Articles | Volume 18, issue 8
https://doi.org/10.5194/acp-18-5391-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-5391-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Considering the future of anthropogenic gas-phase organic compound emissions and the increasing influence of non-combustion sources on urban air quality
Peeyush Khare
Department of Chemical and Environmental Engineering, Yale University, New Haven, CT 06511, USA
Drew R. Gentner
CORRESPONDING AUTHOR
Department of Chemical and Environmental Engineering, Yale University, New Haven, CT 06511, USA
SEARCH (Solutions for Energy, Air, Climate and Health) Center, Yale University, New Haven, CT 06511, USA
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Cited
73 citations as recorded by crossref.
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- Advances in offline approaches for trace measurements of complex organic compound mixtures via soft ionization and high-resolution tandem mass spectrometry P. Khare et al. 10.1016/j.chroma.2019.03.037
- Increasing Contributions of Temperature-Dependent Oxygenated Organic Aerosol to Summertime Particulate Matter in New York City T. Hass-Mitchell et al. 10.1021/acsestair.3c00037
- Outdoor air monitoring: Performance evaluation of a gas sensor to assess episodic nuisance/odorous events using active multi-sorbent bed tube sampling coupled to TD-GC/MS analysis E. Gallego et al. 10.1016/j.scitotenv.2019.133752
- Characterization of the organic functional group composition and sources of summertime aerosols in an eastern city of China K. Xia et al. 10.1016/j.atmosenv.2022.119078
- Highly Resolved Composition during Diesel Evaporation with Modeled Ozone and Secondary Aerosol Formation: Insights into Pollutant Formation from Evaporative Intermediate Volatility Organic Compound Sources G. Drozd et al. 10.1021/acs.est.0c08832
- Secondary organic aerosol production from local emissions dominates the organic aerosol budget over Seoul, South Korea, during KORUS-AQ B. Nault et al. 10.5194/acp-18-17769-2018
- Yields and molecular composition of gas-phase and secondary organic aerosol from the photooxidation of the volatile consumer product benzyl alcohol: formation of highly oxygenated and hydroxy nitro-aromatic compounds M. Jaoui et al. 10.5194/acp-23-4637-2023
- Cleaner Asphalt Production by Suppressing Emissions Using Phenolic Compounds F. Pahlavan et al. 10.1021/acssuschemeng.2c05345
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- Urban Oxidation Flow Reactor Measurements Reveal Significant Secondary Organic Aerosol Contributions from Volatile Emissions of Emerging Importance R. Shah et al. 10.1021/acs.est.9b06531
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- Full-volatility emission framework corrects missing and underestimated secondary organic aerosol sources X. Chang et al. 10.1016/j.oneear.2022.03.015
- Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels R. Miao et al. 10.5194/acp-21-16183-2021
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- Differentiated emissions and secondary organic aerosol formation potential of organic vapor from industrial coatings in China C. Liang et al. 10.1016/j.jhazmat.2024.133668
- Size-fractionated nonpolar organic compounds of traffic aerosol emissions in a highway tunnel X. Li et al. 10.1016/j.envpol.2021.118501
- Global Anthropogenic Emissions of Full-Volatility Organic Compounds L. Huang et al. 10.1021/acs.est.3c04106
- Analysis of reduced and oxidized nitrogen-containing organic compounds at a coastal site in summer and winter J. Ditto et al. 10.5194/acp-22-3045-2022
- Primary and Secondary Organic Aerosol Formation from Asphalt Pavements M. Humes et al. 10.1021/acs.est.3c06037
