Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention, Department of Environmental Science & Engineering, Institute
of Atmospheric Sciences, Fudan University, Shanghai, 200433, China
Tao Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention, Department of Environmental Science & Engineering, Institute
of Atmospheric Sciences, Fudan University, Shanghai, 200433, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention, Department of Environmental Science & Engineering, Institute
of Atmospheric Sciences, Fudan University, Shanghai, 200433, China
Shanghai Institute of Pollution Control and Ecological Security,
Shanghai 200092, China
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology (CICAEET), Nanjing University of Information Science
and Technology, Nanjing 210044, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention, Department of Environmental Science & Engineering, Institute
of Atmospheric Sciences, Fudan University, Shanghai, 200433, China
State Key Laboratory of Organic Geochemistry and Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640,
China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention, Department of Environmental Science & Engineering, Institute
of Atmospheric Sciences, Fudan University, Shanghai, 200433, China
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This study confirmed that SO2 uptake on mineral particles could be greatly enhanced during cloud processing. The large pH fluctuations between the cloud-aerosol modes could significantly modify the microphysical properties of particles, and triggered the formation of reactive Fe particles to accelerate sulfate formation via a self-amplifying process. Results of this study could partly explain the missing source of sulfate and improve agreement between models and field observations.
This study confirmed that SO2 uptake on mineral particles could be greatly enhanced during cloud...
