Articles | Volume 17, issue 15
https://doi.org/10.5194/acp-17-9237-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-9237-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
01 Aug 2017
Research article |
| 01 Aug 2017
Evaluating the impact of new observational constraints on P-S/IVOC emissions, multi-generation oxidation, and chamber wall losses on SOA modeling for Los Angeles, CA
Prettiny K. Ma
Department of Chemistry, Université de Montréal, Montréal,
QC, Canada
Yunliang Zhao
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, USA
Allen L. Robinson
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, USA
David R. Worton
Department of Environmental Science, Policy and Management, University
of California, Berkeley, CA, USA
now at: National Physical Laboratory, Hampton Rd, Teddington,
Middlesex, UK
Allen H. Goldstein
Department of Environmental Science, Policy and Management, University
of California, Berkeley, CA, USA
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA, USA
Amber M. Ortega
Cooperative Institute for Research in the Environmental Sciences and
Dept. of Chemistry and Biochemistry, University of Colorado, Boulder, CO,
USA
now at: Air Pollution Control Division, Colorado Department of Public
Health and Environment, Denver, CO, USA
Jose L. Jimenez
Cooperative Institute for Research in the Environmental Sciences and
Dept. of Chemistry and Biochemistry, University of Colorado, Boulder, CO,
USA
Peter Zotter
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
now at: Lucerne University of Applied Sciences and Arts, School of
Engineering and Architecture, Bioenergy Research, Technikumstrasse 21,
6048 Horw, Switzerland
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Sönke Szidat
Department of Chemistry and Biochemistry & Oeschger Centre for
Climate Change, University of Bern, Bern, Switzerland
Patrick L. Hayes
CORRESPONDING AUTHOR
Department of Chemistry, Université de Montréal, Montréal,
QC, Canada
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Cited
42 citations as recorded by crossref.
- Modified Silica Adsorbents for Toluene Adsorption under Dry and Humid Conditions: Impacts of Pore Size and Surface Chemistry S. Liu et al. 10.1021/acs.langmuir.9b01031
- Semivolatile POA and parameterized total combustion SOA in CMAQv5.2: impacts on source strength and partitioning B. Murphy et al. 10.5194/acp-17-11107-2017
- Contribution of Organic Nitrates to Organic Aerosol over South Korea during KORUS-AQ H. Kenagy et al. 10.1021/acs.est.1c05521
- Comparison of secondary organic aerosol formation from toluene on initially wet and dry ammonium sulfate particles at moderate relative humidity T. Liu et al. 10.5194/acp-18-5677-2018
- Profiles of ambient semi- and intermediate- volatility organic compounds (S/IVOCs) in winter of urban Chengdu Q. Zhou et al. 10.1016/j.scitotenv.2024.177480
- Secondary Organic Aerosol Formation from Urban Roadside Air in Hong Kong T. Liu et al. 10.1021/acs.est.8b06587
- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ C. Jordan et al. 10.1525/elementa.424
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- The newest emission inventory of anthropogenic full-volatility organic in Central China Y. Liu et al. 10.1016/j.atmosres.2024.107245
- An updated comprehensive anthropogenic S/IVOCs emission inventory in Central China: Spatial and Temporal characteristics S. Wang et al. 10.1016/j.atmosres.2022.106546
- Volatile chemical products emerging as largest petrochemical source of urban organic emissions B. McDonald et al. 10.1126/science.aaq0524
- An investigation of petrochemical emissions during KORUS-AQ: Ozone production, reactive nitrogen evolution, and aerosol production Y. Lee et al. 10.1525/elementa.2022.00079
- Secondary organic aerosol production from local emissions dominates the organic aerosol budget over Seoul, South Korea, during KORUS-AQ B. Nault et al. 10.5194/acp-18-17769-2018
