Articles | Volume 18, issue 18
https://doi.org/10.5194/acp-18-13429-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-13429-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Composition and mixing state of atmospheric aerosols determined by electron microscopy: method development and application to aged Saharan dust deposition in the Caribbean boundary layer
Konrad Kandler
CORRESPONDING AUTHOR
Institute for Applied Geosciences, Technical University Darmstadt,
64287 Darmstadt, Germany
Kilian Schneiders
Institute for Applied Geosciences, Technical University Darmstadt,
64287 Darmstadt, Germany
Martin Ebert
Institute for Applied Geosciences, Technical University Darmstadt,
64287 Darmstadt, Germany
Markus Hartmann
Institute for Applied Geosciences, Technical University Darmstadt,
64287 Darmstadt, Germany
now at: Experimental Aerosol and Cloud Microphysics Department, Tropos
Leibniz-Institute für Tropospheric Research (TROPOS), 04318 Leipzig,
Germany
Stephan Weinbruch
Institute for Applied Geosciences, Technical University Darmstadt,
64287 Darmstadt, Germany
Maria Prass
Max Planck Institute for Chemistry, Multiphase Chemistry Department,
55128 Mainz, Germany
Christopher Pöhlker
Max Planck Institute for Chemistry, Multiphase Chemistry Department,
55128 Mainz, Germany
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Cited
36 citations as recorded by crossref.
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- Particle Size Distribution of Various Soil Materials Measured by Laser Diffraction—The Problem of Reproducibility C. Polakowski et al. 10.3390/min11050465
- Analysis of Size Distribution, Chemical Composition, and Optical Properties of Mineral Dust Particles from Dry Deposition Measurement in Tenerife: Determined by Single-Particle Characterization A. Waza et al. 10.3390/atmos14040700
- Field comparison of dry deposition samplers for collection of atmospheric mineral dust: results from single-particle characterization A. Waza et al. 10.5194/amt-12-6647-2019
- Trans‐Regional Transport of Haze Particles From the North China Plain to Yangtze River Delta During Winter J. Zhang et al. 10.1029/2020JD033778
- Complex Aerosol Characterization by Scanning Electron Microscopy Coupled with Energy Dispersive X-ray Spectroscopy A. Brostrøm et al. 10.1038/s41598-020-65383-5
- Impact of various air mass types on cloud condensation nuclei concentrations along coastal southeast Florida E. Edwards et al. 10.1016/j.atmosenv.2021.118371
- Asian and Saharan dust from a chemical/mineralogical point of view: differences and similarities from bulk and single particle measurements K. Kandler et al. 10.1051/e3sconf/20199903001
- A new sample preparation protocol for SEM and TEM particulate matter analysis A. Sinha et al. 10.1016/j.ultramic.2021.113365
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- Remote Sensing of Sea Salt Aerosol below Trade Wind Clouds M. Klingebiel et al. 10.1175/JAS-D-18-0139.1
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- Sun photometer retrievals of Saharan dust properties over Barbados during SALTRACE C. Toledano et al. 10.5194/acp-19-14571-2019
- Climatology of Aerosols over the Caribbean Islands: Aerosol Types, Synoptic Patterns, and Transport A. Rodríguez Vega et al. 10.1175/JAMC-D-21-0015.1
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- Comparison of operator- and computer-controlled scanning electron microscopy of particles from different atmospheric aerosol types S. Eriksen Hammer et al. 10.1007/s00216-019-01614-7
- Atmospheric Transport of North African Dust‐Bearing Supermicron Freshwater Diatoms to South America: Implications for Iron Transport to the Equatorial North Atlantic Ocean A. Barkley et al. 10.1029/2020GL090476
- Characterization of aerosol properties at Cyprus, focusing on cloud condensation nuclei and ice-nucleating particles X. Gong et al. 10.5194/acp-19-10883-2019
- Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements M. Haarig et al. 10.5194/acp-19-13773-2019
- Analysis of Electron Transparent Beam-Sensitive Samples Using Scanning Electron Microscopy Coupled With Energy-Dispersive X-ray Spectroscopy A. Brostrøm et al. 10.1017/S1431927620001464
36 citations as recorded by crossref.
