Articles | Volume 19, issue 19
https://doi.org/10.5194/acp-19-12209-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-12209-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Oct 2019
Research article |
| 02 Oct 2019
| 02 Oct 2019
A large contribution of anthropogenic organo-nitrates to secondary organic aerosol in the Alberta oil sands
Alex K. Y. Lee
CORRESPONDING AUTHOR
Department of Civil and Environmental Engineering, National
University of Singapore, Singapore
NUS Environmental Research Institute, National University of
Singapore, Singapore
Max G. Adam
NUS Environmental Research Institute, National University of
Singapore, Singapore
John Liggio
Air Quality Process Research Section, Environment and Climate Change
Canada, Toronto, ON, Canada
Shao-Meng Li
Air Quality Process Research Section, Environment and Climate Change
Canada, Toronto, ON, Canada
Air Quality Process Research Section, Environment and Climate Change
Canada, Toronto, ON, Canada
Megan D. Willis
Department of Chemistry, University of Toronto, Toronto, ON, Canada
now at: Chemical Sciences
Division, Lawrence Berkeley National Lab, Berkeley, CA, USA
Jonathan P. D. Abbatt
Department of Chemistry, University of Toronto, Toronto, ON, Canada
Travis W. Tokarek
Department of Department of Chemistry, University of Calgary, Calgary, AB, Canada
Charles A. Odame-Ankrah
Department of Department of Chemistry, University of Calgary, Calgary, AB, Canada
Hans D. Osthoff
Department of Department of Chemistry, University of Calgary, Calgary, AB, Canada
Kevin Strawbridge
Air Quality Process Research Section, Environment and Climate Change
Canada, Toronto, ON, Canada
Jeffery R. Brook
Air Quality Process Research Section, Environment and Climate Change
Canada, Toronto, ON, Canada
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Cited
18 citations as recorded by crossref.
- Elemental analysis of oxygenated organic coating on black carbon particles using a soot-particle aerosol mass spectrometer M. Ma et al. 10.5194/amt-14-2799-2021
- Evidence for a kinetically controlled burying mechanism for growth of high viscosity secondary organic aerosol A. Vander Wall et al. 10.1039/C9EM00379G
- Size Distribution and Secondary Formation of Particulate Organic Nitrates in Winter in a Coastal Area A. Shakoor et al. 10.3390/su152416776
- Evidence of Nighttime Production of Organic Nitrates During SEAC4RS, FRAPPÉ, and KORUS‐AQ H. Kenagy et al. 10.1029/2020GL087860
- Unveiling the overlooked direct emissions of particulate organic nitrates from ship J. Chen et al. 10.1016/j.envint.2024.108487
- Estimation of particulate organic nitrates from thermodenuder–aerosol mass spectrometer measurements in the North China Plain W. Xu et al. 10.5194/amt-14-3693-2021
- Aerosols in current and future Arctic climate J. Schmale et al. 10.1038/s41558-020-00969-5
- Evaluating SOA formation from different sources of semi- and intermediate-volatility organic compounds from the Athabasca oil sands J. Sommers et al. 10.1039/D1EA00053E
- A decadal synthesis of atmospheric emissions, ambient air quality, and deposition in the oil sands region E. Horb et al. 10.1002/ieam.4539
- Contribution of Organic Nitrates to Organic Aerosol over South Korea during KORUS-AQ H. Kenagy et al. 10.1021/acs.est.1c05521
- Particulate organic nitrates at Mount Tai in winter and spring: Variation characteristics and effects of mountain-valley breezes and elevated emission sources J. Chen et al. 10.1016/j.envres.2022.113182
- Validation of MAX-DOAS retrievals of aerosol extinction, SO<sub>2</sub>, and NO<sub>2</sub> through comparison with lidar, sun photometer, active DOAS, and aircraft measurements in the Athabasca oil sands region Z. Davis et al. 10.5194/amt-13-1129-2020
- Effect of the “coal to gas” project on atmospheric NOX during the heating period at a suburban site between Beijing and Tianjin S. Zhao et al. 10.1016/j.atmosres.2020.104977
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Detecting and Characterizing Particulate Organic Nitrates with an Aerodyne Long-ToF Aerosol Mass Spectrometer F. Graeffe et al. 10.1021/acsearthspacechem.2c00314
- On the importance of atmospheric loss of organic nitrates by aqueous-phase ●OH oxidation J. González-Sánchez et al. 10.5194/acp-21-4915-2021
- Understanding the Impact of High-NOx Conditions on the Formation of Secondary Organic Aerosol in the Photooxidation of Oil Sand-Related Precursors K. Li et al. 10.1021/acs.est.9b05404
- Principal component analysis of summertime ground site measurements in the Athabasca oil sands with a focus on analytically unresolved intermediate-volatility organic compounds T. Tokarek et al. 10.5194/acp-18-17819-2018
17 citations as recorded by crossref.
