Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15447-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15447-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
17 Dec 2019
Research article |
| 17 Dec 2019
| 17 Dec 2019
The sensitivity of Southern Ocean aerosols and cloud microphysics to sea spray and sulfate aerosol production in the HadGEM3-GA7.1 chemistry–climate model
Laura E. Revell
CORRESPONDING AUTHOR
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Stefanie Kremser
Bodeker Scientific, Alexandra, New Zealand
Sean Hartery
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Mike Harvey
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Jane P. Mulcahy
Met Office, Exeter, UK
Jonny Williams
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Olaf Morgenstern
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Adrian J. McDonald
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Vidya Varma
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Leroy Bird
Bodeker Scientific, Alexandra, New Zealand
Alex Schuddeboom
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
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31 citations as recorded by crossref.
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- Coalescence Scavenging Drives Droplet Number Concentration in Southern Ocean Low Clouds L. Kang et al. 10.1029/2022GL097819
- Are the Significant Ionospheric Anomalies Associated with the 2007 Great Deep-Focus Undersea Jakarta–Java Earthquake? D. Tao et al. 10.3390/rs14092211
- Evaluation of Cloud and Precipitation Simulations in CAM6 and AM4 Using Observations Over the Southern Ocean X. Zhou et al. 10.1029/2020EA001241
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- The biogeochemistry of marine dimethylsulfide F. Hopkins et al. 10.1038/s43017-023-00428-7
- Marine aerosol in Aotearoa New Zealand: implications for air quality, climate change and public health L. Revell et al. 10.1080/03036758.2024.2319753
- UKESM1.1: development and evaluation of an updated configuration of the UK Earth System Model J. Mulcahy et al. 10.5194/gmd-16-1569-2023
- The sensitivity of Southern Ocean atmospheric dimethyl sulfide (DMS) to modeled oceanic DMS concentrations and emissions Y. Bhatti et al. 10.5194/acp-23-15181-2023
- Atmospheric Particle Number Concentrations and New Particle Formation over the Southern Ocean and Antarctica: A Critical Review J. Wang et al. 10.3390/atmos14020402
- Effect of Sodium Dodecyl Benzene Sulfonate on the Production of Cloud Condensation Nuclei from Breaking Waves S. Hartery et al. 10.1021/acsearthspacechem.2c00230
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- Influence of open ocean biogeochemistry on aerosol and clouds: Recent findings and perspectives K. Sellegri et al. 10.1525/elementa.2023.00058
- Polarimetric Backscatter Sonde Observations of Southern Ocean Clouds and Aerosols M. Hamilton et al. 10.3390/atmos11040399
- Low‐Volatility Vapors and New Particle Formation Over the Southern Ocean During the Antarctic Circumnavigation Expedition A. Baccarini et al. 10.1029/2021JD035126
- Influences of Antarctic Ozone Depletion on Southern Ocean Aerosols Y. Bhatti et al. 10.1029/2022JD037199
- The Importance of the Representation of DMS Oxidation in Global Chemistry‐Climate Simulations E. Hoffmann et al. 10.1029/2021GL094068
- The value of remote marine aerosol measurements for constraining radiative forcing uncertainty L. Regayre et al. 10.5194/acp-20-10063-2020
- A Critical Review of Ground Based Observations of Earthquake Precursors L. Conti et al. 10.3389/feart.2021.676766
- Atmosphere‐Ocean Feedback From Wind‐Driven Sea Spray Aerosol Production L. Revell et al. 10.1029/2020GL091900
- Factors controlling marine aerosol size distributions and their climate effects over the northwest Atlantic Ocean region B. Croft et al. 10.5194/acp-21-1889-2021
- Observation on the Droplet Ranging from 2 to 16 μm in Cloud Droplet Size Distribution Based on Digital Holography P. Gao et al. 10.3390/rs14102414
- Rapid growth of Aitken-mode particles during Arctic summer by fog chemical processing and its implication S. Kecorius et al. 10.1093/pnasnexus/pgad124
- The hemispheric contrast in cloud microphysical properties constrains aerosol forcing I. McCoy et al. 10.1073/pnas.1922502117
- Key challenges for tropospheric chemistry in the Southern Hemisphere C. Paton-Walsh et al. 10.1525/elementa.2021.00050
- Summer aerosol measurements over the East Antarctic seasonal ice zone J. Simmons et al. 10.5194/acp-21-9497-2021
- Marine aerosol properties over the Southern Ocean in relation to the wintertime meteorological conditions M. Thomas et al. 10.5194/acp-22-119-2022
- Statistical analysis of the effects of forests on fog I. Hůnová et al. 10.1016/j.scitotenv.2021.146675
- Influences of Recent Particle Formation on Southern Ocean Aerosol Variability and Low Cloud Properties I. McCoy et al. 10.1029/2020JD033529
31 citations as recorded by crossref.
