Articles | Volume 18, issue 19
Atmos. Chem. Phys., 18, 14539–14553, 2018
Atmos. Chem. Phys., 18, 14539–14553, 2018

Research article 11 Oct 2018

Research article | 11 Oct 2018

Heterogeneous OH oxidation of secondary brown carbon aerosol

Elijah G. Schnitzler and Jonathan P. D. Abbatt


Interactive discussion

Status: closed
Status: closed
AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision
AR by Elijah Schnitzler on behalf of the Authors (17 Jul 2018)  Author's response    Manuscript
ED: Publish as is (08 Sep 2018) by Rainer Volkamer
Short summary
Brown carbon (BrC) has significant but poorly constrained effects on climate. In this work, we investigate the effects of the OH radical on optical properties of secondary BrC in a series of smog chamber experiments. At high relative humidity (RH), we find that the evolution of the particles is complex, exhibiting rapid absorption enhancement followed by slow bleaching. At low RH, bleaching does not occur. These results further our understanding of the highly variable evolution of ambient BrC.
Final-revised paper