Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-12185-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-12185-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Aug 2018
Research article |
| 23 Aug 2018
| 23 Aug 2018
Urban influence on the concentration and composition of submicron particulate matter in central Amazonia
Suzane S. de Sá
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Brett B. Palm
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA
Pedro Campuzano-Jost
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA
Douglas A. Day
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA
Weiwei Hu
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA
Gabriel Isaacman-VanWertz
Department of Environmental Science, Policy, and Management, University of California, Berkeley, California, USA
now at: Department of Civil and Environmental Engineering, Virginia Tech, Blacksburg, Virginia, USA
Lindsay D. Yee
Department of Environmental Science, Policy, and Management, University of California, Berkeley, California, USA
Joel Brito
Institute of Physics, University of São Paulo, São Paulo, Brazil
now at: Laboratory for Meteorological Physics (LaMP), University Blaise Pascal, Aubière, France
Samara Carbone
Institute of Physics, University of São Paulo, São Paulo, Brazil
now at: Institute of Agricultural Sciences, Federal University of Uberlândia, Minas Gerais, Brazil
Igor O. Ribeiro
School of Technology, Amazonas State University, Manaus, Amazonas, Brazil
Glauber G. Cirino
National Institute for Amazonian Research, Manaus, Amazonas, Brazil
now at: Department of Meteorology, Geosciences Institute, Federal University of Pará, Belém, Brazil
Yingjun Liu
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
now at: Department of Environmental Science, Policy, and Management, University of California, Berkeley, California, USA
Ryan Thalman
Brookhaven National Laboratory, Upton, New York, USA
now at: Department of Chemistry, Snow College, Richfield, Utah, USA
Arthur Sedlacek
Brookhaven National Laboratory, Upton, New York, USA
Aaron Funk
Department of Atmospheric Sciences, Texas A&M University, College Station, Texas, USA
Courtney Schumacher
Department of Atmospheric Sciences, Texas A&M University, College Station, Texas, USA
John E. Shilling
Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington, USA
Johannes Schneider
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Paulo Artaxo
Institute of Physics, University of São Paulo, São Paulo, Brazil
Allen H. Goldstein
Department of Environmental Science, Policy, and Management, University of California, Berkeley, California, USA
Rodrigo A. F. Souza
School of Technology, Amazonas State University, Manaus, Amazonas, Brazil
Jian Wang
Brookhaven National Laboratory, Upton, New York, USA
Karena A. McKinney
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
now at: Department of Chemistry, Colby College, Waterville, Maine, USA
Henrique Barbosa
Institute of Physics, University of São Paulo, São Paulo, Brazil
M. Lizabeth Alexander
Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington, USA
Jose L. Jimenez
Department of Chemistry and Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA
Scot T. Martin
CORRESPONDING AUTHOR
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Department of Earth and Planetary Sciences, Harvard University, Cambridge, Massachusetts, USA
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Cited
31 citations as recorded by crossref.
- Aircraft-based observations of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX-SOA) in the tropical upper troposphere over the Amazon region C. Schulz et al. 10.5194/acp-18-14979-2018
- Aerosols from anthropogenic and biogenic sources and their interactions – modeling aerosol formation, optical properties, and impacts over the central Amazon basin J. Nascimento et al. 10.5194/acp-21-6755-2021
- Predicting Atmospheric Water-Soluble Organic Mass Reversibly Partitioned to Aerosol Liquid Water in the Eastern United States M. El-Sayed et al. 10.1021/acs.est.3c01259
- Single-particle characterization of aerosols collected at a remote site in the Amazonian rainforest and an urban site in Manaus, Brazil L. Wu et al. 10.5194/acp-19-1221-2019
