
Cryosphere, 10, 2673–2692, https://doi.org/10.5194/tc-10-2673-2016, 2016.
Klemedtsson, L., Arnold, Von, K., Weslien, P., and Gundersen, P.: Soil CN
ratio as a scalar parameter to predict nitrous oxide emissions, Glob. Change
Biol., 11, 1142–1147, https://doi.org/10.1111/j.1365-2486.2005.00973.x, 2005.
Kljun, N., Calanca, P., Rotach, M., and Schmid, H.: A simple parameterization
for flux footprint predictions, Bound.-Lay. Meteorol., 112, 503–523,
https://doi.org/10.1023/B:BOUN.0000030653.71031.96, 2004.
Kroon, P. S., Hensen, A., Jonker, H. J. J., Zahniser, M. S., van 't Veen, W.
H., and Vermeulen, A. T.: Suitability of quantum cascade laser spectroscopy
for CH4 and N2O eddy covariance flux measurements,
Biogeosciences, 4, 715–728, https://doi.org/10.5194/bg-4-715-2007, 2007.
Leise, J. A., Masters, J. M., and Dobosy, R. J.: National Oceanic and
Atmospheric Association. Wind measurements from aircraft, NOAA technical
memorandum OAR ARL-266, 209 pp., https://doi.org/10.7289/V5/TM-OAR-ARL-266, 2013.
Mahrt, L.: Flux Sampling Errors for Aircraft and Towers, J. Atmos. Ocean.
Tech., 15, 416–428, https://doi.org/10.1175/1520-0426(1998)015<0416:FSEFAA>2.0.CO;2,
1998.
Martikainen, P. J., Nykänen, H., Crill, P., and Silvola, J.: Effect of a
lowered water table on nitrous oxide fluxes from northern peatlands, Nature,
366, 51–53, 1993.
Marushchak, M. E., Pitkamaki, A., Koponen, H., Biasi, C., Seppala, M., and
Martikainen, P. J.: Hot spots for nitrous oxide emissions found in different
types of permafrost peatlands, Glob. Change Biol., 17, 2601–2614,
https://doi.org/10.1111/j.1365-2486.2011.02442.x, 2011.
McGuire, A. D., Christensen, T. R., Hayes, D., Heroult, A., Euskirchen, E.,
Kimball, J. S., Koven, C., Lafleur, P., Miller, P. A., Oechel, W., Peylin,
P., Williams, M., and Yi, Y.: An assessment of the carbon balance of Arctic
tundra: comparisons among observations, process models, and atmospheric
inversions, Biogeosciences, 9, 3185–3204, https://doi.org/10.5194/bg-9-3185-2012,
2012.
Meinshausen, M., Smith, S. J., Calvin, K., Daniel, J. S., Kainuma, M. L. T.,
Lamarque, J.-F., Matsumoto, K., Montzka, S. A., Raper, S. C. B., Riahi, K.,
Thomson, A., Velders, G. J. M., and van Vuuren, D. P. P.: The RCP greenhouse
gas concentrations and their extensions from 1765 to 2300, Climatic Change,
109, 213–241, https://doi.org/10.1007/s10584-011-0156-z, 2011.
Morley, N., Baggs, E. M., Dörsch, P., and Bakken, L.: Production of NO,
N2O and N2 by extracted soil bacteria, regulation by
and O2 concentrations, FEMS Microbiol. Ecol., 65,
102–112, https://doi.org/10.1111/j.1574-6941.2008.00495.x, 2008.
Mudelsee, M.: Climate Time Series Analysis: Classical Statistical and
Bootstrap Methods, 2nd edn., Springer, Cham, Switzerland, 474 pp., 2010.
North Slope Science Initiative: North Slope Science Initiative Landcover
Mapping Summary Report, available at:
http://catalog.northslopescience.org/catalog/entries/4616-nssi-landcover-report-landcover-mapping-for-north
(last access: 27 January 2018), 2013.
