Articles | Volume 18, issue 3
https://doi.org/10.5194/acp-18-2225-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-2225-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Feb 2018
Research article |
| 15 Feb 2018
| 15 Feb 2018
Modeling the partitioning of organic chemical species in cloud phases with CLEPS (1.1)
Clémence Rose
Université Clermont Auvergne, CNRS Laboratoire de
Météorologie Physique, 63000 Clermont-Ferrand, France
Nadine Chaumerliac
CORRESPONDING AUTHOR
Université Clermont Auvergne, CNRS Laboratoire de
Météorologie Physique, 63000 Clermont-Ferrand, France
Laurent Deguillaume
CORRESPONDING AUTHOR
Université Clermont Auvergne, CNRS Laboratoire de
Météorologie Physique, 63000 Clermont-Ferrand, France
Hélène Perroux
Université Clermont Auvergne, CNRS Laboratoire de
Météorologie Physique, 63000 Clermont-Ferrand, France
Camille Mouchel-Vallon
Université Clermont Auvergne, CNRS Laboratoire de
Météorologie Physique, 63000 Clermont-Ferrand, France
now at: National Center for Atmospheric Research, Boulder, Colorado,
USA
Maud Leriche
Université de Toulouse, UPS, CNRS, Laboratoire d'Aérologie,
31400 Toulouse, France
Luc Patryl
CEA, DAM, DIF, 91297 Arpajon, France
Patrick Armand
CEA, DAM, DIF, 91297 Arpajon, France
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Cited
15 citations as recorded by crossref.
- Influence of strong iron-binding ligands on cloud water oxidant capacity A. González et al. https://doi.org/10.1016/j.scitotenv.2022.154642
- Treatment of non-ideality in the SPACCIM multiphase model – Part 2: Impacts on the multiphase chemical processing in deliquesced aerosol particles A. Rusumdar et al. https://doi.org/10.5194/acp-20-10351-2020
- Investigating the evolution of water-soluble organic carbon in evaporating cloud water V. Pratap et al. https://doi.org/10.1039/D0EA00005A
- Analysis of Volatile Organic Compounds during the OCTAVE Campaign: Sources and Distributions of Formaldehyde on Reunion Island M. Rocco et al. https://doi.org/10.3390/atmos11020140
- Assessing the efficiency of water-soluble organic compound biodegradation in clouds under various environmental conditions L. Pailler et al. https://doi.org/10.1039/D2EA00153E
- Sources and characteristics of size-resolved particulate organic acids and methanesulfonate in a coastal megacity: Manila, Philippines C. Stahl et al. https://doi.org/10.5194/acp-20-15907-2020
- Atmospherically Relevant Chemistry and Aerosol box model – ARCA box (version 1.2) P. Clusius et al. https://doi.org/10.5194/gmd-15-7257-2022
- Cézeaux-Aulnat-Opme-Puy De Dôme: a multi-site for the long-term survey of the tropospheric composition and climate change J. Baray et al. https://doi.org/10.5194/amt-13-3413-2020
- Predicting reaction rate constants of organic compounds with oxidants in the atmospheric aqueous-phase through multi-task learning L. Gu & Z. Chen https://doi.org/10.1016/j.atmosenv.2024.120775
- Measurement report: Bio-physicochemistry of tropical clouds at Maïdo (Réunion, Indian Ocean): overview of results from the BIO-MAÏDO campaign M. Leriche et al. https://doi.org/10.5194/acp-24-4129-2024
- Classification of Clouds Sampled at the Puy de Dôme Station (France) Based on Chemical Measurements and Air Mass History Matrices P. Renard et al. https://doi.org/10.3390/atmos11070732
- Insights into tropical cloud chemistry in Réunion (Indian Ocean): results from the BIO-MAÏDO campaign P. Dominutti et al. https://doi.org/10.5194/acp-22-505-2022
- Anthropogenic and biogenic hydrophobic VOCs detected in clouds at the puy de Dôme station using Stir Bar Sorptive Extraction: Deviation from the Henry's law prediction M. Wang et al. https://doi.org/10.1016/j.atmosres.2020.104844
- Box Model Intercomparison of Cloud Chemistry M. Barth et al. https://doi.org/10.1029/2021JD035486
- Investigating the role of anthropogenic terpenoids in urban secondary pollution under summer conditions by a box modeling approach M. Farhat et al. https://doi.org/10.1039/D4EA00112E
15 citations as recorded by crossref.
