Articles | Volume 19, issue 19
https://doi.org/10.5194/acp-19-12797-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-12797-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Secondary organic aerosol formation from the laboratory oxidation of biomass burning emissions
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
now at: Department of Chemistry, University of Toronto, Toronto, ON,
Canada
David H. Hagan
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
Matthew M. Coggon
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Abigail R. Koss
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
now at: TOFWERK USA, Boulder, CO, USA
Kanako Sekimoto
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Graduate School of Nanobioscience, Yokohama City University, Yokohama,
Japan
Joost de Gouw
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Carsten Warneke
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Christopher D. Cappa
Department of Civil and Environmental Engineering, University of
California, Davis, CA, USA
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
Publisher's note: the Supplement was exchanged on 28 April 2023.
In the original version of the Supplement, the authors had mistakenly published primary organic aerosol (POA) values that were not corrected for AMS collection efficiency. The error is limited to Table S1 and Figure S9b in the Supplement and does not impact any other figures or conclusions in the paper. In the attached version of the Supplement, the authors have edited Table S1 and Figure S9b to use the properly corrected POA values.
In the original version of the Supplement, the authors had mistakenly published primary organic aerosol (POA) values that were not corrected for AMS collection efficiency. The error is limited to Table S1 and Figure S9b in the Supplement and does not impact any other figures or conclusions in the paper. In the attached version of the Supplement, the authors have edited Table S1 and Figure S9b to use the properly corrected POA values.
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Short summary
Wildfires are a large source of gases and particles to the atmosphere, both of which impact human health and climate. The amount and composition of particles from wildfires can change with time in the atmosphere; however, the impact of aging is not well understood. In a series of controlled laboratory experiments, we show that the particles are oxidized and a significant fraction of the gas-phase carbon (24 %–56 %) is converted to particle mass over the course of several days in the atmosphere.
Wildfires are a large source of gases and particles to the atmosphere, both of which impact...
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