Articles | Volume 17, issue 13
Atmos. Chem. Phys., 17, 8357–8370, 2017
https://doi.org/10.5194/acp-17-8357-2017
Atmos. Chem. Phys., 17, 8357–8370, 2017
https://doi.org/10.5194/acp-17-8357-2017

Research article 10 Jul 2017

Research article | 10 Jul 2017

Comprehensive atmospheric modeling of reactive cyclic siloxanes and their oxidation products

Nathan J. Janechek et al.

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AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment
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AR: Author's response | RR: Referee report | ED: Editor decision
AR by Nathan Janechek on behalf of the Authors (22 Apr 2017)  Author's response    Manuscript
ED: Referee Nomination & Report Request started (25 Apr 2017) by James B. Burkholder
RR by Anonymous Referee #2 (01 May 2017)
RR by Anonymous Referee #1 (06 May 2017)
ED: Publish as is (15 May 2017) by James B. Burkholder
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Short summary
Gas-phase cyclic volatile methyl siloxanes and their oxidation products, which are likely precursors to secondary organic aerosol, were modeled using an atmospheric transport model over North America. Typical concentrations, spatial patterns, seasonal variability, and vertical profiles were quantified. Urban parent compound concentrations were sensitive to transport factors, while rural parent and oxidized product concentrations were sensitive to large-scale seasonal variability in OH.
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