- Influence of strong iron-binding ligands on cloud water oxidant capacity A. González et al. https://doi.org/10.1016/j.scitotenv.2022.154642
- Treatment of non-ideality in the SPACCIM multiphase model – Part 2: Impacts on the multiphase chemical processing in deliquesced aerosol particles A. Rusumdar et al. https://doi.org/10.5194/acp-20-10351-2020
- Investigating the evolution of water-soluble organic carbon in evaporating cloud water V. Pratap et al. https://doi.org/10.1039/D0EA00005A
- Analysis of Volatile Organic Compounds during the OCTAVE Campaign: Sources and Distributions of Formaldehyde on Reunion Island M. Rocco et al. https://doi.org/10.3390/atmos11020140
- Assessing the efficiency of water-soluble organic compound biodegradation in clouds under various environmental conditions L. Pailler et al. https://doi.org/10.1039/D2EA00153E
- Sources and characteristics of size-resolved particulate organic acids and methanesulfonate in a coastal megacity: Manila, Philippines C. Stahl et al. https://doi.org/10.5194/acp-20-15907-2020
- Atmospherically Relevant Chemistry and Aerosol box model – ARCA box (version 1.2) P. Clusius et al. https://doi.org/10.5194/gmd-15-7257-2022
- Cézeaux-Aulnat-Opme-Puy De Dôme: a multi-site for the long-term survey of the tropospheric composition and climate change J. Baray et al. https://doi.org/10.5194/amt-13-3413-2020
- Predicting reaction rate constants of organic compounds with oxidants in the atmospheric aqueous-phase through multi-task learning L. Gu & Z. Chen https://doi.org/10.1016/j.atmosenv.2024.120775
- Measurement report: Bio-physicochemistry of tropical clouds at Maïdo (Réunion, Indian Ocean): overview of results from the BIO-MAÏDO campaign M. Leriche et al. https://doi.org/10.5194/acp-24-4129-2024
- Classification of Clouds Sampled at the Puy de Dôme Station (France) Based on Chemical Measurements and Air Mass History Matrices P. Renard et al. https://doi.org/10.3390/atmos11070732
- Insights into tropical cloud chemistry in Réunion (Indian Ocean): results from the BIO-MAÏDO campaign P. Dominutti et al. https://doi.org/10.5194/acp-22-505-2022
- Anthropogenic and biogenic hydrophobic VOCs detected in clouds at the puy de Dôme station using Stir Bar Sorptive Extraction: Deviation from the Henry's law prediction M. Wang et al. https://doi.org/10.1016/j.atmosres.2020.104844
- Box Model Intercomparison of Cloud Chemistry M. Barth et al. https://doi.org/10.1029/2021JD035486
- Investigating the role of anthropogenic terpenoids in urban secondary pollution under summer conditions by a box modeling approach M. Farhat et al. https://doi.org/10.1039/D4EA00112E
Saved (final revised paper)
Latest update: 14 Oct 2026
Short summary
A detailed aqueous phase mechanism CLEPS 1.1 is coupled with warm microphysics including activation of aerosol particles into cloud droplets. Simulated aqueous concentrations of carboxylic acids are close to the long-term measurements conducted at Puy de Dôme (France). Sensitivity tests show that formic and acetic acids mainly originate from the gas phase with highly variable aqueous-phase reactivity depending on cloud pH, while C3–C4 carboxylic acids mainly originate from the particulate phase.
A detailed aqueous phase mechanism CLEPS 1.1 is coupled with warm microphysics including...
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