Articles | Volume 18, issue 14
https://doi.org/10.5194/acp-18-10483-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-10483-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Fast particulate nitrate formation via N2O5 uptake aloft in winter in Beijing
Haichao Wang
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Xiaorui Chen
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Qindan Zhu
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
now at: the Department of Chemistry, University of California,
Berkeley, CA 94720, USA
Zhijun Wu
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Yusheng Wu
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Kang Sun
China National Environmental Monitoring Centre, Beijing, China
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49 citations as recorded by crossref.
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- Isotopic Evidence for the High Contribution of Wintertime Photochemistry to Particulate Nitrate Formation in Northern China Z. Zhang et al. 10.1029/2021JD035324
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- Atmospheric Δ<sup>17</sup>O(NO<sub>3</sub><sup>−</sup>) reveals nocturnal chemistry dominates nitrate production in Beijing haze P. He et al. 10.5194/acp-18-14465-2018
- Model bias in simulating major chemical components of PM<sub>2.5</sub> in China R. Miao et al. 10.5194/acp-20-12265-2020
- Changes in nitrate accumulation mechanisms as PM2.5 levels increase on the North China Plain: A perspective from the dual isotopic compositions of nitrate L. Luo et al. 10.1016/j.chemosphere.2020.127915
- Low particulate nitrate in the residual layer in autumn over the North China Plain G. Tang et al. 10.1016/j.scitotenv.2021.146845
- Nighttime N2O5 chemistry in an urban site of Beijing in winter based on the measurements by cavity ring-down spectroscopy Z. Li et al. 10.1007/s11869-021-01125-4
- Formation mechanisms of atmospheric nitrate and sulfate during the winter haze pollution periods in Beijing: gas-phase, heterogeneous and aqueous-phase chemistry P. Liu et al. 10.5194/acp-20-4153-2020
- Sources of cellular oxidative potential of water-soluble fine ambient particulate matter in the Midwestern United States Y. Wang et al. 10.1016/j.jhazmat.2021.127777
- The promotion effect of nitrous acid on aerosol formation in wintertime in Beijing: the possible contribution of traffic-related emissions Y. Liu et al. 10.5194/acp-20-13023-2020
- Measurement report: Vertical distribution of biogenic and anthropogenic secondary organic aerosols in the urban boundary layer over Beijing during late summer H. Ren et al. 10.5194/acp-21-12949-2021
- Air pollution scenario over Pakistan: Characterization and ranking of extremely polluted cities using long-term concentrations of aerosols and trace gases M. Bilal et al. 10.1016/j.rse.2021.112617
- Sources and transformation of nitrate aerosol in winter 2017–2018 of megacity Beijing: Insights from an alternative approach Z. Zhang et al. 10.1016/j.atmosenv.2020.117842
- Observations of N2O5 and NO3 at a suburban environment in Yangtze river delta in China: Estimating heterogeneous N2O5 uptake coefficients Z. Li et al. 10.1016/j.jes.2020.04.041
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- Measurements of atmospheric aerosol vertical distribution above North China Plain using hexacopter Y. Zhu et al. 10.1016/j.scitotenv.2019.02.100
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- Nocturnal atmospheric chemistry of NO3 and N2O5 over Changzhou in the Yangtze River Delta in China C. Lin et al. 10.1016/j.jes.2021.09.016
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- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ C. Jordan et al. 10.1525/elementa.424
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- Explosive Secondary Aerosol Formation during Severe Haze in the North China Plain J. Peng et al. 10.1021/acs.est.0c07204
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- Characteristics of aerosol chemistry and acidity in Shanghai after PM2.5 satisfied national guideline: Insight into future emission control Z. Fu et al. 10.1016/j.scitotenv.2022.154319
Latest update: 25 Mar 2023
Short summary
The vertical measurement of NOx and O3 was carried out on a movable carriage on a tower during a winter heavy-haze episode in urban Beijing, China. We found that pNO3- formation via N2O5 uptake was significant at high altitudes (e.g., > 150 m), which was supported by the lower total oxidant
(NO2 + O3) level at high altitudes than at ground level. This study highlights the fact that pNO3- formation via N2O5 uptake may be an important source of pNO3- in the urban airshed during wintertime.
The vertical measurement of NOx and O3 was carried out on a movable carriage on a tower during a...
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