Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-11739-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-11739-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
17 Aug 2018
Research article |
| 17 Aug 2018
| 17 Aug 2018
Characterization of aerosol hygroscopicity, mixing state, and CCN activity at a suburban site in the central North China Plain
Yuying Wang
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
Department of Atmospheric and Oceanic Sciences and ESSIC, University
of Maryland, College Park, Maryland, USA
Yingjie Zhang
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Fang Zhang
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
Haobo Tan
Key Laboratory of Regional Numerical Weather Prediction, Institute of
Tropical and Marine Meteorology, China Meteorological Administration,
Guangzhou 510080, China
Hanbing Xu
Shared Experimental Education Center, Sun Yat-sen University,
Guangzhou 510275, China
Tianyi Fan
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
Xiaoai Jin
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
Xinxin Fan
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
Zipeng Dong
State Key Laboratory of Earth Surface Processes and Resource Ecology,
College of Global Change and Earth System Science, Beijing Normal
University, Beijing 100875, China
Qiuyan Wang
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Nanjing University of Information Science and
Technology, Nanjing 210044, China
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
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Cited
45 citations as recorded by crossref.
- Comparative Analysis of Aerosol Vertical Characteristics over the North China Plain Based on Multi-Source Observation Data F. Wang et al. 10.3390/rs16040609
- The NPF Effect on CCN Number Concentrations: A Review and Re‐Evaluation of Observations From 35 Sites Worldwide J. Ren et al. 10.1029/2021GL095190
- Measurement report: On the difference in aerosol hygroscopicity between high and low relative humidity conditions in the North China Plain J. Shi et al. 10.5194/acp-22-4599-2022
- Characteristics of atmospheric fungi in particle growth events along with new particle formation in the central North China Plain N. Luo et al. 10.1016/j.scitotenv.2019.05.299
- Role of Aerosol Physicochemical Properties on Aerosol Hygroscopicity and Cloud Condensation Nuclei Activity in a Tropical Coastal Atmosphere A. T. C. et al. 10.1021/acsearthspacechem.2c00044
- Vertical profiles of NO<sub>2</sub>, SO<sub>2</sub>, HONO, HCHO, CHOCHO and aerosols derived from MAX-DOAS measurements at a rural site in the central western North China Plain and their relation to emission sources and effects of regional transport Y. Wang et al. 10.5194/acp-19-5417-2019
- Contrasting size-resolved hygroscopicity of fine particles derived by HTDMA and HR-ToF-AMS measurements between summer and winter in Beijing: the impacts of aerosol aging and local emissions X. Fan et al. 10.5194/acp-20-915-2020
- Aerosol activation characteristics and prediction at the central European ACTRIS research station of Melpitz, Germany Y. Wang et al. 10.5194/acp-22-15943-2022
- Observational study of microphysical and chemical characteristics of size-resolved fog in different regional backgrounds in China P. Ge et al. 10.1016/j.scitotenv.2024.175329
- Assessment of Multiple Planetary Boundary Layer Height Retrieval Methods and Their Impact on PM2.5 and Its Chemical Compositions throughout a Year in Nanjing Z. Han et al. 10.3390/rs16183464
- The significant impact of aerosol vertical structure on lower atmosphere stability and its critical role in aerosol–planetary boundary layer (PBL) interactions T. Su et al. 10.5194/acp-20-3713-2020
- Different effects of anthropogenic emissions and aging processes on the mixing state of soot particles in the nucleation and accumulation modes Y. Wang et al. 10.5194/acp-22-14133-2022
- The different sensitivities of aerosol optical properties to particle concentration, humidity, and hygroscopicity between the surface level and the upper boundary layer in Guangzhou, China X. Jin et al. 10.1016/j.scitotenv.2021.150010
- The impact of aerosol size-dependent hygroscopicity and mixing state on the cloud condensation nuclei potential over the north-east Atlantic W. Xu et al. 10.5194/acp-21-8655-2021
- Size-resolved hygroscopic behaviour and mixing state of submicron aerosols in a megacity of the Sichuan Basin during pollution and fireworks episodes L. Yuan et al. 10.1016/j.atmosenv.2020.117393
- Enhancement of secondary aerosol formation by reduced anthropogenic emissions during Spring Festival 2019 and enlightenment for regional PM<sub>2.5</sub> control in Beijing Y. Wang et al. 10.5194/acp-21-915-2021