- Characterization and source identification of submicron aerosol during serious haze pollution periods in Beijing P. Xu et al. 10.1016/j.jes.2021.04.005
- CCN activity and organic hygroscopicity of aerosols downwind of an urban region in central Amazonia: seasonal and diel variations and impact of anthropogenic emissions R. Thalman et al. 10.5194/acp-17-11779-2017
- Major Regional-Scale Production of O3 and Secondary Organic Aerosol in Remote Amazon Regions from the Dynamics and Photochemistry of Urban and Forest Emissions J. Nascimento et al. 10.1021/acs.est.2c01358
- Aerosol optical depth retrievals in central Amazonia from a multi-filter rotating shadow-band radiometer calibrated on-site N. Rosário et al. 10.5194/amt-12-921-2019
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- Mixing states of Amazon basin aerosol particles transported over long distances using transmission electron microscopy K. Adachi et al. 10.5194/acp-20-11923-2020
- Exploration of oxidative chemistry and secondary organic aerosol formation in the Amazon during the wet season: explicit modeling of the Manaus urban plume with GECKO-A C. Mouchel-Vallon et al. 10.5194/acp-20-5995-2020
- Contributions of biomass-burning, urban, and biogenic emissions to the concentrations and light-absorbing properties of particulate matter in central Amazonia during the dry season S. de Sá et al. 10.5194/acp-19-7973-2019
- Impact of Urban Pollution on Organic-Mediated New-Particle Formation and Particle Number Concentration in the Amazon Rainforest B. Zhao et al. 10.1021/acs.est.0c07465
- Extensive urban air pollution footprint evidenced by submicron organic aerosols molecular composition C. Salvador et al. 10.1038/s41612-022-00314-x
- Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency D. Jo et al. 10.5194/acp-21-3395-2021
- Optical properties and spectral dependence of aerosol light absorption over the Brazilian Pantanal R. Palácios et al. 10.1016/j.apr.2022.101413
- Global simulations of monoterpene-derived peroxy radical fates and the distributions of highly oxygenated organic molecules (HOMs) and accretion products R. Xu et al. 10.5194/acp-22-5477-2022
- Effects of different stagnant meteorological conditions on aerosol chemistry and regional transport changes in Beijing, China J. Li et al. 10.1016/j.atmosenv.2021.118483
- Natural and Anthropogenically Influenced Isoprene Oxidation in Southeastern United States and Central Amazon L. Yee et al. 10.1021/acs.est.0c00805
- Chemical composition of ultrafine aerosol particles in central Amazonia during the wet season H. Glicker et al. 10.5194/acp-19-13053-2019
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Gas–particle partitioning of semivolatile organic compounds when wildfire smoke comes to town Y. Liang et al. 10.5194/acp-23-12441-2023
- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
- Urban pollution greatly enhances formation of natural aerosols over the Amazon rainforest M. Shrivastava et al. 10.1038/s41467-019-08909-4
- Overview: On the transport and transformation of pollutants in the outflow of major population centres – observational data from the EMeRGe European intensive operational period in summer 2017 M. Andrés Hernández et al. 10.5194/acp-22-5877-2022
- African biomass burning affects aerosol cycling over the Amazon B. Holanda et al. 10.1038/s43247-023-00795-5
- Fossil and non-fossil sources of the carbonaceous component of PM2.5 in forest and urban areas J. Cha et al. 10.1038/s41598-023-32721-2
- Chemical Signatures of Seasonally Unique Anthropogenic Influences on Organic Aerosol Composition in the Central Amazon E. Franklin et al. 10.1021/acs.est.2c07260
- Unravelling the functions of biogenic volatiles in boreal and temperate forest ecosystems M. Šimpraga et al. 10.1007/s10342-019-01213-2
- Enhanced daytime secondary aerosol formation driven by gas–particle partitioning in downwind urban plumes M. Cai et al. 10.5194/acp-24-13065-2024
- Aircraft observations of the chemical composition and aging of aerosol in the Manaus urban plume during GoAmazon 2014/5 J. Shilling et al. 10.5194/acp-18-10773-2018
30 citations as recorded by crossref.