- Differences and Similarities of Central Asian, African, and Arctic Dust Composition from a Single Particle Perspective K. Kandler et al. 10.3390/atmos11030269
- A review of coarse mineral dust in the Earth system A. Adebiyi et al. 10.1016/j.aeolia.2022.100849
- Measurement report: Characteristics of airborne black-carbon-containing particles during the 2021 summer COVID-19 lockdown in a typical Yangtze River Delta city, China Y. Dai et al. 10.5194/acp-24-9733-2024
- Investigation of an Intense Dust Outbreak in the Mediterranean Using XMed-Dry Network, Multiplatform Observations, and Numerical Modeling U. Rizza et al. 10.3390/app11041566
- Vertical variability of aerosol properties and trace gases over a remote marine region: a case study over Bermuda T. Ajayi et al. 10.5194/acp-24-9197-2024
- Atmospheric Deposition Over the Caribbean Region: Sea Salt and Saharan Dust Are Sources of Essential Elements on the Island of Guadeloupe Y. Xu‐Yang et al. 10.1029/2022JD037175
- Particle Size Distribution of Various Soil Materials Measured by Laser Diffraction—The Problem of Reproducibility C. Polakowski et al. 10.3390/min11050465
- Analysis of Size Distribution, Chemical Composition, and Optical Properties of Mineral Dust Particles from Dry Deposition Measurement in Tenerife: Determined by Single-Particle Characterization A. Waza et al. 10.3390/atmos14040700
- Field comparison of dry deposition samplers for collection of atmospheric mineral dust: results from single-particle characterization A. Waza et al. 10.5194/amt-12-6647-2019
- Trans‐Regional Transport of Haze Particles From the North China Plain to Yangtze River Delta During Winter J. Zhang et al. 10.1029/2020JD033778
- Complex Aerosol Characterization by Scanning Electron Microscopy Coupled with Energy Dispersive X-ray Spectroscopy A. Brostrøm et al. 10.1038/s41598-020-65383-5
- Impact of various air mass types on cloud condensation nuclei concentrations along coastal southeast Florida E. Edwards et al. 10.1016/j.atmosenv.2021.118371
- Asian and Saharan dust from a chemical/mineralogical point of view: differences and similarities from bulk and single particle measurements K. Kandler et al. 10.1051/e3sconf/20199903001
- A new sample preparation protocol for SEM and TEM particulate matter analysis A. Sinha et al. 10.1016/j.ultramic.2021.113365
- Atmospheric phosphorus and its geochemical cycling: Fundamentals, progress, and perspectives X. Diao et al. 10.1016/j.earscirev.2023.104492
- Automated identification and quantification of tire wear particles (TWP) in airborne dust: SEM/EDX single particle analysis coupled to a machine learning classifier J. Rausch et al. 10.1016/j.scitotenv.2021.149832
- Insights into the single-particle composition, size, mixing state, and aspect ratio of freshly emitted mineral dust from field measurements in the Moroccan Sahara using electron microscopy A. Panta et al. 10.5194/acp-23-3861-2023
- Vertical Variability in morphology, chemistry and optical properties of the transported Saharan air layer measured from Cape Verde and the Caribbean S. Aryasree et al. 10.1098/rsos.231433
- Analyzing two decades of dust events on the Southern Great Plains region of West Texas M. Kelley & K. Ardon-Dryer 10.1016/j.apr.2021.101091
- The Discovery of African Dust Transport to the Western Hemisphere and the Saharan Air Layer: A History J. Prospero et al. 10.1175/BAMS-D-19-0309.1
- Retrieving ice-nucleating particle concentration and ice multiplication factors using active remote sensing validated by in situ observations J. Wieder et al. 10.5194/acp-22-9767-2022
- Geochemistry and source contribution of fugitive phosphogypsum particles in Huelva, (SW Spain) R. Torres-Sánchez et al. 10.1016/j.atmosres.2019.104650
- Atmospheric Research Over the Western North Atlantic Ocean Region and North American East Coast: A Review of Past Work and Challenges Ahead A. Sorooshian et al. 10.1029/2019JD031626
- Identifying and Quantifying the Impacts of Advected North African Dust on the Concentration and Composition of Airborne Fine Particulate Matter in Houston and Galveston, Texas A. Bozlaker et al. 10.1029/2019JD030792
- The Influence of Chemical and Mineral Compositions on the Parameterization of Immersion Freezing by Volcanic Ash Particles N. Umo et al. 10.1029/2020JD033356
- Remote Sensing of Sea Salt Aerosol below Trade Wind Clouds M. Klingebiel et al. 10.1175/JAS-D-18-0139.1
- The ice-nucleating activity of African mineral dust in the Caribbean boundary layer A. Harrison et al. 10.5194/acp-22-9663-2022
- Sun photometer retrievals of Saharan dust properties over Barbados during SALTRACE C. Toledano et al. 10.5194/acp-19-14571-2019
- Climatology of Aerosols over the Caribbean Islands: Aerosol Types, Synoptic Patterns, and Transport A. Rodríguez Vega et al. 10.1175/JAMC-D-21-0015.1
- African dust deposition in Puerto Rico: Analysis of a 20-year rainfall chemistry record and comparison with models M. McClintock et al. 10.1016/j.atmosenv.2019.116907
- Characterisation of the filter inlet system on the FAAM BAe-146 research aircraft and its use for size-resolved aerosol composition measurements A. Sanchez-Marroquin et al. 10.5194/amt-12-5741-2019
- Comparison of operator- and computer-controlled scanning electron microscopy of particles from different atmospheric aerosol types S. Eriksen Hammer et al. 10.1007/s00216-019-01614-7
- Atmospheric Transport of North African Dust‐Bearing Supermicron Freshwater Diatoms to South America: Implications for Iron Transport to the Equatorial North Atlantic Ocean A. Barkley et al. 10.1029/2020GL090476
- Characterization of aerosol properties at Cyprus, focusing on cloud condensation nuclei and ice-nucleating particles X. Gong et al. 10.5194/acp-19-10883-2019
- Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements M. Haarig et al. 10.5194/acp-19-13773-2019
- Analysis of Electron Transparent Beam-Sensitive Samples Using Scanning Electron Microscopy Coupled With Energy-Dispersive X-ray Spectroscopy A. Brostrøm et al. 10.1017/S1431927620001464
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Short summary
Aging of transported Saharan dust in the Caribbean was observed by electron microscopy, yielding size, chemical composition and mixing state for each individual particle. Models were developed for assessing mixing relevant for the atmosphere. Particles become internally mixed with sulfate during transport and sea salt in the Caribbean boundary layer. The mixing increases deposition velocity and dust cloud activation, and thus may impact on radiative and cloud nucleating properties.
Aging of transported Saharan dust in the Caribbean was observed by electron microscopy, yielding...
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