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- Watching Paint Dry: Organic Vapor Emissions from Architectural Coatings and their Impact on Secondary Organic Aerosol Formation R. Tanzer-Gruener et al. 10.1021/acs.est.2c02478
- A review of environmental emissions from asphalt plants and paving A. Mohammed & . Saleh 10.15406/mseij.2023.07.00205
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- Siloxane Emissions and Exposures during the Use of Hair Care Products in Buildings J. Jiang et al. 10.1021/acs.est.3c05156
- Using Hybrid PDI-Fe3O4 Nanoparticles for Capturing Aliphatic Alcohols: Halogen Bonding vs. Lone Pair–π Interactions M. Piña et al. 10.3390/ijms25126436
- 2002–2017 anthropogenic emissions data for air quality modeling over the United States K. Foley et al. 10.1016/j.dib.2023.109022
- Full-Volatility Reactive Organic Carbon Emissions from Volatile Chemical Products in Mainland China Y. Wang et al. 10.1021/acsestair.4c00116
- Roles of semivolatile and intermediate-volatility organic compounds in secondary organic aerosol formation and its implication: A review Z. Ling et al. 10.1016/j.jes.2021.08.055
- Rotational spectra of the low energy conformers observed in the (1R)-(−)-myrtenol monomer G. Sedo et al. 10.1016/j.jms.2018.12.005
- Two-year-long high-time-resolution apportionment of primary and secondary carbonaceous aerosols in the Los Angeles Basin using an advanced total carbon–black carbon (TC-BC(λ)) method M. Ivančič et al. 10.1016/j.scitotenv.2022.157606
- Policy-Related Gains in Urban Air Quality May Be Offset by Increased Emissions in a Warming Climate C. Cao et al. 10.1021/acs.est.2c05904
- Behaviour of traffic emitted semi-volatile and intermediate volatility organic compounds within the urban atmosphere R. Xu et al. 10.1016/j.scitotenv.2020.137470
- Towards Solar-Driven Formation of Robust and Self-Healable Waterborne Polyurethane Containing Disulfide Bonds via in-situ Incorporation of 2D Titanium Carbide MXene S. Gong et al. 10.32604/jrm.2022.023011
- Human transport of thirdhand tobacco smoke: A prominent source of hazardous air pollutants into indoor nonsmoking environments R. Sheu et al. 10.1126/sciadv.aay4109
- A novel method for spatial allocation of volatile chemical products emissions: A case study of the Pearl River Delta Z. Cai et al. 10.1016/j.atmosenv.2023.120119
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- Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds Q. Lu et al. 10.5194/acp-20-4313-2020
- Evidence for impacts on surface-level air quality in the northeastern US from long-distance transport of smoke from North American fires during the Long Island Sound Tropospheric Ozone Study (LISTOS) 2018 H. Rogers et al. 10.5194/acp-20-671-2020
- Modeled Emission of Hydroxyl and Ozone Reactivity from Evaporation of Fragrance Mixtures J. Hurley et al. 10.1021/acs.est.1c04004
- Limited Secondary Organic Aerosol Production from Acyclic Oxygenated Volatile Chemical Products M. Humes et al. 10.1021/acs.est.1c07354
- Atmospheric Pollutant Profile of a Road Asphalt Application: Highly Socioeconomic Development-Related Emission D. Wang et al. 10.1021/acs.estlett.3c00011
- Reactive organic carbon emissions from volatile chemical products K. Seltzer et al. 10.5194/acp-21-5079-2021
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- An updated comprehensive anthropogenic S/IVOCs emission inventory in Central China: Spatial and Temporal characteristics S. Wang et al. 10.1016/j.atmosres.2022.106546
- Environmentally persistent free radicals in indoor particulate matter, dust, and on surfaces A. Filippi et al. 10.1039/D1EA00075F
- Evaluating Indoor Air Chemical Diversity, Indoor-to-Outdoor Emissions, and Surface Reservoirs Using High-Resolution Mass Spectrometry R. Sheu et al. 10.1021/acs.est.1c01337
