Articles | Volume 18, issue 4
https://doi.org/10.5194/acp-18-2363-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-2363-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Feb 2018
Research article |
| 19 Feb 2018
| 19 Feb 2018
Measurement–model comparison of stabilized Criegee intermediate and highly oxygenated molecule production in the CLOUD chamber
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Tuija Jokinen
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Jonathan Duplissy
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Tuomo Nieminen
University of Eastern Finland, Department of Applied Physics, P.O. Box 1627, 70211 Kuopio, Finland
Mikael Ehn
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Siegfried Schobesberger
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
University of Eastern Finland, Department of Applied Physics, P.O. Box 1627, 70211 Kuopio, Finland
Department of Atmospheric Sciences, University of Washington, 408 ATG Bldg, Box 351640, Seattle, WA 98195, USA
Martin Heinritzi
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
Sebastian Ehrhart
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
now at: Max-Planck Institute of Chemistry, Atmospheric Chemistry Department,
Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Katrianne Lehtipalo
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland
Jasmin Tröstl
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland
Mario Simon
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
Andreas Kürten
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
Markus Leiminger
University of Innsbruck, Institute for Ion Physics and Applied Physics, Technikerstraße 25, 6020 Innsbruck, Austria
Michael J. Lawler
University of California, Irvine, Department of Chemistry, Irvine, CA 92697, USA
Matti P. Rissanen
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Federico Bianchi
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Arnaud P. Praplan
Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
Jani Hakala
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Antonio Amorim
CENTRA, Faculdade de Ciencias da Universidade de Lisboa, Lisbon, Portugal
Marc Gonin
Tofwerk AG, 3600 Thun, Switzerland
Armin Hansel
University of Innsbruck, Institute for Ion Physics and Applied Physics, Technikerstraße 25, 6020 Innsbruck, Austria
Jasper Kirkby
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
CERN, 1211 Geneva, Switzerland
Josef Dommen
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland
Joachim Curtius
Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhöferallee 1, 60438 Frankfurt am Main, Germany
James N. Smith
University of California, Irvine, Department of Chemistry, Irvine, CA 92697, USA
Tuukka Petäjä
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Douglas R. Worsnop
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Aerodyne Research, Inc., Billerica, MA 01821, USA
Markku Kulmala
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Neil M. Donahue
Carnegie Mellon University Center for Atmospheric Particle Studies, 5000 Forbes Ave, Pittsburgh, PA 15213, USA
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Mikko Sipilä
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
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- Final revised paper (published on 19 Feb 2018)
- Preprint (discussion started on 13 Sep 2017)
Interactive discussion
Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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- Supplement
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RC1: 'Review', Anonymous Referee #2, 15 Oct 2017
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RC2: 'Review of ‘Measurement-model comparison of stabilized Criegee Intermediate and Highly Oxygenated Molecule production in the CLOUD chamber’ by N. Sarnela et al., Atmos. Chem. Phys. Discuss., doi.org/10.5194/acp-2017-780', Anonymous Referee #1, 26 Oct 2017
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AC1: 'The response to the Referees by Nina Sarnela', Nina Sarnela, 19 Dec 2017
Peer-review completion
AR: Author's response | RR: Referee report | ED: Editor decision
AR by Nina Sarnela on behalf of the Authors (21 Dec 2017)
Author's response
Manuscript
ED: Publish subject to minor revisions (review by editor) (02 Jan 2018) by Frank Keutsch
AR by Nina Sarnela on behalf of the Authors (08 Jan 2018)
Author's response
Manuscript
ED: Publish as is (09 Jan 2018) by Frank Keutsch
AR by Nina Sarnela on behalf of the Authors (11 Jan 2018)
Short summary
Atmospheric trace gases can form small molecular clusters, which can grow to larger sizes through the condensation of vapours. This process is called new particle formation. In this paper we studied the formation of sulfuric acid and highly oxygenated molecules, the key compounds in atmospheric new particle formation, in chamber experiments and introduced a way to simulate these ozonolysis products of α-pinene in a simple manner.
Atmospheric trace gases can form small molecular clusters, which can grow to larger sizes...
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