- Vertical profile of particle hygroscopicity and CCN effectiveness during winter in Beijing: insight into the hygroscopicity transition threshold of black carbon D. Hu et al. 10.1039/D0FD00077A
- Measurement report: Aircraft observations of ozone, nitrogen oxides, and volatile organic compounds over Hebei Province, China S. Benish et al. 10.5194/acp-20-14523-2020
- Ozone Pollution in the North China Plain during the 2016 Air Chemistry Research in Asia (ARIAs) Campaign: Observations and a Modeling Study H. He et al. 10.3390/air2020011
- Aerosol hygroscopicity and its link to chemical composition in the coastal atmosphere of Mace Head: marine and continental air masses W. Xu et al. 10.5194/acp-20-3777-2020
- Mathematical derivation and physical interpretation of particle size-resolved activation ratio based on particle hygroscopicity distribution: Application on global characterization of CCN activity X. Jiang et al. 10.1016/j.atmosenv.2020.118137
- Effects of volatile organic compounds and new particle formation on real-time hygroscopicity of PM2.5 particles in Seosan, Republic of Korea J. Kim et al. 10.1016/j.scitotenv.2024.171516
- Significant contribution of organics to aerosol liquid water content in winter in Beijing, China X. Jin et al. 10.5194/acp-20-901-2020
- A New Method for Distinguishing Unactivated Particles in Cloud Condensation Nuclei Measurements: Implications for Aerosol Indirect Effect Evaluation Y. Wang et al. 10.1029/2019GL085379
- In-situ observations reveal weak hygroscopicity in the Southern Tibetan Plateau: implications for aerosol activation and indirect effects Y. Wang et al. 10.1038/s41612-024-00629-x
- Measurement report: The effect of aerosol chemical composition on light scattering due to the hygroscopic swelling effect R. Ren et al. 10.5194/acp-21-9977-2021
- Measurement report: Hygroscopic growth of ambient fine particles measured at five sites in China L. Chen et al. 10.5194/acp-22-6773-2022
- Aerosol hygroscopic growth, contributing factors, and impact on haze events in a severely polluted region in northern China J. Chen et al. 10.5194/acp-19-1327-2019
- Vertical profiles of cloud condensation nuclei number concentration and its empirical estimate from aerosol optical properties over the North China Plain R. Zhang et al. 10.5194/acp-22-14879-2022
- A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations P. Patel et al. 10.5194/acp-24-2861-2024
- Distinct Ultrafine‐ and Accumulation‐Mode Particle Properties in Clean and Polluted Urban Environments Y. Wang et al. 10.1029/2019GL084047
- Measurement report: A multi-year study on the impacts of Chinese New Year celebrations on air quality in Beijing, China B. Foreback et al. 10.5194/acp-22-11089-2022
- Highly significant impact of mineral dust on aerosol hygroscopicity at New Delhi Z. Arub et al. 10.1016/j.atmosenv.2021.118375
- A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements W. Zhou et al. 10.1039/D0EM00212G
- Complex Hygroscopic Behavior of Ambient Aerosol Particles Revealed by a Piezoelectric Technique C. Jose et al. 10.1021/acsearthspacechem.3c00347
- Vertical Distributions of Aerosol and Cloud Microphysical Properties and the Aerosol Impact on a Continental Cumulus Cloud Based on Aircraft Measurements From the Loess Plateau of China Z. Cai et al. 10.3389/fenvs.2021.808861
- Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain (McFAN): integrated analysis and intensive winter campaign 2018 G. Li et al. 10.1039/D0FD00099J
- Closure Investigation on Cloud Condensation Nuclei Ability of Processed Anthropogenic Aerosols D. Hu et al. 10.1029/2020JD032680
- Physicochemical Characteristics and Formation of PM2.5 in Yongin, Korea—A Suburban Metropolitan Area I. Park et al. 10.1007/s13143-024-00371-7
- Predicting cloud condensation nuclei number concentration based on conventional measurements of aerosol properties in the North China Plain Y. Zhang et al. 10.1016/j.scitotenv.2020.137473
- Assessment of submicron aerosol liquid water content and mass-based growth factors in South Asian outflow over the Indian Ocean S. Boreddy et al. 10.1016/j.scitotenv.2023.166461
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Tropospheric aerosol hygroscopicity in China C. Peng et al. 10.5194/acp-20-13877-2020
- Size-resolved characterization of organic aerosol in the North China Plain: new insights from high resolution spectral analysis W. Xu et al. 10.1039/D1EA00025J
- Quantifying particle-to-particle heterogeneity in aerosol hygroscopicity L. Yuan & C. Zhao 10.5194/acp-23-3195-2023
45 citations as recorded by crossref.