- Potential impacts of Arctic warming on Northern Hemisphere mid-latitude aerosol optical depth Y. Chen et al. 10.1007/s00382-019-04706-3
- Roles of semivolatile and intermediate-volatility organic compounds in secondary organic aerosol formation and its implication: A review Z. Ling et al. 10.1016/j.jes.2021.08.055
- Atmospheric oxidation of C10~14 n-alkanes initiated by Cl atoms: Kinetics and mechanism B. Shi et al. 10.1016/j.atmosenv.2019.117166
- Contrasting Reactive Organic Carbon Observations in the Southeast United States (SOAS) and Southern California (CalNex) C. Heald et al. 10.1021/acs.est.0c05027
- Global Simulations of Phase State and Equilibration Time Scales of Secondary Organic Aerosols with GEOS-Chem R. Luu et al. 10.1021/acsearthspacechem.4c00281
- Potential of select intermediate-volatility organic compounds and consumer products for secondary organic aerosol and ozone formation under relevant urban conditions W. Li et al. 10.1016/j.atmosenv.2017.12.019
- Distribution and sources of SVOCs in fine and coarse aerosols in the megacity of Istanbul R. Flores et al. 10.1016/j.atmosres.2022.106100
- Mobile Sources Are Still an Important Source of Secondary Organic Aerosol and Fine Particulate Matter in the Los Angeles Region Y. Zhao et al. 10.1021/acs.est.2c03317
- Elucidating the unexpected importance of intermediate-volatility organic compounds (IVOCs) from refueling procedure X. Yang et al. 10.1016/j.jhazmat.2024.134361
- Marked impacts of transient conditions on potential secondary organic aerosol production during rapid oxidation of gasoline exhausts J. Zhang et al. 10.1038/s41612-023-00385-4
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- How ethanol and gasoline formula changes evaporative emissions of the vehicles H. Man et al. 10.1016/j.apenergy.2018.03.109
- Intermediate-Volatility Organic Compound Emissions from Nonroad Construction Machinery under Different Operation Modes L. Qi et al. 10.1021/acs.est.9b01316
- Sources and Secondary Production of Organic Aerosols in the Northeastern United States during WINTER J. Schroder et al. 10.1029/2018JD028475
- Temperature-dependent emissions dominate aerosol and ozone formation in Los Angeles E. Pfannerstill et al. 10.1126/science.adg8204
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NOx A. Akherati et al. 10.5194/acp-19-4561-2019
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- Evaluating SOA formation from different sources of semi- and intermediate-volatility organic compounds from the Athabasca oil sands J. Sommers et al. 10.1039/D1EA00053E
- Asphalt-related emissions are a major missing nontraditional source of secondary organic aerosol precursors P. Khare et al. 10.1126/sciadv.abb9785
- Chemical Composition of Fresh and Aged Asphalt-Related Organic Aerosols: From Ambient Observations to Laboratory Experiments P. Khare et al. 10.1021/acsestair.4c00193
- Kinetics and mechanisms of the gas-phase reactions of OH radicals with three C15 alkanes B. Shi et al. 10.1016/j.atmosenv.2019.03.028
- Secondary organic aerosols from anthropogenic volatile organic compounds contribute substantially to air pollution mortality B. Nault et al. 10.5194/acp-21-11201-2021
- Reactions of C12–C14 n-Alkylcyclohexanes with Cl Atoms: Kinetics and Secondary Organic Aerosol Formation K. Wang et al. 10.1021/acs.est.1c08958
- Effects of gas–wall interactions on measurements of semivolatile compounds and small polar molecules X. Liu et al. 10.5194/amt-12-3137-2019
- Using observed urban NOx sinks to constrain VOC reactivity and the ozone and radical budget in the Seoul Metropolitan Area B. Nault et al. 10.5194/acp-24-9573-2024
- Widespread Pollution From Secondary Sources of Organic Aerosols During Winter in the Northeastern United States V. Shah et al. 10.1029/2018GL081530
- Oxidation Flow Reactor Results in a Chinese Megacity Emphasize the Important Contribution of S/IVOCs to Ambient SOA Formation W. Hu et al. 10.1021/acs.est.1c03155
42 citations as recorded by crossref.