- Modeling secondary organic aerosol formation from volatile chemical products E. Pennington et al. 10.5194/acp-21-18247-2021
- Anthropogenic secondary organic aerosol and ozone production from asphalt-related emissions K. Seltzer et al. 10.1039/D3EA00066D
- Chlorine-initiated oxidation of <i>n</i>-alkanes under high-NO<sub><i>x</i></sub> conditions: insights into secondary organic aerosol composition and volatility using a FIGAERO–CIMS D. Wang & L. Hildebrandt Ruiz 10.5194/acp-18-15535-2018
- Composition and emission factors of traffic- emitted intermediate volatility and semi-volatile hydrocarbons (C10–C36) at a street canyon and urban background sites in central London, UK R. Xu et al. 10.1016/j.atmosenv.2020.117448
- Volatile Organic Compound Composition and Emissions in a Residential Attic B. Molinier et al. 10.1021/acsestair.4c00040
- Inherently Functionalized Carbon from Algae to Adsorb Precursors of Secondary Organic Aerosols in Noncombustion Sources M. Mousavi et al. 10.1021/acssuschemeng.1c03827
- Measurements of higher alkanes using NO<sup>+</sup> chemical ionization in PTR-ToF-MS: important contributions of higher alkanes to secondary organic aerosols in China C. Wang et al. 10.5194/acp-20-14123-2020
- Atmospheric Photo-Oxidation of 2-Ethoxyethanol: Autoxidation Chemistry of Glycol Ethers H. Yu et al. 10.1021/acs.jpca.3c04456
- Gas-Phase Chlorine Radical Oxidation of Alkanes: Effects of Structural Branching, NOx, and Relative Humidity Observed during Environmental Chamber Experiments L. Jahn et al. 10.1021/acs.jpca.1c03516
- Emission inventory of semi-volatile and intermediate-volatility organic compounds and their effects on secondary organic aerosol over the Pearl River Delta region L. Wu et al. 10.5194/acp-19-8141-2019
- Intermediate-volatility aromatic hydrocarbons from the rubber products industry in China Z. Zhang et al. 10.1016/j.scitotenv.2023.165583
- Volatile organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications C. Stockwell et al. 10.5194/acp-21-6005-2021
- Atmospheric oxidation mechanism and kinetics of indole initiated by ●OH and ●Cl: a computational study J. Xue et al. 10.5194/acp-22-11543-2022
- Oxidized and Unsaturated: Key Organic Aerosol Traits Associated with Cellular Reactive Oxygen Species Production in the Southeastern United States F. Liu et al. 10.1021/acs.est.3c03641
- Asphalt-related emissions are a major missing nontraditional source of secondary organic aerosol precursors P. Khare et al. 10.1126/sciadv.abb9785
73 citations as recorded by crossref.
- VOC emissions by fresh and old asphalt pavements at service temperatures: impacts on urban air quality J. Lasne et al. 10.1039/D3EA00034F
- An updated modeling framework to simulate Los Angeles air quality – Part 1: Model development, evaluation, and source apportionment E. Pennington et al. 10.5194/acp-24-2345-2024
- Preventing emissions of hazardous organic compounds from bituminous composites M. Mousavi & E. Fini 10.1016/j.jclepro.2022.131067
- The effects of photochemical aging and interactions with secondary organic aerosols on cellular toxicity of combustion particles R. Attah et al. 10.1016/j.jaerosci.2024.106473
- A mass-balance-based emission inventory of non-methane volatile organic compounds (NMVOCs) for solvent use in China Z. Mo et al. 10.5194/acp-21-13655-2021
- Advances in offline approaches for trace measurements of complex organic compound mixtures via soft ionization and high-resolution tandem mass spectrometry P. Khare et al. 10.1016/j.chroma.2019.03.037
- Increasing Contributions of Temperature-Dependent Oxygenated Organic Aerosol to Summertime Particulate Matter in New York City T. Hass-Mitchell et al. 10.1021/acsestair.3c00037