Park, S., Boering, K. A., Etheridge, D. M., Ferretti, D., Fraser, P. J., Kim,
K.-R., Krummel, P. B., Langenfelds, R. L., van Ommen, T. D., Steele, L. P.,
and Trudinger, C. M.: Trends and seasonal cycles in the isotopic composition
of nitrous oxide since 1940, Nat. Geosci., 5, 261–265,
https://doi.org/10.1038/ngeo1421, 2012.
Pihlatie, M. K., Kiese, R., Brüggemann, N., Butterbach-Bahl, K.,
Kieloaho, A.-J., Laurila, T., Lohila, A., Mammarella, I., Minkkinen, K.,
Penttilä, T., Schönborn, J., and Vesala, T.: Greenhouse gas fluxes in
a drained peatland forest during spring frost-thaw event, Biogeosciences, 7,
1715–1727, https://doi.org/10.5194/bg-7-1715-2010, 2010.
Potter, C., Matson, P., Vitousek, P., and Davidson, E.: Process modeling of
controls on nitrogen trace gas emissions from soils worldwide, J. Geophys.
Res., 101, 1361–1377, https://doi.org/10.1029/95JD02028, 1996.
Rannik, Ü., Haapanala, S., Shurpali, N. J., Mammarella, I., Lind, S.,
Hyvönen, N., Peltola, O., Zahniser, M., Martikainen, P. J., and Vesala,
T.: Intercomparison of fast response commercial gas analysers for nitrous
oxide flux measurements under field conditions, Biogeosciences, 12, 415–432,
https://doi.org/10.5194/bg-12-415-2015, 2015.
Ravishankara, A. R., Daniel, J. S., and Portmann, R. W.: Nitrous Oxide
(N2O): The Dominant Ozone-Depleting Substance Emitted in the 21st
Century, Science, 326, 123–125, https://doi.org/10.1126/science.1176985, 2009.
Rella, C.: Accurate Greenhouse Gas Measurements in Humid Gas Streams Using
the Picarro G1301 Carbon Dioxide/Methane/Water Vapor Gas Analyzer, Picarro,
Inc, Santa Clara, CA, USA, 2010.
Repo, M. E., Susiluoto, S., Lind, S. E., Jokinen, S., Elsakov, V., Biasi, C.,
Virtanen, T., and Martikainen, P.: Large N2O emissions from
cryoturbated peat soil in tundra, Nat. Geosci., 2, 189–192,
https://doi.org/10.1038/ngeo434, 2009.
Sayres, D. and Dobosy, R.: Alaska 2013 Campaign, Harvard Dataverse, V1,
https://doi.org/10.7910/DVN/YM70Y7, 2018.
Sayres, D. S., Dobosy, R., Healy, C., Dumas, E., Kochendorfer, J., Munster,
J., Wilkerson, J., Baker, B., and Anderson, J. G.: Arctic regional methane
fluxes by ecotope as derived using eddy covariance from a low-flying
aircraft, Atmos. Chem. Phys., 17, 8619–8633, https://doi.org/10.5194/acp-17-8619-2017,
2017.
Schreiber, F., Wunderlin, P., Udert, K. M., and Wells, G. F.: Nitric oxide
and nitrous oxide turnover in natural and engineered microbial communities:
biological pathways, chemical reactions, and novel technologies, Front.
Microbiol., 3, 1–24, https://doi.org/10.3389/fmicb.2012.00372, 2012.
Sellers, P., Hall, F., Kelly, R. D., Black, A., Baldocchi, D., Berry, J.,
Ryan, M., Ranson, K. J., Crill, P. M., Lettenmaier, D. P., Margolis, H.,
Cihlar, J., Newcomer, J., Fitzjarrald, D., Jarvis, P. G., Gower, S. T.,
Halliwell, D., Williams, D., Goodison, B., Wickland, D. E., and Guertin, F.
E.: BOREAS in 1997: Experiment overview, scientific results, and future
directions, J. Geophys. Res., 102, 28731–28769, https://doi.org/10.1029/97JD03300,
1997.
