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ACP | Articles | Volume 18, issue 20
Atmos. Chem. Phys., 18, 14787–14798, 2018
https://doi.org/10.5194/acp-18-14787-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 18, 14787–14798, 2018
https://doi.org/10.5194/acp-18-14787-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 15 Oct 2018

Research article | 15 Oct 2018

Surface fluxes of bromoform and dibromomethane over the tropical western Pacific inferred from airborne in situ measurements

Liang Feng et al.

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Co-ordinated Airborne Studies in the Tropics (CAST) P. Braesicke, N. Harris, J. A. Pyle, A. Robinson, and G. Vaughan http://catalogue.ceda.ac.uk/uuid/565b6bb5a0535b438ad2fae4c852e1b3

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We infer surface fluxes of bromoform (CHBr3) and dibromoform (CH2Br2) from CAST and CONTRAST aircraft observations over the western Pacific, using a tagged version of the GEOS-Chem global 3-D atmospheric chemistry model and a Maximum A Posteriori inverse model. Using the aircraft data, we estimate the regional fluxes about 20–40 % smaller than the prior inventories by Ordóñez et al. (2012). We find no evidence to support a robust linear relationship between CHBr3 and CH2Br2 oceanic emissions.
We infer surface fluxes of bromoform (CHBr3) and dibromoform (CH2Br2) from CAST and CONTRAST...
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