- Comparative Analysis of Aerosol Vertical Characteristics over the North China Plain Based on Multi-Source Observation Data F. Wang et al. 10.3390/rs16040609
- The NPF Effect on CCN Number Concentrations: A Review and Re‐Evaluation of Observations From 35 Sites Worldwide J. Ren et al. 10.1029/2021GL095190
- Measurement report: On the difference in aerosol hygroscopicity between high and low relative humidity conditions in the North China Plain J. Shi et al. 10.5194/acp-22-4599-2022
- Characteristics of atmospheric fungi in particle growth events along with new particle formation in the central North China Plain N. Luo et al. 10.1016/j.scitotenv.2019.05.299
- Role of Aerosol Physicochemical Properties on Aerosol Hygroscopicity and Cloud Condensation Nuclei Activity in a Tropical Coastal Atmosphere A. T. C. et al. 10.1021/acsearthspacechem.2c00044
- Vertical profiles of NO<sub>2</sub>, SO<sub>2</sub>, HONO, HCHO, CHOCHO and aerosols derived from MAX-DOAS measurements at a rural site in the central western North China Plain and their relation to emission sources and effects of regional transport Y. Wang et al. 10.5194/acp-19-5417-2019
- Contrasting size-resolved hygroscopicity of fine particles derived by HTDMA and HR-ToF-AMS measurements between summer and winter in Beijing: the impacts of aerosol aging and local emissions X. Fan et al. 10.5194/acp-20-915-2020
- Aerosol activation characteristics and prediction at the central European ACTRIS research station of Melpitz, Germany Y. Wang et al. 10.5194/acp-22-15943-2022
- Observational study of microphysical and chemical characteristics of size-resolved fog in different regional backgrounds in China P. Ge et al. 10.1016/j.scitotenv.2024.175329
- Assessment of Multiple Planetary Boundary Layer Height Retrieval Methods and Their Impact on PM2.5 and Its Chemical Compositions throughout a Year in Nanjing Z. Han et al. 10.3390/rs16183464
- The significant impact of aerosol vertical structure on lower atmosphere stability and its critical role in aerosol–planetary boundary layer (PBL) interactions T. Su et al. 10.5194/acp-20-3713-2020
- Different effects of anthropogenic emissions and aging processes on the mixing state of soot particles in the nucleation and accumulation modes Y. Wang et al. 10.5194/acp-22-14133-2022
- The different sensitivities of aerosol optical properties to particle concentration, humidity, and hygroscopicity between the surface level and the upper boundary layer in Guangzhou, China X. Jin et al. 10.1016/j.scitotenv.2021.150010
- The impact of aerosol size-dependent hygroscopicity and mixing state on the cloud condensation nuclei potential over the north-east Atlantic W. Xu et al. 10.5194/acp-21-8655-2021
- Size-resolved hygroscopic behaviour and mixing state of submicron aerosols in a megacity of the Sichuan Basin during pollution and fireworks episodes L. Yuan et al. 10.1016/j.atmosenv.2020.117393
- Enhancement of secondary aerosol formation by reduced anthropogenic emissions during Spring Festival 2019 and enlightenment for regional PM<sub>2.5</sub> control in Beijing Y. Wang et al. 10.5194/acp-21-915-2021
- Vertical profile of particle hygroscopicity and CCN effectiveness during winter in Beijing: insight into the hygroscopicity transition threshold of black carbon D. Hu et al. 10.1039/D0FD00077A
- Measurement report: Aircraft observations of ozone, nitrogen oxides, and volatile organic compounds over Hebei Province, China S. Benish et al. 10.5194/acp-20-14523-2020
- Ozone Pollution in the North China Plain during the 2016 Air Chemistry Research in Asia (ARIAs) Campaign: Observations and a Modeling Study H. He et al. 10.3390/air2020011
- Aerosol hygroscopicity and its link to chemical composition in the coastal atmosphere of Mace Head: marine and continental air masses W. Xu et al. 10.5194/acp-20-3777-2020
- Mathematical derivation and physical interpretation of particle size-resolved activation ratio based on particle hygroscopicity distribution: Application on global characterization of CCN activity X. Jiang et al. 10.1016/j.atmosenv.2020.118137
- Effects of volatile organic compounds and new particle formation on real-time hygroscopicity of PM2.5 particles in Seosan, Republic of Korea J. Kim et al. 10.1016/j.scitotenv.2024.171516
