Articles | Volume 18, issue 17
https://doi.org/10.5194/acp-18-13197-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-13197-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Sep 2018
Research article |
| 13 Sep 2018
Molecular insights on aging and aqueous-phase processing from ambient biomass burning emissions-influenced Po Valley fog and aerosol
Matthew Brege
Department of Chemistry, Michigan Technological University, Houghton, MI, USA
Marco Paglione
Institute of Atmospheric Sciences and Climate, Italian National Research Council, Bologna, Italy
Stefania Gilardoni
Institute of Atmospheric Sciences and Climate, Italian National Research Council, Bologna, Italy
Stefano Decesari
Institute of Atmospheric Sciences and Climate, Italian National Research Council, Bologna, Italy
Maria Cristina Facchini
Institute of Atmospheric Sciences and Climate, Italian National Research Council, Bologna, Italy
Department of Chemistry, Michigan Technological University, Houghton, MI, USA
Atmospheric Sciences Program, Michigan Technological University, Houghton, MI, USA
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28 citations as recorded by crossref.
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- High Molecular Diversity of Organic Nitrogen in Urban Snow in North China S. Su et al. 10.1021/acs.est.0c06851
- Measurement report: Molecular characteristics of cloud water in southern China and insights into aqueous-phase processes from Fourier transform ion cyclotron resonance mass spectrometry W. Sun et al. 10.5194/acp-21-16631-2021
- MFAssignR: Molecular formula assignment software for ultrahigh resolution mass spectrometry analysis of environmental complex mixtures S. Schum et al. 10.1016/j.envres.2020.110114
- On the Water-Soluble Organic Matter in Inhalable Air Particles: Why Should Outdoor Experience Motivate Indoor Studies? R. Duarte & A. Duarte 10.3390/app11219917
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- Molecular Characterization of Water‐Soluble Brown Carbon Chromophores in Beijing, China C. Yan et al. 10.1029/2019JD032018
- Strong Deviations from Thermodynamically Expected Phase Partitioning of Low-Molecular-Weight Organic Acids during One Year of Rural Measurements B. Stieger et al. 10.1021/acsearthspacechem.0c00297
- Impact of in-cloud aqueous processes on the chemical compositions and morphology of individual atmospheric aerosols Y. Fu et al. 10.5194/acp-20-14063-2020
- Analysis of reduced and oxidized nitrogen-containing organic compounds at a coastal site in summer and winter J. Ditto et al. 10.5194/acp-22-3045-2022
- Aqueous Photoreactions of Wood Smoke Brown Carbon R. Hems et al. 10.1021/acsearthspacechem.0c00117
- The Roles of N, S, and O in Molecular Absorption Features of Brown Carbon in PM 2.5 in a Typical Semi‐Arid Megacity in Northwestern China Y. Zeng et al. 10.1029/2021JD034791
- Changes in aerosol particle composition during sea fog formation events in the sea ice regions of the Arctic Ocean S. Zhao et al. 10.1016/j.atmosenv.2022.118943
- Detailed NMR analysis of water-soluble organic compounds in size-resolved particulate matter seasonally collected at a suburban site in Prague Š. Horník et al. 10.1016/j.atmosenv.2021.118757
- Atmospheric “HULIS” in Different Environments: Polarities, Molecular Sizes, and Sources Suggest More Than 50% Are Not “Humic-like” T. Spranger et al. 10.1021/acsearthspacechem.9b00299
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- Molecular Speciation of Size Fractionated Particulate Water-Soluble Organic Carbon by Two-Dimensional Nuclear Magnetic Resonance (NMR) Spectroscopy M. Chalbot et al. 10.3390/ijerph18031334
- Multidimensional Analytical Characterization of Water-Soluble Organic Aerosols: Challenges and New Perspectives R. Duarte et al. 10.3390/app11062539
- Nonlinear behavior of organic aerosol in biomass burning plumes: a microphysical model analysis I. Konovalov et al. 10.5194/acp-19-12091-2019
- A multi-year source apportionment of PM2.5 at multiple sites in the southern Po Valley (Italy) F. Scotto et al. 10.1016/j.apr.2021.101192
- Infrared Ion Spectroscopy of Environmental Organic Mixtures: Probing the Composition of α-Pinene Secondary Organic Aerosol E. Walhout et al. 10.1021/acs.est.9b02077
- Molecular Absorption and Evolution Mechanisms of PM 2.5 Brown Carbon Revealed by Electrospray Ionization Fourier Transform–Ion Cyclotron Resonance Mass Spectrometry During a Severe Winter Pollution Episode in Xi'an, China Y. Zeng et al. 10.1029/2020GL087977
- Overview of the French Operational Network for In Situ Observation of PM Chemical Composition and Sources in Urban Environments (CARA Program) O. Favez et al. 10.3390/atmos12020207
- Extreme Molecular Complexity Resulting in a Continuum of Carbonaceous Species in Biomass Burning Tar Balls from Wildfire Smoke M. Brege et al. 10.1021/acsearthspacechem.1c00141
- Molecular and physical characteristics of aerosol at a remote free troposphere site: implications for atmospheric aging S. Schum et al. 10.5194/acp-18-14017-2018
- Advanced instrumental approaches for chemical characterization of indoor particulate matter R. Duarte et al. 10.1080/05704928.2021.2018596
Latest update: 19 Mar 2023
Short summary
The detailed molecular composition of ambient fog and aerosol influenced by regional biomass burning and secondary processes was studied. Aerosol and aqueous-phase functionalization and oxidation were observed, leading to fog compositions that are more "SOA-like" than aerosols. The significance of the aqueous phase in transforming the molecular chemistry and contributing to secondary organic aerosol is demonstrated here.
The detailed molecular composition of ambient fog and aerosol influenced by regional biomass...
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