Articles | Volume 18, issue 14
https://doi.org/10.5194/acp-18-10773-2018
https://doi.org/10.5194/acp-18-10773-2018
Research article
 | 
30 Jul 2018
Research article |  | 30 Jul 2018

Aircraft observations of the chemical composition and aging of aerosol in the Manaus urban plume during GoAmazon 2014/5

John E. Shilling, Mikhail S. Pekour, Edward C. Fortner, Paulo Artaxo, Suzane de Sá, John M. Hubbe, Karla M. Longo, Luiz A. T. Machado, Scot T. Martin, Stephen R. Springston, Jason Tomlinson, and Jian Wang

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AR by John Shilling on behalf of the Authors (26 Jun 2018)  Author's response   Manuscript 
ED: Publish as is (12 Jul 2018) by Tuukka Petäjä
AR by John Shilling on behalf of the Authors (17 Jul 2018)
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Short summary
We report aircraft observations of the evolution of organic aerosol in the Manaus urban plume as it ages. We observe dynamic changes in the organic aerosol. The mean carbon oxidation state of the OA increases from −0.6 to −0.45. Hydrocarbon-like organic aerosol (HOA) mass is lost and is balanced out by formation of oxygenated organic aerosol (OOA). Because HOA loss is balanced by OOA formation, we observe little change in the net Δorg / ΔCO values with aging.
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