- Modified Silica Adsorbents for Toluene Adsorption under Dry and Humid Conditions: Impacts of Pore Size and Surface Chemistry S. Liu et al. 10.1021/acs.langmuir.9b01031
- Semivolatile POA and parameterized total combustion SOA in CMAQv5.2: impacts on source strength and partitioning B. Murphy et al. 10.5194/acp-17-11107-2017
- Contribution of Organic Nitrates to Organic Aerosol over South Korea during KORUS-AQ H. Kenagy et al. 10.1021/acs.est.1c05521
- Comparison of secondary organic aerosol formation from toluene on initially wet and dry ammonium sulfate particles at moderate relative humidity T. Liu et al. 10.5194/acp-18-5677-2018
- Profiles of ambient semi- and intermediate- volatility organic compounds (S/IVOCs) in winter of urban Chengdu Q. Zhou et al. 10.1016/j.scitotenv.2024.177480
- Secondary Organic Aerosol Formation from Urban Roadside Air in Hong Kong T. Liu et al. 10.1021/acs.est.8b06587
- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ C. Jordan et al. 10.1525/elementa.424
- Considering the future of anthropogenic gas-phase organic compound emissions and the increasing influence of non-combustion sources on urban air quality P. Khare & D. Gentner 10.5194/acp-18-5391-2018
- Volatility of Cl-Initiated C12–C14 n-Alkylcyclohexane Secondary Organic Aerosol: Effects of NOx and Photoaging K. Wang et al. 10.1021/acsearthspacechem.2c00035
- The newest emission inventory of anthropogenic full-volatility organic in Central China Y. Liu et al. 10.1016/j.atmosres.2024.107245
- An updated comprehensive anthropogenic S/IVOCs emission inventory in Central China: Spatial and Temporal characteristics S. Wang et al. 10.1016/j.atmosres.2022.106546
- Volatile chemical products emerging as largest petrochemical source of urban organic emissions B. McDonald et al. 10.1126/science.aaq0524
- An investigation of petrochemical emissions during KORUS-AQ: Ozone production, reactive nitrogen evolution, and aerosol production Y. Lee et al. 10.1525/elementa.2022.00079
- Secondary organic aerosol production from local emissions dominates the organic aerosol budget over Seoul, South Korea, during KORUS-AQ B. Nault et al. 10.5194/acp-18-17769-2018
- Potential impacts of Arctic warming on Northern Hemisphere mid-latitude aerosol optical depth Y. Chen et al. 10.1007/s00382-019-04706-3
- Roles of semivolatile and intermediate-volatility organic compounds in secondary organic aerosol formation and its implication: A review Z. Ling et al. 10.1016/j.jes.2021.08.055
- Atmospheric oxidation of C10~14 n-alkanes initiated by Cl atoms: Kinetics and mechanism B. Shi et al. 10.1016/j.atmosenv.2019.117166
- Contrasting Reactive Organic Carbon Observations in the Southeast United States (SOAS) and Southern California (CalNex) C. Heald et al. 10.1021/acs.est.0c05027
- Global Simulations of Phase State and Equilibration Time Scales of Secondary Organic Aerosols with GEOS-Chem R. Luu et al. 10.1021/acsearthspacechem.4c00281
- Potential of select intermediate-volatility organic compounds and consumer products for secondary organic aerosol and ozone formation under relevant urban conditions W. Li et al. 10.1016/j.atmosenv.2017.12.019
- Distribution and sources of SVOCs in fine and coarse aerosols in the megacity of Istanbul R. Flores et al. 10.1016/j.atmosres.2022.106100
- Mobile Sources Are Still an Important Source of Secondary Organic Aerosol and Fine Particulate Matter in the Los Angeles Region Y. Zhao et al. 10.1021/acs.est.2c03317
- Elucidating the unexpected importance of intermediate-volatility organic compounds (IVOCs) from refueling procedure X. Yang et al. 10.1016/j.jhazmat.2024.134361