- Evaluation of SO<sub>2</sub>, SO<sub>4</sub><sup>2−</sup> and an updated SO<sub>2</sub> dry deposition parameterization in the United Kingdom Earth System Model C. Hardacre et al. 10.5194/acp-21-18465-2021
- Coalescence Scavenging Drives Droplet Number Concentration in Southern Ocean Low Clouds L. Kang et al. 10.1029/2022GL097819
- Are the Significant Ionospheric Anomalies Associated with the 2007 Great Deep-Focus Undersea Jakarta–Java Earthquake? D. Tao et al. 10.3390/rs14092211
- Evaluation of Cloud and Precipitation Simulations in CAM6 and AM4 Using Observations Over the Southern Ocean X. Zhou et al. 10.1029/2020EA001241
- The dual-field-of-view polarization lidar technique: a new concept in monitoring aerosol effects in liquid-water clouds – case studies C. Jimenez et al. 10.5194/acp-20-15265-2020
- Untangling the influence of Antarctic and Southern Ocean life on clouds M. Mallet et al. 10.1525/elementa.2022.00130
- The biogeochemistry of marine dimethylsulfide F. Hopkins et al. 10.1038/s43017-023-00428-7
- Marine aerosol in Aotearoa New Zealand: implications for air quality, climate change and public health L. Revell et al. 10.1080/03036758.2024.2319753
- UKESM1.1: development and evaluation of an updated configuration of the UK Earth System Model J. Mulcahy et al. 10.5194/gmd-16-1569-2023
- The sensitivity of Southern Ocean atmospheric dimethyl sulfide (DMS) to modeled oceanic DMS concentrations and emissions Y. Bhatti et al. 10.5194/acp-23-15181-2023
- Atmospheric Particle Number Concentrations and New Particle Formation over the Southern Ocean and Antarctica: A Critical Review J. Wang et al. 10.3390/atmos14020402
- Effect of Sodium Dodecyl Benzene Sulfonate on the Production of Cloud Condensation Nuclei from Breaking Waves S. Hartery et al. 10.1021/acsearthspacechem.2c00230
- Description and evaluation of aerosol in UKESM1 and HadGEM3-GC3.1 CMIP6 historical simulations J. Mulcahy et al. 10.5194/gmd-13-6383-2020
- Modelling wintertime sea-spray aerosols under Arctic haze conditions E. Ioannidis et al. 10.5194/acp-23-5641-2023
- Influence of open ocean biogeochemistry on aerosol and clouds: Recent findings and perspectives K. Sellegri et al. 10.1525/elementa.2023.00058
- Polarimetric Backscatter Sonde Observations of Southern Ocean Clouds and Aerosols M. Hamilton et al. 10.3390/atmos11040399
- Low‐Volatility Vapors and New Particle Formation Over the Southern Ocean During the Antarctic Circumnavigation Expedition A. Baccarini et al. 10.1029/2021JD035126
- Influences of Antarctic Ozone Depletion on Southern Ocean Aerosols Y. Bhatti et al. 10.1029/2022JD037199
- The Importance of the Representation of DMS Oxidation in Global Chemistry‐Climate Simulations E. Hoffmann et al. 10.1029/2021GL094068
- The value of remote marine aerosol measurements for constraining radiative forcing uncertainty L. Regayre et al. 10.5194/acp-20-10063-2020
- A Critical Review of Ground Based Observations of Earthquake Precursors L. Conti et al. 10.3389/feart.2021.676766
- Atmosphere‐Ocean Feedback From Wind‐Driven Sea Spray Aerosol Production L. Revell et al. 10.1029/2020GL091900
- Factors controlling marine aerosol size distributions and their climate effects over the northwest Atlantic Ocean region B. Croft et al. 10.5194/acp-21-1889-2021
- Observation on the Droplet Ranging from 2 to 16 μm in Cloud Droplet Size Distribution Based on Digital Holography P. Gao et al. 10.3390/rs14102414
- Rapid growth of Aitken-mode particles during Arctic summer by fog chemical processing and its implication S. Kecorius et al. 10.1093/pnasnexus/pgad124
- The hemispheric contrast in cloud microphysical properties constrains aerosol forcing I. McCoy et al. 10.1073/pnas.1922502117
- Key challenges for tropospheric chemistry in the Southern Hemisphere C. Paton-Walsh et al. 10.1525/elementa.2021.00050
- Summer aerosol measurements over the East Antarctic seasonal ice zone J. Simmons et al. 10.5194/acp-21-9497-2021
- Marine aerosol properties over the Southern Ocean in relation to the wintertime meteorological conditions M. Thomas et al. 10.5194/acp-22-119-2022
- Statistical analysis of the effects of forests on fog I. Hůnová et al. 10.1016/j.scitotenv.2021.146675
- Influences of Recent Particle Formation on Southern Ocean Aerosol Variability and Low Cloud Properties I. McCoy et al. 10.1029/2020JD033529
Latest update: 14 Dec 2024
Short summary
Aerosols over the Southern Ocean consist primarily of sea salt and sulfate, yet are seasonally biased in our model. We test three sulfate chemistry schemes to investigate DMS oxidation, which forms sulfate aerosol. Simulated cloud droplet number concentrations improve using more complex sulfate chemistry. We also show that a new sea spray aerosol source function, developed from measurements made on a recent Southern Ocean research voyage, improves the model's simulation of aerosol optical depth.
Aerosols over the Southern Ocean consist primarily of sea salt and sulfate, yet are seasonally...
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