Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15447-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15447-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
The sensitivity of Southern Ocean aerosols and cloud microphysics to sea spray and sulfate aerosol production in the HadGEM3-GA7.1 chemistry–climate model
Laura E. Revell
CORRESPONDING AUTHOR
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Stefanie Kremser
Bodeker Scientific, Alexandra, New Zealand
Sean Hartery
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Mike Harvey
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Jane P. Mulcahy
Met Office, Exeter, UK
Jonny Williams
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Olaf Morgenstern
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Adrian J. McDonald
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Vidya Varma
National Institute of Water and Atmospheric Research, Wellington, New Zealand
Leroy Bird
Bodeker Scientific, Alexandra, New Zealand
Alex Schuddeboom
School of Physical and Chemical Sciences, University of Canterbury, Christchurch, New Zealand
Data sets
Cruise data inventory from the R/V Tangaroa 61TG_3052 cruise in the Southern Ocean during 1999 (SOIREE project) P. W. Boyd http://lod.bco-dmo.org/id/dataset/3212
Short summary
Aerosols over the Southern Ocean consist primarily of sea salt and sulfate, yet are seasonally biased in our model. We test three sulfate chemistry schemes to investigate DMS oxidation, which forms sulfate aerosol. Simulated cloud droplet number concentrations improve using more complex sulfate chemistry. We also show that a new sea spray aerosol source function, developed from measurements made on a recent Southern Ocean research voyage, improves the model's simulation of aerosol optical depth.
Aerosols over the Southern Ocean consist primarily of sea salt and sulfate, yet are seasonally...
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