- Outdoor air monitoring: Performance evaluation of a gas sensor to assess episodic nuisance/odorous events using active multi-sorbent bed tube sampling coupled to TD-GC/MS analysis E. Gallego et al. 10.1016/j.scitotenv.2019.133752
- Characterization of the organic functional group composition and sources of summertime aerosols in an eastern city of China K. Xia et al. 10.1016/j.atmosenv.2022.119078
- Highly Resolved Composition during Diesel Evaporation with Modeled Ozone and Secondary Aerosol Formation: Insights into Pollutant Formation from Evaporative Intermediate Volatility Organic Compound Sources G. Drozd et al. 10.1021/acs.est.0c08832
- Secondary organic aerosol production from local emissions dominates the organic aerosol budget over Seoul, South Korea, during KORUS-AQ B. Nault et al. 10.5194/acp-18-17769-2018
- Yields and molecular composition of gas-phase and secondary organic aerosol from the photooxidation of the volatile consumer product benzyl alcohol: formation of highly oxygenated and hydroxy nitro-aromatic compounds M. Jaoui et al. 10.5194/acp-23-4637-2023
- Cleaner Asphalt Production by Suppressing Emissions Using Phenolic Compounds F. Pahlavan et al. 10.1021/acssuschemeng.2c05345
- Distribution and sources of SVOCs in fine and coarse aerosols in the megacity of Istanbul R. Flores et al. 10.1016/j.atmosres.2022.106100
- Urban Oxidation Flow Reactor Measurements Reveal Significant Secondary Organic Aerosol Contributions from Volatile Emissions of Emerging Importance R. Shah et al. 10.1021/acs.est.9b06531
- Differences in Perception of the Environmental and Health Impacts of Decorative Paints among Average Consumers M. Hess & J. Bongaerts 10.3390/su12114495
- Full-volatility emission framework corrects missing and underestimated secondary organic aerosol sources X. Chang et al. 10.1016/j.oneear.2022.03.015
- Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels R. Miao et al. 10.5194/acp-21-16183-2021
- Representing Ozone Formation from Volatile Chemical Products (VCP) in Carbon Bond (CB) Chemical Mechanisms G. Yarwood & K. Tuite 10.3390/atmos15020178
- Indoor Air Sources of Outdoor Air Pollution: Health Consequences, Policy, and Recommendations: An Official American Thoracic Society Workshop Report N. Nassikas et al. 10.1513/AnnalsATS.202312-1067ST
- Volatile Chemical Product Enhancements to Criteria Pollutants in the United States K. Seltzer et al. 10.1021/acs.est.1c04298
- Differentiated emissions and secondary organic aerosol formation potential of organic vapor from industrial coatings in China C. Liang et al. 10.1016/j.jhazmat.2024.133668
- Size-fractionated nonpolar organic compounds of traffic aerosol emissions in a highway tunnel X. Li et al. 10.1016/j.envpol.2021.118501
- Global Anthropogenic Emissions of Full-Volatility Organic Compounds L. Huang et al. 10.1021/acs.est.3c04106
- Analysis of reduced and oxidized nitrogen-containing organic compounds at a coastal site in summer and winter J. Ditto et al. 10.5194/acp-22-3045-2022
- Primary and Secondary Organic Aerosol Formation from Asphalt Pavements M. Humes et al. 10.1021/acs.est.3c06037
- Secondary organic aerosols from anthropogenic volatile organic compounds contribute substantially to air pollution mortality B. Nault et al. 10.5194/acp-21-11201-2021
- Watching Paint Dry: Organic Vapor Emissions from Architectural Coatings and their Impact on Secondary Organic Aerosol Formation R. Tanzer-Gruener et al. 10.1021/acs.est.2c02478
- A review of environmental emissions from asphalt plants and paving A. Mohammed & . Saleh 10.15406/mseij.2023.07.00205
- In the Footsteps of My Countrymen: Atmospheric Chemistry in New England, Los Angeles, and the Southeast United States J. de Gouw 10.1029/2021CN000151
- Ammonium adduct chemical ionization to investigate anthropogenic oxygenated gas-phase organic compounds in urban air P. Khare et al. 10.5194/acp-22-14377-2022
