Articles | Volume 19, issue 4
https://doi.org/10.5194/acp-19-2343-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-2343-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Wintertime secondary organic aerosol formation in Beijing–Tianjin–Hebei (BTH): contributions of HONO sources and heterogeneous reactions
Li Xing
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Jiarui Wu
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Miriam Elser
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Shengrui Tong
State Key Laboratory for Structural Chemistry of Unstable and Stable
Species, Beijing National Laboratory for Molecular Sciences (BNLMS),
Institute of Chemistry, Chinese Academy of Sciences, Beijing, China
Suixin Liu
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Xia Li
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Lang Liu
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Junji Cao
CORRESPONDING AUTHOR
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Jiamao Zhou
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
Imad El-Haddad
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Rujin Huang
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
State Key Laboratory for Structural Chemistry of Unstable and Stable
Species, Beijing National Laboratory for Molecular Sciences (BNLMS),
Institute of Chemistry, Chinese Academy of Sciences, Beijing, China
Xuexi Tie
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Guohui Li
CORRESPONDING AUTHOR
Key Laboratory of Aerosol Chemistry and Physics, SKLLQG, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
CAS Center for Excellence in Quaternary Science and Global Change, Xi'an,
China
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Latest update: 16 Aug 2024
Short summary
We used the WRF-CHEM model to simulate wintertime secondary organic aerosol (SOA) concentrations over Beijing–Tianjin–Hebei (BTH), China. Heterogeneous HONO sources increased the near-surface SOA by 46.3 % in BTH. Direct emissions of glyoxal and methylglyoxal from residential sources contributed 25.5 % to the total SOA mass. Our study highlights the importance of heterogeneous HONO sources and primary residential emissions of glyoxal and methylglyoxal to SOA formation in winter over BTH.
We used the WRF-CHEM model to simulate wintertime secondary organic aerosol (SOA) concentrations...
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