- Aircraft-based observations of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX-SOA) in the tropical upper troposphere over the Amazon region C. Schulz et al. 10.5194/acp-18-14979-2018
- Aerosols from anthropogenic and biogenic sources and their interactions – modeling aerosol formation, optical properties, and impacts over the central Amazon basin J. Nascimento et al. 10.5194/acp-21-6755-2021
- Predicting Atmospheric Water-Soluble Organic Mass Reversibly Partitioned to Aerosol Liquid Water in the Eastern United States M. El-Sayed et al. 10.1021/acs.est.3c01259
- Single-particle characterization of aerosols collected at a remote site in the Amazonian rainforest and an urban site in Manaus, Brazil L. Wu et al. 10.5194/acp-19-1221-2019
- Characterization and source identification of submicron aerosol during serious haze pollution periods in Beijing P. Xu et al. 10.1016/j.jes.2021.04.005
- CCN activity and organic hygroscopicity of aerosols downwind of an urban region in central Amazonia: seasonal and diel variations and impact of anthropogenic emissions R. Thalman et al. 10.5194/acp-17-11779-2017
- Major Regional-Scale Production of O3 and Secondary Organic Aerosol in Remote Amazon Regions from the Dynamics and Photochemistry of Urban and Forest Emissions J. Nascimento et al. 10.1021/acs.est.2c01358
- Aerosol optical depth retrievals in central Amazonia from a multi-filter rotating shadow-band radiometer calibrated on-site N. Rosário et al. 10.5194/amt-12-921-2019
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- Mixing states of Amazon basin aerosol particles transported over long distances using transmission electron microscopy K. Adachi et al. 10.5194/acp-20-11923-2020
- Exploration of oxidative chemistry and secondary organic aerosol formation in the Amazon during the wet season: explicit modeling of the Manaus urban plume with GECKO-A C. Mouchel-Vallon et al. 10.5194/acp-20-5995-2020
- Contributions of biomass-burning, urban, and biogenic emissions to the concentrations and light-absorbing properties of particulate matter in central Amazonia during the dry season S. de Sá et al. 10.5194/acp-19-7973-2019
- Impact of Urban Pollution on Organic-Mediated New-Particle Formation and Particle Number Concentration in the Amazon Rainforest B. Zhao et al. 10.1021/acs.est.0c07465
- Extensive urban air pollution footprint evidenced by submicron organic aerosols molecular composition C. Salvador et al. 10.1038/s41612-022-00314-x
- Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency D. Jo et al. 10.5194/acp-21-3395-2021
- Optical properties and spectral dependence of aerosol light absorption over the Brazilian Pantanal R. Palácios et al. 10.1016/j.apr.2022.101413
- Global simulations of monoterpene-derived peroxy radical fates and the distributions of highly oxygenated organic molecules (HOMs) and accretion products R. Xu et al. 10.5194/acp-22-5477-2022
- Effects of different stagnant meteorological conditions on aerosol chemistry and regional transport changes in Beijing, China J. Li et al. 10.1016/j.atmosenv.2021.118483
- Natural and Anthropogenically Influenced Isoprene Oxidation in Southeastern United States and Central Amazon L. Yee et al. 10.1021/acs.est.0c00805
- Chemical composition of ultrafine aerosol particles in central Amazonia during the wet season H. Glicker et al. 10.5194/acp-19-13053-2019
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Gas–particle partitioning of semivolatile organic compounds when wildfire smoke comes to town Y. Liang et al. 10.5194/acp-23-12441-2023
- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
- Urban pollution greatly enhances formation of natural aerosols over the Amazon rainforest M. Shrivastava et al. 10.1038/s41467-019-08909-4
- Overview: On the transport and transformation of pollutants in the outflow of major population centres – observational data from the EMeRGe European intensive operational period in summer 2017 M. Andrés Hernández et al. 10.5194/acp-22-5877-2022
- African biomass burning affects aerosol cycling over the Amazon B. Holanda et al. 10.1038/s43247-023-00795-5
- Fossil and non-fossil sources of the carbonaceous component of PM2.5 in forest and urban areas J. Cha et al. 10.1038/s41598-023-32721-2
- Chemical Signatures of Seasonally Unique Anthropogenic Influences on Organic Aerosol Composition in the Central Amazon E. Franklin et al. 10.1021/acs.est.2c07260
- Unravelling the functions of biogenic volatiles in boreal and temperate forest ecosystems M. Šimpraga et al. 10.1007/s10342-019-01213-2
- Enhanced daytime secondary aerosol formation driven by gas–particle partitioning in downwind urban plumes M. Cai et al. 10.5194/acp-24-13065-2024
Discussed (preprint)
Latest update: 10 Dec 2024
Short summary
This study aimed at understanding and quantifying the changes in mass concentration and composition of submicron airborne particulate matter (PM) in Amazonia due to urban pollution. Downwind of Manaus, PM concentrations increased by up to 200 % under polluted compared with background conditions. The observed changes included contributions from both primary and secondary processes. The differences in organic PM composition suggested a shift in the pathways of secondary production with pollution.
This study aimed at understanding and quantifying the changes in mass concentration and...
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