- Marked impacts of transient conditions on potential secondary organic aerosol production during rapid oxidation of gasoline exhausts J. Zhang et al. 10.1038/s41612-023-00385-4
- Improving air quality model predictions of organic species using measurement-derived organic gaseous and particle emissions in a petrochemical-dominated region C. Stroud et al. 10.5194/acp-18-13531-2018
- Measurements of higher alkanes using NO+ chemical ionization in PTR-ToF-MS: important contributions of higher alkanes to secondary organic aerosols in China C. Wang et al. 10.5194/acp-20-14123-2020
- How ethanol and gasoline formula changes evaporative emissions of the vehicles H. Man et al. 10.1016/j.apenergy.2018.03.109
- Intermediate-Volatility Organic Compound Emissions from Nonroad Construction Machinery under Different Operation Modes L. Qi et al. 10.1021/acs.est.9b01316
- Sources and Secondary Production of Organic Aerosols in the Northeastern United States during WINTER J. Schroder et al. 10.1029/2018JD028475
- Temperature-dependent emissions dominate aerosol and ozone formation in Los Angeles E. Pfannerstill et al. 10.1126/science.adg8204
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NOx A. Akherati et al. 10.5194/acp-19-4561-2019
- Simulation of secondary organic aerosol over the Yangtze River Delta region: The impacts from the emissions of intermediate volatility organic compounds and the SOA modeling framework L. Huang et al. 10.1016/j.atmosenv.2020.118079
- Evaluating SOA formation from different sources of semi- and intermediate-volatility organic compounds from the Athabasca oil sands J. Sommers et al. 10.1039/D1EA00053E
- Asphalt-related emissions are a major missing nontraditional source of secondary organic aerosol precursors P. Khare et al. 10.1126/sciadv.abb9785
- Chemical Composition of Fresh and Aged Asphalt-Related Organic Aerosols: From Ambient Observations to Laboratory Experiments P. Khare et al. 10.1021/acsestair.4c00193
- Kinetics and mechanisms of the gas-phase reactions of OH radicals with three C15 alkanes B. Shi et al. 10.1016/j.atmosenv.2019.03.028
- Secondary organic aerosols from anthropogenic volatile organic compounds contribute substantially to air pollution mortality B. Nault et al. 10.5194/acp-21-11201-2021
- Reactions of C12–C14 n-Alkylcyclohexanes with Cl Atoms: Kinetics and Secondary Organic Aerosol Formation K. Wang et al. 10.1021/acs.est.1c08958
- Effects of gas–wall interactions on measurements of semivolatile compounds and small polar molecules X. Liu et al. 10.5194/amt-12-3137-2019
- Using observed urban NOx sinks to constrain VOC reactivity and the ozone and radical budget in the Seoul Metropolitan Area B. Nault et al. 10.5194/acp-24-9573-2024
- Widespread Pollution From Secondary Sources of Organic Aerosols During Winter in the Northeastern United States V. Shah et al. 10.1029/2018GL081530
- Oxidation Flow Reactor Results in a Chinese Megacity Emphasize the Important Contribution of S/IVOCs to Ambient SOA Formation W. Hu et al. 10.1021/acs.est.1c03155
Discussed (final revised paper)
Discussed (preprint)
Latest update: 27 Jun 2025
Short summary
Airborne particulate matter (PM) negatively impacts air quality in cities throughout the world. An important fraction of PM is organic aerosol. We have evaluated and developed several new models for secondary organic aerosol (SOA), which is formed from the chemical processing of gaseous precursors. Using our model results, we have quantified important SOA sources and precursors and also identified possible model parameterizations that could be used for air quality predictions.
Airborne particulate matter (PM) negatively impacts air quality in cities throughout the world....
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