Articles | Volume 19, issue 22
https://doi.org/10.5194/acp-19-14403-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-19-14403-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
28 Nov 2019
Research article |
| 28 Nov 2019
| 28 Nov 2019
Impact of anthropogenic emissions on biogenic secondary organic aerosol: observation in the Pearl River Delta, southern China
Yu-Qing Zhang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Duo-Hong Chen
State Environmental Protection Key Laboratory of Regional Air Quality Monitoring, Guangdong Environmental Monitoring Center,
Guangzhou 510308, China
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Tao Zhang
State Environmental Protection Key Laboratory of Regional Air Quality Monitoring, Guangdong Environmental Monitoring Center,
Guangzhou 510308, China
Jun-Qi Wang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Qian Cheng
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Hao Jiang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Wei Song
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Yu-Bo Ou
State Environmental Protection Key Laboratory of Regional Air Quality Monitoring, Guangdong Environmental Monitoring Center,
Guangzhou 510308, China
Peng-Lin Ye
Aerodyne Research Inc., Billerica, Massachusetts 01821, USA
Gan Zhang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Xin-Ming Wang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Viewed
Total article views: 2,592 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 03 Jul 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,737 | 814 | 41 | 2,592 | 342 | 47 | 88 |
- HTML: 1,737
- PDF: 814
- XML: 41
- Total: 2,592
- Supplement: 342
- BibTeX: 47
- EndNote: 88
Total article views: 2,182 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 28 Nov 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,525 | 623 | 34 | 2,182 | 237 | 39 | 73 |
- HTML: 1,525
- PDF: 623
- XML: 34
- Total: 2,182
- Supplement: 237
- BibTeX: 39
- EndNote: 73
Total article views: 410 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 03 Jul 2019)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 212 | 191 | 7 | 410 | 105 | 8 | 15 |
- HTML: 212
- PDF: 191
- XML: 7
- Total: 410
- Supplement: 105
- BibTeX: 8
- EndNote: 15
Viewed (geographical distribution)
Total article views: 2,592 (including HTML, PDF, and XML)
Thereof 2,667 with geography defined
and -75 with unknown origin.
Total article views: 2,182 (including HTML, PDF, and XML)
Thereof 2,076 with geography defined
and 106 with unknown origin.
Total article views: 410 (including HTML, PDF, and XML)
Thereof 591 with geography defined
and -181 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
32 citations as recorded by crossref.
- Contrasting compositions and sources of organic aerosol markers in summertime PM2.5 from urban and mountainous regions in the North China Plain Y. Yi et al. 10.1016/j.scitotenv.2020.144187
- Insight into the characteristics of carbonaceous aerosols at urban and regional sites in the downwind area of Pearl River Delta region, China M. Lu et al. 10.1016/j.scitotenv.2021.146251
- Time‐Resolved Measurements of PM2.5 Chemical Composition and Brown Carbon Absorption in Nanjing, East China: Diurnal Variations and Organic Tracer‐Based PMF Analysis W. Feng et al. 10.1029/2023JD039092
- Contrasting molecular characteristics and formation mechanisms of biogenic and anthropogenic secondary organic aerosols at the summit and foot of Mt. Huang, East China Y. Wang et al. 10.1016/j.scitotenv.2023.165116
- Different roles of primary and secondary sources in reducing PM2.5: Insights from molecular markers in Pearl River Delta, South China K. Yang et al. 10.1016/j.atmosenv.2022.119487
- Diurnal Variations in High Time-Resolved Molecular Distributions and Formation Mechanisms of Biogenic Secondary Organic Aerosols at Mt. Huang, East China Y. Li et al. 10.3390/molecules28165939
- Characteristics of PM2.5-bound secondary organic aerosol tracers in a coastal city in Southeastern China: Seasonal patterns and pollution identification T. Liu et al. 10.1016/j.atmosenv.2020.117710
- Diurnal variations in primary and secondary organic aerosols in an eastern China coastal city: The impact of land-sea breezes Q. Zhang et al. 10.1016/j.envpol.2023.121016
- Evolution of Brown Carbon Aerosols during Atmospheric Long-Range Transport in the South Asian Outflow and Himalayan Cryosphere V. Choudhary et al. 10.1021/acsearthspacechem.2c00047
- Secondary organic aerosols in PM2.5 on a coastal island in southeastern China: Impact of atmospheric process and biomass burning N. Chen et al. 10.1016/j.atmosenv.2023.119841
- Tracer-based characterization of source variations of PM2.5 and organic carbon in Shanghai influenced by the COVID-19 lockdown S. Zhu et al. 10.1039/D0FD00091D
