Secondary organic aerosol formation from the laboratory oxidation of biomass burning emissions

Lim, Christopher Y.; Hagan, David H.; Coggon, Matthew M.; Koss, Abigail R.; Sekimoto, Kanako; de Gouw, Joost; Warneke, Carsten; Cappa, Christopher D.; Kroll, Jesse H.

doi:https://doi.org/10.5194/acp-19-12797-2019

Articles | Volume 19, issue 19

https://doi.org/10.5194/acp-19-12797-2019

© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

https://doi.org/10.5194/acp-19-12797-2019

© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

Articles | Volume 19, issue 19

Research article

|

14 Oct 2019

Research article |

| 14 Oct 2019

Secondary organic aerosol formation from the laboratory oxidation of biomass burning emissions

Christopher Y. Lim, David H. Hagan, Matthew M. Coggon, Abigail R. Koss, Kanako Sekimoto, Joost de Gouw, Carsten Warneke, Christopher D. Cappa, and Jesse H. Kroll

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Final revised paper (published on 14 Oct 2019)
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Preprint (discussion started on 09 Apr 2019)
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Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC1: 'Engaging paper, some thoughts', Anonymous Referee #1, 07 May 2019
RC2: 'Review of Lim et al. acd-2019-326', Anonymous Referee #2, 13 Jun 2019
AC1: 'Final author comments', Christopher Lim, 25 Jul 2019

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Christopher Lim on behalf of the Authors (26 Jul 2019) Author's response

ED: Referee Nomination & Report Request started (29 Jul 2019) by Ryan Sullivan

RR by Anonymous Referee #1 (16 Aug 2019)

ED: Publish subject to minor revisions (review by editor) (26 Aug 2019) by Ryan Sullivan

AR by Christopher Lim on behalf of the Authors (09 Sep 2019) Author's response Manuscript

ED: Publish as is (15 Sep 2019) by Ryan Sullivan

AR by Christopher Lim on behalf of the Authors (17 Sep 2019) Manuscript

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Short summary

Wildfires are a large source of gases and particles to the atmosphere, both of which impact human health and climate. The amount and composition of particles from wildfires can change with time in the atmosphere; however, the impact of aging is not well understood. In a series of controlled laboratory experiments, we show that the particles are oxidized and a significant fraction of the gas-phase carbon (24 %–56 %) is converted to particle mass over the course of several days in the atmosphere.