- Elemental analysis of oxygenated organic coating on black carbon particles using a soot-particle aerosol mass spectrometer M. Ma et al. 10.5194/amt-14-2799-2021
- Evidence for a kinetically controlled burying mechanism for growth of high viscosity secondary organic aerosol A. Vander Wall et al. 10.1039/C9EM00379G
- Size Distribution and Secondary Formation of Particulate Organic Nitrates in Winter in a Coastal Area A. Shakoor et al. 10.3390/su152416776
- Evidence of Nighttime Production of Organic Nitrates During SEAC4RS, FRAPPÉ, and KORUS‐AQ H. Kenagy et al. 10.1029/2020GL087860
- Unveiling the overlooked direct emissions of particulate organic nitrates from ship J. Chen et al. 10.1016/j.envint.2024.108487
- Estimation of particulate organic nitrates from thermodenuder–aerosol mass spectrometer measurements in the North China Plain W. Xu et al. 10.5194/amt-14-3693-2021
- Aerosols in current and future Arctic climate J. Schmale et al. 10.1038/s41558-020-00969-5
- Evaluating SOA formation from different sources of semi- and intermediate-volatility organic compounds from the Athabasca oil sands J. Sommers et al. 10.1039/D1EA00053E
- A decadal synthesis of atmospheric emissions, ambient air quality, and deposition in the oil sands region E. Horb et al. 10.1002/ieam.4539
- Contribution of Organic Nitrates to Organic Aerosol over South Korea during KORUS-AQ H. Kenagy et al. 10.1021/acs.est.1c05521
- Particulate organic nitrates at Mount Tai in winter and spring: Variation characteristics and effects of mountain-valley breezes and elevated emission sources J. Chen et al. 10.1016/j.envres.2022.113182
- Validation of MAX-DOAS retrievals of aerosol extinction, SO<sub>2</sub>, and NO<sub>2</sub> through comparison with lidar, sun photometer, active DOAS, and aircraft measurements in the Athabasca oil sands region Z. Davis et al. 10.5194/amt-13-1129-2020
- Effect of the “coal to gas” project on atmospheric NOX during the heating period at a suburban site between Beijing and Tianjin S. Zhao et al. 10.1016/j.atmosres.2020.104977
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Detecting and Characterizing Particulate Organic Nitrates with an Aerodyne Long-ToF Aerosol Mass Spectrometer F. Graeffe et al. 10.1021/acsearthspacechem.2c00314
- On the importance of atmospheric loss of organic nitrates by aqueous-phase ●OH oxidation J. González-Sánchez et al. 10.5194/acp-21-4915-2021
- Understanding the Impact of High-NOx Conditions on the Formation of Secondary Organic Aerosol in the Photooxidation of Oil Sand-Related Precursors K. Li et al. 10.1021/acs.est.9b05404
Latest update: 22 Nov 2024
Short summary
This work provides the first direct field evidence that anthropogenic organo-nitrate contributed up to half of secondary organic aerosol (SOA) mass that was freshly produced within the emission plumes of oil sands facilities in Alberta, Canada. The findings illustrate the central role of organo-nitrate in SOA production from the oil and gas industry, with relevance for other urban and industrial regions with significant intermediate-volatility organic compounds (IVOCs) and NOx emissions.
This work provides the first direct field evidence that anthropogenic organo-nitrate contributed...
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