- Measurement report: Effects of anthropogenic emissions and environmental factors on the formation of biogenic secondary organic aerosol (BSOA) in a coastal city of southeastern China Y. Hong et al. 10.5194/acp-22-7827-2022
- Chemical Characteristics and Source Apportionment of Biogenic Primary and Secondary Organic Aerosols in an Alpine Ecosystem of Tibetan Plateau L. Cui et al. 10.1029/2022JD037897
- Short-term source apportionment of fine particulate matter with time-dependent profiles using SoFi Pro: exploring the reliability of rolling positive matrix factorization (PMF) applied to bihourly molecular and elemental tracer data Q. Wang et al. 10.5194/acp-24-475-2024
- Observational Insights into Isoprene Secondary Organic Aerosol Formation through the Epoxide Pathway at Three Urban Sites from Northern to Southern China Y. Zhang et al. 10.1021/acs.est.1c06974
- Interactions of organosulfates with water vapor under sub- and supersaturated conditions C. Peng et al. 10.5194/acp-21-7135-2021
- Chemical components and source identification of PM2.5 in non-heating season in Beijing: The influences of biomass burning and dust Y. Ren et al. 10.1016/j.atmosres.2020.105412
- Modeling Analysis of Biogenic Secondary Organic Aerosol Dependence on Anthropogenic Emissions in China X. Dong et al. 10.1021/acs.estlett.2c00104
- Impact of the COVID-19 on the vertical distributions of major pollutants from a tower in the Pearl River Delta L. Li et al. 10.1016/j.atmosenv.2022.119068
- Tracer-based characterization of fine carbonaceous aerosol in Beijing during a strict emission control period H. Ren et al. 10.1016/j.scitotenv.2022.156638
- Shipping-related pollution decreased but mortality increased in Chinese port cities Z. Luo et al. 10.1038/s44284-024-00050-8
- Molecular and Elemental Tracers‐Based Receptor Modeling of PM2.5 in Suburban Hong Kong With Hourly Time‐Scale Air Quality Considerations S. Wang et al. 10.1029/2023JD039875
- Spatiotemporal distribution and influencing factors of secondary organic aerosols in the summer atmosphere from the Bering Sea to the western North Pacific C. Hu et al. 10.1016/j.scitotenv.2022.160138
- NH3 Weakens the Enhancing Effect of SO2 on Biogenic Secondary Organic Aerosol Formation L. Du et al. 10.1021/acs.estlett.2c00959
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- Accelerated reduction of air pollutants in China, 2017-2020 C. Li et al. 10.1016/j.scitotenv.2021.150011
- Organic Molecular Tracers in PM2.5 at Urban Sites during Spring and Summer in Japan: Impact of Secondary Organic Aerosols on Water-Soluble Organic Carbon F. Ikemori et al. 10.3390/atmos12050579
- New formation and fate of Isoprene SOA markers revealed by field data-constrained modeling J. Zhang et al. 10.1038/s41612-023-00394-3
- Temporal trends of the concentration and sources of secondary organic aerosols in PM2.5 in Shanghai during 2012 and 2018 Y. Zhong et al. 10.1016/j.atmosenv.2021.118596
- Anthropogenic–Biogenic Interactions at Night: Enhanced Formation of Secondary Aerosols and Particulate Nitrogen- and Sulfur-Containing Organics from β-Pinene Oxidation L. Xu et al. 10.1021/acs.est.0c07879
- Seasonal characteristics and provenance of organic aerosols in the urban atmosphere of Liaocheng in the North China Plain: Significant effect of biomass burning Y. Li et al. 10.1016/j.partic.2022.07.012
- Size distributions of molecular markers for biogenic secondary organic aerosol in urban Beijing D. Liu et al. 10.1016/j.envpol.2023.121569
32 citations as recorded by crossref.
- Contrasting compositions and sources of organic aerosol markers in summertime PM2.5 from urban and mountainous regions in the North China Plain Y. Yi et al. 10.1016/j.scitotenv.2020.144187
- Insight into the characteristics of carbonaceous aerosols at urban and regional sites in the downwind area of Pearl River Delta region, China M. Lu et al. 10.1016/j.scitotenv.2021.146251
- Time‐Resolved Measurements of PM2.5 Chemical Composition and Brown Carbon Absorption in Nanjing, East China: Diurnal Variations and Organic Tracer‐Based PMF Analysis W. Feng et al. 10.1029/2023JD039092
- Contrasting molecular characteristics and formation mechanisms of biogenic and anthropogenic secondary organic aerosols at the summit and foot of Mt. Huang, East China Y. Wang et al. 10.1016/j.scitotenv.2023.165116
- Different roles of primary and secondary sources in reducing PM2.5: Insights from molecular markers in Pearl River Delta, South China K. Yang et al. 10.1016/j.atmosenv.2022.119487
- Diurnal Variations in High Time-Resolved Molecular Distributions and Formation Mechanisms of Biogenic Secondary Organic Aerosols at Mt. Huang, East China Y. Li et al. 10.3390/molecules28165939
- Characteristics of PM2.5-bound secondary organic aerosol tracers in a coastal city in Southeastern China: Seasonal patterns and pollution identification T. Liu et al. 10.1016/j.atmosenv.2020.117710