- Siloxane Emissions and Exposures during the Use of Hair Care Products in Buildings J. Jiang et al. 10.1021/acs.est.3c05156
- Using Hybrid PDI-Fe3O4 Nanoparticles for Capturing Aliphatic Alcohols: Halogen Bonding vs. Lone Pair–π Interactions M. Piña et al. 10.3390/ijms25126436
- 2002–2017 anthropogenic emissions data for air quality modeling over the United States K. Foley et al. 10.1016/j.dib.2023.109022
- Full-Volatility Reactive Organic Carbon Emissions from Volatile Chemical Products in Mainland China Y. Wang et al. 10.1021/acsestair.4c00116
- Roles of semivolatile and intermediate-volatility organic compounds in secondary organic aerosol formation and its implication: A review Z. Ling et al. 10.1016/j.jes.2021.08.055
- Rotational spectra of the low energy conformers observed in the (1R)-(−)-myrtenol monomer G. Sedo et al. 10.1016/j.jms.2018.12.005
- Two-year-long high-time-resolution apportionment of primary and secondary carbonaceous aerosols in the Los Angeles Basin using an advanced total carbon–black carbon (TC-BC(λ)) method M. Ivančič et al. 10.1016/j.scitotenv.2022.157606
- Policy-Related Gains in Urban Air Quality May Be Offset by Increased Emissions in a Warming Climate C. Cao et al. 10.1021/acs.est.2c05904
- Behaviour of traffic emitted semi-volatile and intermediate volatility organic compounds within the urban atmosphere R. Xu et al. 10.1016/j.scitotenv.2020.137470
- Towards Solar-Driven Formation of Robust and Self-Healable Waterborne Polyurethane Containing Disulfide Bonds via in-situ Incorporation of 2D Titanium Carbide MXene S. Gong et al. 10.32604/jrm.2022.023011
- Human transport of thirdhand tobacco smoke: A prominent source of hazardous air pollutants into indoor nonsmoking environments R. Sheu et al. 10.1126/sciadv.aay4109
- A novel method for spatial allocation of volatile chemical products emissions: A case study of the Pearl River Delta Z. Cai et al. 10.1016/j.atmosenv.2023.120119
- Effects of Molecular-Level Compositional Variability in Organic Aerosol on Phase State and Thermodynamic Mixing Behavior J. Ditto et al. 10.1021/acs.est.9b02664
- Emission characteristics of reactive organic gases (ROGs) from industrial volatile chemical products (VCPs) in the Pearl River Delta (PRD), China S. Wang et al. 10.5194/acp-24-7101-2024
- Impact of Solvent Emissions on Reactive Aromatics and Ozone in the Great Lakes Region C. Stroud et al. 10.3390/atmos14071094
- Investigation of Anthropogenic Monoterpenes in Canadian Cities O. Jo et al. 10.1021/acsearthspacechem.3c00181
- Impact of OA on the Temperature Dependence of PM 2.5 in the Los Angeles Basin C. Nussbaumer & R. Cohen 10.1021/acs.est.0c07144
- Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds Q. Lu et al. 10.5194/acp-20-4313-2020
- Evidence for impacts on surface-level air quality in the northeastern US from long-distance transport of smoke from North American fires during the Long Island Sound Tropospheric Ozone Study (LISTOS) 2018 H. Rogers et al. 10.5194/acp-20-671-2020
- Modeled Emission of Hydroxyl and Ozone Reactivity from Evaporation of Fragrance Mixtures J. Hurley et al. 10.1021/acs.est.1c04004
- Limited Secondary Organic Aerosol Production from Acyclic Oxygenated Volatile Chemical Products M. Humes et al. 10.1021/acs.est.1c07354
- Atmospheric Pollutant Profile of a Road Asphalt Application: Highly Socioeconomic Development-Related Emission D. Wang et al. 10.1021/acs.estlett.3c00011
- Reactive organic carbon emissions from volatile chemical products K. Seltzer et al. 10.5194/acp-21-5079-2021
- Impact of improved representation of volatile organic compound emissions and production of NOx reservoirs on modeled urban ozone production K. Travis et al. 10.5194/acp-24-9555-2024
