Articles | Volume 18, issue 3
Atmos. Chem. Phys., 18, 2225–2242, 2018
https://doi.org/10.5194/acp-18-2225-2018
Atmos. Chem. Phys., 18, 2225–2242, 2018
https://doi.org/10.5194/acp-18-2225-2018
Research article
15 Feb 2018
Research article | 15 Feb 2018

Modeling the partitioning of organic chemical species in cloud phases with CLEPS (1.1)

Clémence Rose et al.

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Short summary
A detailed aqueous phase mechanism CLEPS 1.1 is coupled with warm microphysics including activation of aerosol particles into cloud droplets. Simulated aqueous concentrations of carboxylic acids are close to the long-term measurements conducted at Puy de Dôme (France). Sensitivity tests show that formic and acetic acids mainly originate from the gas phase with highly variable aqueous-phase reactivity depending on cloud pH, while C3–C4 carboxylic acids mainly originate from the particulate phase.
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