- Diurnal variations in primary and secondary organic aerosols in an eastern China coastal city: The impact of land-sea breezes Q. Zhang et al. 10.1016/j.envpol.2023.121016
- Evolution of Brown Carbon Aerosols during Atmospheric Long-Range Transport in the South Asian Outflow and Himalayan Cryosphere V. Choudhary et al. 10.1021/acsearthspacechem.2c00047
- Secondary organic aerosols in PM2.5 on a coastal island in southeastern China: Impact of atmospheric process and biomass burning N. Chen et al. 10.1016/j.atmosenv.2023.119841
- Tracer-based characterization of source variations of PM2.5 and organic carbon in Shanghai influenced by the COVID-19 lockdown S. Zhu et al. 10.1039/D0FD00091D
- Measurement report: Effects of anthropogenic emissions and environmental factors on the formation of biogenic secondary organic aerosol (BSOA) in a coastal city of southeastern China Y. Hong et al. 10.5194/acp-22-7827-2022
- Chemical Characteristics and Source Apportionment of Biogenic Primary and Secondary Organic Aerosols in an Alpine Ecosystem of Tibetan Plateau L. Cui et al. 10.1029/2022JD037897
- Short-term source apportionment of fine particulate matter with time-dependent profiles using SoFi Pro: exploring the reliability of rolling positive matrix factorization (PMF) applied to bihourly molecular and elemental tracer data Q. Wang et al. 10.5194/acp-24-475-2024
- Observational Insights into Isoprene Secondary Organic Aerosol Formation through the Epoxide Pathway at Three Urban Sites from Northern to Southern China Y. Zhang et al. 10.1021/acs.est.1c06974
- Interactions of organosulfates with water vapor under sub- and supersaturated conditions C. Peng et al. 10.5194/acp-21-7135-2021
- Chemical components and source identification of PM2.5 in non-heating season in Beijing: The influences of biomass burning and dust Y. Ren et al. 10.1016/j.atmosres.2020.105412
- Modeling Analysis of Biogenic Secondary Organic Aerosol Dependence on Anthropogenic Emissions in China X. Dong et al. 10.1021/acs.estlett.2c00104
- Impact of the COVID-19 on the vertical distributions of major pollutants from a tower in the Pearl River Delta L. Li et al. 10.1016/j.atmosenv.2022.119068
- Tracer-based characterization of fine carbonaceous aerosol in Beijing during a strict emission control period H. Ren et al. 10.1016/j.scitotenv.2022.156638
- Shipping-related pollution decreased but mortality increased in Chinese port cities Z. Luo et al. 10.1038/s44284-024-00050-8
- Molecular and Elemental Tracers‐Based Receptor Modeling of PM2.5 in Suburban Hong Kong With Hourly Time‐Scale Air Quality Considerations S. Wang et al. 10.1029/2023JD039875
- Spatiotemporal distribution and influencing factors of secondary organic aerosols in the summer atmosphere from the Bering Sea to the western North Pacific C. Hu et al. 10.1016/j.scitotenv.2022.160138
- NH3 Weakens the Enhancing Effect of SO2 on Biogenic Secondary Organic Aerosol Formation L. Du et al. 10.1021/acs.estlett.2c00959
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- Accelerated reduction of air pollutants in China, 2017-2020 C. Li et al. 10.1016/j.scitotenv.2021.150011
- Organic Molecular Tracers in PM2.5 at Urban Sites during Spring and Summer in Japan: Impact of Secondary Organic Aerosols on Water-Soluble Organic Carbon F. Ikemori et al. 10.3390/atmos12050579
- New formation and fate of Isoprene SOA markers revealed by field data-constrained modeling J. Zhang et al. 10.1038/s41612-023-00394-3
- Temporal trends of the concentration and sources of secondary organic aerosols in PM2.5 in Shanghai during 2012 and 2018 Y. Zhong et al. 10.1016/j.atmosenv.2021.118596
- Anthropogenic–Biogenic Interactions at Night: Enhanced Formation of Secondary Aerosols and Particulate Nitrogen- and Sulfur-Containing Organics from β-Pinene Oxidation L. Xu et al. 10.1021/acs.est.0c07879
- Seasonal characteristics and provenance of organic aerosols in the urban atmosphere of Liaocheng in the North China Plain: Significant effect of biomass burning Y. Li et al. 10.1016/j.partic.2022.07.012
- Size distributions of molecular markers for biogenic secondary organic aerosol in urban Beijing D. Liu et al. 10.1016/j.envpol.2023.121569
Latest update: 15 Apr 2024
Short summary
BSOA formation is affected by human activities, which are not well understood in polluted areas. In the polluted PRD region, we find that monoterpene SOA is aged, which probably results from high Ox and sulfate levels. NOx levels significantly affect isoprene SOA formation pathways. An unexpected increase of β-caryophyllene SOA in winter is also highly associated with enhanced biomass burning, Ox, and sulfate. Our results indicate that BSOA could be reduced by lowering anthropogenic emissions.
BSOA formation is affected by human activities, which are not well understood in polluted areas....
Altmetrics
Final-revised paper
Preprint