- Significant contribution of organics to aerosol liquid water content in winter in Beijing, China X. Jin et al. 10.5194/acp-20-901-2020
- A New Method for Distinguishing Unactivated Particles in Cloud Condensation Nuclei Measurements: Implications for Aerosol Indirect Effect Evaluation Y. Wang et al. 10.1029/2019GL085379
- In-situ observations reveal weak hygroscopicity in the Southern Tibetan Plateau: implications for aerosol activation and indirect effects Y. Wang et al. 10.1038/s41612-024-00629-x
- Measurement report: The effect of aerosol chemical composition on light scattering due to the hygroscopic swelling effect R. Ren et al. 10.5194/acp-21-9977-2021
- Measurement report: Hygroscopic growth of ambient fine particles measured at five sites in China L. Chen et al. 10.5194/acp-22-6773-2022
- Aerosol hygroscopic growth, contributing factors, and impact on haze events in a severely polluted region in northern China J. Chen et al. 10.5194/acp-19-1327-2019
- Vertical profiles of cloud condensation nuclei number concentration and its empirical estimate from aerosol optical properties over the North China Plain R. Zhang et al. 10.5194/acp-22-14879-2022
- A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations P. Patel et al. 10.5194/acp-24-2861-2024
- Distinct Ultrafine‐ and Accumulation‐Mode Particle Properties in Clean and Polluted Urban Environments Y. Wang et al. 10.1029/2019GL084047
- Measurement report: A multi-year study on the impacts of Chinese New Year celebrations on air quality in Beijing, China B. Foreback et al. 10.5194/acp-22-11089-2022
- Highly significant impact of mineral dust on aerosol hygroscopicity at New Delhi Z. Arub et al. 10.1016/j.atmosenv.2021.118375
- A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements W. Zhou et al. 10.1039/D0EM00212G
- Complex Hygroscopic Behavior of Ambient Aerosol Particles Revealed by a Piezoelectric Technique C. Jose et al. 10.1021/acsearthspacechem.3c00347
- Vertical Distributions of Aerosol and Cloud Microphysical Properties and the Aerosol Impact on a Continental Cumulus Cloud Based on Aircraft Measurements From the Loess Plateau of China Z. Cai et al. 10.3389/fenvs.2021.808861
- Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain (McFAN): integrated analysis and intensive winter campaign 2018 G. Li et al. 10.1039/D0FD00099J
- Closure Investigation on Cloud Condensation Nuclei Ability of Processed Anthropogenic Aerosols D. Hu et al. 10.1029/2020JD032680
- Physicochemical Characteristics and Formation of PM2.5 in Yongin, Korea—A Suburban Metropolitan Area I. Park et al. 10.1007/s13143-024-00371-7
- Predicting cloud condensation nuclei number concentration based on conventional measurements of aerosol properties in the North China Plain Y. Zhang et al. 10.1016/j.scitotenv.2020.137473
- Assessment of submicron aerosol liquid water content and mass-based growth factors in South Asian outflow over the Indian Ocean S. Boreddy et al. 10.1016/j.scitotenv.2023.166461
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Tropospheric aerosol hygroscopicity in China C. Peng et al. 10.5194/acp-20-13877-2020
- Size-resolved characterization of organic aerosol in the North China Plain: new insights from high resolution spectral analysis W. Xu et al. 10.1039/D1EA00025J
- Quantifying particle-to-particle heterogeneity in aerosol hygroscopicity L. Yuan & C. Zhao 10.5194/acp-23-3195-2023
Saved (final revised paper)
Latest update: 14 Dec 2024
Short summary
Very different aerosol hygroscopicities and mixing states were found at these sites in the North China Plain. The PDF for 40–200 nm particles showed the particles were highly aged and internally mixed at Xingtai because of high pollution and strong photochemical reactions. A good proxy for the chemical comical composition (kappa = 0.31) in calculating CCN concentration was found. Importantly, our study investigated the influence of industrial emissions on the aerosol properties.
Very different aerosol hygroscopicities and mixing states were found at these sites in the North...
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