- An updated comprehensive anthropogenic S/IVOCs emission inventory in Central China: Spatial and Temporal characteristics S. Wang et al. 10.1016/j.atmosres.2022.106546
- Environmentally persistent free radicals in indoor particulate matter, dust, and on surfaces A. Filippi et al. 10.1039/D1EA00075F
- Evaluating Indoor Air Chemical Diversity, Indoor-to-Outdoor Emissions, and Surface Reservoirs Using High-Resolution Mass Spectrometry R. Sheu et al. 10.1021/acs.est.1c01337
- Modeling secondary organic aerosol formation from volatile chemical products E. Pennington et al. 10.5194/acp-21-18247-2021
- Anthropogenic secondary organic aerosol and ozone production from asphalt-related emissions K. Seltzer et al. 10.1039/D3EA00066D
- Chlorine-initiated oxidation of <i>n</i>-alkanes under high-NO<sub><i>x</i></sub> conditions: insights into secondary organic aerosol composition and volatility using a FIGAERO–CIMS D. Wang & L. Hildebrandt Ruiz 10.5194/acp-18-15535-2018
- Composition and emission factors of traffic- emitted intermediate volatility and semi-volatile hydrocarbons (C10–C36) at a street canyon and urban background sites in central London, UK R. Xu et al. 10.1016/j.atmosenv.2020.117448
- Volatile Organic Compound Composition and Emissions in a Residential Attic B. Molinier et al. 10.1021/acsestair.4c00040
- Inherently Functionalized Carbon from Algae to Adsorb Precursors of Secondary Organic Aerosols in Noncombustion Sources M. Mousavi et al. 10.1021/acssuschemeng.1c03827
- Measurements of higher alkanes using NO<sup>+</sup> chemical ionization in PTR-ToF-MS: important contributions of higher alkanes to secondary organic aerosols in China C. Wang et al. 10.5194/acp-20-14123-2020
- Atmospheric Photo-Oxidation of 2-Ethoxyethanol: Autoxidation Chemistry of Glycol Ethers H. Yu et al. 10.1021/acs.jpca.3c04456
- Gas-Phase Chlorine Radical Oxidation of Alkanes: Effects of Structural Branching, NOx, and Relative Humidity Observed during Environmental Chamber Experiments L. Jahn et al. 10.1021/acs.jpca.1c03516
- Emission inventory of semi-volatile and intermediate-volatility organic compounds and their effects on secondary organic aerosol over the Pearl River Delta region L. Wu et al. 10.5194/acp-19-8141-2019
- Intermediate-volatility aromatic hydrocarbons from the rubber products industry in China Z. Zhang et al. 10.1016/j.scitotenv.2023.165583
- Volatile organic compound emissions from solvent- and water-borne coatings – compositional differences and tracer compound identifications C. Stockwell et al. 10.5194/acp-21-6005-2021
- Atmospheric oxidation mechanism and kinetics of indole initiated by ●OH and ●Cl: a computational study J. Xue et al. 10.5194/acp-22-11543-2022
- Oxidized and Unsaturated: Key Organic Aerosol Traits Associated with Cellular Reactive Oxygen Species Production in the Southeastern United States F. Liu et al. 10.1021/acs.est.3c03641
- Asphalt-related emissions are a major missing nontraditional source of secondary organic aerosol precursors P. Khare et al. 10.1126/sciadv.abb9785
Discussed (final revised paper)
Latest update: 12 Dec 2024
Short summary
Following decades of successful regulatory policies focused on combustion-related sources (e.g. motor vehicles), emissions from non-combustion sources have become increasingly important for urban air quality. Using multiple approaches, we demonstrate that emissions from consumer, commercial, and industrial products and materials have become prominent contributors to the formation of photochemical smog (i.e. secondary organic particulate matter and ozone) and its associated health effects.
Following decades of successful regulatory policies focused on combustion-related sources (e.g....
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