Serreze, M. C. and Barry, R. G.: Processes and impacts of Arctic
amplification: A research synthesis, Global Planet. Change, 77, 85–96,
https://doi.org/10.1016/j.gloplacha.2011.03.004, 2011.
Syakila, A. and Kroeze, C.: The global nitrous oxide budget revisited,
Greenhouse Gas Measurement and Management, 1, 17–26,
https://doi.org/10.3763/ghgmm.2010.0007, 2011.
Vellinga, O., Dobosy, R., Dumas, E. J., Gioli, B., Elbers, J. A., and Hutjes,
R. W. A..: Calibration and quality assurance of flux observations from a
small research aircraft, J. Atmos. Ocean. Tech., 30, 161–181,
https://doi.org/10.1175/JTECH-D-11-00138.1, 2013.
Voigt, C., Lamprecht, R. E., Marushchak, M. E., Lind, S. E., Novakovskiy, A.,
Aurela, M., Martikainen, P. J., and Biasi, C.: Warming of subarctic tundra
increases emissions of all three important greenhouse gases – carbon
dioxide, methane, and nitrous oxide, Glob. Change Biol., 23, 3121–3138,
https://doi.org/10.1111/gcb.13563, 2016.
Voigt, C., Marushchak, M. E., Lamprecht, R. E., Jackowicz-Korczyński, M.,
Lindgren, A., Mastepanov, M., Granlund, L., Christensen, T., Tahvanainen, T.,
Martikainen, P. J., and Biasi, C.: Increased nitrous oxide emissions from
Arctic peatlands after permafrost thaw, P. Natl. Acad. Sci. USA, 114,
6238–6243, https://doi.org/10.1073/pnas.1702902114, 2017.
Webb, E., Pearman, G., and Leuning, R.: Correction of flux measurements for
density effects due to heat and water vapour transfer, Q. J. Roy. Meteor.
Soc., 106, 85–100, https://doi.org/10.1002/qj.49710644707, 1980.
Weinstock, E., Smith, J. B., Sayres, D. S., Pittman, J. V., Spackman, J. R.,
Hinsta, E. J., Hanisco, T. F., Moyer, E. J., St. Clair, J. M., Sargent, M.
R., and Anderson, J. G.: Validation of the Harvard Lyman-α in situ
water vapor instrument: Implications for the mechanism that control
stratospheric water vapor, J. Geophys. Res., 114, D23301,
https://doi.org/10.1029/2009JD012427, 2009.
Yang, G., Peng, Y., Marushchak, M.E., Chen, Y., Wang, G., Li, F., Zhang, D.,
Wang, J., Yu, J., Liu, L., Qin, S., Kou, D., and Yang, Y.: Magnitude and
Pathways of Increased Nitrous Oxide Emissions from Uplands Following
Permafrost Thaw, Environ. Sci. Technol., 52, 9162–9169,
https://doi.org/10.1021/acs.est.8b02271, 2018.
Zhuang, Q., Lu, Y., and Chen, M.: An inventory of global N2O
emissions from the soils of natural terrestrial ecosystems, Atmos. Environ.,
47, 66–75, 2012.
Zona, D., Jannsens, I.A., Aubinet, M., Gioli, B., Vicca, S., Fichot, R., and
Ceulemans, R.: Fluxes of the greenhouse gases (CO2, CH4 and
N2O) above a short-rotation poplar plantation after conversion from
agricultural land, Agr. Forest Meteorol., 164, 100–110,
https://doi.org/10.1016/j.agrformet.2012.10.008, 2013.
Short summary
As frozen soil, called permafrost, increasingly thaws over the years, scientists have put much effort into understanding how this may increase carbon emissions, which would exacerbate climate change. Our work supports the emerging view that these efforts should also include nitrous oxide (N2O), a more potent greenhouse gas. Using a low-flying aircraft to study thousands of acres of Alaskan permafrost, we observed average N2O emissions higher than typically assumed for regions such as this.
As frozen soil, called permafrost, increasingly thaws over the years, scientists have put much...
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